From 2be5b10eab9f3f79202cce9200cb5814c40724ad Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Fri, 17 Apr 2026 14:47:21 +0200 Subject: [PATCH 001/119] started with ECM --- .../EquivalentCircuitModel.m | 135 ++++++++++++++++++ .../EquivalentCircuitModelInputParams.m | 53 +++++++ .../EquivalentCircuitModel/exampleECM.json | 15 ++ Battery/EquivalentCircuitModel/exampleECM.m | 12 ++ 4 files changed, 215 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/EquivalentCircuitModel.m create mode 100644 Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m create mode 100644 Battery/EquivalentCircuitModel/exampleECM.json create mode 100644 Battery/EquivalentCircuitModel/exampleECM.m diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m new file mode 100644 index 000000000..7c108bee5 --- /dev/null +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -0,0 +1,135 @@ +classdef EquivalentCircuitModel < BaseModel + + properties + + nominalcellcapacity + + OCP + R0 + R1 + C1 + R2 + C2 + + initSOC + initOverpotential2 + lowerVoltageCutoff + + %% helpers + OCPfunc + end + + methods + + function model = EquivalentCircuitModel(inputparams) + + model = model@BaseModel(); + + %% Setup the model using the input parameters + + fdnames = {'nominalcellcapacity', ... + 'OCP' , ... + 'R0' , ... + 'R1' , ... + 'C1' , ... + 'R2' , ... + 'C2' , ... + 'initSOC' , ... + 'initOverpotential2' , ... + 'lowerVoltageCutoff'}; + + model = dispatchParams(model, inputparams, fdnames); + + model.OCPfunc = setupFunction(model.OCP); + + end + + function model = registerVarAndPropfuncNames(model) + + model = registerVarAndPropfuncNames@BaseModel(model); + + varnames = {}; + % Current + varnames{end + 1} = 'I'; + % + varnames{end + 1} = 'OCP'; + % + varnames{end + 1} = 'U'; + + varnames{end + 1} = 'UR'; + varnames{end + 1} = 'U1'; + varnames{end + 1} = 'U2'; + varnames{end + 1} = 'SOC'; + + varnames{end + 1} = 'dU1dt'; + varnames{end + 1} = 'dU2dt'; + varnames{end + 1} = 'dSOCdt'; + + model = model.registerVarNames(varnames); + + fn = @EquivalentCircuitModel.updateUR; + inputnames = {'I'}; + model = model.registerPropFunction({'UR', fn, inputnames}); + + fn = @EquivalentCircuitModel.updatedU1dt; + inputnames = {'U1', 'I'}; + model = model.registerPropFunction({'dU1dt', fn, inputnames}); + + fn = @EquivalentCircuitModel.updatedU2dt; + inputnames = {'U2', 'I'}; + model = model.registerPropFunction({'dU2dt', fn, inputnames}); + + fn = @EquivalentCircuitModel.updatedSOCdt; + inputnames = {'I'}; + model = model.registerPropFunction({'dSOCdt', fn, inputnames}); + + fn = @EquivalentCircuitModel.updateU; + inputnames = {'SOC', 'U1', 'U2', 'UR'}; + model = model.registerPropFunction({'U', fn, inputnames}); + + end + + function state = updateUR(model, state) + + state.UR = model.R0*state.I; + + end + + function state = updatedU1dt(model, state) + + state.dU2dt = model.updatedUdt(state.U2, model.R2, model.C2, state.I); + + end + + function state = updatedU2dt(model, state) + + state.dU1dt = model.updatedUdt(state.U1, model.R1, model.C1, state.I); + + end + + function state = updatedSOCdt(model, state) + + Qmax = model.nominalcellcapacity; + + state.dSOCdt = -(1 / Qmax) * state.I; + + end + + function state = updateU(model, state) + + OCP = model.OCPfunc(state.SOC); + state.U = OCP - (state.U1 + state.U2 + state.UR); + + end + + end + + methods (Static) + + function dUdt = updatedUdt(U, R, C, I) + dUdt = -(1 / (R * C)) * U + (1 / C) * I; + end + + end + +end diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m new file mode 100644 index 000000000..f6e5092b3 --- /dev/null +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m @@ -0,0 +1,53 @@ +classdef EquivalentCircuitModelInputParams < InputParams +% +% Input parameter class for the :code:`Battery` model. +% + + properties + + nominalcellcapacity + OCP + R0 + R1 + C1 + R2 + C2 + initSOC + initOverpotential2 + lowerVoltageCutoff + + end + + methods + + function inputparams = EquivalentCircuitModelInputParams(jsonstruct) + + inputparams = inputparams@InputParams(jsonstruct); + + end + + end + +end + + + +%{ +Copyright 2021-2024 SINTEF Industry, Sustainable Energy Technology +and SINTEF Digital, Mathematics & Cybernetics. + +This file is part of The Battery Modeling Toolbox BattMo + +BattMo is free software: you can redistribute it and/or modify +it under the terms of the GNU General Public License as published by +the Free Software Foundation, either version 3 of the License, or +(at your option) any later version. + +BattMo is distributed in the hope that it will be useful, +but WITHOUT ANY WARRANTY; without even the implied warranty of +MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the +GNU General Public License for more details. + +You should have received a copy of the GNU General Public License +along with BattMo. If not, see . +%} diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json new file mode 100644 index 000000000..656df760a --- /dev/null +++ b/Battery/EquivalentCircuitModel/exampleECM.json @@ -0,0 +1,15 @@ +{ "nominalcellcapacity" : 63.7, + "OCP" : { + "functionFormat" : "tabulated", + "argumentList" : ["SOC"], + "dataX" : [0.000000, 0.020000, 0.040000, 0.060000, 0.080000, 0.100000, 0.120000, 0.140000, 0.160000, 0.180000, 0.200000, 0.220000, 0.240000, 0.260000, 0.280000, 0.300000, 0.320000, 0.340000, 0.360000, 0.380000, 0.400000, 0.420000, 0.440000, 0.460000, 0.480000, 0.500000, 0.520000, 0.540000, 0.560000, 0.580000, 0.600000, 0.620000, 0.640000, 0.660000, 0.680000, 0.700000, 0.720000, 0.740000, 0.760000, 0.780000, 0.800000, 0.820000, 0.840000, 0.860000, 0.880000, 0.900000, 0.920000, 0.940000, 0.960000, 0.980000, 1.000000], + "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]}, + + "R0" : 10, + "R1" : 10, + "C1" : 10, + "R2" : 10, + "C2" : 10, + "initSOC" : 10, + "initOverpotential2" : 10, + "lowerVoltageCutoff" : 10} diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m new file mode 100644 index 000000000..ee1d3f4f0 --- /dev/null +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -0,0 +1,12 @@ +jsonstruct = parseBattmoJson('exampleECM.json'); +inputparams = EquivalentCircuitModelInputParams(jsonstruct); +model = EquivalentCircuitModel(inputparams); + +cgit = model.cgit; + +clear state; +state.I = 3; + + +state = model.evalVarName(state, {'dSOCdt'}); +state = model.evalVarName(state, {'U'}); From 07ab3f213d4855aa55ed8b17236b6f0daff0007c Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Fri, 17 Apr 2026 14:54:32 +0200 Subject: [PATCH 002/119] update in ECM --- .../EquivalentCircuitModel.m | 14 ++++++++++++++ Battery/EquivalentCircuitModel/exampleECM.m | 1 - 2 files changed, 14 insertions(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index 7c108bee5..277513813 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -121,6 +121,20 @@ state.U = OCP - (state.U1 + state.U2 + state.UR); end + + function state0 = setupInitialCondition(model, SOC0) + + state0.U1 = 0; + state0.U2 = 0; + state0.SOC = SOC0; + + end + + function solve(model, SOC0) + + state0 = model.setupInitialCondition(SOC0); + + end end diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index ee1d3f4f0..4d7a9fc8f 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -7,6 +7,5 @@ clear state; state.I = 3; - state = model.evalVarName(state, {'dSOCdt'}); state = model.evalVarName(state, {'U'}); From 1fd72380d587e2400c05ff9798e231c92c7bbe65 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Fri, 17 Apr 2026 16:19:47 +0200 Subject: [PATCH 003/119] update in ecm --- .../EquivalentCircuitModel.m | 71 ++++++++++++++++++- .../EquivalentCircuitModelInputParams.m | 1 + .../EquivalentCircuitModel/exampleECM.json | 10 ++- Battery/EquivalentCircuitModel/exampleECM.m | 8 +-- 4 files changed, 79 insertions(+), 11 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index 277513813..67af03d0a 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -15,8 +15,12 @@ initOverpotential2 lowerVoltageCutoff + I + totalTime + %% helpers OCPfunc + Ifunc end methods @@ -36,11 +40,13 @@ 'C2' , ... 'initSOC' , ... 'initOverpotential2' , ... - 'lowerVoltageCutoff'}; + 'lowerVoltageCutoff' , ... + 'I'}; model = dispatchParams(model, inputparams, fdnames); model.OCPfunc = setupFunction(model.OCP); + model.Ifunc = setupFunction(model.I); end @@ -129,10 +135,69 @@ state0.SOC = SOC0; end + + function state = setupStateFromY(model, y) + + state.U1 = y(1); + state.U2 = y(2); + state.SOC = y(3); + + end + + function y = setupYfromState(model, state) + + y(1) = state.U1; + y(2) = state.U2; + y(3) = state.SOC; + + end - function solve(model, SOC0) + function y = setupFfromState(model, state) - state0 = model.setupInitialCondition(SOC0); + y(1) = state.dU1dt; + y(2) = state.dU2dt; + y(3) = state.dSOCdt; + + end + + function f = ode(model, t, y) + + state = model.setupStateFromY(y); + + state.I = model.Ifunc(t); + + state = model.evalVarName(state, 'dU1dt'); + state = model.evalVarName(state, 'dU2dt'); + state = model.evalVarName(state, 'dSOCdt'); + + f = model.setupFromState(state); + + end + + function U = solve(model) + + if isempty(model.computationalGraph) + model = setupComputationalGraph(model) + end + + % setup initial condition + state0 = model.setupInitialCondition(model.initSOC); + y0 = model.setupYfromState(state0); + + % setup time span + tspan = [0, model.totalTime]; + + % solve ode + [t_out, y_out] = ode45(@(t, y) model.ode(t, y), tspan, y0) + + for i = 1:length(t_out) + + state = model.setupStateFromY(y_out(i, :)); + state.I = model.Ifunc(t_out(i)); + state = model.evalVarName(state, 'U'); + U(i) = state.U; + + end end diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m index f6e5092b3..06e831c40 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m @@ -15,6 +15,7 @@ initSOC initOverpotential2 lowerVoltageCutoff + I end diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json index 656df760a..29cf61aed 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.json +++ b/Battery/EquivalentCircuitModel/exampleECM.json @@ -12,4 +12,12 @@ "C2" : 10, "initSOC" : 10, "initOverpotential2" : 10, - "lowerVoltageCutoff" : 10} + "lowerVoltageCutoff" : 10, + "I" : { + "functionFormat" : "tabulated", + "argumentList" : ["time"], + "dataX" : [0, 500, 500.1, 1000, 1000.1, 1500], + "dataY" : [1, 1, 0, 0, -0.5, -0.5] + }, + "totalTime" : 1500 +} diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 4d7a9fc8f..63bbcacb2 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -2,10 +2,4 @@ inputparams = EquivalentCircuitModelInputParams(jsonstruct); model = EquivalentCircuitModel(inputparams); -cgit = model.cgit; - -clear state; -state.I = 3; - -state = model.evalVarName(state, {'dSOCdt'}); -state = model.evalVarName(state, {'U'}); +model.solve() From ca45a81aff6e9909bfbbb891f12eae300d9be79d Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Fri, 17 Apr 2026 16:30:07 +0200 Subject: [PATCH 004/119] update in ecm --- .../EquivalentCircuitModel.m | 19 +++++++++++-------- .../EquivalentCircuitModelInputParams.m | 3 ++- .../EquivalentCircuitModel/exampleECM.json | 10 +++++----- Battery/EquivalentCircuitModel/exampleECM.m | 10 +++++++++- 4 files changed, 27 insertions(+), 15 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index 67af03d0a..3a6821dab 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -41,7 +41,8 @@ 'initSOC' , ... 'initOverpotential2' , ... 'lowerVoltageCutoff' , ... - 'I'}; + 'I' , ... + 'totalTime'}; model = dispatchParams(model, inputparams, fdnames); @@ -157,6 +158,7 @@ y(1) = state.dU1dt; y(2) = state.dU2dt; y(3) = state.dSOCdt; + y = y'; end @@ -170,14 +172,14 @@ state = model.evalVarName(state, 'dU2dt'); state = model.evalVarName(state, 'dSOCdt'); - f = model.setupFromState(state); + f = model.setupFfromState(state); end - function U = solve(model) + function [t, U, I] = solve(model) if isempty(model.computationalGraph) - model = setupComputationalGraph(model) + model = setupComputationalGraph(model); end % setup initial condition @@ -188,17 +190,18 @@ tspan = [0, model.totalTime]; % solve ode - [t_out, y_out] = ode45(@(t, y) model.ode(t, y), tspan, y0) + [t_out, y_out] = ode45(@(t, y) model.ode(t, y), tspan, y0); for i = 1:length(t_out) state = model.setupStateFromY(y_out(i, :)); - state.I = model.Ifunc(t_out(i)); + I(i) = model.Ifunc(t_out(i)); + state.I = I(i); state = model.evalVarName(state, 'U'); U(i) = state.U; - end - + + t = t_out; end end diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m index 06e831c40..10b6a0e12 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m @@ -15,7 +15,8 @@ initSOC initOverpotential2 lowerVoltageCutoff - I + I + totalTime end diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json index 29cf61aed..1b74e3a53 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.json +++ b/Battery/EquivalentCircuitModel/exampleECM.json @@ -5,11 +5,11 @@ "dataX" : [0.000000, 0.020000, 0.040000, 0.060000, 0.080000, 0.100000, 0.120000, 0.140000, 0.160000, 0.180000, 0.200000, 0.220000, 0.240000, 0.260000, 0.280000, 0.300000, 0.320000, 0.340000, 0.360000, 0.380000, 0.400000, 0.420000, 0.440000, 0.460000, 0.480000, 0.500000, 0.520000, 0.540000, 0.560000, 0.580000, 0.600000, 0.620000, 0.640000, 0.660000, 0.680000, 0.700000, 0.720000, 0.740000, 0.760000, 0.780000, 0.800000, 0.820000, 0.840000, 0.860000, 0.880000, 0.900000, 0.920000, 0.940000, 0.960000, 0.980000, 1.000000], "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]}, - "R0" : 10, - "R1" : 10, - "C1" : 10, - "R2" : 10, - "C2" : 10, + "R0" : 5e-3, + "R1" : 5e-3, + "C1" : 4e3, + "R2" : 5e-3, + "C2" : 1.44e5, "initSOC" : 10, "initOverpotential2" : 10, "lowerVoltageCutoff" : 10, diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 63bbcacb2..0213ab512 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -2,4 +2,12 @@ inputparams = EquivalentCircuitModelInputParams(jsonstruct); model = EquivalentCircuitModel(inputparams); -model.solve() +[t, U, I] = model.solve(); + +%% + +tiledlayout(1, 2); +nexttile +plot(t, U) +nexttile +plot(t, I) From c058e246a0a8df21092debb1a980a8cb48c7fcbf Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Fri, 17 Apr 2026 16:55:56 +0200 Subject: [PATCH 005/119] added ecm notebook in doc --- Battery/EquivalentCircuitModel/exampleECM.m | 10 +- .../notebooks/exampleECM.ipynb | 104 ++++++++++++++++++ .../notebooks/exampleECM.mlx | Bin 0 -> 22373 bytes Documentation/batteryphysics.rst | 8 +- Documentation/exampleECM.nblink | 3 + 5 files changed, 123 insertions(+), 2 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb create mode 100644 Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx create mode 100644 Documentation/exampleECM.nblink diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 0213ab512..73b5ab5c7 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -1,10 +1,18 @@ +%% Equivalent Circuit Model +% + +%% Load data set jsonstruct = parseBattmoJson('exampleECM.json'); inputparams = EquivalentCircuitModelInputParams(jsonstruct); + + +%% Setup model model = EquivalentCircuitModel(inputparams); +%% run Simulation [t, U, I] = model.solve(); -%% +%% Plotting tiledlayout(1, 2); nexttile diff --git a/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb b/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb new file mode 100644 index 000000000..6dafa2118 --- /dev/null +++ b/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb @@ -0,0 +1,104 @@ +{ + "cells": [ + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "# Equivalent Circuit Model\n", + "\n", + "## Load data set" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "jsonstruct = parseBattmoJson('exampleECM.json');\n", + "inputparams = EquivalentCircuitModelInputParams(jsonstruct);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "## Setup model" + ] + }, + { + "cell_type": "code", + "execution_count": 2, + "metadata": {}, + "source": [ + "model = EquivalentCircuitModel(inputparams);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "## run Simulation" + ] + }, + { + "cell_type": "code", + "execution_count": 3, + "metadata": {}, + "source": [ + "[t, U, I] = model.solve();" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "## Plotting" + ] + }, + { + "cell_type": "code", + "execution_count": 4, + "metadata": {}, + "source": [ + "tiledlayout(1, 2);\n", + "nexttile\n", + "plot(t, U)\n", + "nexttile\n", + "plot(t, I)" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
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z%-gmnOhb++wUl{^jO1x@gmP#RZKaol)Gp&{+LbIA4FV8>5|D2q6B=>yjm`+m# z^{#dN|6tU+Fi`G7`M=}8U{dcJ+-H9NQU0%i_1*1n1kn4!`)td` - + + .. grid-item-card:: + :padding: 2 + + :ref:`Equivalent Circuit Model ` + diff --git a/Documentation/exampleECM.nblink b/Documentation/exampleECM.nblink new file mode 100644 index 000000000..dafcad3e0 --- /dev/null +++ b/Documentation/exampleECM.nblink @@ -0,0 +1,3 @@ +{ + "path" : "../Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb" +} From 0d2c22daa48a40d5c74b7298372c7151d2a14e23 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 20 Apr 2026 11:08:32 +0200 Subject: [PATCH 006/119] little bug changes --- Battery/EquivalentCircuitModel/EquivalentCircuitModel.m | 7 +++++-- 1 file changed, 5 insertions(+), 2 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index 3a6821dab..31d328e13 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -102,13 +102,13 @@ end - function state = updatedU1dt(model, state) + function state = updatedU2dt(model, state) state.dU2dt = model.updatedUdt(state.U2, model.R2, model.C2, state.I); end - function state = updatedU2dt(model, state) + function state = updatedU1dt(model, state) state.dU1dt = model.updatedUdt(state.U1, model.R1, model.C1, state.I); @@ -192,6 +192,9 @@ % solve ode [t_out, y_out] = ode45(@(t, y) model.ode(t, y), tspan, y0); + + U = zeros(length(t_out), 1); + I = zeros(length(t_out), 1); %gagne du temps en allouant déjà la mémoire for i = 1:length(t_out) state = model.setupStateFromY(y_out(i, :)); From c2798645354914e7a4438e4a755dd295aeded7ea Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 20 Apr 2026 14:07:50 +0200 Subject: [PATCH 007/119] fixed capacity definition --- .../EquivalentCircuitModel.m | 8 ++-- .../EquivalentCircuitModel/exampleECM.json | 19 ++++----- Battery/EquivalentCircuitModel/exampleECM.m | 40 +++++++++++++------ 3 files changed, 43 insertions(+), 24 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index 31d328e13..bad1dc0df 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -118,7 +118,7 @@ Qmax = model.nominalcellcapacity; - state.dSOCdt = -(1 / Qmax) * state.I; + state.dSOCdt = -(1 / (Qmax*3600)) * state.I; end @@ -176,7 +176,7 @@ end - function [t, U, I] = solve(model) + function [t, U, I, SOC] = solve(model) if isempty(model.computationalGraph) model = setupComputationalGraph(model); @@ -192,7 +192,7 @@ % solve ode [t_out, y_out] = ode45(@(t, y) model.ode(t, y), tspan, y0); - + SOC = zeros(length(t_out), 1); U = zeros(length(t_out), 1); I = zeros(length(t_out), 1); %gagne du temps en allouant déjà la mémoire for i = 1:length(t_out) @@ -202,6 +202,8 @@ state.I = I(i); state = model.evalVarName(state, 'U'); U(i) = state.U; + state = model.evalVarName(state, 'SOC'); + SOC(i) = state.SOC; end t = t_out; diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json index 1b74e3a53..37717d39c 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.json +++ b/Battery/EquivalentCircuitModel/exampleECM.json @@ -1,23 +1,24 @@ -{ "nominalcellcapacity" : 63.7, +{ + "nominalcellcapacity" : 63.7, "OCP" : { "functionFormat" : "tabulated", "argumentList" : ["SOC"], "dataX" : [0.000000, 0.020000, 0.040000, 0.060000, 0.080000, 0.100000, 0.120000, 0.140000, 0.160000, 0.180000, 0.200000, 0.220000, 0.240000, 0.260000, 0.280000, 0.300000, 0.320000, 0.340000, 0.360000, 0.380000, 0.400000, 0.420000, 0.440000, 0.460000, 0.480000, 0.500000, 0.520000, 0.540000, 0.560000, 0.580000, 0.600000, 0.620000, 0.640000, 0.660000, 0.680000, 0.700000, 0.720000, 0.740000, 0.760000, 0.780000, 0.800000, 0.820000, 0.840000, 0.860000, 0.880000, 0.900000, 0.920000, 0.940000, 0.960000, 0.980000, 1.000000], - "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]}, - + "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000] + }, "R0" : 5e-3, "R1" : 5e-3, "C1" : 4e3, "R2" : 5e-3, "C2" : 1.44e5, - "initSOC" : 10, - "initOverpotential2" : 10, - "lowerVoltageCutoff" : 10, + "initSOC" : 1, + "initOverpotential2" : 0, + "lowerVoltageCutoff" : 1.0, "I" : { "functionFormat" : "tabulated", "argumentList" : ["time"], - "dataX" : [0, 500, 500.1, 1000, 1000.1, 1500], - "dataY" : [1, 1, 0, 0, -0.5, -0.5] + "dataX" : [0, 500, 500.1, 1000, 1000.1, 1500], + "dataY" : [30, 30, 0, 0, -15, -15] }, "totalTime" : 1500 -} +} \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 73b5ab5c7..34fc38036 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -1,21 +1,37 @@ -%% Equivalent Circuit Model -% +%% Equivalent Circuit Model Simulation -%% Load data set -jsonstruct = parseBattmoJson('exampleECM.json'); +% Load data set +jsonstruct = jsondecode(fileread('exampleECM.json')); inputparams = EquivalentCircuitModelInputParams(jsonstruct); - -%% Setup model +% Setup model model = EquivalentCircuitModel(inputparams); -%% run Simulation -[t, U, I] = model.solve(); +% Run Simulation +[t, U, I, SOC] = model.solve(); + -%% Plotting +% Plotting +figure; +tiledlayout(3, 1); -tiledlayout(1, 2); nexttile -plot(t, U) +plot(t, U, 'LineWidth', 2) +title('Tension de la Batterie') +xlabel('Temps (s)') +ylabel('Tension (V)') +grid on + +nexttile +plot(t, I, 'LineWidth', 2, 'Color', 'r') +title('Courant Appliqué') +xlabel('Temps (s)') +ylabel('Courant (A)') +grid on + nexttile -plot(t, I) +plot(t, SOC, 'LineWidth', 2, 'Color', 'g') +title('SOC') +xlabel('Temps (s)') +ylabel('SOC') +grid on \ No newline at end of file From be32715f4d1be986b6f1d4c98653395a14b8b5a8 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 20 Apr 2026 14:42:01 +0200 Subject: [PATCH 008/119] Translation --- .../EquivalentCircuitModel.m | 1 - Battery/EquivalentCircuitModel/exampleECM.m | 14 +++++++------- 2 files changed, 7 insertions(+), 8 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index bad1dc0df..bb274ef0c 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -10,7 +10,6 @@ C1 R2 C2 - initSOC initOverpotential2 lowerVoltageCutoff diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 34fc38036..6fcc97046 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -17,21 +17,21 @@ nexttile plot(t, U, 'LineWidth', 2) -title('Tension de la Batterie') -xlabel('Temps (s)') -ylabel('Tension (V)') +title('Battery Voltage') +xlabel('Time /s') +ylabel('Voltage /V') grid on nexttile plot(t, I, 'LineWidth', 2, 'Color', 'r') -title('Courant Appliqué') -xlabel('Temps (s)') -ylabel('Courant (A)') +title('Applied Current') +xlabel('Time /s') +ylabel('Current /A') grid on nexttile plot(t, SOC, 'LineWidth', 2, 'Color', 'g') title('SOC') -xlabel('Temps (s)') +xlabel('Time /s') ylabel('SOC') grid on \ No newline at end of file From 7f99366a3e1c69f27d637e4e2622522f32e9fd28 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 20 Apr 2026 16:22:46 +0200 Subject: [PATCH 009/119] changed parameters in vectors --- .../EquivalentCircuitModel.m | 16 +++++++++--- .../EquivalentCircuitModel/exampleECM.json | 13 ++++------ Battery/EquivalentCircuitModel/exampleECM.m | 25 ++++++++++++++++++- 3 files changed, 42 insertions(+), 12 deletions(-) diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index bb274ef0c..ff38ffcc0 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -20,6 +20,11 @@ %% helpers OCPfunc Ifunc + R0func + R1func + C1func + R2func + C2func end methods @@ -47,6 +52,11 @@ model.OCPfunc = setupFunction(model.OCP); model.Ifunc = setupFunction(model.I); + model.R0func = setupFunction(model.R0); + model.R1func = setupFunction(model.R1); + model.C1func = setupFunction(model.C1); + model.R2func = setupFunction(model.R2); + model.C2func = setupFunction(model.C2); end @@ -97,19 +107,19 @@ function state = updateUR(model, state) - state.UR = model.R0*state.I; + state.UR = model.R0func(state.SOC)*state.I; end function state = updatedU2dt(model, state) - state.dU2dt = model.updatedUdt(state.U2, model.R2, model.C2, state.I); + state.dU2dt = model.updatedUdt(state.U2, model.R2func(state.SOC), model.C2func(state.SOC), state.I); end function state = updatedU1dt(model, state) - state.dU1dt = model.updatedUdt(state.U1, model.R1, model.C1, state.I); + state.dU1dt = model.updatedUdt(state.U1, model.R1func(state.SOC), model.C1func(state.SOC), state.I); end diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json index 37717d39c..c569583b6 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.json +++ b/Battery/EquivalentCircuitModel/exampleECM.json @@ -1,4 +1,5 @@ { + "nominalcellcapacity" : 63.7, "OCP" : { "functionFormat" : "tabulated", @@ -6,19 +7,15 @@ "dataX" : [0.000000, 0.020000, 0.040000, 0.060000, 0.080000, 0.100000, 0.120000, 0.140000, 0.160000, 0.180000, 0.200000, 0.220000, 0.240000, 0.260000, 0.280000, 0.300000, 0.320000, 0.340000, 0.360000, 0.380000, 0.400000, 0.420000, 0.440000, 0.460000, 0.480000, 0.500000, 0.520000, 0.540000, 0.560000, 0.580000, 0.600000, 0.620000, 0.640000, 0.660000, 0.680000, 0.700000, 0.720000, 0.740000, 0.760000, 0.780000, 0.800000, 0.820000, 0.840000, 0.860000, 0.880000, 0.900000, 0.920000, 0.940000, 0.960000, 0.980000, 1.000000], "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000] }, - "R0" : 5e-3, - "R1" : 5e-3, - "C1" : 4e3, - "R2" : 5e-3, - "C2" : 1.44e5, + "initSOC" : 1, "initOverpotential2" : 0, "lowerVoltageCutoff" : 1.0, "I" : { "functionFormat" : "tabulated", "argumentList" : ["time"], - "dataX" : [0, 500, 500.1, 1000, 1000.1, 1500], - "dataY" : [30, 30, 0, 0, -15, -15] + "dataX" : [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200], + "dataY" : [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0] }, - "totalTime" : 1500 + "totalTime" : 4200 } \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index 6fcc97046..dafe84224 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -2,8 +2,31 @@ % Load data set jsonstruct = jsondecode(fileread('exampleECM.json')); + +R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; +R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; +tau1_tot=[4.9,11,12,17,15;4.9,11,12,18,17;4.9,13,14,17,18;4.9,13,20,16,19;4.9,12,17,16,18;3.7,13,16,14,15;3.2,14,17,15,14;3.2,16,18,15,15;4.3,16,17,15,15;5.9,16,17,15,13;8.8,17,17,15,15;14,18,17,16,15;18,20,18,16,14;21,23,22,18,16;23,24,24,19,17;23,26,25,20,16;23,26,24,23,21;22,26,23,23,23;22,24,22,24,22;21,23,21,22,20;19,23,20,21,19;19,23,20,20,17;18,23,19,19,16;17,23,19,18,15;16,23,19,18,15;15,24,19,17,14;15,25,20,17,14;17,26,20,18,15;17,27,22,18,14;20,27,24,20,16;25,29,25,26,21;23,27,22,22,23;21,22,20,27,24;21,21,21,24,21;21,23,25,22,18;22,26,26,20,18;24,28,23,21,18;27,27,21,20,18;31,25,21,21,17;31,24,20,21,18;29,23,19,21,17;26,23,20,20,18;24,23,20,21,19;22,23,20,20,19;21,23,20,22,19;19,23,21,23,17;19,24,21,21,18;18,24,20,20,18;17,24,21,23,19;17,23,15,22,19;17,23,14,15,17]; +R2_tot = [0.00465917,0.00296137,0.00671937,0.00670953,0.00638318;0.00465917,0.00296137,0.0049358,0.00369832,0.00345545;0.00465917,0.00360752,0.00337953,0.00232382,0.00217768;0.00465917,0.00385934,0.00299688,0.00165026,0.00141804;0.00465917,0.00279048,0.00167985,0.000868944,0.00062913;0.00344996,0.00198995,0.00127818,0.000602667,0.000490827;0.00243925,0.00173739,0.00100247,0.000502448,0.000400199;0.00195174,0.0016195,0.00117991,0.000653807,0.000522623;0.00196127,0.00143448,0.00090563,0.000593035,0.000515238;0.00210982,0.0013075,0.000808184,0.000489967,0.000453458;0.00266036,0.00121596,0.000742684,0.000416342,0.000378914;0.00344871,0.00125469,0.00074347,0.000401257,0.000350742;0.00389231,0.00126885,0.000696434,0.000379638,0.000337394;0.00392122,0.00188842,0.00105021,0.000512664,0.000344475;0.00377053,0.00200223,0.00129526,0.00051701,0.000287237;0.00349905,0.00192787,0.00134563,0.000629481,0.000378992;0.00314826,0.00181955,0.00130909,0.000850741,0.000526779;0.00285045,0.00175597,0.00125321,0.000856617,0.000718745;0.00255589,0.00161788,0.00119344,0.000887228,0.000640541;0.00227795,0.00154717,0.00113057,0.000748643,0.000532106;0.00204687,0.00150239,0.00108992,0.000741976,0.00046544;0.00179717,0.00147648,0.00104268,0.000650899,0.000408277;0.00166159,0.00146907,0.00104974,0.000648536,0.000425937;0.00154212,0.0014479,0.00100709,0.000584535,0.000365088;0.00142178,0.00147631,0.000971539,0.000574467,0.000359385;0.00138252,0.00149249,0.000966175,0.000567393,0.00034615;0.00135213,0.00150963,0.000946023,0.000509391,0.00032513;0.00161978,0.00157701,0.000973037,0.000512528,0.000321927;0.0018797,0.00176393,0.00107455,0.000552517,0.000360338;0.00233758,0.00204923,0.00128005,0.000575555,0.000345665;0.00303428,0.00251452,0.00155042,0.00101129,0.000740204;0.00397936,0.0023618,0.00194514,0.00167676,0.00124506;0.00494525,0.00268869,0.00239193,0.00146285,0.000987005;0.00575857,0.00294003,0.00244425,0.0011978,0.000867504;0.00596764,0.00278034,0.00213064,0.00106735,0.000733011;0.00569216,0.00241023,0.00177033,0.00095135,0.00066496;0.00494613,0.00199842,0.00153419,0.000885069,0.000648523;0.00403546,0.00176577,0.00135467,0.000898499,0.000675215;0.00326917,0.00161032,0.00130149,0.000889941,0.000633382;0.00274124,0.00153081,0.001227,0.000919164,0.000697074;0.00244927,0.00150333,0.0012413,0.000897664,0.000705495;0.00220336,0.00150596,0.00124922,0.000957534,0.000664272;0.00199516,0.00153147,0.00127479,0.000917949,0.0007466;0.00184088,0.0015754,0.00130798,0.000984517,0.000675919;0.00173782,0.00161791,0.00131662,0.000949267,0.000741;0.0017013,0.00158804,0.00133677,0.000999377,0.000704756;0.00162086,0.00170525,0.00138481,0.000946432,0.000736538;0.00152086,0.00166043,0.00128942,0.00097447,0.000683679;0.00150632,0.00176676,0.00137887,0.00096943,0.000718854;0.00128553,0.00167337,0.0016092,0.000944572,0.000726751;0.00128553,0.00167337,0.00170989,0.00124241,0.000828314]; +tau2_tot = [95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,4.4e+02,7.2e+02,7.2e+02,7.2e+02;95,5.3e+02,7e+02,6.9e+02,7.2e+02;95,5.3e+02,6.4e+02,5.8e+02,6.9e+02;1.2e+02,5.4e+02,5.8e+02,4.5e+02,5.5e+02;1.8e+02,5.8e+02,5.8e+02,4.4e+02,5.4e+02;2.5e+02,6.2e+02,6.2e+02,5.6e+02,6e+02;3.7e+02,6e+02,5.7e+02,5.6e+02,6.2e+02;5.3e+02,5.6e+02,5.1e+02,5e+02,6.4e+02;6.7e+02,5.6e+02,4.8e+02,4.3e+02,6e+02;7.2e+02,5.9e+02,4.6e+02,3.8e+02,5.7e+02;7.2e+02,6.4e+02,4.9e+02,3.7e+02,5.2e+02;7.2e+02,6.9e+02,6.4e+02,4.6e+02,4.3e+02;7.2e+02,7.2e+02,6.9e+02,5e+02,3.9e+02;7.2e+02,7e+02,7e+02,6.4e+02,5.5e+02;7.2e+02,7e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.1e+02,7e+02,6.9e+02,7.1e+02;7.2e+02,7e+02,7e+02,7e+02,6.8e+02;7.1e+02,7e+02,6.9e+02,6.5e+02,6e+02;6.8e+02,7.1e+02,6.8e+02,6.4e+02,5e+02;6.3e+02,7.1e+02,6.6e+02,6.1e+02,4.8e+02;6e+02,7e+02,6.6e+02,5.6e+02,5e+02;5.6e+02,6.9e+02,6.4e+02,5.3e+02,4.3e+02;5.3e+02,6.9e+02,6.1e+02,5.4e+02,4.2e+02;5.2e+02,6.8e+02,6e+02,5.2e+02,4.1e+02;5.7e+02,6.7e+02,5.9e+02,4.6e+02,3.9e+02;7e+02,6.9e+02,6e+02,4.9e+02,4.1e+02;7.2e+02,7.1e+02,6.3e+02,5e+02,4.2e+02;7.2e+02,7.2e+02,6.6e+02,5.9e+02,5.5e+02;7.2e+02,7.2e+02,7e+02,6.3e+02,6.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,7e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,6.5e+02;7.2e+02,7.2e+02,7.2e+02,6.9e+02,6.1e+02;7.2e+02,7.2e+02,7.1e+02,6.8e+02,6.3e+02;7.2e+02,7e+02,6.8e+02,6.9e+02,6.6e+02;7e+02,6.7e+02,6.8e+02,7e+02,6.4e+02;6.6e+02,6.5e+02,6.7e+02,7.2e+02,7.1e+02;6e+02,6.4e+02,6.7e+02,7.2e+02,6.9e+02;5.6e+02,6.5e+02,6.7e+02,7.2e+02,6.9e+02;5.4e+02,6.6e+02,6.8e+02,7.2e+02,7.2e+02;5.3e+02,6.7e+02,7e+02,7.2e+02,6.5e+02;5.4e+02,6.7e+02,7e+02,7.2e+02,7.1e+02;5.5e+02,6.5e+02,7.1e+02,7.2e+02,6.4e+02;5.3e+02,6.7e+02,7e+02,6.9e+02,6.8e+02;5.2e+02,6.4e+02,6.3e+02,6.8e+02,5.9e+02;4.9e+02,6.2e+02,6.5e+02,6.7e+02,5.8e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02]; + +R0 = R0_tot(:,3); +R1 = R1_tot(:,3); +tau1 = tau1_tot(:,3); +R2 = R2_tot(:,3); +tau2 = tau2_tot(:,3); +C1 = tau1 ./ R1; +C2 = tau2 ./ R2; + +axe_SOC = jsonstruct.OCP.dataX; inputparams = EquivalentCircuitModelInputParams(jsonstruct); +inputparams.R0 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R0); +inputparams.R1 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R1); +inputparams.C1 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', C1); +inputparams.R2 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R2); +inputparams.C2 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', C2); + + % Setup model model = EquivalentCircuitModel(inputparams); @@ -12,7 +35,7 @@ % Plotting -figure; +figure(Name='Highlighting the difference in resistance depending on the state of charge'); tiledlayout(3, 1); nexttile From c06f07afbbf73d10cf162582aebc5fdf6831a92c Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 20 Apr 2026 16:58:31 +0200 Subject: [PATCH 010/119] new funtion create_parameters instead of json file to allow calculs --- .../create_parameters.m | 59 +++++++++++++++++++ .../EquivalentCircuitModel/exampleECM.json | 21 ------- Battery/EquivalentCircuitModel/exampleECM.m | 26 +------- 3 files changed, 61 insertions(+), 45 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/create_parameters.m delete mode 100644 Battery/EquivalentCircuitModel/exampleECM.json diff --git a/Battery/EquivalentCircuitModel/create_parameters.m b/Battery/EquivalentCircuitModel/create_parameters.m new file mode 100644 index 000000000..8fa694884 --- /dev/null +++ b/Battery/EquivalentCircuitModel/create_parameters.m @@ -0,0 +1,59 @@ +function p = create_parameters() + + p.nominalcellcapacity = 63.7; + p.initSOC = 1.0; + p.lowerVoltageCutoff = 3.0; + p.initOverpotential2 = 0; + p.totalTime = 4200; + + p.I.functionFormat = 'tabulated'; + p.I.argumentList = {'time'}; + p.I.dataX = [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200]; + p.I.dataY = [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0]; + + p.OCP.functionFormat = 'tabulated'; + p.OCP.argumentList = {'SOC'}; + p.OCP.dataX = [0.00, 0.02, 0.04, 0.06, 0.08, 0.10, 0.12, 0.14, 0.16, 0.18, 0.20, 0.22, 0.24, 0.26, 0.28, 0.30, 0.32, 0.34, 0.36, 0.38, 0.40, 0.42, 0.44, 0.46, 0.48, 0.50, 0.52, 0.54, 0.56, 0.58, 0.60, 0.62, 0.64, 0.66, 0.68, 0.70, 0.72, 0.74, 0.76, 0.78, 0.80, 0.82, 0.84, 0.86, 0.88, 0.90, 0.92, 0.94, 0.96, 0.98, 1.00]; + p.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000] + + R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; + R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; + tau1_tot=[4.9,11,12,17,15;4.9,11,12,18,17;4.9,13,14,17,18;4.9,13,20,16,19;4.9,12,17,16,18;3.7,13,16,14,15;3.2,14,17,15,14;3.2,16,18,15,15;4.3,16,17,15,15;5.9,16,17,15,13;8.8,17,17,15,15;14,18,17,16,15;18,20,18,16,14;21,23,22,18,16;23,24,24,19,17;23,26,25,20,16;23,26,24,23,21;22,26,23,23,23;22,24,22,24,22;21,23,21,22,20;19,23,20,21,19;19,23,20,20,17;18,23,19,19,16;17,23,19,18,15;16,23,19,18,15;15,24,19,17,14;15,25,20,17,14;17,26,20,18,15;17,27,22,18,14;20,27,24,20,16;25,29,25,26,21;23,27,22,22,23;21,22,20,27,24;21,21,21,24,21;21,23,25,22,18;22,26,26,20,18;24,28,23,21,18;27,27,21,20,18;31,25,21,21,17;31,24,20,21,18;29,23,19,21,17;26,23,20,20,18;24,23,20,21,19;22,23,20,20,19;21,23,20,22,19;19,23,21,23,17;19,24,21,21,18;18,24,20,20,18;17,24,21,23,19;17,23,15,22,19;17,23,14,15,17]; + R2_tot = [0.00465917,0.00296137,0.00671937,0.00670953,0.00638318;0.00465917,0.00296137,0.0049358,0.00369832,0.00345545;0.00465917,0.00360752,0.00337953,0.00232382,0.00217768;0.00465917,0.00385934,0.00299688,0.00165026,0.00141804;0.00465917,0.00279048,0.00167985,0.000868944,0.00062913;0.00344996,0.00198995,0.00127818,0.000602667,0.000490827;0.00243925,0.00173739,0.00100247,0.000502448,0.000400199;0.00195174,0.0016195,0.00117991,0.000653807,0.000522623;0.00196127,0.00143448,0.00090563,0.000593035,0.000515238;0.00210982,0.0013075,0.000808184,0.000489967,0.000453458;0.00266036,0.00121596,0.000742684,0.000416342,0.000378914;0.00344871,0.00125469,0.00074347,0.000401257,0.000350742;0.00389231,0.00126885,0.000696434,0.000379638,0.000337394;0.00392122,0.00188842,0.00105021,0.000512664,0.000344475;0.00377053,0.00200223,0.00129526,0.00051701,0.000287237;0.00349905,0.00192787,0.00134563,0.000629481,0.000378992;0.00314826,0.00181955,0.00130909,0.000850741,0.000526779;0.00285045,0.00175597,0.00125321,0.000856617,0.000718745;0.00255589,0.00161788,0.00119344,0.000887228,0.000640541;0.00227795,0.00154717,0.00113057,0.000748643,0.000532106;0.00204687,0.00150239,0.00108992,0.000741976,0.00046544;0.00179717,0.00147648,0.00104268,0.000650899,0.000408277;0.00166159,0.00146907,0.00104974,0.000648536,0.000425937;0.00154212,0.0014479,0.00100709,0.000584535,0.000365088;0.00142178,0.00147631,0.000971539,0.000574467,0.000359385;0.00138252,0.00149249,0.000966175,0.000567393,0.00034615;0.00135213,0.00150963,0.000946023,0.000509391,0.00032513;0.00161978,0.00157701,0.000973037,0.000512528,0.000321927;0.0018797,0.00176393,0.00107455,0.000552517,0.000360338;0.00233758,0.00204923,0.00128005,0.000575555,0.000345665;0.00303428,0.00251452,0.00155042,0.00101129,0.000740204;0.00397936,0.0023618,0.00194514,0.00167676,0.00124506;0.00494525,0.00268869,0.00239193,0.00146285,0.000987005;0.00575857,0.00294003,0.00244425,0.0011978,0.000867504;0.00596764,0.00278034,0.00213064,0.00106735,0.000733011;0.00569216,0.00241023,0.00177033,0.00095135,0.00066496;0.00494613,0.00199842,0.00153419,0.000885069,0.000648523;0.00403546,0.00176577,0.00135467,0.000898499,0.000675215;0.00326917,0.00161032,0.00130149,0.000889941,0.000633382;0.00274124,0.00153081,0.001227,0.000919164,0.000697074;0.00244927,0.00150333,0.0012413,0.000897664,0.000705495;0.00220336,0.00150596,0.00124922,0.000957534,0.000664272;0.00199516,0.00153147,0.00127479,0.000917949,0.0007466;0.00184088,0.0015754,0.00130798,0.000984517,0.000675919;0.00173782,0.00161791,0.00131662,0.000949267,0.000741;0.0017013,0.00158804,0.00133677,0.000999377,0.000704756;0.00162086,0.00170525,0.00138481,0.000946432,0.000736538;0.00152086,0.00166043,0.00128942,0.00097447,0.000683679;0.00150632,0.00176676,0.00137887,0.00096943,0.000718854;0.00128553,0.00167337,0.0016092,0.000944572,0.000726751;0.00128553,0.00167337,0.00170989,0.00124241,0.000828314]; + tau2_tot = [95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,4.4e+02,7.2e+02,7.2e+02,7.2e+02;95,5.3e+02,7e+02,6.9e+02,7.2e+02;95,5.3e+02,6.4e+02,5.8e+02,6.9e+02;1.2e+02,5.4e+02,5.8e+02,4.5e+02,5.5e+02;1.8e+02,5.8e+02,5.8e+02,4.4e+02,5.4e+02;2.5e+02,6.2e+02,6.2e+02,5.6e+02,6e+02;3.7e+02,6e+02,5.7e+02,5.6e+02,6.2e+02;5.3e+02,5.6e+02,5.1e+02,5e+02,6.4e+02;6.7e+02,5.6e+02,4.8e+02,4.3e+02,6e+02;7.2e+02,5.9e+02,4.6e+02,3.8e+02,5.7e+02;7.2e+02,6.4e+02,4.9e+02,3.7e+02,5.2e+02;7.2e+02,6.9e+02,6.4e+02,4.6e+02,4.3e+02;7.2e+02,7.2e+02,6.9e+02,5e+02,3.9e+02;7.2e+02,7e+02,7e+02,6.4e+02,5.5e+02;7.2e+02,7e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.1e+02,7e+02,6.9e+02,7.1e+02;7.2e+02,7e+02,7e+02,7e+02,6.8e+02;7.1e+02,7e+02,6.9e+02,6.5e+02,6e+02;6.8e+02,7.1e+02,6.8e+02,6.4e+02,5e+02;6.3e+02,7.1e+02,6.6e+02,6.1e+02,4.8e+02;6e+02,7e+02,6.6e+02,5.6e+02,5e+02;5.6e+02,6.9e+02,6.4e+02,5.3e+02,4.3e+02;5.3e+02,6.9e+02,6.1e+02,5.4e+02,4.2e+02;5.2e+02,6.8e+02,6e+02,5.2e+02,4.1e+02;5.7e+02,6.7e+02,5.9e+02,4.6e+02,3.9e+02;7e+02,6.9e+02,6e+02,4.9e+02,4.1e+02;7.2e+02,7.1e+02,6.3e+02,5e+02,4.2e+02;7.2e+02,7.2e+02,6.6e+02,5.9e+02,5.5e+02;7.2e+02,7.2e+02,7e+02,6.3e+02,6.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,7e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,6.5e+02;7.2e+02,7.2e+02,7.2e+02,6.9e+02,6.1e+02;7.2e+02,7.2e+02,7.1e+02,6.8e+02,6.3e+02;7.2e+02,7e+02,6.8e+02,6.9e+02,6.6e+02;7e+02,6.7e+02,6.8e+02,7e+02,6.4e+02;6.6e+02,6.5e+02,6.7e+02,7.2e+02,7.1e+02;6e+02,6.4e+02,6.7e+02,7.2e+02,6.9e+02;5.6e+02,6.5e+02,6.7e+02,7.2e+02,6.9e+02;5.4e+02,6.6e+02,6.8e+02,7.2e+02,7.2e+02;5.3e+02,6.7e+02,7e+02,7.2e+02,6.5e+02;5.4e+02,6.7e+02,7e+02,7.2e+02,7.1e+02;5.5e+02,6.5e+02,7.1e+02,7.2e+02,6.4e+02;5.3e+02,6.7e+02,7e+02,6.9e+02,6.8e+02;5.2e+02,6.4e+02,6.3e+02,6.8e+02,5.9e+02;4.9e+02,6.2e+02,6.5e+02,6.7e+02,5.8e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02]; + + R0 = R0_tot(:,3)'; + R1 = R1_tot(:,3)'; + tau1 = tau1_tot(:,3)'; + R2 = R2_tot(:,3)'; + tau2 = tau2_tot(:,3)'; + C1 = tau1 ./ R1; + C2 = tau2 ./ R2; + + + p.R0.functionFormat = 'tabulated'; + p.R0.argumentList = {'SOC'}; + p.R0.dataX = p.OCP.dataX; % same axis as SOC + p.R0.dataY = R0; + + p.R1.functionFormat = 'tabulated'; + p.R1.argumentList = {'SOC'}; + p.R1.dataX = p.OCP.dataX; + p.R1.dataY = R1; + + p.C1.functionFormat = 'tabulated'; + p.C1.argumentList = {'SOC'}; + p.C1.dataX = p.OCP.dataX; + p.C1.dataY = C1; + + p.R2.functionFormat = 'tabulated'; + p.R2.argumentList = {'SOC'}; + p.R2.dataX = p.OCP.dataX; + p.R2.dataY = R2; + + p.C2.functionFormat = 'tabulated'; + p.C2.argumentList = {'SOC'}; + p.C2.dataX = p.OCP.dataX; + p.C2.dataY = C2; + +end diff --git a/Battery/EquivalentCircuitModel/exampleECM.json b/Battery/EquivalentCircuitModel/exampleECM.json deleted file mode 100644 index c569583b6..000000000 --- a/Battery/EquivalentCircuitModel/exampleECM.json +++ /dev/null @@ -1,21 +0,0 @@ -{ - - "nominalcellcapacity" : 63.7, - "OCP" : { - "functionFormat" : "tabulated", - "argumentList" : ["SOC"], - "dataX" : [0.000000, 0.020000, 0.040000, 0.060000, 0.080000, 0.100000, 0.120000, 0.140000, 0.160000, 0.180000, 0.200000, 0.220000, 0.240000, 0.260000, 0.280000, 0.300000, 0.320000, 0.340000, 0.360000, 0.380000, 0.400000, 0.420000, 0.440000, 0.460000, 0.480000, 0.500000, 0.520000, 0.540000, 0.560000, 0.580000, 0.600000, 0.620000, 0.640000, 0.660000, 0.680000, 0.700000, 0.720000, 0.740000, 0.760000, 0.780000, 0.800000, 0.820000, 0.840000, 0.860000, 0.880000, 0.900000, 0.920000, 0.940000, 0.960000, 0.980000, 1.000000], - "dataY" : [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000] - }, - - "initSOC" : 1, - "initOverpotential2" : 0, - "lowerVoltageCutoff" : 1.0, - "I" : { - "functionFormat" : "tabulated", - "argumentList" : ["time"], - "dataX" : [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200], - "dataY" : [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0] - }, - "totalTime" : 4200 -} \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/exampleECM.m index dafe84224..31a5d82f8 100644 --- a/Battery/EquivalentCircuitModel/exampleECM.m +++ b/Battery/EquivalentCircuitModel/exampleECM.m @@ -1,31 +1,9 @@ %% Equivalent Circuit Model Simulation % Load data set -jsonstruct = jsondecode(fileread('exampleECM.json')); - -R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; -R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; -tau1_tot=[4.9,11,12,17,15;4.9,11,12,18,17;4.9,13,14,17,18;4.9,13,20,16,19;4.9,12,17,16,18;3.7,13,16,14,15;3.2,14,17,15,14;3.2,16,18,15,15;4.3,16,17,15,15;5.9,16,17,15,13;8.8,17,17,15,15;14,18,17,16,15;18,20,18,16,14;21,23,22,18,16;23,24,24,19,17;23,26,25,20,16;23,26,24,23,21;22,26,23,23,23;22,24,22,24,22;21,23,21,22,20;19,23,20,21,19;19,23,20,20,17;18,23,19,19,16;17,23,19,18,15;16,23,19,18,15;15,24,19,17,14;15,25,20,17,14;17,26,20,18,15;17,27,22,18,14;20,27,24,20,16;25,29,25,26,21;23,27,22,22,23;21,22,20,27,24;21,21,21,24,21;21,23,25,22,18;22,26,26,20,18;24,28,23,21,18;27,27,21,20,18;31,25,21,21,17;31,24,20,21,18;29,23,19,21,17;26,23,20,20,18;24,23,20,21,19;22,23,20,20,19;21,23,20,22,19;19,23,21,23,17;19,24,21,21,18;18,24,20,20,18;17,24,21,23,19;17,23,15,22,19;17,23,14,15,17]; -R2_tot = [0.00465917,0.00296137,0.00671937,0.00670953,0.00638318;0.00465917,0.00296137,0.0049358,0.00369832,0.00345545;0.00465917,0.00360752,0.00337953,0.00232382,0.00217768;0.00465917,0.00385934,0.00299688,0.00165026,0.00141804;0.00465917,0.00279048,0.00167985,0.000868944,0.00062913;0.00344996,0.00198995,0.00127818,0.000602667,0.000490827;0.00243925,0.00173739,0.00100247,0.000502448,0.000400199;0.00195174,0.0016195,0.00117991,0.000653807,0.000522623;0.00196127,0.00143448,0.00090563,0.000593035,0.000515238;0.00210982,0.0013075,0.000808184,0.000489967,0.000453458;0.00266036,0.00121596,0.000742684,0.000416342,0.000378914;0.00344871,0.00125469,0.00074347,0.000401257,0.000350742;0.00389231,0.00126885,0.000696434,0.000379638,0.000337394;0.00392122,0.00188842,0.00105021,0.000512664,0.000344475;0.00377053,0.00200223,0.00129526,0.00051701,0.000287237;0.00349905,0.00192787,0.00134563,0.000629481,0.000378992;0.00314826,0.00181955,0.00130909,0.000850741,0.000526779;0.00285045,0.00175597,0.00125321,0.000856617,0.000718745;0.00255589,0.00161788,0.00119344,0.000887228,0.000640541;0.00227795,0.00154717,0.00113057,0.000748643,0.000532106;0.00204687,0.00150239,0.00108992,0.000741976,0.00046544;0.00179717,0.00147648,0.00104268,0.000650899,0.000408277;0.00166159,0.00146907,0.00104974,0.000648536,0.000425937;0.00154212,0.0014479,0.00100709,0.000584535,0.000365088;0.00142178,0.00147631,0.000971539,0.000574467,0.000359385;0.00138252,0.00149249,0.000966175,0.000567393,0.00034615;0.00135213,0.00150963,0.000946023,0.000509391,0.00032513;0.00161978,0.00157701,0.000973037,0.000512528,0.000321927;0.0018797,0.00176393,0.00107455,0.000552517,0.000360338;0.00233758,0.00204923,0.00128005,0.000575555,0.000345665;0.00303428,0.00251452,0.00155042,0.00101129,0.000740204;0.00397936,0.0023618,0.00194514,0.00167676,0.00124506;0.00494525,0.00268869,0.00239193,0.00146285,0.000987005;0.00575857,0.00294003,0.00244425,0.0011978,0.000867504;0.00596764,0.00278034,0.00213064,0.00106735,0.000733011;0.00569216,0.00241023,0.00177033,0.00095135,0.00066496;0.00494613,0.00199842,0.00153419,0.000885069,0.000648523;0.00403546,0.00176577,0.00135467,0.000898499,0.000675215;0.00326917,0.00161032,0.00130149,0.000889941,0.000633382;0.00274124,0.00153081,0.001227,0.000919164,0.000697074;0.00244927,0.00150333,0.0012413,0.000897664,0.000705495;0.00220336,0.00150596,0.00124922,0.000957534,0.000664272;0.00199516,0.00153147,0.00127479,0.000917949,0.0007466;0.00184088,0.0015754,0.00130798,0.000984517,0.000675919;0.00173782,0.00161791,0.00131662,0.000949267,0.000741;0.0017013,0.00158804,0.00133677,0.000999377,0.000704756;0.00162086,0.00170525,0.00138481,0.000946432,0.000736538;0.00152086,0.00166043,0.00128942,0.00097447,0.000683679;0.00150632,0.00176676,0.00137887,0.00096943,0.000718854;0.00128553,0.00167337,0.0016092,0.000944572,0.000726751;0.00128553,0.00167337,0.00170989,0.00124241,0.000828314]; -tau2_tot = [95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,4.4e+02,7.2e+02,7.2e+02,7.2e+02;95,5.3e+02,7e+02,6.9e+02,7.2e+02;95,5.3e+02,6.4e+02,5.8e+02,6.9e+02;1.2e+02,5.4e+02,5.8e+02,4.5e+02,5.5e+02;1.8e+02,5.8e+02,5.8e+02,4.4e+02,5.4e+02;2.5e+02,6.2e+02,6.2e+02,5.6e+02,6e+02;3.7e+02,6e+02,5.7e+02,5.6e+02,6.2e+02;5.3e+02,5.6e+02,5.1e+02,5e+02,6.4e+02;6.7e+02,5.6e+02,4.8e+02,4.3e+02,6e+02;7.2e+02,5.9e+02,4.6e+02,3.8e+02,5.7e+02;7.2e+02,6.4e+02,4.9e+02,3.7e+02,5.2e+02;7.2e+02,6.9e+02,6.4e+02,4.6e+02,4.3e+02;7.2e+02,7.2e+02,6.9e+02,5e+02,3.9e+02;7.2e+02,7e+02,7e+02,6.4e+02,5.5e+02;7.2e+02,7e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.1e+02,7e+02,6.9e+02,7.1e+02;7.2e+02,7e+02,7e+02,7e+02,6.8e+02;7.1e+02,7e+02,6.9e+02,6.5e+02,6e+02;6.8e+02,7.1e+02,6.8e+02,6.4e+02,5e+02;6.3e+02,7.1e+02,6.6e+02,6.1e+02,4.8e+02;6e+02,7e+02,6.6e+02,5.6e+02,5e+02;5.6e+02,6.9e+02,6.4e+02,5.3e+02,4.3e+02;5.3e+02,6.9e+02,6.1e+02,5.4e+02,4.2e+02;5.2e+02,6.8e+02,6e+02,5.2e+02,4.1e+02;5.7e+02,6.7e+02,5.9e+02,4.6e+02,3.9e+02;7e+02,6.9e+02,6e+02,4.9e+02,4.1e+02;7.2e+02,7.1e+02,6.3e+02,5e+02,4.2e+02;7.2e+02,7.2e+02,6.6e+02,5.9e+02,5.5e+02;7.2e+02,7.2e+02,7e+02,6.3e+02,6.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,7e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,6.5e+02;7.2e+02,7.2e+02,7.2e+02,6.9e+02,6.1e+02;7.2e+02,7.2e+02,7.1e+02,6.8e+02,6.3e+02;7.2e+02,7e+02,6.8e+02,6.9e+02,6.6e+02;7e+02,6.7e+02,6.8e+02,7e+02,6.4e+02;6.6e+02,6.5e+02,6.7e+02,7.2e+02,7.1e+02;6e+02,6.4e+02,6.7e+02,7.2e+02,6.9e+02;5.6e+02,6.5e+02,6.7e+02,7.2e+02,6.9e+02;5.4e+02,6.6e+02,6.8e+02,7.2e+02,7.2e+02;5.3e+02,6.7e+02,7e+02,7.2e+02,6.5e+02;5.4e+02,6.7e+02,7e+02,7.2e+02,7.1e+02;5.5e+02,6.5e+02,7.1e+02,7.2e+02,6.4e+02;5.3e+02,6.7e+02,7e+02,6.9e+02,6.8e+02;5.2e+02,6.4e+02,6.3e+02,6.8e+02,5.9e+02;4.9e+02,6.2e+02,6.5e+02,6.7e+02,5.8e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02]; - -R0 = R0_tot(:,3); -R1 = R1_tot(:,3); -tau1 = tau1_tot(:,3); -R2 = R2_tot(:,3); -tau2 = tau2_tot(:,3); -C1 = tau1 ./ R1; -C2 = tau2 ./ R2; - -axe_SOC = jsonstruct.OCP.dataX; -inputparams = EquivalentCircuitModelInputParams(jsonstruct); - -inputparams.R0 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R0); -inputparams.R1 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R1); -inputparams.C1 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', C1); -inputparams.R2 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', R2); -inputparams.C2 = struct('functionFormat', 'tabulated', 'argumentList', {{'SOC'}}, 'dataX', axe_SOC, 'dataY', C2); +params = create_parameters(); +inputparams = EquivalentCircuitModelInputParams(params); % Setup model model = EquivalentCircuitModel(inputparams); From b69906b9ceda42ce547c3fbb5a949bf3f58edf17 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 29 Apr 2026 10:59:25 +0200 Subject: [PATCH 011/119] push of EIS --- .../EquivalentCircuitModel.m | 2 +- .../EquivalentCircuitModel/cost_function.m | 29 +++++++ .../EquivalentCircuitModel/plotexperience.m | 76 +++++++++++++++++++ Battery/EquivalentCircuitModel/run_fitting.m | 48 ++++++++++++ .../spectral_analysis/cost_function_eis.m | 14 ++++ .../load_experimental_data.m | 34 +++++++++ .../spectral_analysis/load_nyquist.m | 15 ++++ .../spectral_analysis/plot_nyquist_ank.m | 24 ++++++ .../spectral_analysis/plot_nyquist_params.m | 26 +++++++ .../spectral_analysis/run_fitting_eis.m | 72 ++++++++++++++++++ 10 files changed, 339 insertions(+), 1 deletion(-) create mode 100644 Battery/EquivalentCircuitModel/cost_function.m create mode 100644 Battery/EquivalentCircuitModel/plotexperience.m create mode 100644 Battery/EquivalentCircuitModel/run_fitting.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m index ff38ffcc0..ab2715ac3 100644 --- a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m @@ -1,4 +1,4 @@ -classdef EquivalentCircuitModel < BaseModel +calassdef EquivalentCircuitModel < BaseModel properties diff --git a/Battery/EquivalentCircuitModel/cost_function.m b/Battery/EquivalentCircuitModel/cost_function.m new file mode 100644 index 000000000..1bb8d6a18 --- /dev/null +++ b/Battery/EquivalentCircuitModel/cost_function.m @@ -0,0 +1,29 @@ +function total_error = cost_function(params_test, parameters, initial_values, t_exp, V_exp) + + + parameters.R0 = abs(params_test(1)); + parameters.R1 = abs(params_test(2)); + parameters.C1 = max(abs(params_test(3)), 0.1); + parameters.R2 = abs(params_test(4)); + parameters.C2 = max(abs(params_test(5)), 0.1); + + + inputparams = EquivalentCircuitModelInputParams(parameters); + model = EquivalentCircuitModel(inputparams); + [t_sim, V_sim, ~] = model.solve(); + + % Time synchronization + V_sim_aligne = interp1(t_sim, V_sim, t_exp, 'linear', 'extrap'); + + + voltage_error = sum((V_exp - V_sim_aligne).^2); + + lambda = 0.5; + + rel_error = sum((params_test-initial_values)./initial_values); + + tikhonov_error = lambda * rel_error.^2; + + total_error = voltage_error + tikhonov_error; + +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/plotexperience.m b/Battery/EquivalentCircuitModel/plotexperience.m new file mode 100644 index 000000000..d18f714cc --- /dev/null +++ b/Battery/EquivalentCircuitModel/plotexperience.m @@ -0,0 +1,76 @@ +function experience = plotexperience() + + + json_jp3 = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-params\jp3-opt-1d-full.json'; + jsonstruct = parseBattmoJson(json_jp3); + + % 1. Construction du modèle + [model, inputparams] = setupModelFromJson(jsonstruct); + + model.NegativeElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.argumentList = {'c'}; + model.NegativeElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.numberOfArguments = 1; + + model.PositiveElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.argumentList = {'c'}; + model.PositiveElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.numberOfArguments = 1; + + model.Electrolyte.computeDiffusionCoefficientFunc.argumentList = {'c', 'T'}; + model.Electrolyte.computeConductivityFunc.argumentList = {'c', 'T'}; + + % 3. Initialisation de l'état (maintenant le modèle sait quoi envoyer !) + state0 = setupInitialState(model); + + inputparams.Control.controlPolicy = 'CCDischarge'; + inputparams.Control.DRate = 2; + inputparams.Control.tmax = 30; + inputparams.Control.rampupTime = 0.1; + inputparams.Control.lowerCutoffVoltage = 2.5; + + schedule1 = setupSchedule(model, inputparams); + [~, states1] = simulateBattery(model, state0, schedule1); + state_after_pulse = states1{end}; + + inputparams.Control.DRate = 0; + inputparams.Control.tmax = 600; + inputparams.Control.rampupTime = 0.1; + + + schedule2 = setupSchedule(model, inputparams); + disp('Simulation du Repos en cours...'); + [~, states2] = simulateBattery(model, state_after_pulse, schedule2); + + all_states = [states1(:); states2(:)]; + N = length(all_states); + + time = zeros(N, 1); + voltage = zeros(N, 1); + current = zeros(N, 1); + + + for i = 1:N + time(i) = all_states{i}.time; + try + % Dans BattMo, les données du circuit extérieur sont dans "Control" + voltage(i) = all_states{i}.Control.E; + current(i) = all_states{i}.Control.I; + catch + % Alternative si les variables sont stockées à la racine + voltage(i) = all_states{i}.voltage; + current(i) = all_states{i}.current; + end + end + + figure; + subplot(2,1,1); + plot(time, voltage); + xlabel('Time (s)'); + ylabel('Voltage (V)'); + title('Voltage vs Time'); + + subplot(2,1,2); + plot(time, current); + xlabel('Time (s)'); + ylabel('Current (A)'); + title('Current vs Time'); + + experience = [current, voltage, time]; +end diff --git a/Battery/EquivalentCircuitModel/run_fitting.m b/Battery/EquivalentCircuitModel/run_fitting.m new file mode 100644 index 000000000..6b7d6747d --- /dev/null +++ b/Battery/EquivalentCircuitModel/run_fitting.m @@ -0,0 +1,48 @@ +%% Fitting Script + +% Charge les données expérimentales +t_exp = [0:1:1000]'; % Temps en secondes +V_exp = 4.1 * ones(1001, 1) - 0.1 * (t_exp/1000); % Fausse courbe de tension +I_exp = ones(1001, 1); % Courant expérimental + + +parameters = create_parameters(); + +% Remplacer le courant du modèle par le courant expérimental +parameters.I.dataX = t_exp; +parameters.I.dataY = I_exp; + +% Valeurs initiales [R0, R1, C1, R2, C2] +initial_values = [0.010, 0.010, 3000, 0.010, 100000]; + +options = optimset('Display', 'iter', 'TolX', 1e-4); +disp('beginning of optimization'); + +% Optimization with fminsearch +best_params = fminsearch(@(p) cost_function(p, parameters, initial_values, t_exp, V_exp), initial_values, options); + +fprintf('\n=== PARAMETERS FOUND ===\n'); +fprintf('R0 = %.5f Ohms\n', best_params(1)); +fprintf('R1 = %.5f Ohms\n', best_params(2)); +fprintf('C1 = %.1f Farads\n', best_params(3)); +fprintf('R2 = %.5f Ohms\n', best_params(4)); +fprintf('C2 = %.1f Farads\n', best_params(5)); + +%% Vérification Graphique + + +parameters.R0 = best_params(1); +parameters.R1 = best_params(2); +parameters.C1 = best_params(3); +parameters.R2 = best_params(4); +parameters.C2 = best_params(5); + +inputparams = EquivalentCircuitModelInputParams(parameters); +model = EquivalentCircuitModel(inputparams); +[t_sim, V_sim, ~] = model.solve(); + +figure; +plot(t_exp, V_exp, 'k', 'LineWidth', 2); hold on; +plot(t_sim, V_sim, 'r--', 'LineWidth', 2); +legend('Expérimental', 'Modèle (Fitted)'); +title('Résultat du Fitting'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m new file mode 100644 index 000000000..f4263fe0b --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m @@ -0,0 +1,14 @@ + +function [total_error, Z_re_exp, Z_im_exp] = cost_function_eis(best_params) + + +Z_re_exp = plot_nyquist_ank.Z_real; +Z_im_exp = plot_nyquist_ank.Z_imag; + + +omega = logspace(-2, 4, 100) + +Z_re_params = plot_nyquist_params.Z_real(best_params); +Z_im_params = plot_nyquist_params.Z_imag(best_params); + +totalerror = sum((Z_re_exp(omega)-Z_re_params(omega)).^2) + sum((Z_im_exp(omega)-Z_im_params(omega))^2) \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m new file mode 100644 index 000000000..4cea34683 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m @@ -0,0 +1,34 @@ +function [Z_real, Z_imag, omega] = load_experimental_data() + % --- 1. Configuration et Importation des données --- + filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; + + % Le délimiteur est la tabulation ('\t') + opts = detectImportOptions(filename, 'Delimiter', '\t'); + data = readtable(filename, opts); + + % --- 2. Identification des colonnes --- + % L'impédance réelle est dans Var26 et l'imaginaire dans Var27. + Z_real_raw = data.Var26; + Z_imag_raw = data.Var27; + omega_raw = data.Var16; + % --- 3. Gestion des virgules --- + % On remplace les virgules par des points, puis on convertit le texte en nombres + Z_real = str2double(strrep(Z_real_raw, ',', '.')); + Z_imag = str2double(strrep(Z_imag_raw, ',', '.')); + omega = str2double(strrep(omega_raw, ',', '.')); + + % --- 4. Nettoyage des données --- + % S'il y a des lignes de cyclage sans données EIS, on filtre les zéros ou NaN + idx_valides = (Z_real ~= 0) & ~isnan(Z_real); + Z_real = Z_real(idx_valides); + Z_imag = Z_imag(idx_valides); + + Z_real = Z_real(8:60); + Z_imag = Z_imag(8:60); + omega = 2*pi*omega(8:60); + + Z_real = Z_real(:); + Z_imag = Z_imag(:); + omega = omega(:); + +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m new file mode 100644 index 000000000..f5bb28400 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m @@ -0,0 +1,15 @@ +function [Z_real, Z_imag] = load_nyquist(params, omega) + + R_0 = params(1); + R_1 = params(2); + C_1 = params(3); + R_2 = params(4); + C_2 = params(5); + + + + Z_real = R_0 + R_1 ./ (1+(R_1* C_1.*omega).^2) + R_2 ./ (1+(R_2* C_2.*omega).^2); + Z_imag = (R_1*R_1*C_1.*omega ./ (1+(R_1* C_1.*omega).^2)) ... + + (R_2*R_2*C_2.*omega ./ (1+(R_2* C_2.*omega).^2)); + +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m new file mode 100644 index 000000000..2044245c4 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m @@ -0,0 +1,24 @@ + + + +load_experimental_data(); + +% --- 5. Tracé du diagramme de Nyquist --- +figure('Name', 'EIS', 'Color', 'w'); + +% On trace -Im(Z) en fonction de Re(Z) +plot(Z_real, Z_imag, 'o', ... + 'LineWidth', 1.5, ... + 'MarkerSize', 2, ... + 'MarkerFaceColor', [0 0.4470 0.7410], ... + 'MarkerEdgeColor', 'k'); +grid on; +axis equal; % Force la même échelle en X et Y + +% Ajout des labels +xlabel('Z_{re} ', 'FontSize', 12, 'FontWeight', 'bold'); +ylabel('-Z_{im}', 'FontSize', 12, 'FontWeight', 'bold'); +title('Nyquist diagram from data', 'FontSize', 14); + +% Amélioration des axes +set(gca, 'FontSize', 11, 'LineWidth', 1); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m new file mode 100644 index 000000000..3250ec09d --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m @@ -0,0 +1,26 @@ + +% params = [6.2261e-3, 0.3e-3, 10000.1264, 0.00097, 2e5]; % best params +% handmade + +params = [0.003, 0.00134, 5, 0.00330, 20000] +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(); +omega = logspace(-2, 4, 100) + +[Z_real, Z_imag] = load_nyquist(params, omega) + +figure; +plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); +hold on; +plot(Z_real, Z_imag, '-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'b'); +axis equal; % Essentiel pour Nyquist +grid on; +xlabel('Z_{réel} (\Omega)', 'FontWeight', 'bold'); +ylabel('-Z_{imaginaire} (\Omega)', 'FontWeight', 'bold'); +title('Nyquist diagram simulated'); + + + + + + + diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m new file mode 100644 index 000000000..4ea8d8fe9 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -0,0 +1,72 @@ +%% Fitting Script + +% initial values [R0, R1, C1, R2, C2] + params0 = [8.2e-3, 1.5e-3, 1, 1.5e-2, 200]; % handmade best ones + +% params0 = [6.2261e-3, 0.3e-3, 10000.1264, 0.00097, 2e5]; + + +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(); +%lengthZ = length(Z_im_exp); + +scales = [1e-3, 1e-3, 1000, 1e-3, 10000]; + +params0_norm = params0 ./ scales; + +lb_true = [1e-5, 1e-5, 1e-5, 1e-5, 1e-5]; +lb_norm = lb_true ./ scales; +ub_norm = []; + +delta = @(p_norm) compute_residuals(p_norm .* scales, Z_re_exp, Z_im_exp, omega); + +options = optimoptions('lsqnonlin', 'Display', 'iter', 'MaxFunctionEvaluations', 20000); + +best_params_norm = lsqnonlin(delta, params0_norm, lb_norm, ub_norm, options); + +best_params = best_params_norm .* scales; + + +fprintf('\n=== PARAMETERS FOUND ===\n'); +fprintf('R0 = %.5f Ohms\n', best_params(1)); +fprintf('R1 = %.5f Ohms\n', best_params(2)); +fprintf('C1 = %.1f Farads\n', best_params(3)); +fprintf('R2 = %.5f Ohms\n', best_params(4)); +fprintf('C2 = %.1f Farads\n', best_params(5)); + +%% Graphique + + +parameters.R0 = best_params(1); +parameters.R1 = best_params(2); +parameters.C1 = best_params(3); +parameters.R2 = best_params(4); +parameters.C2 = best_params(5); + +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, logspace(-2, 4, 100)); % doesn't work with omega which is strange + + +%% +figure; +plot(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); +hold on; +plot(omega, Z_re_fit, 'b-', 'LineWidth', 2); +legend('Expérimental', 'Modèle (Fitted)'); +title('Fitting results'); +xlabel('Z_{re} (\Omega)'); +ylabel('-Z_{im} (\Omega)'); +grid on; +axis equal; + + + +function res = compute_residuals(p, Z_re_exp, Z_im_exp, omega) + + [Z_re_param, Z_Im_param] = load_nyquist(p, omega); + + Module_Z = sqrt(Z_re_exp.^2 + Z_im_exp.^2); + + err_re = (Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); + err_im = (Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); + + res = [err_re; err_im]; +end \ No newline at end of file From 77864feff41c9ae7940100476196b33a5b481f9f Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 29 Apr 2026 11:15:45 +0200 Subject: [PATCH 012/119] problem with omega loading fixed --- .../load_experimental_data.m | 3 +- .../spectral_analysis/run_fitting_eis.m | 30 +++++++++++++++---- 2 files changed, 27 insertions(+), 6 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m index 4cea34683..604eec019 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m @@ -22,7 +22,8 @@ idx_valides = (Z_real ~= 0) & ~isnan(Z_real); Z_real = Z_real(idx_valides); Z_imag = Z_imag(idx_valides); - + omega = omega(idx_valides); + Z_real = Z_real(8:60); Z_imag = Z_imag(8:60); omega = 2*pi*omega(8:60); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m index 4ea8d8fe9..9b3f34d73 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -42,21 +42,41 @@ parameters.R2 = best_params(4); parameters.C2 = best_params(5); -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, logspace(-2, 4, 100)); % doesn't work with omega which is strange +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); % doesn't work with omega which is strange %% figure; +subplot(3,1,1); plot(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; -plot(omega, Z_re_fit, 'b-', 'LineWidth', 2); +plot(omega, Z_re_fit, 'bo', 'LineWidth', 2); legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); -xlabel('Z_{re} (\Omega)'); -ylabel('-Z_{im} (\Omega)'); -grid on; +xlabel('Omega'); +ylabel('Z_{re} '); + +subplot(3,1,2); +plot(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); +hold on; +plot(omega, Z_im_fit, 'bo', 'LineWidth', 2); +legend('Expérimental', 'Modèle (Fitted)'); +title('Fitting results'); +xlabel('Omega'); +ylabel('-Z_{im} '); + +subplot(3,1,3); +plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); +hold on; +plot(Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); +legend('Expérimental', 'Modèle (Fitted)'); +title('Nyquist'); +xlabel('Z_{re}'); +ylabel('-Z_{im} '); axis equal; +grid on; + function res = compute_residuals(p, Z_re_exp, Z_im_exp, omega) From 5bff6e5b86fa9a483d5c79b493580741c937fbbe Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 4 May 2026 11:19:25 +0200 Subject: [PATCH 013/119] fitting with unitboxBFGS, limit: C1<10*C2 --- .../spectral_analysis/run_fitting_eis.m | 83 ++- .../spectral_analysis/unitBoxBFGS.m | 578 ++++++++++++++++++ 2 files changed, 647 insertions(+), 14 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m index 9b3f34d73..85678bd9a 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -1,15 +1,21 @@ %% Fitting Script % initial values [R0, R1, C1, R2, C2] - params0 = [8.2e-3, 1.5e-3, 1, 1.5e-2, 200]; % handmade best ones +% params0 = [8.2e-3, 1.5e-3, 1, 1.5e-2, 200]; % handmade best ones -% params0 = [6.2261e-3, 0.3e-3, 10000.1264, 0.00097, 2e5]; +params0 = [3e-3, 0.00260, 100, 0.00132, 1]; [Z_re_exp, Z_im_exp, omega] = load_experimental_data(); %lengthZ = length(Z_im_exp); -scales = [1e-3, 1e-3, 1000, 1e-3, 10000]; +% synthetic data +% opti_params = [0.00341, 0.00260, 5663.9, 0.00132, 0.9]; +% [Z_re_exp, Z_im_exp] = load_nyquist(opti_params, omega); + +%% + +scales = [10e-2, 10e-3, 15000, 10e-3, 5]; params0_norm = params0 ./ scales; @@ -17,13 +23,21 @@ lb_norm = lb_true ./ scales; ub_norm = []; -delta = @(p_norm) compute_residuals(p_norm .* scales, Z_re_exp, Z_im_exp, omega); +f_opt = @(p_norm) optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) ; + +% best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); +params0_norm = params0_norm(:); -options = optimoptions('lsqnonlin', 'Display', 'iter', 'MaxFunctionEvaluations', 20000); +[min_value, best_params_norm, history] = unitBoxBFGS(... + params0_norm, ... + f_opt, ... + 'maximize', false, ... + 'linIneq', struct('A', [0, 0, -1, 0, 10], 'b', 0), ... + 'enforceFeasible', true ... +); -best_params_norm = lsqnonlin(delta, params0_norm, lb_norm, ub_norm, options); -best_params = best_params_norm .* scales; +best_params = best_params_norm(:) .* scales(:); fprintf('\n=== PARAMETERS FOUND ===\n'); @@ -48,18 +62,18 @@ %% figure; subplot(3,1,1); -plot(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); +semilogx(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; -plot(omega, Z_re_fit, 'bo', 'LineWidth', 2); +semilogx(omega, Z_re_fit, 'bo', 'LineWidth', 2); legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); ylabel('Z_{re} '); subplot(3,1,2); -plot(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); +semilogx(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; -plot(omega, Z_im_fit, 'bo', 'LineWidth', 2); +semilogx(omega, Z_im_fit, 'bo', 'LineWidth', 2); legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); @@ -79,14 +93,55 @@ -function res = compute_residuals(p, Z_re_exp, Z_im_exp, omega) +function [v, g_norm] = optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) + + p = p_norm(:) .* scales(:); [Z_re_param, Z_Im_param] = load_nyquist(p, omega); Module_Z = sqrt(Z_re_exp.^2 + Z_im_exp.^2); + Module_Z = Module_Z(:); err_re = (Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); err_im = (Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); - res = [err_re; err_im]; -end \ No newline at end of file + v = sum(err_re.^2 + err_im.^2); + + +if nargout > 1 + w = omega(:); + R0 = p(1); + R1 = p(2); + C1 = p(3); + R2 = p(4); + C2 = p(5); + + + g_re_dR0 = -ones(size(w)); + g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; + g_re_dC1 = (2*C1*R1^3.*w.^2) ./ (1+(R1*C1.*w).^2).^2; + g_re_dR2 = -(1-(R2*C2.*w).^2) ./ (1+(R2*C2.*w).^2).^2; + g_re_dC2 = (2*C2*R2^3.*w.^2) ./ (1+(R2*C2.*w).^2).^2; + + J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; + + + g_im_dR0 = zeros(size(w)); + g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; + g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; + g_im_dR2 = -(2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; + g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; + + J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; + derr_re_dp = J_re ./ Module_Z; + derr_im_dp = J_im ./ Module_Z; + + + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); + g_norm = g_true .* scales(:); +end + +end + + + diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m b/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m new file mode 100644 index 000000000..d020d1a6f --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m @@ -0,0 +1,578 @@ +function [v, u, history] = unitBoxBFGS(u0, f, varargin) +% Iterative line search optimization using BFGS intended for scaled +% problems, i.e., 0<=u<=1 and f~O(1) +% +% SYNOPSIS: +% [v, u, history] = unitBoxBFGS(u0, f, ...) +% +% PARAMETERS +% u0 : inital guess nx1 vector with 0<= u0 <= 1 and feasible wrt +% any additional constraints +% f : function handle s.t., [v,g] = f(u) returns +% v : objective value +% g : objective nx1 gradient vector +% KEYWORD ARGUMENTS: +% 'maximize' : Boolean option (false will minimize objective) +% Default: true +% 'stepInit' : Initial step (gradient scaling). If not provided +% (or set to nan), the following scaling will be used: +% stepInit = maxInitialUpdate/max(|initial gradient|) +% 'maxInitialUpdate' : as described above. Default: 0.05 +% 'history' : Option for 'warm starting' based on previous +% optimization (must have been run with option +% 'outputHessian' = true) +% Stopping criteria options +% 'gradTol' : Absolute tollerance of inf-norm of projected gradient. +% Default: 1e-3 +% 'objChangeTol' : Absolute objective update tollerance. Default: 5e-4 +% 'maxIt' : Maximal number of iterations. Default: 25 +% Line-search options +% 'lineSearchMaxIt' : Maximal number of line-search iterations. Default: 5 +% 'stepIncreaseTol' : Maximal step increase factor between line +% search iterations. Deafult: 10 +% 'wolfe1', : Objective improvement condition. Default: 1e-4 +% 'wolfe2', : Gradient reduction condition. Default: 0.9 +% Hessian approximation options +% 'useBFGS' : If false pure gradient search will be used. +% Deafult: true +% 'limitedMemory' : If false, full Hessian approximations will be +% made (in general not recommended), otherwise +% L-BFGS (see LimitedMemoryHessian.m). +% Default: true +% 'lbfgsNum' : Number of vector-pairs stored for L-BFGS. +% : Default: 5 +% 'lbfgsStrategy' : 'static' or 'dynamic' (see LimitedMemoryHessian.m) +% Default: 'dynamic' +% Linear constraints options +% 'linEq' : Linear equality constraints given as structure with +% fields 'A' and 'b' to enforce A*u=b +% 'linIneq' : Linear inequality constraints *in addition to* the default +% box constraints (0 <= u <= 1). Given as structure with +% fields 'A' and 'b' to enforce A*u<=b +% 'enforceFeasible' : If true, will attempt to repair problematic +% constraint handling/violations by projection. A +% NOTE: A non-feasible initial guess, will always be +% attempted to be made feasible. +% Default: false +% Plotting and output options +% 'plotEvolution' : Plot progess of optimization in figure. +% Default: true +% 'logPlot' : Use logarithmic y-axis when plotting objective +% Default: false +% 'outputHessian' : Output Hessian approximation for each iteration +% in history-structure. Deafault: false +% +% RETURNS: +% v : Optimal or best objective value +% u : Control/parameter vector corresponding to v +% history : Structure containing for each iteration: +% 'val' : objective value +% 'u' : control/parameter vector +% 'pg' : norm of projected gradient +% 'alpha' : line-search step length +% 'lsit' : number of line-search iterations +% 'lsfl' : line-search flag +% 'hess' : Hessian inverse approximation (if requested) + +%{ +Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. + +This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). + +MRST is free software: you can redistribute it and/or modify +it under the terms of the GNU General Public License as published by +the Free Software Foundation, either version 3 of the License, or +(at your option) any later version. + +MRST is distributed in the hope that it will be useful, +but WITHOUT ANY WARRANTY; without even the implied warranty of +MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the +GNU General Public License for more details. + +You should have received a copy of the GNU General Public License +along with MRST. If not, see . +%} +opt = struct( 'maximize', true, ... + 'stepInit', nan, ... + 'maxInitialUpdate', 0.05, ... + 'gradTol', 1e-3, ... + 'objChangeTol', 5e-4, ... + 'objChangeTolRel', -inf, ... + 'maxIt', 25, ... + 'lineSearchMaxIt', 5, ... + 'wolfe1', 1e-4, ... + 'wolfe2', 0.9, ... + 'safeguardFac', 1e-5, ... + 'stepIncreaseTol', 10, ... + 'useBFGS', true, ... + 'limitedMemory', true, ... + 'lbfgsNum', 5, ... + 'lbfgsStrategy', 'dynamic', ... + 'linEq', [], ... + 'enforceFeasible', true, ... + 'linIneq', [], ... + 'plotEvolution', true, ... + 'logPlot', false, ... + 'outputHessian', false, ... + 'history', [] ); +opt = merge_options(opt, varargin{:}); +objSign = 1; +if opt.maximize + f = @(u)fNegative(u, f); + objSign = -1; +end +c = getConstraints(u0, opt); +if isempty(opt.history) + % Setup constraint struct + [u0, ~, consOK] = checkFeasible(u0, c, opt.enforceFeasible, 'Initial guess'); + assert(consOK, 'Infeasible initial guess') + + % Perform initial evaluation of objective and gradient: + [v0,g0] = f(u0); + % If not provided, set initial step + step = opt.stepInit; + if isnan(step) || step <= 0 + step = opt.maxInitialUpdate/max(abs(g0)); + end + % Initial Hessian-approximation + if ~opt.limitedMemory + Hi = step; + else + Hi = LimitedMemoryHessian('initScale', step, ... + 'm', opt.lbfgsNum, ... + 'initStrategy', opt.lbfgsStrategy); + end + HiPrev = Hi; + it = 0; + % Setup struct for gathering optimization history + history = gatherInfo([], objSign*v0, u0, norm(g0), nan, nan, nan, Hi, opt.outputHessian); +else + history = opt.history; + it = numel(history.val); + Hi = history.hess{it}; + assert(~isempty(Hi), ... + 'Warm start based on history requires Hessian approximations'); + u0 = history.u{it}; + [v0, g0] = f(u0); + HiPrev = history.hess{max(it-1,1)}; + opt.maxIt = opt.maxIt + it; +end +[v, u] = deal(v0,u0); +if opt.plotEvolution >0 + evFig = figure; + plotInfo(evFig, history, opt.logPlot) +end +printInfo(history, it); + +success = false; +g = g0; +while ~success + it = it+1; + [d, Hi, pg, opt.maxStep] = getSearchDirection(u0, g0, Hi, HiPrev, c); + %if isempty(d), break; end + if ~(norm(pg,inf) < opt.gradTol) && ~isempty(d) + % Perform line-search + [tmp, flag, fixed] = checkFeasible(u0+d, c, opt.enforceFeasible); + if ~flag && fixed + d = tmp - u0; + end + [u, v, g, lsinfo] = lineSearch(u0, v0, g0, d, f, opt); + % Update Hessian approximation + if opt.useBFGS %&& lsinfo.flag == 1 + [du, dg] = deal(u-u0, g-g0); + % if any of the gradient entries are not defined, we set + % the difference to zero + dg(~isfinite(dg)) = 0; + if du'*dg > sqrt(eps)*norm(du)*norm(dg) + HiPrev = Hi; + if isa(Hi, 'LimitedMemoryHessian') + Hi = Hi.update(du, dg); + else + r = 1/(du'*dg); + V = eye(numel(u)) - r*dg*du'; + Hi = V'*Hi*V + r*(du*du'); + end + else + fprintf('Hessian not updated during iteration %d.\n', it) + end + end + % Update history + history = gatherInfo(history, objSign*v, u, norm(pg,inf), lsinfo.step, ... + lsinfo.nits, lsinfo.flag, Hi, opt.outputHessian); + else + history = gatherInfo(history, objSign*v, u, norm(pg,inf), 0, 0, 0, ... + Hi, opt.outputHessian); + end + + %Check stopping criteria + success = (it >= opt.maxIt) || (norm(pg,inf) < opt.gradTol) || ... + (abs(v-v0) < opt.objChangeTol) || ... + (abs((v-v0)./v) < opt.objChangeTolRel); + + [u0, v0, g0] = deal(u, v, g); + if opt.plotEvolution > 0 + plotInfo(evFig, history, opt.logPlot) + end + printInfo(history, it); +end +end +%-------------------------------------------------------------------------- + +function [d, Hi, pg, maxStep] = getSearchDirection(u0, g0, Hi, HiPrev, c) +% Find search-direction which is (sum of) the projection(s) of Hi*g0 +% restricted to directions with non-active constraints. +cnt = 1; +for k = 1:3 + if k==2 + Hi = HiPrev; + elseif k==3 + if isa(Hi, 'LimitedMemoryHessian') + Hi = Hi.reset(); + else + Hi = 1; + end + end + % Project gradient and search direction onto nullspace of equality + % constraints + Q = c.e.Q; + pg = -projQ(g0, Q); + d = -projQ(g0, Q, Hi); + % The following loop(s) should project onto nullspace of additional + % active constraints. First for gradient direction, then for search + % direction which may have additional constraints active. While-loop + % will in most cases only be traversed once, so we don't worry too much + % about efficiency + isActive = false; + for kd = 1:2 + [na, na_prev] = deal(0, -1); + while na > na_prev + if kd == 1 + [~, active_cur] = classifyConstraints(c.i.A, c.i.b, u0, pg); + else + [~, active_cur] = classifyConstraints(c.i.A, c.i.b, u0, d); + end + isActive = isActive | active_cur; + na_prev = na; + na = nnz(isActive); + if na > na_prev % redo projection for all active + [Q, s] = svd([c.i.A(isActive,:)', c.e.A'], 0); + s = diag(s); + Q = Q(:, s > sqrt(eps)*s(1)); + if kd == 1 + pg = -projQ(g0, Q); + else + d = -projQ(g0, Q, Hi); + end + end + end + end + % Check for tiny projected gradient + if norm(pg, inf) <= sqrt(eps)*norm(g0, inf) % nothing more to do + [d, maxStep] = deal([]); + return + end + % Iteratively find all constraints that become active from u0 to u0+d, + % and project remaining line segments accordingly. + [dr, gr] = deal(d, g0); + becomesActive = isActive; + d = 0; + done = false; + while ~done + if norm(dr) > sqrt(eps) + sgn = classifyConstraints(c.i.A, c.i.b, u0+d, dr); + [ix, s] = findNextConstraint(c.i.A, c.i.b, u0+d, dr, sgn<=0 | becomesActive); + else + [ix, s] = deal([], 0); + end + if ~isempty(ix) && s <= 1+sqrt(eps) + becomesActive(ix) = true; + d = d + s*dr; + gr = (1-s)*gr; + Q = expandQ(Q, c.i.A(ix,:)'); + dr = -projQ(gr, Q, Hi); + else + d = d+dr; + done = true; + end + end + % find maximal step length we can take with d before hitting the next + % constraint (should be >= 1) + sgn = classifyConstraints(c.i.A, c.i.b, u0, d); + [~, maxStep] = findNextConstraint(c.i.A, c.i.b, u0, d, sgn<=0); + if maxStep < .95 + warning('Problematic constraint handling, relative step length: %6.5f', maxStep); + end + if maxStep < 1 + [d, maxStep] = deal(maxStep*d, 1); + end + + isDecreasing = d'*g0 <= 0; + isZero = norm(d, inf) <= sqrt(eps)*norm(Hi*g0, inf); + if isDecreasing && ~isZero % decreasing search direction found, exit + break; + else + % retry with other Hessian approx + if ~isZero + str = 'Small norm of search direction'; + else + str = 'Non-inceasing search direction'; + end + switch cnt + case 1 + fprintf('%s, trying previous Hessian approximation.\n', str) + case 2 + fprintf('%s, trying to reset Hessian to identity.\n', str) + case 3 + fprintf('Exiting: %s.\n', str) + [d, maxStep] = deal([]); + end + end +end +end +%-------------------------------------------------------------------------- + +function w = projQ(v, Q, H) +if nargin < 3 + H = 1; +end +if isempty(Q) + w = H*v; +else + if ~isa(H, 'LimitedMemoryHessian') + tmp = H*(v-Q*(Q'*v)); + w = tmp - Q*(Q'*tmp); + else + H = H.setNullspace(Q); + w = H*v; + end +end +end +%-------------------------------------------------------------------------- + +function c = getConstraints(u, opt) +% Box constraints, always 0<= u <= 1 +nu = numel(u); +c.i.A = [diag(-ones(nu,1)); diag(ones(nu,1))]; +c.i.b = [zeros(nu,1); ones(nu,1)]; +% Add general linear constraints +if ~isempty(opt.linIneq) + % scale by norm(A) + sc = norm(opt.linIneq.A); + c.i.A = [c.i.A; opt.linIneq.A/sc]; + c.i.b = [c.i.b; opt.linIneq.b/sc]; +end +% Equality constraints (always active) +if ~isempty(opt.linEq) + sc = norm(opt.linEq.A); + c.e.A = opt.linEq.A/sc; + c.e.b = opt.linEq.b/sc; + [Q, s] = svd(c.e.A', 0); + s = diag(s); + c.e.Q = Q(:, s> sqrt(eps) * s(1)); +else + c.e.A = zeros(0, nu); + c.e.b = []; + c.e.Q = zeros(nu, 0); +end +end +%-------------------------------------------------------------------------- + +function [u, flag, fixed] = checkFeasible(u, c, enforce, nm) +% Check that u is feasible. If not and enforce == true, try to fix. Ideally +% should be solved as ||u-u*|| st c.e and c.i, but since we don't have a +% QP-solver resort to (costly) iterative projections in active subspaces. +% Intended for fixing mild violations. +if nargin < 4 + nm = 'Vector u'; +end +if nargin < 3 + enforce = false; +end +hasEC = ~isempty(c.e.A); +hasIC = ~isempty(c.i.A); +[ecOK, icOK] = deal(true); + +if hasEC + [Ae, be] = deal(c.e.A, c.e.b); + if any(abs(c.e.A*u-c.e.b) > sqrt(eps)) + % find closest u that fulfills c.e. + u = u + Ae'*((Ae*Ae')\(be-Ae*u)); + ecOK = false; %now OK, but warn + end +end + +flag = ecOK; +fixed = false; +maxIt = 100; +for it = 1:maxIt + if hasIC + icOK = ~any(c.i.A*u-c.i.b > sqrt(eps)); + flag = flag && icOK; + end + if ~enforce + break + else + if ~icOK + Q = zeros(numel(u), 0); + proj = @(v)v; + if hasEC + Q = c.e.Q; + proj = @(v)v-Q*(Q'*v); + end + % Loop through each violating and project. If there are no more + % availabe directions, restart while-loop from current point + done = false; + cnt = 0; + while ~done + if cnt == 0 + icIx = find(c.i.A*u-c.i.b > sqrt(eps)); + icIx = circshift(icIx, it); + end + if isempty(icIx) || cnt == numel(icIx) + done = true; + else + % + ix = icIx(cnt+1); + [a, b] = deal(c.i.A(ix,:)', c.i.b(ix)); + pa = proj(a); + if norm(pa) < sqrt(eps)*norm(a) + % skip + cnt = cnt +1; + else + cnt = 0; + u = u + pa*((b-a'*u)/(a'*pa)); + if size(Q,2) < size(Q,1)-1 + Q = expandQ(Q, pa); + proj = @(v)v-Q*(Q'*v); + else + % possibly restart while-loop + done = true; + end + end + end + end + else + fixed = true; + break + end + end +end + + +if it == maxIt + warning('Failed attempt to fix feasibility of %s, continuing anyway ...', nm); +elseif ~flag + if ~enforce + warning('%s is not feasible within tollerance. %s', nm, ... + 'Consider running with option ''enforceFeasible''=true'); + else + warning('%s was not feasible, fixed feasibility in %d iteration(s)', ... + nm, it-1); + end +end +end +%-------------------------------------------------------------------------- +function [sgn, act] = classifyConstraints(A, b, u, v) +% classify inequality constraints for point u with direction v +% sgn: -1: in, 0: parallell, 1: out +% act: true for active +sgn = A*v; +sgn(abs(sgn) -sqrt(eps) & sgn > 0; +end +%-------------------------------------------------------------------------- + +function [ix, s] = findNextConstraint(A, b, u, d, ac) +s = (b-A*u)./(A*d); +s(ac) = inf; +s(s sqrt(eps) + Q = [Q, v/norm(v)]; +else + fprintf('Newly active constraint is linear combination of other active constraints ??!!\n') +end +end +%-------------------------------------------------------------------------- + +function [v, g] = fNegative(u, f) +if nargout == 1 + v = -f(u); +elseif nargout == 2 + [v, g] = f(u); + [v, g] = deal(-v, -g); +end +end +%-------------------------------------------------------------------------- + +function [] = plotInfo(fig, hst, logPlot) +if ~ishandle(fig) + figure(fig) +else + % Avoid stealing focus if figure already exists + set(0, 'CurrentFigure', fig); +end +xt = 0:(numel(hst.val)-1); +xlim = [-.2, xt(end)+.5]; +ch = abs(hst.val(2:end)-hst.val(1:end-1)); +popt = {'o-', 'LineWidth', 2, 'MarkerSize', 6, ... + 'MarkerFaceColor', [1 1 1]}; +subplot(5,1,1), +if ~logPlot + plot(xt, hst.val, popt{:}); +else + semilogy(xt, abs(hst.val), popt{:}); +end +title('Objective'); +set(gca, 'XLim', xlim) +subplot(5,1,2), semilogy(xt,hst.pg, popt{:}), title('Gradient norm'); +set(gca, 'XLim', xlim) +subplot(5,1,3), semilogy(xt(2:end)-.5,ch, popt{:}), title('Objective change'); +set(gca, 'XLim', xlim) +subplot(5,1,4), bar(xt,hst.lsit), title('Line search iterations'); +set(gca, 'XLim', xlim) +subplot(5,1,5), col = [0.8500 0.3250 0.0980]; +if numel(hst.u{end}) < 50 + bar(hst.u{end}, 'FaceColor', col); +else + plot(hst.u{end}, '.-', 'Color', col); +end +title('Current scaled controls'); +set(gca, 'YLim', [0, 1]) +drawnow +end +%-------------------------------------------------------------------------- + +function hst = gatherInfo(hst, val, u, pg, alpha, lsit, lsfl, hess, outputH) +% obj.val | contr | norm proj.grad | ls-step | ls-its | ls-flag | hessian +if ~outputH + hess = []; +end +if isempty(hst) + hst = struct('val', val, 'u', {{u}}, 'pg', pg, ... + 'alpha', alpha, 'lsit', lsit, 'lsfl', lsfl, ... + 'hess', {{hess}}); +else + hst.val = [hst.val , val ]; + hst.u = [hst.u , {u} ]; + hst.pg = [hst.pg , pg ]; + hst.alpha = [hst.alpha, alpha]; + hst.lsit = [hst.lsit , lsit ]; + hst.lsfl = [hst.lsfl , lsfl ]; + hst.hess = [hst.hess ,{hess}]; +end +end +%-------------------------------------------------------------------------- + +function printInfo(history, it) +fprintf('It: %2.1d | val: %4.3e | ls-its: %3.1d | pgrad: %4.3e\n', ... + it, history.val(end), history.lsit(end), ... + history.pg(end)); +end From 53693506c5158001b7f1376b95b319f5d5f6234e Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 5 May 2026 13:34:38 +0200 Subject: [PATCH 014/119] details --- .../spectral_analysis/run_fitting_eis.m | 36 +++++++++++++++---- 1 file changed, 30 insertions(+), 6 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m index 85678bd9a..1e287449a 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -7,10 +7,22 @@ [Z_re_exp, Z_im_exp, omega] = load_experimental_data(); + + %lengthZ = length(Z_im_exp); % synthetic data -% opti_params = [0.00341, 0.00260, 5663.9, 0.00132, 0.9]; +% opti_params = [0.00341, 0.00260, 5663.9, 0.00132, 0.9]; % params with +% lsqnonlin +% +% params with unitboxBFGS: +% R0 = 0.00318 Ohms +% R1 = 0.00247 Ohms +% C1 = 10654.4 Farads +% R2 = 0.00155 Ohms +% C2 = 0.4 Farads +% + % [Z_re_exp, Z_im_exp] = load_nyquist(opti_params, omega); %% @@ -32,13 +44,17 @@ params0_norm, ... f_opt, ... 'maximize', false, ... - 'linIneq', struct('A', [0, 0, -1, 0, 10], 'b', 0), ... + 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... 'enforceFeasible', true ... ); best_params = best_params_norm(:) .* scales(:); +[v_opt, g_opt] = optifunc(best_params, scales, Z_re_exp, Z_im_exp, omega) + +fprintf('\n=== FITTING SCORE ===\n'); +fprintf('Error : %e\n', v_opt); fprintf('\n=== PARAMETERS FOUND ===\n'); fprintf('R0 = %.5f Ohms\n', best_params(1)); @@ -56,7 +72,7 @@ parameters.R2 = best_params(4); parameters.C2 = best_params(5); -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); % doesn't work with omega which is strange +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); %% @@ -65,7 +81,7 @@ semilogx(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; semilogx(omega, Z_re_fit, 'bo', 'LineWidth', 2); -legend('Expérimental', 'Modèle (Fitted)'); +% legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); ylabel('Z_{re} '); @@ -74,7 +90,7 @@ semilogx(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; semilogx(omega, Z_im_fit, 'bo', 'LineWidth', 2); -legend('Expérimental', 'Modèle (Fitted)'); +% legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); ylabel('-Z_{im} '); @@ -83,7 +99,7 @@ plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; plot(Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); -legend('Expérimental', 'Modèle (Fitted)'); +% legend('Expérimental', 'Modèle (Fitted)'); title('Nyquist'); xlabel('Z_{re}'); ylabel('-Z_{im} '); @@ -91,7 +107,15 @@ grid on; +text_error = sprintf('Fitting error : %.2e', v_opt); + +subplot(3,1,3); +text(0.05, 0.90, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); function [v, g_norm] = optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) From b78424bc70f6267ce78986a5c6628f428907f23f Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 5 May 2026 13:58:34 +0200 Subject: [PATCH 015/119] added iterations --- .../spectral_analysis/run_fitting_eis.m | 10 ++++++---- 1 file changed, 6 insertions(+), 4 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m index 1e287449a..6fa9ee303 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -43,15 +43,17 @@ [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... f_opt, ... - 'maximize', false, ... - 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... - 'enforceFeasible', true ... + 'maximize', false, ... + 'enforceFeasible', true, ... + 'maxIt', 300, ... + 'objChangeTol', 1e-6, ... + 'gradTol', 1e-5 ... ); best_params = best_params_norm(:) .* scales(:); -[v_opt, g_opt] = optifunc(best_params, scales, Z_re_exp, Z_im_exp, omega) +[v_opt, g_opt] = optifunc(best_params_norm, scales, Z_re_exp, Z_im_exp, omega) fprintf('\n=== FITTING SCORE ===\n'); fprintf('Error : %e\n', v_opt); From 67075aca614cec60793f4ba44278f6624a5bc8b3 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 5 May 2026 13:59:47 +0200 Subject: [PATCH 016/119] iterations and constraints --- .../EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m | 3 ++- 1 file changed, 2 insertions(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m index 6fa9ee303..9a6a0ab46 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m @@ -43,7 +43,8 @@ [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... f_opt, ... - 'maximize', false, ... + 'maximize', false, ... + 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... 'enforceFeasible', true, ... 'maxIt', 300, ... 'objChangeTol', 1e-6, ... From 6b3d582a74acdd964eec67f97dd299050c88af9a Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 10:29:43 +0200 Subject: [PATCH 017/119] classe fitting_eis --- .../spectral_analysis/fitting_eis.m | 159 ++++++++++++++++++ 1 file changed, 159 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m new file mode 100644 index 000000000..c83c4399e --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m @@ -0,0 +1,159 @@ +classdef fitting_eis + + properties + params0 + Z_re_exp + Z_im_exp + omega + scales + lb_true + end + + + + methods + + + function [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega) + + f_opt = @(p_norm) optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) ; + + params0_norm = params0 ./ scales; + % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); + params0_norm = params0_norm(:); + + [min_value, best_params_norm, history] = unitBoxBFGS(... + params0_norm, ... + f_opt, ... + 'maximize', false, ... + 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... + 'enforceFeasible', true, ... + 'maxIt', 300, ... + 'objChangeTol', 1e-6, ... + 'gradTol', 1e-5 ... + ); + best_params = best_params_norm(:) .* scales(:); + + end + + function plotresults(params0, scales, Z_re_exp, Z_im_exp, omega) + + [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega); + parameters.R0 = best_params(1); + parameters.R1 = best_params(2); + parameters.C1 = best_params(3); + parameters.R2 = best_params(4); + parameters.C2 = best_params(5); + + [Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); + + figure; + subplot(3,1,1); + semilogx(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); + hold on; + semilogx(omega, Z_re_fit, 'bo', 'LineWidth', 2); + % legend('Expérimental', 'Modèle (Fitted)'); + title('Fitting results'); + xlabel('Omega'); + ylabel('Z_{re} '); + + subplot(3,1,2); + semilogx(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + hold on; + semilogx(omega, Z_im_fit, 'bo', 'LineWidth', 2); + % legend('Expérimental', 'Modèle (Fitted)'); + title('Fitting results'); + xlabel('Omega'); + ylabel('-Z_{im} '); + + subplot(3,1,3); + plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + hold on; + plot(Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); + % legend('Expérimental', 'Modèle (Fitted)'); + title('Nyquist'); + xlabel('Z_{re}'); + ylabel('-Z_{im} '); + axis equal; + + grid on; + + text_error = sprintf('Fitting error : %.2e', v_opt); + + subplot(3,1,3); + + text(0.05, 0.90, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + end + + function GiveResults(params0, scales, Z_re_exp, Z_im_exp, omega) + + [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega); + [v_opt, g_opt] = optifunc(best_params_norm, scales, Z_re_exp, Z_im_exp, omega); + + fprintf('\n=== FITTING SCORE ===\n'); + fprintf('Error : %e\n', v_opt); + + fprintf('\n=== PARAMETERS FOUND ===\n'); + fprintf('R0 = %.5f Ohms\n', best_params(1)); + fprintf('R1 = %.5f Ohms\n', best_params(2)); + fprintf('C1 = %.1f Farads\n', best_params(3)); + fprintf('R2 = %.5f Ohms\n', best_params(4)); + fprintf('C2 = %.1f Farads\n', best_params(5)); + + + end + + + function [v, g_norm] = optifunc(p, scales, Z_re_exp, Z_im_exp, omega) + + [Z_re_param, Z_Im_param] = load_nyquist(p, omega); + + Module_Z = sqrt(Z_re_exp.^2 + Z_im_exp.^2); + Module_Z = Module_Z(:); + + err_re = (Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); + err_im = (Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); + + v = sum(err_re.^2 + err_im.^2); + + + if nargout > 1 + w = omega(:); + R0 = p(1); + R1 = p(2); + C1 = p(3); + R2 = p(4); + C2 = p(5); + + + g_re_dR0 = -ones(size(w)); + g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; + g_re_dC1 = (2*C1*R1^3.*w.^2) ./ (1+(R1*C1.*w).^2).^2; + g_re_dR2 = -(1-(R2*C2.*w).^2) ./ (1+(R2*C2.*w).^2).^2; + g_re_dC2 = (2*C2*R2^3.*w.^2) ./ (1+(R2*C2.*w).^2).^2; + + J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; + + + g_im_dR0 = zeros(size(w)); + g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; + g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; + g_im_dR2 = -(2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; + g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; + + J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; + derr_re_dp = J_re ./ Module_Z; + derr_im_dp = J_im ./ Module_Z; + + + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); + g_norm = g_true .* scales(:); + end + end + + end +end \ No newline at end of file From 7595336daabbfb8ee10a5900c54c1b0d6937e715 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 13:32:38 +0200 Subject: [PATCH 018/119] =?UTF-8?q?classe=20lmoins=20incoh=C3=A9rente=3F?= MIME-Version: 1.0 Content-Type: text/plain; charset=UTF-8 Content-Transfer-Encoding: 8bit --- .../spectral_analysis/fitting_eis.m | 91 +++++++++++-------- 1 file changed, 52 insertions(+), 39 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m index c83c4399e..19e8c9e9b 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m @@ -1,4 +1,4 @@ -classdef fitting_eis +classdef fitting_eis < handle properties params0 @@ -6,19 +6,31 @@ Z_im_exp omega scales - lb_true + + best_params_found = [] + fitting_error = [] end methods + function feis = fitting_eis(params0, scales, Z_re_exp, Z_im_exp, omega) + feis.params0 = params0(:); + feis.scales = scales(:); + feis.Z_re_exp = Z_re_exp(:); + feis.Z_im_exp = Z_im_exp(:); + feis.omega = omega(:); + end + - function [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega) + function [min_value, best_params, history] = optimizationBFGS(feis) + + - f_opt = @(p_norm) optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) ; + f_opt = @(p_norm) feis.optifunc(p_norm.* feis.scales) ; - params0_norm = params0 ./ scales; + params0_norm = feis.params0 ./ feis.scales; % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); @@ -26,50 +38,50 @@ params0_norm, ... f_opt, ... 'maximize', false, ... - 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... + 'linIneq', struct('A', [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)], 'b', 0), ... 'enforceFeasible', true, ... 'maxIt', 300, ... 'objChangeTol', 1e-6, ... 'gradTol', 1e-5 ... ); - best_params = best_params_norm(:) .* scales(:); + best_params = best_params_norm(:) .* feis.scales(:); - end + feis.best_params_found = best_params; + [feis.fitting_error, ~] = feis.optifunc(best_params); + - function plotresults(params0, scales, Z_re_exp, Z_im_exp, omega) + end - [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega); - parameters.R0 = best_params(1); - parameters.R1 = best_params(2); - parameters.C1 = best_params(3); - parameters.R2 = best_params(4); - parameters.C2 = best_params(5); + function plotresults(feis) + if isempty(feis.best_params_found) + feis.optimizationBFGS(); + end - [Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); + [Z_re_fit, Z_im_fit] = load_nyquist(feis.best_params_found, feis.omega); figure; subplot(3,1,1); - semilogx(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); + semilogx(feis.omega, feis.Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; - semilogx(omega, Z_re_fit, 'bo', 'LineWidth', 2); + semilogx(feis.omega, Z_re_fit, 'bo', 'LineWidth', 2); % legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); ylabel('Z_{re} '); subplot(3,1,2); - semilogx(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + semilogx(feis.omega, feis.Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; - semilogx(omega, Z_im_fit, 'bo', 'LineWidth', 2); + semilogx(feis.omega, Z_im_fit, 'bo', 'LineWidth', 2); % legend('Expérimental', 'Modèle (Fitted)'); title('Fitting results'); xlabel('Omega'); ylabel('-Z_{im} '); subplot(3,1,3); - plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + plot(feis.Z_re_exp, feis.Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); hold on; - plot(Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); + plot(feis.Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); % legend('Expérimental', 'Modèle (Fitted)'); title('Nyquist'); xlabel('Z_{re}'); @@ -78,7 +90,7 @@ function plotresults(params0, scales, Z_re_exp, Z_im_exp, omega) grid on; - text_error = sprintf('Fitting error : %.2e', v_opt); + text_error = sprintf('Fitting error : %.2e', feis.fitting_error); subplot(3,1,3); @@ -89,40 +101,41 @@ function plotresults(params0, scales, Z_re_exp, Z_im_exp, omega) 'FontWeight', 'bold'); end - function GiveResults(params0, scales, Z_re_exp, Z_im_exp, omega) + function GiveResults(feis) + if isempty(feis.best_params_found) + feis.optimizationBFGS(); + end - [min_value, best_params, history] = optimizationBFGS(params0, scales, Z_re_exp, Z_im_exp, omega); - [v_opt, g_opt] = optifunc(best_params_norm, scales, Z_re_exp, Z_im_exp, omega); fprintf('\n=== FITTING SCORE ===\n'); - fprintf('Error : %e\n', v_opt); + fprintf('Error : %e\n', feis.fitting_error); fprintf('\n=== PARAMETERS FOUND ===\n'); - fprintf('R0 = %.5f Ohms\n', best_params(1)); - fprintf('R1 = %.5f Ohms\n', best_params(2)); - fprintf('C1 = %.1f Farads\n', best_params(3)); - fprintf('R2 = %.5f Ohms\n', best_params(4)); - fprintf('C2 = %.1f Farads\n', best_params(5)); + fprintf('R0 = %.5f Ohms\n', feis.best_params_found(1)); + fprintf('R1 = %.5f Ohms\n', feis.best_params_found(2)); + fprintf('C1 = %.1f Farads\n', feis.best_params_found(3)); + fprintf('R2 = %.5f Ohms\n', feis.best_params_found(4)); + fprintf('C2 = %.1f Farads\n', feis.best_params_found(5)); end - function [v, g_norm] = optifunc(p, scales, Z_re_exp, Z_im_exp, omega) + function [v, g_norm] = optifunc(feis, p) - [Z_re_param, Z_Im_param] = load_nyquist(p, omega); + [Z_re_param, Z_Im_param] = load_nyquist(p, feis.omega); - Module_Z = sqrt(Z_re_exp.^2 + Z_im_exp.^2); + Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); Module_Z = Module_Z(:); - err_re = (Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); - err_im = (Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); + err_im = (feis.Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); v = sum(err_re.^2 + err_im.^2); if nargout > 1 - w = omega(:); + w = feis.omega(:); R0 = p(1); R1 = p(2); C1 = p(3); @@ -151,7 +164,7 @@ function GiveResults(params0, scales, Z_re_exp, Z_im_exp, omega) g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); - g_norm = g_true .* scales(:); + g_norm = g_true .* feis.scales(:); end end From 2eca284801688b7607726248588ecdbbf7b01ad9 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 13:53:59 +0200 Subject: [PATCH 019/119] modif --- Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m | 2 -- 1 file changed, 2 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m index 19e8c9e9b..47af8a49a 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m @@ -26,8 +26,6 @@ function [min_value, best_params, history] = optimizationBFGS(feis) - - f_opt = @(p_norm) feis.optifunc(p_norm.* feis.scales) ; params0_norm = feis.params0 ./ feis.scales; From d31ee97300138e702ba3049d4ea6de6879dd0e15 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 14:08:50 +0200 Subject: [PATCH 020/119] commentaire --- Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m | 1 + 1 file changed, 1 insertion(+) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m index 47af8a49a..0b2141e7a 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m @@ -6,6 +6,7 @@ Z_im_exp omega scales + %commentaire best_params_found = [] fitting_error = [] From 0a1441d6b269ad84d298a1c49445e109dea3f002 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 14:09:44 +0200 Subject: [PATCH 021/119] 2 --- Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m | 2 +- 1 file changed, 1 insertion(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m index 0b2141e7a..b5895944c 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m @@ -6,7 +6,7 @@ Z_im_exp omega scales - %commentaire + %commentaire2 best_params_found = [] fitting_error = [] From d4a46f9a72eddbc09c6991251dc9a118b4cee59e Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 14:13:51 +0200 Subject: [PATCH 022/119] run file added --- .../spectral_analysis/runclassfitting.m | 14 ++++++++++++++ 1 file changed, 14 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m new file mode 100644 index 000000000..091800ff4 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -0,0 +1,14 @@ +params0 = [3e-3, 0.00260, 100, 0.00132, 1]; + + +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(); + +scales = [10e-2, 10e-3, 15000, 10e-3, 5]; + +feis = fitting_eis(params0, scales, Z_re_exp, Z_im_exp, omega); + +fitting_eis.optimizationBFGS(feis); + +fitting_eis.plotresults(feis); + +fitting_eis.GiveResults(feis); \ No newline at end of file From 037c138c88ebf932f8c345d91c31d3527755820e Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 6 May 2026 14:10:34 +0200 Subject: [PATCH 023/119] renamed file --- .../spectral_analysis/{fitting_eis.m => FittingEIS.m} | 0 1 file changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/spectral_analysis/{fitting_eis.m => FittingEIS.m} (100%) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/fitting_eis.m rename to Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m From c8edd2d133fa5c619ba035836710a75141c05222 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 6 May 2026 14:17:35 +0200 Subject: [PATCH 024/119] some updates --- .../spectral_analysis/FittingEIS.m | 21 ++++++++++--------- 1 file changed, 11 insertions(+), 10 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index b5895944c..3b464ab3b 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -1,4 +1,4 @@ -classdef fitting_eis < handle +classdef FittingEIS < handle properties params0 @@ -6,22 +6,23 @@ Z_im_exp omega scales - %commentaire2 best_params_found = [] fitting_error = [] + end methods - function feis = fitting_eis(params0, scales, Z_re_exp, Z_im_exp, omega) - feis.params0 = params0(:); - feis.scales = scales(:); - feis.Z_re_exp = Z_re_exp(:); - feis.Z_im_exp = Z_im_exp(:); - feis.omega = omega(:); + function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) + + feis.params0 = params0; + feis.scales = scales; + feis.Z_re_exp = Z_re_exp; + feis.Z_im_exp = Z_im_exp; + feis.omega = omega; end @@ -48,10 +49,10 @@ feis.best_params_found = best_params; [feis.fitting_error, ~] = feis.optifunc(best_params); - end function plotresults(feis) + if isempty(feis.best_params_found) feis.optimizationBFGS(); end @@ -168,4 +169,4 @@ function GiveResults(feis) end end -end \ No newline at end of file +end From f226093427ba1a8a3e6e500c1aec5378c5e02580 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 6 May 2026 14:30:59 +0200 Subject: [PATCH 025/119] added filename input in load_experimental_data --- .../spectral_analysis/load_experimental_data.m | 7 ++++--- 1 file changed, 4 insertions(+), 3 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m index 604eec019..1dc719fc4 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m @@ -1,6 +1,7 @@ -function [Z_real, Z_imag, omega] = load_experimental_data() +function [Z_real, Z_imag, omega] = load_experimental_data(filename) + % --- 1. Configuration et Importation des données --- - filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; + % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; % Le délimiteur est la tabulation ('\t') opts = detectImportOptions(filename, 'Delimiter', '\t'); @@ -32,4 +33,4 @@ Z_imag = Z_imag(:); omega = omega(:); -end \ No newline at end of file +end From 68ae254f7734bf2aa7c8acd02a492a399f4e527e Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 6 May 2026 14:31:12 +0200 Subject: [PATCH 026/119] some changes runclassfitting --- .../spectral_analysis/runclassfitting.m | 12 +++++++----- 1 file changed, 7 insertions(+), 5 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 091800ff4..b45557b4d 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -1,14 +1,16 @@ params0 = [3e-3, 0.00260, 100, 0.00132, 1]; +filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; +% filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; -[Z_re_exp, Z_im_exp, omega] = load_experimental_data(); +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); scales = [10e-2, 10e-3, 15000, 10e-3, 5]; -feis = fitting_eis(params0, scales, Z_re_exp, Z_im_exp, omega); +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); -fitting_eis.optimizationBFGS(feis); +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); -fitting_eis.plotresults(feis); +feis.plotresults(best_params, fitting_error); -fitting_eis.GiveResults(feis); \ No newline at end of file +feis.printResults(best_params, fitting_error); From 96f329a6f334b2ca8e3987561bffa8c036cc8190 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 6 May 2026 14:31:23 +0200 Subject: [PATCH 027/119] some clean-up in FittingEIS --- .../spectral_analysis/FittingEIS.m | 87 ++++++++----------- 1 file changed, 37 insertions(+), 50 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 3b464ab3b..79e94ca98 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -1,14 +1,14 @@ -classdef FittingEIS < handle +classdef FittingEIS properties - params0 - Z_re_exp - Z_im_exp - omega - scales - - best_params_found = [] - fitting_error = [] + params0 + Z_re_exp + Z_im_exp + omega + scales + + % best_params_found = [] + % fitting_error = [] end @@ -23,10 +23,11 @@ feis.Z_re_exp = Z_re_exp; feis.Z_im_exp = Z_im_exp; feis.omega = omega; + end - function [min_value, best_params, history] = optimizationBFGS(feis) + function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) f_opt = @(p_norm) feis.optifunc(p_norm.* feis.scales) ; @@ -43,21 +44,16 @@ 'maxIt', 300, ... 'objChangeTol', 1e-6, ... 'gradTol', 1e-5 ... - ); + ); best_params = best_params_norm(:) .* feis.scales(:); - feis.best_params_found = best_params; - [feis.fitting_error, ~] = feis.optifunc(best_params); - + fitting_error = feis.optifunc(best_params); + end - function plotresults(feis) + function plotresults(feis, best_params, fitting_error) - if isempty(feis.best_params_found) - feis.optimizationBFGS(); - end - - [Z_re_fit, Z_im_fit] = load_nyquist(feis.best_params_found, feis.omega); + [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); figure; subplot(3,1,1); @@ -90,39 +86,33 @@ function plotresults(feis) grid on; - text_error = sprintf('Fitting error : %.2e', feis.fitting_error); + text_error = sprintf('Fitting error : %.2e', fitting_error); subplot(3,1,3); text(0.05, 0.90, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); end - function GiveResults(feis) - if isempty(feis.best_params_found) - feis.optimizationBFGS(); - end - + function printResults(feis, best_params, fitting_error) fprintf('\n=== FITTING SCORE ===\n'); - fprintf('Error : %e\n', feis.fitting_error); + fprintf('Error : %e\n', fitting_error); fprintf('\n=== PARAMETERS FOUND ===\n'); - fprintf('R0 = %.5f Ohms\n', feis.best_params_found(1)); - fprintf('R1 = %.5f Ohms\n', feis.best_params_found(2)); - fprintf('C1 = %.1f Farads\n', feis.best_params_found(3)); - fprintf('R2 = %.5f Ohms\n', feis.best_params_found(4)); - fprintf('C2 = %.1f Farads\n', feis.best_params_found(5)); + fprintf('R0 = %.5f Ohms\n', best_params(1)); + fprintf('R1 = %.5f Ohms\n', best_params(2)); + fprintf('C1 = %.1f Farads\n', best_params(3)); + fprintf('R2 = %.5f Ohms\n', best_params(4)); + fprintf('C2 = %.1f Farads\n', best_params(5)); - end - function [v, g_norm] = optifunc(feis, p) - + [Z_re_param, Z_Im_param] = load_nyquist(p, feis.omega); Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); @@ -132,26 +122,24 @@ function GiveResults(feis) err_im = (feis.Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); v = sum(err_re.^2 + err_im.^2); - - - if nargout > 1 + + if nargout > 1 + w = feis.omega(:); R0 = p(1); R1 = p(2); C1 = p(3); R2 = p(4); C2 = p(5); - - + g_re_dR0 = -ones(size(w)); g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; g_re_dC1 = (2*C1*R1^3.*w.^2) ./ (1+(R1*C1.*w).^2).^2; g_re_dR2 = -(1-(R2*C2.*w).^2) ./ (1+(R2*C2.*w).^2).^2; g_re_dC2 = (2*C2*R2^3.*w.^2) ./ (1+(R2*C2.*w).^2).^2; - + J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; - g_im_dR0 = zeros(size(w)); g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; @@ -161,12 +149,11 @@ function GiveResults(feis) J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; derr_re_dp = J_re ./ Module_Z; derr_im_dp = J_im ./ Module_Z; - - + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); g_norm = g_true .* feis.scales(:); + + end end - end - end end From 5318a926712408535880379e0d4cbf7f8a6d27cc Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 6 May 2026 16:50:41 +0200 Subject: [PATCH 028/119] class efficient --- .../spectral_analysis/FittingEIS.m | 45 +++- .../spectral_analysis/LimitedMemoryHessian.m | 217 ++++++++++++++++++ .../spectral_analysis/argmaxCubic.m | 66 ++++++ .../spectral_analysis/lineSearch.m | 147 ++++++++++++ .../spectral_analysis/runclassfitting.m | 2 +- 5 files changed, 468 insertions(+), 9 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 79e94ca98..097b74dfc 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -18,12 +18,26 @@ function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) - feis.params0 = params0; - feis.scales = scales; - feis.Z_re_exp = Z_re_exp; - feis.Z_im_exp = Z_im_exp; - feis.omega = omega; - + % feis.params0 = params0; + % feis.scales = scales; + % feis.Z_re_exp = Z_re_exp; + % feis.Z_im_exp = Z_im_exp; + % feis.omega = omega; + + + if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end + if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end + if istable(omega), omega = table2array(omega); end + if istable(params0), params0 = table2array(params0); end + if istable(scales), scales = table2array(scales); end + + % Everything has to be "double" and colon (:) + feis.params0 = double(params0(:)); + feis.scales = double(scales(:)); + feis.Z_re_exp= double(Z_re_exp(:)); + feis.Z_im_exp= double(Z_im_exp(:)); + feis.omega = double(omega(:)); + end @@ -113,13 +127,28 @@ function printResults(feis, best_params, fitting_error) function [v, g_norm] = optifunc(feis, p) - [Z_re_param, Z_Im_param] = load_nyquist(p, feis.omega); + [Z_re_param, Z_im_param] = load_nyquist(p, feis.omega); + + + if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end + if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end + + + Z_re_param = double(Z_re_param(:)); + Z_im_param = double(Z_im_param(:)); + + + if ~isnumeric(Z_re_param) || ~isreal(Z_re_param) || any(isnan(Z_re_param(:))) + v = 1e10; + g_norm = zeros(5,1); + return; + end Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); Module_Z = Module_Z(:); err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); - err_im = (feis.Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Module_Z(:); v = sum(err_re.^2 + err_im.^2); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m b/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m new file mode 100644 index 000000000..b181be464 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m @@ -0,0 +1,217 @@ +classdef LimitedMemoryHessian +% LimitedMemoryHessian: simple implementation of limited memory +% approxiamtion of invere Hessian (for use in L-BFGS) +% see: unitBoxBFGS (option limitedMemory) +properties + initScale % scaling for H0 (defualt 1) + initStrategy % 'static' : H0k = H0 (default) + % 'dynamic': H0k = gamma_k*I + nullspace = []; % nullspace of active subspace +end +properties (SetAccess = private) + m % number of vectors stored (default 5) + S = []; % m recent control/param diffs + Y = []; % m recent gradient diffs + itCount = 0; % update iteration count + sign % sign of Hessian(default 1) +end + +methods + function H = LimitedMemoryHessian(varargin) + opt = struct('initScale', 1, ... + 'initStrategy', 'static', ... + 'm', 5, ... + 'sign', 1); + opt = merge_options(opt, varargin{:}); + fn = fieldnames(opt); + for k = 1:numel(fn) + H.(fn{k}) = opt.(fn{k}); + end + end + % --------------------------------------------------------------------- + + function H = update(H, s ,y) + % store new vectors + H.itCount = H.itCount +1; + pix = ':'; + if H.itCount > H.m + pix = 2:H.m; + end + H.S = [H.S(:, pix), s]; + H.Y = [H.Y(:, pix), y]; + if H.itCount == 1 % limit m to number of vars + if H.m > numel(s) + H.m = numel(s); + dispif(mrstVerbose, 'Resetting ''m'' to number of parameters (%d)\n', H.m); + end + end + end + + % --------------------------------------------------------------------- + function H = reset(H) + [H.S, H.Y] = deal([]); + H.itCount = 0; + H.nullspace = []; + end + + % --------------------------------------------------------------------- + function r = mtimes(H, v) + % apply mulitplication H*v + if isa(v, 'LimitedMemoryHessian') + error('Only right-multiplciation is supported'); + else + if H.itCount == 0 + r = (H.sign*H.initScale)*v; + if ~isempty(H.nullspace) + if islogical(H.nullspace) + r = r.*(~H.nullspace); + else + r = r - H.nullspace*(H.nullspace'*r); + end + end + else + assert(all(size(v)==[size(H.S, 1), 1]), ... + 'Dimension mismatch'); + if isempty(H.nullspace) % do standard L-BFGS + nVec = size(H.S, 2); + [rho, alpha] = deal(nan(1, nVec)); + for k = nVec:-1:1 + rho(k) = 1/(H.S(:,k)'*H.Y(:,k)); + alpha(k) = rho(k)*(H.S(:,k)'*v); + v = v - alpha(k)*H.Y(:,k); + end + r = H.applyInitial(v); + for k = 1:nVec + beta = rho(k)*(H.Y(:,k)'*r); + r = r + (alpha(k)-beta)*H.S(:,k); + end + else % do subspace version + th = H.applyInitial(1); + r = subspaceProd(H.S, H.Y, th, H.nullspace, v); + end + end + end + end + + % --------------------------------------------------------------------- + function H = uminus(H) + H.sign = -H.sign; + end + + % --------------------------------------------------------------------- + function r = applyInitial(H, v) + if strcmp(H.initStrategy, 'static') + r = (H.sign*H.initScale)*v; + elseif strcmp(H.initStrategy, 'dynamic') + [s,y] = deal(H.S(:,end), H.Y(:,end)); + r = ((s'*y)/(y'*y))*v; + else + error('Unknown strategy: %s', H.initStrategy); + end + end + + % --------------------------------------------------------------------- + function H = setNullspace(H, Q) + if nargin < 2 + H.nullspace = []; + else + if H.itCount > 0 && ~islogical(Q) + assert(size(Q,1)==size(H.S, 1), 'Dimension mismatch'); + assert(size(Q,1)>=size(Q,2), ... + 'Number of columns in nullspace matrix exceeds number of rows'); + end + H.nullspace = Q; + end + end + + % --------------------------------------------------------------------- + function M = full(H) + % Create full matrix, only intended for debugging purposes + if H.itCount == 0 + M = H*1; + else + n = size(H.S, 1); + M = zeros(n); + for k = 1:n + ek = zeros(n,1); + ek(k) = 1; + M(:,k) = H*ek; + end + end + end +end +end +% ------------------------------------------------------------------------- +% ------------------------------------------------------------------------- +function r = subspaceProd(S, Y, th, Q, v) +% Perform product restricted to nullspace of Q-colunms, i.e., +% r = Z * (Z'*Hessian*Z)^-1 * Z'*v +% with Z = null(Q') +% Formula from: +% Byrd, R. H., Lu, P., Nocedal, J., & Zhu, C. (1995). +% A limited memory algorithm for bound constrained optimization. +% SIAM Journal on scientific computing, 16(5), 1190-1208. +% +% S : control diffs +% Y : gradient diffs +% th : inverse Hessian scaling +% Q : nullspace of active subspace +% v : vector +if size(Q,1) <= size(Q,2) + % null(Q')=[], return zero; + r = 0*v; +else + n = size(S,2); + W = [Y, S/th]; + tmp = S'*Y; + L = tril(tmp, -1); + D = diag(diag(tmp)); + M = [-D, L'; L, (S'*S)/th]; + % projection onto active subspace (u -> Z*Z'*u) + if islogical(Q) + projSub = @(u)u.*(~Q); + else + projSub = @(u)u-Q*(Q'*u); + end + r = M\(W'*projSub(v)); + r = (eye(2*n) - th*(M\(W'*projSub(W))))\r; + r = projSub(th*v + th^2*(W*r)); +end +end + +%{ +% For reference: +% should be equal to subspaceProd, but at the additional cost of doing null(Q') +Z = null(Q'); +n = size(S,2); +W = [Y, S/th]; +tmp = S'*Y; +L = tril(tmp, -1); +D = diag(diag(tmp)); +M = [-D, L'; L, (S'*S)/th]; +WtZ = W'*Z; +Ztv = Z'*v; +r = M\(WtZ*Ztv); +r = (eye(2*n)-th*(M\(WtZ*WtZ')))\r; +r = th*Ztv + (th^2)*WtZ'*r; +r = Z*r; +%} + +%{ +Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. + +This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). + +MRST is free software: you can redistribute it and/or modify +it under the terms of the GNU General Public License as published by +the Free Software Foundation, either version 3 of the License, or +(at your option) any later version. + +MRST is distributed in the hope that it will be useful, +but WITHOUT ANY WARRANTY; without even the implied warranty of +MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the +GNU General Public License for more details. + +You should have received a copy of the GNU General Public License +along with MRST. If not, see . +%} diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m b/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m new file mode 100644 index 000000000..3903d6d30 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m @@ -0,0 +1,66 @@ +function [xOpt, poly] = argmaxCubic(p1, p2) +% find max of cubic polynomial through p1, p2 +% shift values: +%{ +Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. + +This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). + +MRST is free software: you can redistribute it and/or modify +it under the terms of the GNU General Public License as published by +the Free Software Foundation, either version 3 of the License, or +(at your option) any later version. + +MRST is distributed in the hope that it will be useful, +but WITHOUT ANY WARRANTY; without even the implied warranty of +MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the +GNU General Public License for more details. + +You should have received a copy of the GNU General Public License +along with MRST. If not, see . +%} +shift = p1.a; +p1.a = 0; +p2.a = p2.a-shift; +poly = zeros(4,1); +poly(3:4) = [p1.dv; p1.v]; +a = p2.a; +poly(1:2) = [a^3, a^2; 3*a^2 2*a]\[p2.v-p1.dv*a-p1.v; p2.dv-p1.dv]; +xe = roots(polyder(poly)); +if numel(xe) == 0 + xe = -inf; +elseif any(imag(xe)~=0) + xe = inf; +elseif xe(1) == xe(end) % single root + if poly(1) ~= 0 + xe = inf; + elseif poly(2) < 0 + xe = xe(1); + else + xe = -inf; + end +else % two roots + [~,ix] = max(polyval(poly,xe)); + xe = xe(ix); + if xe < p1.a + xe = -inf; + end +end +xOpt = xe + shift; + +%-------------------------------------------------------------------------- +% % Uncomment for debugging purposes: +% figure(99), clf, hold on +% x1 = p1.a; x2 = p2.a; +% xi = x1/2:(x2-x1)/50:2*x2; +% plot(xi+shift, polyval(poly, xi)); +% plot(xe+shift, polyval(poly, xe), 'o', 'Markersize', 14, 'MarkerEdgeColor', 'r'); +% plot(p1.a+shift, p1.v, 'o', 'Markersize', 14); +% plot(p2.a+shift, p2.v, 'o', 'Markersize', 14); +% l0 = p1.dv*xi + p1.v -p1.dv*p1.a; +% lx = p2.dv*xi + p2.v -p2.dv*p2.a; +% plot(xi+shift, l0, '--k') +% plot(xi+shift, lx, '--k') +% drawnow +end + diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m b/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m new file mode 100644 index 000000000..9e20938ac --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m @@ -0,0 +1,147 @@ +function [u, v, g, info] = lineSearch(u0, v0, g0, d, f, opt) +% lineSearch -- helper function which performs line search based on +% Wolfe-conditions. +% +% SYNOPSIS: +% [u, v, g, info] = lineSearch(u0, v0, g0, d, f, c, opt) +% +% PARAMETERS: +% u0 : current control vector +% v0 : current objective value +% g0 : current gradient +% d : search direction, returns an error unless d'*g0 > 0 +% f : objective function s.t. [v,g] = f(u) +% c : struct with linear inequality and equality constraints +% opt: struct of parameters for line search +% +% RETURNS: +% u : control vector found along d +% v : objective value for u +% g : gradient for u +% info : struct containing fields: +% flag : 1 for success (Wolfe conditions satisfied) +% -1 max step-length reached without satisfying Wolfe-conds +% -2 line search failed in maxIt iterations (returns most recent +% control without further considerations) +% step : step-length +% nits : number of iterations used + +%{ +Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. + +This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). + +MRST is free software: you can redistribute it and/or modify +it under the terms of the GNU General Public License as published by +the Free Software Foundation, either version 3 of the License, or +(at your option) any later version. + +MRST is distributed in the hope that it will be useful, +but WITHOUT ANY WARRANTY; without even the implied warranty of +MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the +GNU General Public License for more details. + +You should have received a copy of the GNU General Public License +along with MRST. If not, see . +%} +c1 = opt.wolfe1; +c2 = opt.wolfe2; +sgf = opt.safeguardFac; +incTol = opt.stepIncreaseTol; +maxIt = opt.lineSearchMaxIt; +aMax = opt.maxStep; + +% Assert search direction is increasing +assert(d'*g0 <= 0) + +% Define convenience-function to gather info for a "point", where a is the +% step-length, v is the value and dv is the dirctional derivative: +assignPoint = @(a,v,dv)struct('a', a, 'v', v, 'dv', dv); +p0 = assignPoint(0, v0, d'*g0); % 0-point + +% Function handles for wolfe conditions wrt p0 +w1 = @(p) p.v <= p0.v + c1*p.a*p0.dv; +w2 = @(p) abs(p.dv) <= c2*abs(p0.dv); + +% End-points of initial interval +p1 = p0; +p2 = assignPoint(aMax, inf, inf); +% Initial step-length: +a = 1; +lineSearchDone = false; +it = 0; +vals = nan(1, maxIt); +while ~lineSearchDone && it < maxIt + it = it +1; + u = u0 + a*d; + [v, g] = f(u); % function evaluation / simulation + vals(it) = v; + p = assignPoint(a, v, d'*g); % new point + if w1(p) && w2(p) + lineSearchDone = true; + flag = 1; + else + if abs(aMax - p.a) < sqrt(eps) && ... % max step-length reached + (p.v < p0.v) && ... % the step yielded an improvement + (p.dv < 0) % continuing further would improve (but not allowed) + lineSearchDone = true; + flag = -1; + fprintf('Line search at max step size, Wolfe conditions not satisfied for this step.\n'); + else % logic for refining/expanding interval of interest [p1 p2] + if p.a > p2.a + % if we have extrapolated p1.v >= p2.v + [p1, p2] = deal(p2, p); + else + if p.dv >= 0 + p2 = p; + else % keep best + if p1.v <= p2.v + p2 = p; + else + p1 = p; + end + end + end + % Find next candidate-step by interpolation + if p1.v > p2.v && p1.dv >= p2.dv + % Just getting steeper, no need to interpolate + a = inf; + else + a = argmaxCubic(negatePnt(p1), negatePnt(p2)); + end + % Safe-guarding and thresholding: + if a > p2.a + a = max(a, (1+sgf)*p2.a); + a = min(a, min(incTol*p2.a, aMax)); + elseif a > p1.a + a = max(a, p1.a + sgf*(p2.a-p1.a)); + a = min(a, p2.a - sgf*(p2.a-p1.a)); + else + a = (p1.a+p2.a)/2; + fprintf('Cubic interpolation failed, cutting interval in half ...') + end + end + end +end +% Check if line search succeeded +if ~lineSearchDone + flag = -2; + fprintf('Line search unable to succeed in %d iterations ...\n', maxIt); + % Although line search did not succeed in maxIt iterations, we ensure + % to return the greater of p1 and p2's objective value none the less. + if p1.v < p2.v + u = u0 + p1.a*d; + % and we will re-compute the gradients for these controls + [v, g] = f(u); + end +end +info = struct('flag', flag, 'step', a, 'nits', it, 'objVals', vals(1:it)); +end + +function p = negatePnt(p) +[p.v, p.dv] = deal(-p.v, -p.dv); +end + + + + \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index b45557b4d..bb26f8fce 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,7 +5,7 @@ [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -scales = [10e-2, 10e-3, 15000, 10e-3, 5]; +scales = [10e-2, 10e-3, 5000, 100e-3, 50]; feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); From dff9f8ec38e5532067ee234b804847bbaae3b4ca Mon Sep 17 00:00:00 2001 From: Alexandre Date: Thu, 7 May 2026 13:51:35 +0200 Subject: [PATCH 029/119] load more flexible --- .../load_experimental_data.m | 47 +++++++++++++------ 1 file changed, 33 insertions(+), 14 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m index 1dc719fc4..d1d9c0ea5 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m @@ -5,32 +5,51 @@ % Le délimiteur est la tabulation ('\t') opts = detectImportOptions(filename, 'Delimiter', '\t'); + + opts.VariableNamesLine = 1; + opts.DataLine = 2; + opts.VariableNamingRule = 'preserve'; data = readtable(filename, opts); + colNames = data.Properties.VariableNames; + + + idx_real = contains(colNames, 'Re(Z)', 'IgnoreCase', true); + idx_imag = contains(colNames, 'Im(Z)', 'IgnoreCase', true); + idx_freq = contains(colNames, 'freq', 'IgnoreCase', true); - % --- 2. Identification des colonnes --- - % L'impédance réelle est dans Var26 et l'imaginaire dans Var27. - Z_real_raw = data.Var26; - Z_imag_raw = data.Var27; - omega_raw = data.Var16; - % --- 3. Gestion des virgules --- - % On remplace les virgules par des points, puis on convertit le texte en nombres - Z_real = str2double(strrep(Z_real_raw, ',', '.')); - Z_imag = str2double(strrep(Z_imag_raw, ',', '.')); - omega = str2double(strrep(omega_raw, ',', '.')); + % Extraction des données brutes (peu importe où elles se trouvent) + Z_real_raw = data{:, idx_real}; + Z_imag_raw = data{:, idx_imag}; + freq_raw = data{:, idx_freq}; + + if iscell(Z_real_raw) || isstring(Z_real_raw) + Z_real = str2double(strrep(Z_real_raw, ',', '.')); + Z_imag = str2double(strrep(Z_imag_raw, ',', '.')); + freq = str2double(strrep(freq_raw, ',', '.')); + else + Z_real = Z_real_raw; + Z_imag = Z_imag_raw; + freq = freq_raw; + end - % --- 4. Nettoyage des données --- - % S'il y a des lignes de cyclage sans données EIS, on filtre les zéros ou NaN idx_valides = (Z_real ~= 0) & ~isnan(Z_real); Z_real = Z_real(idx_valides); Z_imag = Z_imag(idx_valides); - omega = omega(idx_valides); + freq = freq(idx_valides); Z_real = Z_real(8:60); Z_imag = Z_imag(8:60); - omega = 2*pi*omega(8:60); + omega = 2*pi*freq(8:60); Z_real = Z_real(:); Z_imag = Z_imag(:); omega = omega(:); +%% Figure test + % figure; + % semilogx(omega, Z_real, 'ro', 'MarkerFaceColor', 'r'); + % % legend('Expérimental', 'Modèle (Fitted)'); + % title('Fitting results'); + % xlabel('Omega'); + % ylabel('Z_{re} '); end From 2de7702b971c289319e1a207a9be634c6c85a7a6 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 11 May 2026 10:56:27 +0200 Subject: [PATCH 030/119] runImpedance working --- Examples/Advanced/Impedance/runImpedanceScript.m | 4 ++-- Utilities/FunctionInterface/NamedFunction.m | 1 - 2 files changed, 2 insertions(+), 3 deletions(-) diff --git a/Examples/Advanced/Impedance/runImpedanceScript.m b/Examples/Advanced/Impedance/runImpedanceScript.m index c91a2c43f..706dcfcf8 100644 --- a/Examples/Advanced/Impedance/runImpedanceScript.m +++ b/Examples/Advanced/Impedance/runImpedanceScript.m @@ -2,8 +2,8 @@ close all mrstModule add ad-core mrst-gui mpfa agmg linearsolvers - -jsonstruct = parseBattmoJson(fullfile('ParameterData','BatteryCellParameters','LithiumIonBatteryCell','lithium_ion_battery_nmc_graphite.json')); +addpath('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-eis'); +jsonstruct = parseBattmoJson('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-eis\jp3-opt-1d-full.json'); % We define some shorthand names for simplicity. ne = 'NegativeElectrode'; diff --git a/Utilities/FunctionInterface/NamedFunction.m b/Utilities/FunctionInterface/NamedFunction.m index 1918c35ec..2bc75df9f 100644 --- a/Utilities/FunctionInterface/NamedFunction.m +++ b/Utilities/FunctionInterface/NamedFunction.m @@ -20,7 +20,6 @@ fdnames = {'functionName'}; fn = dispatchParams(fn, jsonstruct, fdnames); - fn.functionHandler = str2func(fn.functionName); end From ff7c9a7ae1c4f36ab05e683f3ed1bafada0a72d6 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 12 May 2026 14:05:34 +0200 Subject: [PATCH 031/119] Comparison with Ank's experimental data --- .../Advanced/Impedance/runImpedanceScript.m | 74 +++++++++++++++++-- 1 file changed, 69 insertions(+), 5 deletions(-) diff --git a/Examples/Advanced/Impedance/runImpedanceScript.m b/Examples/Advanced/Impedance/runImpedanceScript.m index 706dcfcf8..65aa1c1c4 100644 --- a/Examples/Advanced/Impedance/runImpedanceScript.m +++ b/Examples/Advanced/Impedance/runImpedanceScript.m @@ -3,7 +3,9 @@ mrstModule add ad-core mrst-gui mpfa agmg linearsolvers addpath('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-eis'); -jsonstruct = parseBattmoJson('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-eis\jp3-opt-1d-full.json'); + +filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\2026-alexandre-fichter\jp3-eis\jp3-opt-1d-full.json'; +jsonstruct = parseBattmoJson(filename); % We define some shorthand names for simplicity. ne = 'NegativeElectrode'; @@ -27,23 +29,85 @@ set(0, 'defaultlinelinewidth', 3); + +params0 = [3e-3, 0.00260, 100, 0.00132, 1]; + +filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; +% filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; + +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); + +scales = [10e-2, 10e-3, 5000, 100e-3, 50]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + +%% Comparison with Ank's experimental data + figure + + +subplot(3,1,1); +legtxt = sprintf('exp data'); +semilogx(feis.omega, feis.Z_re_exp,'r', 'displayname', legtxt); +hold on; +legtxt = sprintf('fitted data'); +semilogx(feis.omega, Z_re_fit, 'b', 'displayname', legtxt); +xlabel('Omega'); +ylabel('Z_{re} '); + +subplot(3,1,2); +legtxt = sprintf('exp data'); +semilogx(feis.omega, feis.Z_im_exp, 'r', 'displayname', legtxt); +hold on; +legtxt = sprintf('fitted data'); +semilogx(feis.omega, Z_im_fit, 'b', 'displayname', legtxt); +xlabel('Omega'); +ylabel('-Z_{im} '); + +subplot(3,1,3); +legtxt = sprintf('exp data'); +plot(feis.Z_re_exp, feis.Z_im_exp, 'r', 'displayname', legtxt); +hold on; +legtxt = sprintf('fitted data'); +plot(feis.Z_re_exp, Z_im_fit, 'b', 'displayname', legtxt); +axis equal; + + + + hold on -socs = linspace(0.1, 1, 5); +socs = linspace(0.1, 1, 2); -for isoc = 1 : numel(socs) +socs = [socs, 0.2]; +for isoc = 1 : numel(socs) soc = socs(isoc); impsolv = ImpedanceSolver(inputparams, 'soc', soc, 'computeSteadyState', false); - omegas = linspace(-3, 6, 500); + omegas = linspace(-2, 4, 500); omegas = 10.^omegas; Z = impsolv.computeImpedance(omegas); - Z = (Z*gen.faceArea)/((centi*meter)^2); + % Z = (Z*gen.faceArea)/((centi*meter)^2); + Z = (Z*gen.faceArea); + + subplot(3,1,1); + legtxt = sprintf('SOC=%g', soc); + semilogx(omegas, real(Z), 'displayname', legtxt); + + + subplot(3,1,2); + legtxt = sprintf('SOC=%g', soc); + semilogx(omegas, -imag(Z), 'displayname', legtxt); + + subplot(3,1,3); legtxt = sprintf('SOC=%g', soc); plot(real(Z), -imag(Z), 'displayname', legtxt); xlabel('real(Z) / Ωcm^2') From d3c3de3e239b74048673b9bb70e5c7fcf99db5c9 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 13 May 2026 11:38:26 +0200 Subject: [PATCH 032/119] first try to fit an ecm circuit with chen data --- .../spectral_analysis/FittingEIS.m | 56 +++++++++---------- .../spectral_analysis/load_chen_data.m | 51 +++++++++++++++++ .../spectral_analysis/plot_nyquist_params.m | 4 +- .../spectral_analysis/runclassfitting.m | 13 +++-- .../Advanced/Impedance/runImpedanceChen.m | 21 +++++-- 5 files changed, 107 insertions(+), 38 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 097b74dfc..b2c510dbf 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -18,25 +18,25 @@ function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) - % feis.params0 = params0; - % feis.scales = scales; - % feis.Z_re_exp = Z_re_exp; - % feis.Z_im_exp = Z_im_exp; - % feis.omega = omega; - - - if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end - if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end - if istable(omega), omega = table2array(omega); end - if istable(params0), params0 = table2array(params0); end - if istable(scales), scales = table2array(scales); end - - % Everything has to be "double" and colon (:) - feis.params0 = double(params0(:)); - feis.scales = double(scales(:)); - feis.Z_re_exp= double(Z_re_exp(:)); - feis.Z_im_exp= double(Z_im_exp(:)); - feis.omega = double(omega(:)); + feis.params0 = params0; + feis.scales = scales; + feis.Z_re_exp = Z_re_exp; + feis.Z_im_exp = Z_im_exp; + feis.omega = omega; + + + % if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end + % if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end + % if istable(omega), omega = table2array(omega); end + % if istable(params0), params0 = table2array(params0); end + % if istable(scales), scales = table2array(scales); end + % + % % Everything has to be "double" and colon (:) + % feis.params0 = double(params0(:)); + % feis.scales = double(scales(:)); + % feis.Z_re_exp= double(Z_re_exp(:)); + % feis.Z_im_exp= double(Z_im_exp(:)); + % feis.omega = double(omega(:)); end @@ -71,28 +71,28 @@ function plotresults(feis, best_params, fitting_error) figure; subplot(3,1,1); - semilogx(feis.omega, feis.Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); + semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - semilogx(feis.omega, Z_re_fit, 'bo', 'LineWidth', 2); - % legend('Expérimental', 'Modèle (Fitted)'); + semilogx(feis.omega, Z_re_fit, 'b', 'LineWidth', 2); + legend('experience', 'fitted model'); title('Fitting results'); xlabel('Omega'); ylabel('Z_{re} '); subplot(3,1,2); - semilogx(feis.omega, feis.Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + semilogx(feis.omega, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - semilogx(feis.omega, Z_im_fit, 'bo', 'LineWidth', 2); - % legend('Expérimental', 'Modèle (Fitted)'); + semilogx(feis.omega, Z_im_fit, 'b', 'LineWidth', 2); + legend('experience', 'fitted model'); title('Fitting results'); xlabel('Omega'); ylabel('-Z_{im} '); subplot(3,1,3); - plot(feis.Z_re_exp, feis.Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); + plot(feis.Z_re_exp, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - plot(feis.Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); - % legend('Expérimental', 'Modèle (Fitted)'); + plot(feis.Z_re_exp, Z_im_fit, 'b', 'LineWidth', 2); + legend('experience', 'fitted model'); title('Nyquist'); xlabel('Z_{re}'); ylabel('-Z_{im} '); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m new file mode 100644 index 000000000..65617a943 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m @@ -0,0 +1,51 @@ +function [Z_real, Z_imag, omegas] = load_chen_data() + + + % We define some shorthand names for simplicity. + ne = 'NegativeElectrode'; + pe = 'PositiveElectrode'; + elyte = 'Electrolyte'; + thermal = 'ThermalModel'; + co = 'Coating'; + am = 'ActiveMaterial'; + itf = 'Interface'; + sd = 'SolidDiffusion'; + ctrl = 'Control'; + cc = 'CurrentCollector'; + + mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + + jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + + includeDoubleLayer = false; + + if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + + end + + [model, inputparams, ~] = setupModelFromJson(jsonstruct); + + c_ne = 29.866*mol/litre; % initial concentration at negative electrode + c_pe = 17.038*mol/litre; % initial concentration at positive electrode + + initstate = initStateChen2020(model, c_ne, c_pe); + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + + omegas = linspace(-4, 2, 50); + omegas = 10.^omegas; + Z = impsolv.computeImpedance(omegas); + + Z_real = real(Z); + Z_imag = - imag(Z); +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m index 3250ec09d..2afa33f60 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m @@ -2,9 +2,9 @@ % params = [6.2261e-3, 0.3e-3, 10000.1264, 0.00097, 2e5]; % best params % handmade -params = [0.003, 0.00134, 5, 0.00330, 20000] +params = [0.003, 0.00134, 5, 0.00330, 20000]; [Z_re_exp, Z_im_exp, omega] = load_experimental_data(); -omega = logspace(-2, 4, 100) +omega = logspace(-2, 4, 100); [Z_real, Z_imag] = load_nyquist(params, omega) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index bb26f8fce..d12928427 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -1,16 +1,21 @@ -params0 = [3e-3, 0.00260, 100, 0.00132, 1]; -filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; + +% filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; % filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; +% +% [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); + +params0 = [3e-2, 1e-1, 1e2, 1e-2, 1e2]; -[Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); +[Z_re_exp, Z_im_exp, omega] = load_chen_data(); -scales = [10e-2, 10e-3, 5000, 100e-3, 50]; +scales = [1e-1, 1, 1e3, 1e-1, 1000]; feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +%% feis.plotresults(best_params, fitting_error); feis.printResults(best_params, fitting_error); diff --git a/Examples/Advanced/Impedance/runImpedanceChen.m b/Examples/Advanced/Impedance/runImpedanceChen.m index c0bc1ed7d..16a10a49a 100644 --- a/Examples/Advanced/Impedance/runImpedanceChen.m +++ b/Examples/Advanced/Impedance/runImpedanceChen.m @@ -1,6 +1,9 @@ clear all % close all + + + % We define some shorthand names for simplicity. ne = 'NegativeElectrode'; pe = 'PositiveElectrode'; @@ -39,23 +42,33 @@ impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); -%% + + + + + set(0, 'defaultlinelinewidth', 3); + + +figure + + omegas = linspace(-4, 2, 30); omegas = 10.^omegas; Z = impsolv.computeImpedance(omegas); - -figure hold on plot(real(Z), -imag(Z), 'displayname', 'battmo'); +axis equal; + + docompare = true; if docompare p = fileparts(mfilename('fullpath')); - data = load(fullfile(p, 'utils', 'pybamm_chen_impedances.mat')); + data = load('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\matlab\BattMo\Examples\Advanced\Impedance\utils\pybamm_chen_impedances.mat'); Zpybamm = data.impedances; plot(real(Zpybamm), -imag(Zpybamm), 'displayname', 'pybamm'); end From 81ff6914d7752503dcee17f3c0f82e3a7bc7060f Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 13 May 2026 14:50:21 +0200 Subject: [PATCH 033/119] try with lsqnonlin, it works --- .../spectral_analysis/FittingEIS.m | 112 ++++++++++++++++-- .../spectral_analysis/runclassfitting.m | 9 +- .../spectral_analysis/unitBoxBFGS.m | 2 +- 3 files changed, 111 insertions(+), 12 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index b2c510dbf..be5852dc7 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -48,16 +48,28 @@ params0_norm = feis.params0 ./ feis.scales; % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); + + + A_custom = [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)]; + b_custom = 0; + limite_basse = 1e-5; + A_lim = -eye(5); + b_lim = -limite_basse * ones(5, 1); + + A_total = [A_custom; A_lim]; + b_total = [b_custom; b_lim]; + [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... f_opt, ... 'maximize', false, ... - 'linIneq', struct('A', [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)], 'b', 0), ... + 'linIneq', struct('A', A_total, 'b', b_total), ... 'enforceFeasible', true, ... 'maxIt', 300, ... 'objChangeTol', 1e-6, ... - 'gradTol', 1e-5 ... + 'gradTol', 1e-5, ... + 'lineSearchMaxIt', 100 ... ); best_params = best_params_norm(:) .* feis.scales(:); @@ -153,36 +165,120 @@ function printResults(feis, best_params, fitting_error) v = sum(err_re.^2 + err_im.^2); if nargout > 1 - + w = feis.omega(:); R0 = p(1); R1 = p(2); C1 = p(3); R2 = p(4); C2 = p(5); - + g_re_dR0 = -ones(size(w)); g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; g_re_dC1 = (2*C1*R1^3.*w.^2) ./ (1+(R1*C1.*w).^2).^2; g_re_dR2 = -(1-(R2*C2.*w).^2) ./ (1+(R2*C2.*w).^2).^2; g_re_dC2 = (2*C2*R2^3.*w.^2) ./ (1+(R2*C2.*w).^2).^2; - + J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; - + g_im_dR0 = zeros(size(w)); g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; g_im_dR2 = -(2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; - + J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; derr_re_dp = J_re ./ Module_Z; derr_im_dp = J_im ./ Module_Z; - + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); g_norm = g_true .* feis.scales(:); end + + + % finite difference method + % if nargout > 1 + % g_norm = zeros(5,1); + % dp_norm = 1e-6; + % + % for i = 1:5 + % p_perturb = p; + % p_perturb(i) = p_perturb(i) + dp_norm * feis.scales(i); + % + % [Z_re_pert, Z_im_pert] = load_nyquist(p_perturb, feis.omega); + % + % err_re_pert = (feis.Z_re_exp(:) - double(Z_re_pert(:))) ./ Module_Z; + % err_im_pert = (feis.Z_im_exp(:) - double(Z_im_pert(:))) ./ Module_Z; + % + % v_perturb = sum(err_re_pert.^2 + err_im_pert.^2); + % + % g_norm = (v_perturb - v) / dp_norm; + % end + % end + end + + function residuals = optifunc_lsq(feis, p) + % 1. On empêche physiquement les paramètres de valoir zéro + p = max(p, 1e-8); + + % 2. Chargement du modèle + [Z_re_param, Z_im_param] = load_nyquist(p, feis.omega); + if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end + if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end + + Z_re_param = double(Z_re_param(:)); + Z_im_param = double(Z_im_param(:)); + + % Si le modèle renvoie du NaN (physiquement impossible), on pénalise + if ~isnumeric(Z_re_param) || ~isreal(Z_re_param) || any(isnan(Z_re_param(:))) + residuals = 1e10 * ones(2 * length(feis.omega), 1); + return; + end + + % 3. Calcul du module pour l'erreur relative + Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); + Module_Z = Module_Z(:); + + % 4. Vecteurs de résidus (Non mis au carré, lsqnonlin s'en charge) + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Module_Z; + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Module_Z; + + % 5. On empile les parties réelles et imaginaires en un seul vecteur colonne + residuals = [err_re; err_im]; + end + + function [min_value, best_params, resnorm] = optimizationLsqnonlin(feis) + % Fonction objectif : renvoie le vecteur de résidus + f_res = @(p_norm) feis.optifunc_lsq(p_norm(:) .* feis.scales(:)); + + % Paramètres initiaux normés + params0_norm = feis.params0(:) ./ feis.scales(:); + + % Bornes (Limites inférieures strictes > 0 pour éviter les crashs) + lb_norm = ones(5,1) * 1e-5; + ub_norm = inf(5,1); + + % Options de lsqnonlin + options = optimoptions('lsqnonlin', ... + 'Display', 'iter-detailed', ... % Affichage très détaillé + 'Algorithm', 'trust-region-reflective', ... % Parfait pour l'EIS + 'MaxFunctionEvaluations', 3000, ... + 'MaxIterations', 500, ... + 'StepTolerance', 1e-8, ... + 'FunctionTolerance', 1e-6); + + % Lancement de l'optimiseur natif MATLAB + [best_params_norm, resnorm, ~, exitflag, output] = lsqnonlin(... + f_res, params0_norm, lb_norm, ub_norm, options); + + % Récupération des vraies valeurs (dénormalisation) + best_params = best_params_norm(:) .* feis.scales(:); + min_value = resnorm; % Erreur finale (somme des carrés des résidus) + + % Affichage du statut de fin + disp('=== RAISON DE FIN DE LSQNONLIN ==='); + disp(output.message); end end end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index d12928427..e54110310 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,15 +5,18 @@ % % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -params0 = [3e-2, 1e-1, 1e2, 1e-2, 1e2]; +params0 = [3e-2, 1e-1, 3e1, 1e-2, 1e1]; [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -scales = [1e-1, 1, 1e3, 1e-1, 1000]; +scales = [1e-1, 1, 1e2, 1e-1, 1e2]; feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +% [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +%% Lancement avec LSQNONLIN +[min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); %% feis.plotresults(best_params, fitting_error); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m b/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m index d020d1a6f..867264599 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m @@ -284,7 +284,7 @@ This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). else [ix, s] = deal([], 0); end - if ~isempty(ix) && s <= 1+sqrt(eps) + if ~isempty(ix) && s <= 1+sqrt(eps) becomesActive(ix) = true; d = d + s*dr; gr = (1-s)*gr; From e8d3e28a8943343424644a1f7f6be0b5ec809915 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 13 May 2026 17:35:04 +0200 Subject: [PATCH 034/119] nonworking try with unitbox --- .../spectral_analysis/FittingEIS.m | 42 +++++++++---------- .../spectral_analysis/runclassfitting.m | 25 ++++++++--- 2 files changed, 40 insertions(+), 27 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index be5852dc7..3969e5657 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -50,21 +50,15 @@ params0_norm = params0_norm(:); - A_custom = [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)]; + A_custom = [0, 0, 2*feis.scales(3)/feis.scales(5), 0, -1]; b_custom = 0; - limite_basse = 1e-5; - A_lim = -eye(5); - b_lim = -limite_basse * ones(5, 1); - - A_total = [A_custom; A_lim]; - b_total = [b_custom; b_lim]; [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... f_opt, ... 'maximize', false, ... - 'linIneq', struct('A', A_total, 'b', b_total), ... + 'linIneq', struct('A', A_custom, 'b', b_custom), ... 'enforceFeasible', true, ... 'maxIt', 300, ... 'objChangeTol', 1e-6, ... @@ -139,7 +133,11 @@ function printResults(feis, best_params, fitting_error) function [v, g_norm] = optifunc(feis, p) - [Z_re_param, Z_im_param] = load_nyquist(p, feis.omega); + + % Preventing physical values to get too close from 0 + p_safe = max(p, 1e-8); + + [Z_re_param, Z_im_param] = load_nyquist(p_safe, feis.omega); if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end @@ -156,11 +154,11 @@ function printResults(feis, best_params, fitting_error) return; end - Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); - Module_Z = Module_Z(:); + Modulus_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); + Modulus_Z = Modulus_Z(:); - err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); - err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Module_Z(:); + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); v = sum(err_re.^2 + err_im.^2); @@ -188,8 +186,8 @@ function printResults(feis, best_params, fitting_error) g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; - derr_re_dp = J_re ./ Module_Z; - derr_im_dp = J_im ./ Module_Z; + derr_re_dp = J_re ./ Modulus_Z; + derr_im_dp = J_im ./ Modulus_Z; g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); g_norm = g_true .* feis.scales(:); @@ -208,8 +206,8 @@ function printResults(feis, best_params, fitting_error) % % [Z_re_pert, Z_im_pert] = load_nyquist(p_perturb, feis.omega); % - % err_re_pert = (feis.Z_re_exp(:) - double(Z_re_pert(:))) ./ Module_Z; - % err_im_pert = (feis.Z_im_exp(:) - double(Z_im_pert(:))) ./ Module_Z; + % err_re_pert = (feis.Z_re_exp(:) - double(Z_re_pert(:))) ./ Modulus_Z; + % err_im_pert = (feis.Z_im_exp(:) - double(Z_im_pert(:))) ./ Modulus_Z; % % v_perturb = sum(err_re_pert.^2 + err_im_pert.^2); % @@ -237,17 +235,17 @@ function printResults(feis, best_params, fitting_error) end % 3. Calcul du module pour l'erreur relative - Module_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); - Module_Z = Module_Z(:); + Modulus_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); + Modulus_Z = Modulus_Z(:); % 4. Vecteurs de résidus (Non mis au carré, lsqnonlin s'en charge) - err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Module_Z; - err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Module_Z; + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z; + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z; % 5. On empile les parties réelles et imaginaires en un seul vecteur colonne residuals = [err_re; err_im]; end - + function [min_value, best_params, resnorm] = optimizationLsqnonlin(feis) % Fonction objectif : renvoie le vecteur de résidus f_res = @(p_norm) feis.optifunc_lsq(p_norm(:) .* feis.scales(:)); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index e54110310..3167147b7 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,20 +5,35 @@ % % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -params0 = [3e-2, 1e-1, 3e1, 1e-2, 1e1]; +params0 = [3e-2, 1, 1e4, 1e-2, 3e4]; [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -scales = [1e-1, 1, 1e2, 1e-1, 1e2]; +scales = [1e-1, 10, 1e5, 1e-1, 1e5]; feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); -% [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +% % Lancement avec LSQNONLIN +% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); + + +% result with lsqnonlin: +% === FITTING SCORE === +% Error : 7.324871e-02 +% +% === PARAMETERS FOUND === +% R0 = 0.05052 Ohms +% R1 = 1.12673 Ohms +% C1 = 59119.9 Farads +% R2 = 0.03155 Ohms +% C2 = 11054.0 Farads -%% Lancement avec LSQNONLIN -[min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); %% feis.plotresults(best_params, fitting_error); feis.printResults(best_params, fitting_error); + + From d44938412bb28ca0de1568b236c5488464735103 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 19 May 2026 13:30:35 +0200 Subject: [PATCH 035/119] error with chen data lowered --- .../spectral_analysis/FittingEIS.m | 63 ++++++++++--------- .../spectral_analysis/runclassfitting.m | 14 ++--- 2 files changed, 40 insertions(+), 37 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 3969e5657..4b677b770 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -18,25 +18,28 @@ function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) - feis.params0 = params0; - feis.scales = scales; - feis.Z_re_exp = Z_re_exp; - feis.Z_im_exp = Z_im_exp; - feis.omega = omega; - - - % if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end - % if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end - % if istable(omega), omega = table2array(omega); end - % if istable(params0), params0 = table2array(params0); end - % if istable(scales), scales = table2array(scales); end - % - % % Everything has to be "double" and colon (:) - % feis.params0 = double(params0(:)); - % feis.scales = double(scales(:)); - % feis.Z_re_exp= double(Z_re_exp(:)); - % feis.Z_im_exp= double(Z_im_exp(:)); - % feis.omega = double(omega(:)); + % feis.params0 = params0; + % feis.scales = scales; + % feis.Z_re_exp = Z_re_exp; + % feis.Z_im_exp = Z_im_exp; + % feis.omega = omega; + + + if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end + if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end + if istable(omega), omega = table2array(omega); end + if istable(params0), params0 = table2array(params0); end + if istable(scales), scales = table2array(scales); end + + % Everything has to be "double" and colon (:) + feis.params0 = double(params0(:)); + feis.scales = double(scales(:)); + feis.Z_re_exp= double(Z_re_exp(:)); + feis.Z_im_exp= double(Z_im_exp(:)); + feis.omega = double(omega(:)); + + %pb here because the way I take exp data changes a lot the + %result... end @@ -50,7 +53,7 @@ params0_norm = params0_norm(:); - A_custom = [0, 0, 2*feis.scales(3)/feis.scales(5), 0, -1]; + A_custom = [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)]; b_custom = 0; @@ -58,7 +61,7 @@ params0_norm, ... f_opt, ... 'maximize', false, ... - 'linIneq', struct('A', A_custom, 'b', b_custom), ... + 'linIneq', struct('A', A_custom, 'b', b_custom), ... %A*u<=b 'enforceFeasible', true, ... 'maxIt', 300, ... 'objChangeTol', 1e-6, ... @@ -79,7 +82,7 @@ function plotresults(feis, best_params, fitting_error) subplot(3,1,1); semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - semilogx(feis.omega, Z_re_fit, 'b', 'LineWidth', 2); + semilogx(feis.omega, Z_re_fit, 'b'); legend('experience', 'fitted model'); title('Fitting results'); xlabel('Omega'); @@ -88,7 +91,7 @@ function plotresults(feis, best_params, fitting_error) subplot(3,1,2); semilogx(feis.omega, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - semilogx(feis.omega, Z_im_fit, 'b', 'LineWidth', 2); + semilogx(feis.omega, Z_im_fit, 'b'); legend('experience', 'fitted model'); title('Fitting results'); xlabel('Omega'); @@ -97,7 +100,7 @@ function plotresults(feis, best_params, fitting_error) subplot(3,1,3); plot(feis.Z_re_exp, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); hold on; - plot(feis.Z_re_exp, Z_im_fit, 'b', 'LineWidth', 2); + plot(feis.Z_re_exp, Z_im_fit, 'b'); legend('experience', 'fitted model'); title('Nyquist'); xlabel('Z_{re}'); @@ -165,11 +168,11 @@ function printResults(feis, best_params, fitting_error) if nargout > 1 w = feis.omega(:); - R0 = p(1); - R1 = p(2); - C1 = p(3); - R2 = p(4); - C2 = p(5); + R0 = p_safe(1); + R1 = p_safe(2); + C1 = p_safe(3); + R2 = p_safe(4); + C2 = p_safe(5); g_re_dR0 = -ones(size(w)); g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; @@ -255,7 +258,7 @@ function printResults(feis, best_params, fitting_error) % Bornes (Limites inférieures strictes > 0 pour éviter les crashs) lb_norm = ones(5,1) * 1e-5; - ub_norm = inf(5,1); + ub_norm = ones(5,1) * 1e5./ feis.scales(:); % Options de lsqnonlin options = optimoptions('lsqnonlin', ... diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 3167147b7..8b0df6ccd 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,18 +5,18 @@ % % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -params0 = [3e-2, 1, 1e4, 1e-2, 3e4]; +params0 = [3e-2, 1, 3e3, 1e-1, 1e3]; [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -scales = [1e-1, 10, 1e5, 1e-1, 1e5]; +scales = [1e-1, 1e1, 1e5, 1e0, 1e5]; -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +% feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); +% +% [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); -% % Lancement avec LSQNONLIN -% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); +% Lancement avec LSQNONLIN +[min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); % result with lsqnonlin: From aed07b6480a094f605a987412528b98787766e54 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Fri, 29 May 2026 17:08:56 +0200 Subject: [PATCH 036/119] beginning of change with scales, all programs _impact --- .../spectral_analysis/FittingEIS.m | 341 ++++++++++++++---- .../spectral_analysis/load_chen_data.m | 2 +- .../spectral_analysis/load_nyquist.m | 4 +- .../spectral_analysis/load_santoni_data.m | 12 + .../activationEnergyOfReaction_impact.m | 48 +++ .../pxdparams_impact/bruggeman_impact.m | 46 +++ .../electronicConductivity_impact.m | 46 +++ .../pxdparams_impact/param_dependency.m | 88 +++++ .../pxdparams_impact/porosity_impact.m | 45 +++ .../reactionRateConstant_impact.m | 47 +++ .../referenceDiffusionCoefficient_impact.m | 46 +++ .../saturationConcentration_impact.m | 47 +++ .../pxdparams_impact/volumefraction_impact.m | 46 +++ .../volumetricSurfaceArea_impact.m | 47 +++ .../spectral_analysis/runclassfitting.m | 45 ++- .../Advanced/Impedance/runImpedanceChen.m | 3 +- 16 files changed, 831 insertions(+), 82 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 4b677b770..67877839e 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -16,6 +16,7 @@ methods + function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) % feis.params0 = params0; @@ -43,12 +44,22 @@ end + function p_norm = unscaled2scaled(feis, p) + p_norm = (p-feis.params0./feis.scales)./(feis.scales*feis.params0-feis.params0/feis.scales); + end + + function p = scaled2unscaled(feis, p_norm) + a = feis.scales; + p0 = feis.params0; + p = (a*p0-p0/a).*p_norm +p0/a; + end + function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) - f_opt = @(p_norm) feis.optifunc(p_norm.* feis.scales) ; + f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm)) ; - params0_norm = feis.params0 ./ feis.scales; + params0_norm = unscaled2scaled(feis, feis.params0); % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); @@ -68,71 +79,13 @@ 'gradTol', 1e-5, ... 'lineSearchMaxIt', 100 ... ); - best_params = best_params_norm(:) .* feis.scales(:); + best_params = scaled2unscaled(feis, best_params_norm(:) ); fitting_error = feis.optifunc(best_params); end - function plotresults(feis, best_params, fitting_error) - - [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); - - figure; - subplot(3,1,1); - semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - semilogx(feis.omega, Z_re_fit, 'b'); - legend('experience', 'fitted model'); - title('Fitting results'); - xlabel('Omega'); - ylabel('Z_{re} '); - - subplot(3,1,2); - semilogx(feis.omega, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - semilogx(feis.omega, Z_im_fit, 'b'); - legend('experience', 'fitted model'); - title('Fitting results'); - xlabel('Omega'); - ylabel('-Z_{im} '); - - subplot(3,1,3); - plot(feis.Z_re_exp, feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - plot(feis.Z_re_exp, Z_im_fit, 'b'); - legend('experience', 'fitted model'); - title('Nyquist'); - xlabel('Z_{re}'); - ylabel('-Z_{im} '); - axis equal; - - grid on; - - text_error = sprintf('Fitting error : %.2e', fitting_error); - - subplot(3,1,3); - - text(0.05, 0.90, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); - end - - function printResults(feis, best_params, fitting_error) - - fprintf('\n=== FITTING SCORE ===\n'); - fprintf('Error : %e\n', fitting_error); - - fprintf('\n=== PARAMETERS FOUND ===\n'); - fprintf('R0 = %.5f Ohms\n', best_params(1)); - fprintf('R1 = %.5f Ohms\n', best_params(2)); - fprintf('C1 = %.1f Farads\n', best_params(3)); - fprintf('R2 = %.5f Ohms\n', best_params(4)); - fprintf('C2 = %.1f Farads\n', best_params(5)); - - end + function [v, g_norm] = optifunc(feis, p) @@ -193,7 +146,7 @@ function printResults(feis, best_params, fitting_error) derr_im_dp = J_im ./ Modulus_Z; g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); - g_norm = g_true .* feis.scales(:); + g_norm = unscaled2scaled(feis, g_true); end @@ -219,6 +172,119 @@ function printResults(feis, best_params, fitting_error) % end end +%% Warburg Model + + function [min_value, history, best_params, fitting_error] = optimizationBFGS_warburg(feis) + + f_opt = @(p_norm) feis.optifunc_warburg(p_norm.* feis.scales) ; + + params0_norm = feis.params0 ./ feis.scales; + params0_norm = params0_norm(:); + + + + [min_value, best_params_norm, history] = unitBoxBFGS(... + params0_norm, ... + f_opt, ... + 'maximize', false, ... + 'enforceFeasible', true, ... + 'maxIt', 300, ... + 'objChangeTol', 1e-6, ... + 'gradTol', 1e-5, ... + 'lineSearchMaxIt', 200 ... + ); + best_params = best_params_norm(:) .* feis.scales(:); + + fitting_error = feis.optifunc_warburg(best_params); + + end + + function [v, g_norm] = optifunc_warburg(feis, p) + + % Preventing physical values to get too close from 0 + p_safe = max(p, 1e-7); + + + w = feis.omega(:); + R0 = p_safe(1); + R1 = p_safe(2); + Q1 = p_safe(3); + a1 = p_safe(4); + R2 = p_safe(5); + Q2 = p_safe(6); + a2 = p_safe(7); + Q = p_safe(8); + L = p_safe(9); + + s = 1i .* w; + s = s(:); + + sa1 = s.^a1; + sa2 = s.^a2; + + Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); + + Z_re_param = real(Z_param_cplx); + Z_im_param = imag(Z_param_cplx); + + if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end + if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end + + + Z_re_param = double(Z_re_param(:)); + Z_im_param = double(Z_im_param(:)); + + Modulus_Z = sqrt(Z_re_param.^2 + Z_im_param.^2); + Modulus_Z = Modulus_Z(:); + + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); + + v = sum(err_re.^2 + err_im.^2); + + + if nargout > 1 + + den1 = (1 + R1 .* Q1 .* sa1).^2; + den2 = (1 + R2 .* Q2 .* sa2).^2; + + + dZ_dR0 = ones(size(s)); % R0 + dZ_dR1 = 1 ./ den1; % R1 + dZ_dR2 = 1 ./ den2; % R2 + + dZ_dQ1 = - (R1^2 .* sa1) ./ den1; % Q1 + dZ_dQ2 = - (R2^2 .* sa2) ./ den2; % Q2 + + dZ_da1 = - (Q1 * R1^2 .* sa1 .* log(s)) ./ den1; % a1 + dZ_da2 = - (Q2 * R2^2 .* sa2 .* log(s)) ./ den2; % a2 + + dZ_dQ = - 1 ./ (Q^2 .* (s.^0.5)); % Q + dZ_dL = s; % L + + J = [dZ_dR0, dZ_dR1, dZ_dQ1, dZ_da1, dZ_dR2, dZ_dQ2, dZ_da2, dZ_dQ, dZ_dL]; + + J_im = imag(J); + J_re = real(J); + + derr_re_dp = -J_re ./ Modulus_Z; + derr_im_dp = -J_im ./ Modulus_Z; + + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); + g_norm = g_true .* feis.scales(:); + + + if any(isinf(g_norm)) || any(isnan(g_norm)) || isinf(v) || isnan(v) v = 1e10; + g_norm = zeros(9,1); + return; + end + end + end + + + + %% lsq method + function residuals = optifunc_lsq(feis, p) % 1. On empêche physiquement les paramètres de valoir zéro p = max(p, 1e-8); @@ -281,5 +347,154 @@ function printResults(feis, best_params, fitting_error) disp('=== RAISON DE FIN DE LSQNONLIN ==='); disp(output.message); end + +%% lsq method warburg + function v = optifunclsq_warburg(feis, p) + p_safe = max(p, 1e-15); + + R0 = p_safe(1); R1 = p_safe(2); Q1 = p_safe(3); a1 = p_safe(4); + R2 = p_safe(5); Q2 = p_safe(6); a2 = p_safe(7); Q = p_safe(8); L = p_safe(9); + + w = feis.omega(:); + s = 1i .* w; + + sa1 = s.^a1; + sa2 = s.^a2; + Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); + + Z_re_param = real(Z_param_cplx); + Z_im_param = imag(Z_param_cplx); + + if any(isnan(Z_re_param)) || any(isnan(Z_im_param)) || any(isinf(Z_re_param)) || any(isinf(Z_im_param)) + v = 1e6; % Pénalité forte mais gérable + return; + end + + Modulus_Z = sqrt(Z_re_param.^2 + Z_im_param.^2); + Modulus_Z = Modulus_Z(:); + + err_re = (feis.Z_re_exp(:) - Z_re_param) ./ Modulus_Z; + err_im = (feis.Z_im_exp(:) - Z_im_param) ./ Modulus_Z; + + v = sum(err_re.^2 + err_im.^2); + + end + + + function [min_value, history, best_params, fitting_error] = optimizationlsq_warburg(feis) + f_opt = @(p_norm) feis.optifunclsq_warburg(p_norm .* feis.scales); + + params0_norm = feis.params0 ./ feis.scales; + params0_norm = params0_norm(:); + + if length(params0_norm) ~= 9 + error('feis.params0 should have 9 parameters but it has %d).', length(params0_norm)); + end + + lb_norm = [1e-10; 1e-10; 1e-10; 1e-3; 1e-10; 1e-10; 0.01; 1e-5; 1e-15] ./ feis.scales; + ub_norm = [1e5; 1e5; 1e6; 1.0; 1e5; 1e6; 1.0; 1e15; 1e-2 ] ./ feis.scales; + + options = optimoptions('fmincon', ... + 'Display', 'iter', ... + 'Algorithm', 'sqp', ... % Très bon pour ce type de fitting + 'SpecifyObjectiveGradient', false, ... + 'MaxFunctionEvaluations', 10000, ... + 'MaxIterations', 1000); + + [best_params_norm, min_value] = fmincon(f_opt, params0_norm, [], [], [], [], lb_norm, ub_norm, [], options); + + history = []; % Si vous n'en avez pas besoin + best_params = best_params_norm(:) .* feis.scales(:); + fitting_error = feis.optifunclsq_warburg(best_params); + end + + %% showing the results + + function plotresults(feis, best_params, fitting_error) + + % [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + w = feis.omega(:); + R0 = best_params(1); + R1 = best_params(2); + Q1 = best_params(3); + a1 = best_params(4); + R2 = best_params(5); + Q2 = best_params(6); + a2 = best_params(7); + Q = best_params(8); + L = best_params(9); + s = 1i .* w; + s = s(:); + + sa1 = s.^a1; + sa2 = s.^a2; + + Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); + + Z_re_fit = real(Z_param_cplx); + Z_im_fit = imag(Z_param_cplx); + + + figure; + subplot(3,1,1); + semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, Z_re_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('Z_{re} '); + + subplot(3,1,2); + semilogx(feis.omega, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('-Z_{im} '); + + subplot(3,1,3); + plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + plot(Z_re_fit, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Nyquist'); + xlabel('Z_{re}'); + ylabel('-Z_{im} '); + axis equal; + + grid on; + text_error = sprintf('Fitting error : %.2e', fitting_error); + text(0.05, 0.85, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + end + + function printResults(feis, best_params, fitting_error) + + fprintf('\n=== FITTING SCORE ===\n'); + fprintf('Error : %e\n', fitting_error); + + % fprintf('\n=== PARAMETERS FOUND ===\n'); + % fprintf('R0 = %.5f Ohms\n', best_params(1)); + % fprintf('R1 = %.5f Ohms\n', best_params(2)); + % fprintf('C1 = %.1f Farads\n', best_params(3)); + % fprintf('R2 = %.5f Ohms\n', best_params(4)); + % fprintf('C2 = %.1f Farads\n', best_params(5)); + + fprintf('\n=== PARAMETERS FOUND ===\n'); + fprintf('R0 = %.4e Ohms\n', best_params(1)); + fprintf('R1 = %.4e Ohms\n', best_params(2)); + fprintf('Q1 = %.4e s^a/Ohm\n', best_params(3)); + fprintf('a1 = %.4f \n', best_params(4)); % %f suffit pour 'a' car il est entre 0 et 1 + fprintf('R2 = %.4e Ohms\n', best_params(5)); + fprintf('Q2 = %.4e s^a/Ohm\n', best_params(6)); + fprintf('a2 = %.4f \n', best_params(7)); + fprintf('Q = %.4e \n', best_params(8)); + fprintf('L = %.4e Henrys\n', best_params(9)); + end end end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m index 65617a943..5cec30862 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m @@ -47,5 +47,5 @@ Z = impsolv.computeImpedance(omegas); Z_real = real(Z); - Z_imag = - imag(Z); + Z_imag = imag(Z); end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m index f5bb28400..1cad56a49 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m @@ -9,7 +9,7 @@ Z_real = R_0 + R_1 ./ (1+(R_1* C_1.*omega).^2) + R_2 ./ (1+(R_2* C_2.*omega).^2); - Z_imag = (R_1*R_1*C_1.*omega ./ (1+(R_1* C_1.*omega).^2)) ... - + (R_2*R_2*C_2.*omega ./ (1+(R_2* C_2.*omega).^2)); + Z_imag = -(R_1*R_1*C_1.*omega ./ (1+(R_1* C_1.*omega).^2)) ... + - (R_2*R_2*C_2.*omega ./ (1+(R_2* C_2.*omega).^2)); end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m new file mode 100644 index 000000000..5a84bcf63 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m @@ -0,0 +1,12 @@ +function [Z_real, Z_imag, omegas] = load_santoni_data() + + path_data = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\papers\LiPo Battery LP-503562-IS-3 EIS, Capacity, ECM Data\LiPO_1\EIS_Charge_discharge\EIS_45\1_EIS.csv'; + data_exp = readtable(path_data, 'Delimiter', '\t'); + + + freq = table2array(data_exp(:, 1)); + Z_real = table2array(data_exp(:, 2)); + Z_imag = table2array(data_exp(:, 3)); + + omegas = 2 * pi .* freq; +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m new file mode 100644 index 000000000..6ff436588 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m @@ -0,0 +1,48 @@ + +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); + +b = linspace(1e4, 5e4, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.Interface.activationEnergyOfReaction = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.Interface.activationEnergyOfReaction = b(i)/2; %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('activation Energy Of Reaction = %.2e', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m new file mode 100644 index 000000000..1412d6644 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m @@ -0,0 +1,46 @@ + +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); +b = linspace(0.5,2,10); + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.bruggemanCoefficient = b(i); + inputparams.PositiveElectrode.Coating.bruggemanCoefficient = b(i); + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('Bruggeman coefficient = %.2f', b(i)); + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m new file mode 100644 index 000000000..df70d8b3f --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m @@ -0,0 +1,46 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); +b = linspace(10, 1000, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.electronicConductivity = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.electronicConductivity = b(i); %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('Electronic Conductivity = %.2f', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m new file mode 100644 index 000000000..6cdcc3915 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m @@ -0,0 +1,88 @@ +function param_dependency() + mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + + jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + + includeDoubleLayer = false; + + if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + + end + + + [~, inputparams, ~] = setupModelFromJson(jsonstruct); + + c_ne = 29.866*mol/litre; % initial concentration at negative electrode + c_pe = 17.038*mol/litre; % initial concentration at positive electrode + + % 2. Création de l'interface graphique + fig = uifigure('Name', 'Impedance explorer', 'Position', [100, 100, 600, 450]); + ax = uiaxes(fig, 'Position', [50, 150, 500, 250]); + title(ax, 'Diagramme de Nyquist (Chen 2020)'); + xlabel(ax, 'Z'' (\Omega)'); + ylabel(ax, '-Z" (\Omega)'); + grid(ax, 'on'); + + % 3. Création du curseur (-1 à +1 ordre de grandeur) + sld = uislider(fig, ... + 'Position', [100, 80, 400, 3], ... + 'Limits', [-1, 1], ... + 'Value', 0); + + lbl = uilabel(fig, 'Position', [100, 100, 400, 22], 'Text', 'Prêt. Bougez le curseur pour lancer un calcul.'); + + % 4. Connexion au relâchement de la souris (ValueChangedFcn) + % On passe la structure inputparams complète à notre fonction + sld.ValueChangedFcn = @(src, event) updatePlot(ax, lbl, inputparams, event.Value); + + % (Optionnel) Lancer un premier calcul d'initialisation + % updatePlot(ax, lbl, inputparams, 0); +end + +% --- Fonction de mise à jour lourde --- +function updatePlot(ax, lbl, inputparams, slider_val) + + % 1. Avertir l'utilisateur et figer l'affichage + lbl.Text = 'Calcul en cours... Veuillez patienter (cela peut prendre quelques secondes).'; + drawnow; % CRUCIAL : Force MATLAB à afficher le texte avant de bloquer + + % 2. Calculer la nouvelle valeur et modifier la structure + % On modifie ici le SolidDiffusion.referenceDiffusionCoefficient + valeur_initiale = 3.3e-14; + nouvelle_valeur = valeur_initiale * (10^slider_val); + + % On navigue dans l'arborescence exacte de votre fichier JSON + inputparams.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = nouvelle_valeur; + + % 3. APPEL DE VOS FONCTIONS + try + [model, ~, ~] = setupModelFromJson(jsonstruct); + initstate = initStateChen2020(model, c_ne, c_pe); + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + % Définition des fréquences et calcul de l'impédance + frequences = logspace(-2, 3, 30); + Z = impsolv.computeImpedance(frequences); + + % 4. Tracer le vrai résultat + % On utilise -imag(Z) car on trace traditionnellement l'opposé de la partie imaginaire + plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#D95319'); + + % Restaurer le texte + lbl.Text = sprintf('Calcul terminé. Diffusion = %.2e (10^{%.2f}x)', nouvelle_valeur, slider_val); + + catch ME + % Si le solveur plante (par exemple si la nouvelle valeur rend le système instable) + lbl.Text = 'Erreur lors du calcul (paramètre hors limites ?)'; + disp(ME.message); % Affiche l'erreur dans la console MATLAB + end +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m new file mode 100644 index 000000000..47d1a7cce --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m @@ -0,0 +1,45 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); +b = linspace(0.1, 0.9, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.Separator.porosity = b(i); %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('porosity = %.2f', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m new file mode 100644 index 000000000..12baa2706 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m @@ -0,0 +1,47 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); + +b = linspace(1e-11, 1e-12, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = b(i)*5; %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('reactionRateConstant = %.2e', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m new file mode 100644 index 000000000..88aebd8d1 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m @@ -0,0 +1,46 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); +b = logspace(-15, -10, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = b(i)/10; %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('Diffusion Coefficient = %.2e', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m new file mode 100644 index 000000000..ac40f3e89 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m @@ -0,0 +1,47 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); + +b = linspace(3e4, 7e4, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.Interface.saturationConcentration = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.Interface.saturationConcentration = b(i)+2e4; %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('saturation Concentration = %.2e', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m new file mode 100644 index 000000000..3eff22ccb --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m @@ -0,0 +1,46 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); +b = linspace(0.5,0.95,10); + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.volumeFraction = b(i); + inputparams.PositiveElectrode.Coating.volumeFraction = b(i); + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('Volume Fraction = %.2f', b(i)); + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m new file mode 100644 index 000000000..3e949d075 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m @@ -0,0 +1,47 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = false; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); + +b = linspace(1e5, 7e5, 20); %change here + +frequences = logspace(-2, 4, 30); +figure; +hold on; +for i = 1:length(b) + + inputparams.NegativeElectrode.Coating.ActiveMaterial.Interface.volumetricSurfaceArea = b(i); %change here + inputparams.PositiveElectrode.Coating.ActiveMaterial.Interface.volumetricSurfaceArea = b(i); %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('volumetric Surface Area = %.2e', b(i)); %change here + plot(Z_re, -Z_im, 'DisplayName', curve); +end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 8b0df6ccd..b53b9d10e 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -2,21 +2,34 @@ % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; % filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; -% -% [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -params0 = [3e-2, 1, 3e3, 1e-1, 1e3]; +% [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); +% [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); [Z_re_exp, Z_im_exp, omega] = load_chen_data(); + +params0 = [3e-2, 1, 3e3, 1e-1, 1e3]; scales = [1e-1, 1e1, 1e5, 1e0, 1e5]; -% feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); -% -% [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; +scales_w = params0_w*10; %to be changed between lsq and bfgs + +feis = FittingEIS(params0_w, scales_w, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS_warburg(); + +% % Lancement avec LSQNONLIN +% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); + + + + +%% +feis.plotresults(best_params, fitting_error); + +feis.printResults(best_params, fitting_error); -% Lancement avec LSQNONLIN -[min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); % result with lsqnonlin: @@ -31,9 +44,13 @@ % C2 = 11054.0 Farads -%% -feis.plotresults(best_params, fitting_error); - -feis.printResults(best_params, fitting_error); - - +% results warburg chen +% 4.7197e-02 ... +% 1.0000e-2 ... +% 2.3392e-03 ... +% 0.0103 ... +% 6.8573e-04 ... +% 1.0000e-1 ... +% 0.0307 ... +% 7.0505e+02 ... +% 2.9134e-06 \ No newline at end of file diff --git a/Examples/Advanced/Impedance/runImpedanceChen.m b/Examples/Advanced/Impedance/runImpedanceChen.m index 16a10a49a..b53ea7ba7 100644 --- a/Examples/Advanced/Impedance/runImpedanceChen.m +++ b/Examples/Advanced/Impedance/runImpedanceChen.m @@ -55,8 +55,7 @@ figure -omegas = linspace(-4, 2, 30); -omegas = 10.^omegas; +omegas = logspace(-4, 2, 30); Z = impsolv.computeImpedance(omegas); hold on From 70a5efed969bd09077f753558d1949cb41ccf714 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 1 Jun 2026 15:23:05 +0200 Subject: [PATCH 037/119] new boxing working for thevenin model --- .../spectral_analysis/FittingEIS.m | 137 ++++++++++++++---- .../spectral_analysis/runclassfitting.m | 16 +- 2 files changed, 119 insertions(+), 34 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 67877839e..fa5727f0b 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -45,7 +45,9 @@ end function p_norm = unscaled2scaled(feis, p) - p_norm = (p-feis.params0./feis.scales)./(feis.scales*feis.params0-feis.params0/feis.scales); + a = feis.scales; + p0 = feis.params0; + p_norm = (p-p0./a)./(a*p0-p0/a); end function p = scaled2unscaled(feis, p_norm) @@ -54,6 +56,7 @@ p = (a*p0-p0/a).*p_norm +p0/a; end + %% Thevenin Model function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) @@ -63,10 +66,16 @@ % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); + a = feis.scales; + p03 = feis.params0(3); + p05 = feis.params0(5); - A_custom = [0, 0, -1, 0, 2*feis.scales(5)/feis.scales(3)]; - b_custom = 0; + A_custom = [0, 0, -1, 0, 2*(a*p05 - p05/a)/(a*p03- p03/a)]; + b_custom = (p03-2*p05)/(a^2*p03 - p03); + max_iter = 300; + tol_obj = 1e-7; + tol_grad = 1e-5; [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... @@ -74,15 +83,36 @@ 'maximize', false, ... 'linIneq', struct('A', A_custom, 'b', b_custom), ... %A*u<=b 'enforceFeasible', true, ... - 'maxIt', 300, ... - 'objChangeTol', 1e-6, ... - 'gradTol', 1e-5, ... + 'maxIt', max_iter, ... + 'objChangeTol', tol_obj, ... + 'gradTol', tol_grad, ... 'lineSearchMaxIt', 100 ... ); best_params = scaled2unscaled(feis, best_params_norm(:) ); fitting_error = feis.optifunc(best_params); + it_count = length(history.val) - 1; + final_pg = history.pg(end); + + % Cost function variation + if it_count >= 1 + delta_v = abs(history.val(end) - history.val(end-1)); + else + delta_v = inf; + end + + if it_count >= max_iter + fprintf('Stopped because %d iterations reached.\n', max_iter); + elseif final_pg < tol_grad + fprintf('Stopped because reached gradTol = %e.\n', tol_grad); + elseif delta_v < tol_obj + fprintf('Stopped because reached objChangeTol = %e.\n', tol_obj); + else + fprintf('Unexpected error or relative tolerance reached.\n'); + end + + end @@ -136,17 +166,21 @@ J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; g_im_dR0 = zeros(size(w)); - g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; - g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; - g_im_dR2 = -(2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; - g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; + g_im_dR1 = (2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; + g_im_dC1 = (R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; + g_im_dR2 = (2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; + g_im_dC2 = (R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; derr_re_dp = J_re ./ Modulus_Z; derr_im_dp = J_im ./ Modulus_Z; g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); - g_norm = unscaled2scaled(feis, g_true); + % Chain rule : + a = feis.scales; + p0 = feis.params0(:); + dp_dpnorm = (a * p0 - p0 / a); % Dérivée de p par rapport à p_norm + g_norm = g_true .* dp_dpnorm; end @@ -410,7 +444,54 @@ %% showing the results - function plotresults(feis, best_params, fitting_error) + function plotresults_thevenin(feis, best_params, fitting_error) + + [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + + figure; + subplot(3,1,1); + semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, Z_re_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('Z_{re} '); + + subplot(3,1,2); + semilogx(feis.omega, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('-Z_{im} '); + + subplot(3,1,3); + plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + plot(feis.Z_re_exp, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Nyquist'); + xlabel('Z_{re}'); + ylabel('-Z_{im} '); + axis equal; + + grid on; + + text_error = sprintf('Fitting error : %.2e', fitting_error); + + subplot(3,1,3); + + text(0.05, 0.90, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + end + + + function plotresults_warburg(feis, best_params, fitting_error) % [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); w = feis.omega(:); @@ -478,23 +559,23 @@ function printResults(feis, best_params, fitting_error) fprintf('\n=== FITTING SCORE ===\n'); fprintf('Error : %e\n', fitting_error); - % fprintf('\n=== PARAMETERS FOUND ===\n'); - % fprintf('R0 = %.5f Ohms\n', best_params(1)); - % fprintf('R1 = %.5f Ohms\n', best_params(2)); - % fprintf('C1 = %.1f Farads\n', best_params(3)); - % fprintf('R2 = %.5f Ohms\n', best_params(4)); - % fprintf('C2 = %.1f Farads\n', best_params(5)); - fprintf('\n=== PARAMETERS FOUND ===\n'); - fprintf('R0 = %.4e Ohms\n', best_params(1)); - fprintf('R1 = %.4e Ohms\n', best_params(2)); - fprintf('Q1 = %.4e s^a/Ohm\n', best_params(3)); - fprintf('a1 = %.4f \n', best_params(4)); % %f suffit pour 'a' car il est entre 0 et 1 - fprintf('R2 = %.4e Ohms\n', best_params(5)); - fprintf('Q2 = %.4e s^a/Ohm\n', best_params(6)); - fprintf('a2 = %.4f \n', best_params(7)); - fprintf('Q = %.4e \n', best_params(8)); - fprintf('L = %.4e Henrys\n', best_params(9)); + fprintf('R0 = %.5f Ohms\n', best_params(1)); + fprintf('R1 = %.5f Ohms\n', best_params(2)); + fprintf('C1 = %.1f Farads\n', best_params(3)); + fprintf('R2 = %.5f Ohms\n', best_params(4)); + fprintf('C2 = %.1f Farads\n', best_params(5)); + + % fprintf('\n=== PARAMETERS FOUND ===\n'); + % fprintf('R0 = %.4e Ohms\n', best_params(1)); + % fprintf('R1 = %.4e Ohms\n', best_params(2)); + % fprintf('Q1 = %.4e s^a/Ohm\n', best_params(3)); + % fprintf('a1 = %.4f \n', best_params(4)); % %f suffit pour 'a' car il est entre 0 et 1 + % fprintf('R2 = %.4e Ohms\n', best_params(5)); + % fprintf('Q2 = %.4e s^a/Ohm\n', best_params(6)); + % fprintf('a2 = %.4f \n', best_params(7)); + % fprintf('Q = %.4e \n', best_params(8)); + % fprintf('L = %.4e Henrys\n', best_params(9)); end end end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index b53b9d10e..ee1a5ae0b 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -9,15 +9,19 @@ [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -params0 = [3e-2, 1, 3e3, 1e-1, 1e3]; -scales = [1e-1, 1e1, 1e5, 1e0, 1e5]; +params0 = [2, ... + 1, ... + 5e2, ... + 1, ... + 1e2]; % initial condition: C1>2*C2 +scales = 100; params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; scales_w = params0_w*10; %to be changed between lsq and bfgs -feis = FittingEIS(params0_w, scales_w, Z_re_exp, Z_im_exp, omega); +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); -[~, ~, best_params, fitting_error] = feis.optimizationBFGS_warburg(); +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); % % Lancement avec LSQNONLIN % [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); @@ -26,9 +30,9 @@ %% -feis.plotresults(best_params, fitting_error); +feis.plotresults_thevenin(best_params, fitting_error); -feis.printResults(best_params, fitting_error); +feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin From 64e095875c74be3f4b28b2c18c8963a8b273a23f Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 2 Jun 2026 14:28:28 +0200 Subject: [PATCH 038/119] scaling changed to pmin and pmax, try to normalize the error (doesn't work..) --- .../spectral_analysis/FittingEIS.m | 49 ++++++++++++------- .../spectral_analysis/runclassfitting.m | 14 ++++-- 2 files changed, 39 insertions(+), 24 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index fa5727f0b..950fae7c9 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -45,33 +45,37 @@ end function p_norm = unscaled2scaled(feis, p) - a = feis.scales; - p0 = feis.params0; - p_norm = (p-p0./a)./(a*p0-p0/a); + pmin = feis.scales(1:5); + pmax = feis.scales(6:10); + p_norm = (p-pmin)./(pmax-pmin); end function p = scaled2unscaled(feis, p_norm) - a = feis.scales; - p0 = feis.params0; - p = (a*p0-p0/a).*p_norm +p0/a; + pmin = feis.scales(1:5); + pmax = feis.scales(6:10); + p = (pmax-pmin).*p_norm +pmin; end %% Thevenin Model function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) + [v0, g0] = feis.optifunc(feis.params0); - f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm)) ; + f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm), v0, g0); params0_norm = unscaled2scaled(feis, feis.params0); % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); - a = feis.scales; - p03 = feis.params0(3); - p05 = feis.params0(5); + pmin = feis.scales(1:5); + pmax = feis.scales(6:10); + p03min = pmin(3); + p03max = pmax(3); + p05min = pmin(5); + p05max = pmax(5); - A_custom = [0, 0, -1, 0, 2*(a*p05 - p05/a)/(a*p03- p03/a)]; - b_custom = (p03-2*p05)/(a^2*p03 - p03); + A_custom = [0, 0, -1, 0, 2*(p05max - p05min)/(p03max- p03min)]; + b_custom = (p03min-2*p05min)/(p03max - p03min); max_iter = 300; tol_obj = 1e-7; @@ -90,6 +94,7 @@ ); best_params = scaled2unscaled(feis, best_params_norm(:) ); + % explications of why it stopped fitting_error = feis.optifunc(best_params); it_count = length(history.val) - 1; @@ -117,9 +122,12 @@ - function [v, g_norm] = optifunc(feis, p) + function [v, g_norm] = optifunc(feis, p, v0, g0) - + if nargin < 4 + v0 = 1; + g0 = 1; + end % Preventing physical values to get too close from 0 p_safe = max(p, 1e-8); @@ -146,8 +154,10 @@ err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); - v = sum(err_re.^2 + err_im.^2); - + v_abs = sum(err_re.^2 + err_im.^2); + v = v_abs / v0; + + if nargout > 1 w = feis.omega(:); @@ -177,10 +187,11 @@ g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); % Chain rule : - a = feis.scales; - p0 = feis.params0(:); - dp_dpnorm = (a * p0 - p0 / a); % Dérivée de p par rapport à p_norm + pmin = feis.scales(1:5); + pmax = feis.scales(6:10); + dp_dpnorm = (pmax - pmin); % Dérivée de p par rapport à p_norm g_norm = g_true .* dp_dpnorm; + g_norm = g_norm ./g0; end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index ee1a5ae0b..44b3c2bda 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -10,11 +10,15 @@ params0 = [2, ... - 1, ... - 5e2, ... - 1, ... - 1e2]; % initial condition: C1>2*C2 -scales = 100; + 1, ... + 7e3, ... + 1, ... + 1.5e3]; % initial condition: C1>2*C2 + +a = 100; +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; scales_w = params0_w*10; %to be changed between lsq and bfgs From daa45b8a5f577aad34c86d5c340e66c8bf1f63dc Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 3 Jun 2026 09:27:39 +0200 Subject: [PATCH 039/119] fitting robuste pour thevenin --- .../spectral_analysis/FittingEIS.m | 17 +++---- .../spectral_analysis/load_chen_data.m | 3 +- .../doubleLayerCapacitance_impact.m | 47 +++++++++++++++++++ .../spectral_analysis/runclassfitting.m | 10 ++-- .../Advanced/Impedance/runImpedanceChen.m | 2 +- 5 files changed, 61 insertions(+), 18 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 950fae7c9..56f896c3b 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -59,9 +59,9 @@ %% Thevenin Model function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) - [v0, g0] = feis.optifunc(feis.params0); + - f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm), v0, g0); + f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm)); params0_norm = unscaled2scaled(feis, feis.params0); % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); @@ -78,7 +78,7 @@ b_custom = (p03min-2*p05min)/(p03max - p03min); max_iter = 300; - tol_obj = 1e-7; + tol_obj = 1e-15; tol_grad = 1e-5; [min_value, best_params_norm, history] = unitBoxBFGS(... @@ -122,12 +122,8 @@ - function [v, g_norm] = optifunc(feis, p, v0, g0) + function [v, g_norm] = optifunc(feis, p) - if nargin < 4 - v0 = 1; - g0 = 1; - end % Preventing physical values to get too close from 0 p_safe = max(p, 1e-8); @@ -154,8 +150,7 @@ err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); - v_abs = sum(err_re.^2 + err_im.^2); - v = v_abs / v0; + v = sum(err_re.^2 + err_im.^2); if nargout > 1 @@ -191,7 +186,7 @@ pmax = feis.scales(6:10); dp_dpnorm = (pmax - pmin); % Dérivée de p par rapport à p_norm g_norm = g_true .* dp_dpnorm; - g_norm = g_norm ./g0; + end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m index 5cec30862..d93dc9035 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m @@ -42,8 +42,7 @@ impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); - omegas = linspace(-4, 2, 50); - omegas = 10.^omegas; + omegas = logspace(-4, 2, 50); Z = impsolv.computeImpedance(omegas); Z_real = real(Z); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m new file mode 100644 index 000000000..a4c856f22 --- /dev/null +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m @@ -0,0 +1,47 @@ +mrstModule add ad-core mrst-gui mpfa agmg linearsolvers + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + + +includeDoubleLayer = true; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); + +c_ne = 29.866*mol/litre; % initial concentration at negative electrode +c_pe = 17.038*mol/litre; % initial concentration at positive electrode + +initstate = initStateChen2020(model, c_ne, c_pe); + +b = logspace(-2, 2, 20); %change here + +frequences = logspace(-2, 4, 30); + + +for i = 1:length(b) + + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here + + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + Z = impsolv.computeImpedance(frequences); + Z_re = real(Z); + Z_im = imag(Z); + curve = sprintf('doubleLayerCapacitance = %.2e', b(i)); %change here + figure; + plot(Z_re, -Z_im, 'DisplayName', curve); + legend('show'); + +end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 44b3c2bda..46612168e 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,17 +5,19 @@ % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); % [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); - [Z_re_exp, Z_im_exp, omega] = load_chen_data(); +% omega = logspace(-4, 2, 50); +% params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; +% [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); params0 = [2, ... 1, ... - 7e3, ... + 7e2, ... 1, ... - 1.5e3]; % initial condition: C1>2*C2 - + 1.5e2]; % initial condition: C1>2*C2 a = 100; + pmin = params0 / a; pmax = params0 * a; scales = [pmin, pmax]; diff --git a/Examples/Advanced/Impedance/runImpedanceChen.m b/Examples/Advanced/Impedance/runImpedanceChen.m index b53ea7ba7..1f52b1093 100644 --- a/Examples/Advanced/Impedance/runImpedanceChen.m +++ b/Examples/Advanced/Impedance/runImpedanceChen.m @@ -24,7 +24,7 @@ jsonstruct = mergeJsonStructs({jsonstruct_material, ... jsonstruct_geometry}); -includeDoubleLayer = false; +includeDoubleLayer = true; if includeDoubleLayer From e9e4a96ab3cdbc2f0ce14a0e473826216d412978 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Wed, 3 Jun 2026 16:56:18 +0200 Subject: [PATCH 040/119] fix in doubleLayerCapacitance --- .../doubleLayerCapacitance_impact.m | 14 +++++++++++--- 1 file changed, 11 insertions(+), 3 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m index a4c856f22..a3638f660 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m @@ -30,13 +30,21 @@ frequences = logspace(-2, 4, 30); -for i = 1:length(b) - - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here +for i = 18:20 + + fprintf('compute impedance for doubleLayerCapacitance = %.2e ... ', b(i)); %change here + + tic + % jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here + % [model, inputparams, ~] = setupModelFromJson(jsonstruct); + inputparams.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); Z = impsolv.computeImpedance(frequences); + + fprintf('done in %g s\n', toc); + Z_re = real(Z); Z_im = imag(Z); curve = sprintf('doubleLayerCapacitance = %.2e', b(i)); %change here From 86de364467de4264abc7704eee3c802d52535e79 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Thu, 4 Jun 2026 09:29:07 +0200 Subject: [PATCH 041/119] little changes --- .../doubleLayerCapacitance_impact.m | 9 +- .../pxdparams_impact/param_dependency.m | 141 +++++++++++------- .../spectral_analysis/runclassfitting.m | 18 +-- 3 files changed, 98 insertions(+), 70 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m index a4c856f22..76b88ec94 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m @@ -29,7 +29,7 @@ frequences = logspace(-2, 4, 30); - +figure; for i = 1:length(b) jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here @@ -40,8 +40,9 @@ Z_re = real(Z); Z_im = imag(Z); curve = sprintf('doubleLayerCapacitance = %.2e', b(i)); %change here - figure; - plot(Z_re, -Z_im, 'DisplayName', curve); - legend('show'); + plot(Z_re, -Z_im, 'DisplayName', curve); + end + +legend('show'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m index 6cdcc3915..9a07c3fe1 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m @@ -1,88 +1,115 @@ function param_dependency() mrstModule add ad-core mrst-gui mpfa agmg linearsolvers - + + % 1. Chargement des données (Conservez votre méthode de chargement ici) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); - jsonstruct = mergeJsonStructs({jsonstruct_material, ... - jsonstruct_geometry}); - - - - includeDoubleLayer = false; - - if includeDoubleLayer - - jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; - - end - + c_ne = 29.866*mol/litre; + c_pe = 17.038*mol/litre; - [~, inputparams, ~] = setupModelFromJson(jsonstruct); + % 2. Création de l'interface graphique (Fenêtre plus haute pour accueillir les curseurs) + fig = uifigure('Name', 'Impedance Explorer', 'Position', [100, 50, 600, 650]); - c_ne = 29.866*mol/litre; % initial concentration at negative electrode - c_pe = 17.038*mol/litre; % initial concentration at positive electrode - - % 2. Création de l'interface graphique - fig = uifigure('Name', 'Impedance explorer', 'Position', [100, 100, 600, 450]); - ax = uiaxes(fig, 'Position', [50, 150, 500, 250]); - title(ax, 'Diagramme de Nyquist (Chen 2020)'); - xlabel(ax, 'Z'' (\Omega)'); - ylabel(ax, '-Z" (\Omega)'); + % Graphique + ax = uiaxes(fig, 'Position', [50, 350, 500, 250]); + title(ax, 'Nyquist Diagram'); + xlabel(ax, 'Re(Z)'); + ylabel(ax, '-Im(Z)'); grid(ax, 'on'); + + % Label de statut + lbl = uilabel(fig, 'Position', [50, 310, 500, 22], 'Text', 'Ready, use slider to start.'); + lbl.FontWeight = 'bold'; + + % --- CURSEUR 1 : Diffusion Solide (Anode) --- + % Modifie le transport du Lithium dans les particules de graphite. + uilabel(fig, 'Position', [50, 260, 500, 40], 'WordWrap', 'on', ... + 'Text', '1. refDiffusionCoefficient * 10^x'); - % 3. Création du curseur (-1 à +1 ordre de grandeur) - sld = uislider(fig, ... - 'Position', [100, 80, 400, 3], ... - 'Limits', [-1, 1], ... + sld1 = uislider(fig, 'Position', [50, 240, 500, 3], ... + 'Limits', [-10, 10], ... % Définit le minimum et le maximum + 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 + 'Value', 0); + + % --- CURSEUR 2 : Taux de réaction (Anode) --- + % Modifie la cinétique de transfert de charge. + uilabel(fig, 'Position', [50, 170, 500, 40], 'WordWrap', 'on', ... + 'Text', '2. Anode reactionRateConstant * 10^x'); + sld2 = uislider(fig, 'Position', [50, 150, 500, 3],... + 'Limits', [-10, 10], ... % Définit le minimum et le maximum + 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 'Value', 0); - lbl = uilabel(fig, 'Position', [100, 100, 400, 22], 'Text', 'Prêt. Bougez le curseur pour lancer un calcul.'); + % --- CURSEUR 3 : Taux de réaction (Cathode) --- + % Modifie la cinétique de transfert de charge. + uilabel(fig, 'Position', [50, 80, 500, 40], 'WordWrap', 'on', ... + 'Text', '3. Cathode reactionRateConstant * 10^x'); + sld3 = uislider(fig, 'Position', [50, 60, 500, 3], ... + 'Limits', [-10, 10], ... % Définit le minimum et le maximum + 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 + 'Value', 0); - % 4. Connexion au relâchement de la souris (ValueChangedFcn) - % On passe la structure inputparams complète à notre fonction - sld.ValueChangedFcn = @(src, event) updatePlot(ax, lbl, inputparams, event.Value); + % 4. Connexion aux événements + % On crée une fonction anonyme qui passe TOUS les curseurs + callback_fcn = @(src, event) updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3); + + sld1.ValueChangedFcn = callback_fcn; + sld2.ValueChangedFcn = callback_fcn; + sld3.ValueChangedFcn = callback_fcn; - % (Optionnel) Lancer un premier calcul d'initialisation - % updatePlot(ax, lbl, inputparams, 0); + % Optionnel : Tracer l'état initial + % updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3); end -% --- Fonction de mise à jour lourde --- -function updatePlot(ax, lbl, inputparams, slider_val) +% --- Fonction de mise à jour --- +function updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3) - % 1. Avertir l'utilisateur et figer l'affichage - lbl.Text = 'Calcul en cours... Veuillez patienter (cela peut prendre quelques secondes).'; - drawnow; % CRUCIAL : Force MATLAB à afficher le texte avant de bloquer + % Figer l'affichage + lbl.Text = 'Processing... '; + lbl.FontColor = '#D95319'; + drawnow; - % 2. Calculer la nouvelle valeur et modifier la structure - % On modifie ici le SolidDiffusion.referenceDiffusionCoefficient - valeur_initiale = 3.3e-14; - nouvelle_valeur = valeur_initiale * (10^slider_val); + % 1. Récupération des valeurs de base depuis votre JSON + base_diff_anode = 1.3135e-15; + base_rate_anode = 5.031e-11; + base_rate_cathode = 2.33e-11; - % On navigue dans l'arborescence exacte de votre fichier JSON - inputparams.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = nouvelle_valeur; + % 2. Application des multiplicateurs (10^slider_val) + val_diff_anode = base_diff_anode * (10^(sld1.Value)); + val_rate_anode = base_rate_anode * (10^(sld2.Value)); + val_rate_cathode = base_rate_cathode * (10^(sld3.Value)); + + % 3. Injection dans la structure JSON AVANT de construire le modèle + jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode; + jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; + jsonstruct.PositiveElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_cathode; - % 3. APPEL DE VOS FONCTIONS try - [model, ~, ~] = setupModelFromJson(jsonstruct); + % 4. Exécution de BattMo + [model, inputparams, ~] = setupModelFromJson(jsonstruct); initstate = initStateChen2020(model, c_ne, c_pe); + impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); - % Définition des fréquences et calcul de l'impédance frequences = logspace(-2, 3, 30); Z = impsolv.computeImpedance(frequences); - % 4. Tracer le vrai résultat - % On utilise -imag(Z) car on trace traditionnellement l'opposé de la partie imaginaire - plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#D95319'); + % 5. Tracé + plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); - % Restaurer le texte - lbl.Text = sprintf('Calcul terminé. Diffusion = %.2e (10^{%.2f}x)', nouvelle_valeur, slider_val); + % Retour à la normale + lbl.Text = 'Done'; + lbl.FontColor = '#77AC30'; catch ME - % Si le solveur plante (par exemple si la nouvelle valeur rend le système instable) - lbl.Text = 'Erreur lors du calcul (paramètre hors limites ?)'; - disp(ME.message); % Affiche l'erreur dans la console MATLAB + lbl.Text = 'Erreur lors du calcul (vérifiez la console).'; + lbl.FontColor = '#A2142F'; + disp('--- ERREUR DANS LE CALCUL ---'); + disp(ME.message); + for k = 1:length(ME.stack) + disp(['Ligne ', num2str(ME.stack(k).line), ' dans ', ME.stack(k).name]); + end end end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 46612168e..247541164 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -5,18 +5,18 @@ % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); % [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); -[Z_re_exp, Z_im_exp, omega] = load_chen_data(); +% [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -% omega = logspace(-4, 2, 50); -% params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; -% [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); +omega = logspace(-4, 2, 50); +params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; +[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); -params0 = [2, ... +params0 = [5, ... + 10, ... + 7e1, ... 1, ... - 7e2, ... - 1, ... - 1.5e2]; % initial condition: C1>2*C2 -a = 100; + 1.5e1]; % initial condition: C1>2*C2 +a = 1000; pmin = params0 / a; pmax = params0 * a; From 19b7a0003481ac585ae0764b36740d66e4897a35 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 16 Jun 2026 09:33:47 +0200 Subject: [PATCH 042/119] Recet changes and notebook added --- .../spectral_analysis/FittingEIS.m | 16 +++---- .../spectral_analysis/load_chen_data.m | 4 +- .../load_experimental_data.m | 4 +- .../doubleLayerCapacitance_impact.m | 20 ++++----- .../pxdparams_impact/param_dependency.m | 39 +++++++++++----- .../spectral_analysis/runclassfitting.m | 42 ++++++++++++------ Notebook.mlx | Bin 0 -> 244295 bytes 7 files changed, 76 insertions(+), 49 deletions(-) create mode 100644 Notebook.mlx diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index 56f896c3b..a084da688 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -460,7 +460,7 @@ function plotresults_thevenin(feis, best_params, fitting_error) hold on; semilogx(feis.omega, Z_re_fit, 'b'); legend('experience', 'fitted model'); - title('Fitting results'); + title('Fitting Real Impedance'); xlabel('Omega'); ylabel('Z_{re} '); @@ -469,7 +469,7 @@ function plotresults_thevenin(feis, best_params, fitting_error) hold on; semilogx(feis.omega, -Z_im_fit, 'b'); legend('experience', 'fitted model'); - title('Fitting results'); + title('Fitting Imaginary Impedance'); xlabel('Omega'); ylabel('-Z_{im} '); @@ -478,7 +478,7 @@ function plotresults_thevenin(feis, best_params, fitting_error) hold on; plot(feis.Z_re_exp, -Z_im_fit, 'b'); legend('experience', 'fitted model'); - title('Nyquist'); + title('Nyquist Diagram'); xlabel('Z_{re}'); ylabel('-Z_{im} '); axis equal; @@ -566,11 +566,11 @@ function printResults(feis, best_params, fitting_error) fprintf('Error : %e\n', fitting_error); fprintf('\n=== PARAMETERS FOUND ===\n'); - fprintf('R0 = %.5f Ohms\n', best_params(1)); - fprintf('R1 = %.5f Ohms\n', best_params(2)); - fprintf('C1 = %.1f Farads\n', best_params(3)); - fprintf('R2 = %.5f Ohms\n', best_params(4)); - fprintf('C2 = %.1f Farads\n', best_params(5)); + fprintf('R0 = %.2e Ohms\n', best_params(1)); + fprintf('R1 = %.2e Ohms\n', best_params(2)); + fprintf('C1 = %.2e Farads\n', best_params(3)); + fprintf('R2 = %.2e Ohms\n', best_params(4)); + fprintf('C2 = %.2e Farads\n', best_params(5)); % fprintf('\n=== PARAMETERS FOUND ===\n'); % fprintf('R0 = %.4e Ohms\n', best_params(1)); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m index d93dc9035..52a7a65a4 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m @@ -23,12 +23,12 @@ - includeDoubleLayer = false; + includeDoubleLayer = true; if includeDoubleLayer jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 30; end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m index d1d9c0ea5..b2e0c2643 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m @@ -28,13 +28,13 @@ freq = str2double(strrep(freq_raw, ',', '.')); else Z_real = Z_real_raw; - Z_imag = Z_imag_raw; + Z_imag = Z_imag_raw; freq = freq_raw; end idx_valides = (Z_real ~= 0) & ~isnan(Z_real); Z_real = Z_real(idx_valides); - Z_imag = Z_imag(idx_valides); + Z_imag = -Z_imag(idx_valides); % in the file is given -Im freq = freq(idx_valides); Z_real = Z_real(8:60); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m index f8eb5ff77..df5714137 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m @@ -6,7 +6,10 @@ jsonstruct = mergeJsonStructs({jsonstruct_material, ... jsonstruct_geometry}); - +ne = 'NegativeElectrode'; +co = 'Coating'; +am = 'ActiveMaterial'; +itf = 'Interface'; includeDoubleLayer = true; @@ -29,23 +32,18 @@ frequences = logspace(-2, 4, 30); -<<<<<<< HEAD + figure; +hold on; for i = 1:length(b) - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here -======= - -for i = 18:20 ->>>>>>> e9e4a96ab3cdbc2f0ce14a0e473826216d412978 - fprintf('compute impedance for doubleLayerCapacitance = %.2e ... ', b(i)); %change here tic - % jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here - % [model, inputparams, ~] = setupModelFromJson(jsonstruct); + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here + [model, inputparams, ~] = setupModelFromJson(jsonstruct); - inputparams.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); + % inputparams.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); Z = impsolv.computeImpedance(frequences); diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m index 9a07c3fe1..8a44ae62d 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m @@ -5,7 +5,22 @@ function param_dependency() jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + ne = 'NegativeElectrode'; + co = 'Coating'; + am = 'ActiveMaterial'; + itf = 'Interface'; + includeDoubleLayer = true; + + if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + + end + + + c_ne = 29.866*mol/litre; c_pe = 17.038*mol/litre; @@ -26,29 +41,29 @@ function param_dependency() % --- CURSEUR 1 : Diffusion Solide (Anode) --- % Modifie le transport du Lithium dans les particules de graphite. uilabel(fig, 'Position', [50, 260, 500, 40], 'WordWrap', 'on', ... - 'Text', '1. refDiffusionCoefficient * 10^x'); + 'Text', '1. Anode refDiffusionCoefficient * 10^x (initial value: 1.3135e-15)'); sld1 = uislider(fig, 'Position', [50, 240, 500, 3], ... - 'Limits', [-10, 10], ... % Définit le minimum et le maximum - 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 + 'Limits', [-5, 5], ... % Définit le minimum et le maximum + 'MajorTicks', -5:0.5:5, ... % Ajoute une graduation tous les 1 'Value', 0); % --- CURSEUR 2 : Taux de réaction (Anode) --- % Modifie la cinétique de transfert de charge. uilabel(fig, 'Position', [50, 170, 500, 40], 'WordWrap', 'on', ... - 'Text', '2. Anode reactionRateConstant * 10^x'); + 'Text', '2. Anode reactionRateConstant * 10^x (initial value: 5.031e-11) '); sld2 = uislider(fig, 'Position', [50, 150, 500, 3],... - 'Limits', [-10, 10], ... % Définit le minimum et le maximum - 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 + 'Limits', [-5, 5], ... % Définit le minimum et le maximum + 'MajorTicks', -5:0.5:5, ... % Ajoute une graduation tous les 1 'Value', 0); % --- CURSEUR 3 : Taux de réaction (Cathode) --- % Modifie la cinétique de transfert de charge. uilabel(fig, 'Position', [50, 80, 500, 40], 'WordWrap', 'on', ... - 'Text', '3. Cathode reactionRateConstant * 10^x'); + 'Text', '3. doubleLayerCapacitance * x (initial value: 0.2)'); sld3 = uislider(fig, 'Position', [50, 60, 500, 3], ... - 'Limits', [-10, 10], ... % Définit le minimum et le maximum - 'MajorTicks', -10:1:10, ... % Ajoute une graduation tous les 1 + 'Limits', [-5, 5], ... % Définit le minimum et le maximum + 'MajorTicks', -5:0.5:5, ... % Ajoute une graduation tous les 1 'Value', 0); % 4. Connexion aux événements @@ -74,17 +89,17 @@ function updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3) % 1. Récupération des valeurs de base depuis votre JSON base_diff_anode = 1.3135e-15; base_rate_anode = 5.031e-11; - base_rate_cathode = 2.33e-11; + base_doubleLayerCapacitance = 0.2; % 2. Application des multiplicateurs (10^slider_val) val_diff_anode = base_diff_anode * (10^(sld1.Value)); val_rate_anode = base_rate_anode * (10^(sld2.Value)); - val_rate_cathode = base_rate_cathode * (10^(sld3.Value)); + val_doubleLayerCapacitance = base_doubleLayerCapacitance * 10^(sld3.Value); % 3. Injection dans la structure JSON AVANT de construire le modèle jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode; jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; - jsonstruct.PositiveElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_cathode; + jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_doubleLayerCapacitance; try % 4. Exécution de BattMo diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m index 247541164..59dbedd95 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m @@ -1,21 +1,19 @@ +%% Main code: % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; % filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; - +% % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); % [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); -% [Z_re_exp, Z_im_exp, omega] = load_chen_data(); +[Z_re_exp, Z_im_exp, omega] = load_chen_data(); + +% omega = logspace(-4, 2, 50); +% params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; +% [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); -omega = logspace(-4, 2, 50); -params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; -[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 -params0 = [5, ... - 10, ... - 7e1, ... - 1, ... - 1.5e1]; % initial condition: C1>2*C2 a = 1000; pmin = params0 / a; @@ -29,19 +27,35 @@ [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); -% % Lancement avec LSQNONLIN -% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); - +% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); +% % Lancement avec LSQNONLIN -%% +%% Printing results feis.plotresults_thevenin(best_params, fitting_error); feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin + +%% Robustness test +% for i = 1:5 + % params0 = pmin + (pmax - pmin) .* rand(1, 5); + % disp(['Tour ', num2str(i), ' - params0 :']); + % disp(params0); + % feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + % + % [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + % feis.plotresults_thevenin(best_params, fitting_error); + % feis.printResults(best_params, fitting_error); + % + % drawnow; + +% end +%% + % result with lsqnonlin: % === FITTING SCORE === % Error : 7.324871e-02 diff --git a/Notebook.mlx b/Notebook.mlx new file mode 100644 index 0000000000000000000000000000000000000000..b020cb83e3291b5e30e49ec5a71bf6eafe8ba79a GIT binary patch literal 244295 zcmZ6xQ>-vd&~CYH+qP}nwr$(CZQHhO+qU&?<9z3wNoM}J=wb2mo*d3;=-q-;cJiy`77xor}JTr-P}pE}e(1O{?;x+%N+|?;ACZ zzT(jkAYn=iI9epMN`=orf(&x?o{4w{qxsNRI`AAmBO0AWIF~&ww&0g&ox8C1Y6+=ZDKbXkqWI9M5n98k(psH zSX8lnNU#+oY*h5)yOPQp0@f6T<-=q|;}IJA0;LiA4^?Hl&XtH`+2M^Ha{X6=B^rP7 z04FJRK?EwbvOi?K5rJDJ)z)6@O$yEb|7Kgciw_dih-Z>-krWCFJCK$YwvW8fJh*43?& zDJ3>v-b{gF!v$2x;}eh1&N$}R!s|)wENzNR<&r$*Af)O=iK=q?Z1K(7QZ>Mo1*%BS zULw+yT@g*@HiI7|+U#3M@`-Hat{|4e#(-N#6i%K 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00:00:00 2001 From: Alexandre Date: Tue, 16 Jun 2026 11:55:42 +0200 Subject: [PATCH 043/119] codes added to notebook --- Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m | 4 ++-- 1 file changed, 2 insertions(+), 2 deletions(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m index a084da688..c1812db7a 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m @@ -189,7 +189,7 @@ end - + end % finite difference method % if nargout > 1 @@ -210,7 +210,7 @@ % g_norm = (v_perturb - v) / dp_norm; % end % end - end + %% Warburg Model From a7e1d769317bba5f4531748ba8e24fe90cc3fc5a Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 16 Jun 2026 14:40:52 +0200 Subject: [PATCH 044/119] Code added to Notebook --- Notebook.mlx | Bin 244295 -> 305419 bytes 1 file changed, 0 insertions(+), 0 deletions(-) diff --git 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| 2 +- Notebook.mlx | Bin 305419 -> 625125 bytes 2 files changed, 1 insertion(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m index 52a7a65a4..45b210d80 100644 --- a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m @@ -28,7 +28,7 @@ if includeDoubleLayer jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 30; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; end diff --git a/Notebook.mlx b/Notebook.mlx index c6f6742ed17351e01ef88d35d83b03433928447f..d9e75187949c382022356ce5ec5e8b0ff912add2 100644 GIT binary patch delta 333669 zcmV(pK=8kd(h}v9Ca}{23N?eQb~XV30M`eT-2x?ll}m2JAP_+JJ_TZ5#-GG-Dm&R# ziqveP^Z?W*wiWX!Saoyz(som)nyxICqk%UMW(4K_Lk{F!Sl4S+(S*g62vzH*S8YXK 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056/119] more cleaning --- .../{examples => }/notebooks/calibrationECM.mlx | Bin .../{examples => }/notebooks/exampleECM.ipynb | 0 .../{examples => }/notebooks/exampleECM.mlx | Bin 3 files changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/{examples => }/notebooks/calibrationECM.mlx (100%) rename Battery/EquivalentCircuitModel/{examples => }/notebooks/exampleECM.ipynb (100%) rename Battery/EquivalentCircuitModel/{examples => }/notebooks/exampleECM.mlx (100%) diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/calibrationECM.mlx b/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/examples/notebooks/calibrationECM.mlx rename to Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.ipynb b/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb similarity index 100% rename from Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.ipynb rename to Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.mlx b/Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.mlx rename to Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx From f5913f5ad5cb06cce8752a853c2e0dc5524ded34 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 22 Jun 2026 14:35:51 +0200 Subject: [PATCH 057/119] more cleaning 2 --- .../calibration/FittingEIS.m | 19 -- .../calibration/runFittingEIS.m | 172 ------------------ 2 files changed, 191 deletions(-) delete mode 100644 Battery/EquivalentCircuitModel/calibration/runFittingEIS.m diff --git a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m index c1812db7a..53564e67a 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m @@ -191,25 +191,6 @@ end end - % finite difference method - % if nargout > 1 - % g_norm = zeros(5,1); - % dp_norm = 1e-6; - % - % for i = 1:5 - % p_perturb = p; - % p_perturb(i) = p_perturb(i) + dp_norm * feis.scales(i); - % - % [Z_re_pert, Z_im_pert] = load_nyquist(p_perturb, feis.omega); - % - % err_re_pert = (feis.Z_re_exp(:) - double(Z_re_pert(:))) ./ Modulus_Z; - % err_im_pert = (feis.Z_im_exp(:) - double(Z_im_pert(:))) ./ Modulus_Z; - % - % v_perturb = sum(err_re_pert.^2 + err_im_pert.^2); - % - % g_norm = (v_perturb - v) / dp_norm; - % end - % end %% Warburg Model diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m b/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m deleted file mode 100644 index 33c8d940a..000000000 --- a/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m +++ /dev/null @@ -1,172 +0,0 @@ -%% Fitting Script - -% initial values [R0, R1, C1, R2, C2] -% params0 = [8.2e-3, 1.5e-3, 1, 1.5e-2, 200]; % handmade best ones - -params0 = [3e-3, 0.00260, 100, 0.00132, 1]; - -[Z_re_exp, Z_im_exp, omega] = load_experimental_data(); - -% lengthZ = length(Z_im_exp); - -% synthetic data -% opti_params = [0.00341, 0.00260, 5663.9, 0.00132, 0.9]; % params with -% lsqnonlin -% -% params with unitboxBFGS: -% R0 = 0.00318 Ohms -% R1 = 0.00247 Ohms -% C1 = 10654.4 Farads -% R2 = 0.00155 Ohms -% C2 = 0.4 Farads -% - -% [Z_re_exp, Z_im_exp] = load_nyquist(opti_params, omega); - -%% - -scales = [10e-2, 10e-3, 15000, 10e-3, 5]; - -params0_norm = params0 ./ scales; - -lb_true = [1e-5, 1e-5, 1e-5, 1e-5, 1e-5]; -lb_norm = lb_true ./ scales; -ub_norm = []; - -f_opt = @(p_norm) optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) ; - -% best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); -params0_norm = params0_norm(:); - -[min_value, best_params_norm, history] = unitBoxBFGS(... - params0_norm, ... - f_opt, ... - 'maximize', false, ... - 'linIneq', struct('A', [0, 0, -1, 0, 2*scales(5)/scales(3)], 'b', 0), ... - 'enforceFeasible', true, ... - 'maxIt', 300, ... - 'objChangeTol', 1e-6, ... - 'gradTol', 1e-5 ... -); - - -best_params = best_params_norm(:) .* scales(:); - -[v_opt, g_opt] = optifunc(best_params_norm, scales, Z_re_exp, Z_im_exp, omega) - -fprintf('\n=== FITTING SCORE ===\n'); -fprintf('Error : %e\n', v_opt); - -fprintf('\n=== PARAMETERS FOUND ===\n'); -fprintf('R0 = %.5f Ohms\n', best_params(1)); -fprintf('R1 = %.5f Ohms\n', best_params(2)); -fprintf('C1 = %.1f Farads\n', best_params(3)); -fprintf('R2 = %.5f Ohms\n', best_params(4)); -fprintf('C2 = %.1f Farads\n', best_params(5)); - -%% Graphique - - -parameters.R0 = best_params(1); -parameters.R1 = best_params(2); -parameters.C1 = best_params(3); -parameters.R2 = best_params(4); -parameters.C2 = best_params(5); - -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, omega); - - -%% -figure; -subplot(3,1,1); -semilogx(omega, Z_re_exp, 'ro', 'MarkerFaceColor', 'r'); -hold on; -semilogx(omega, Z_re_fit, 'bo', 'LineWidth', 2); -% legend('Expérimental', 'Modèle (Fitted)'); -title('Fitting results'); -xlabel('Omega'); -ylabel('Z_{re} '); - -subplot(3,1,2); -semilogx(omega, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); -hold on; -semilogx(omega, Z_im_fit, 'bo', 'LineWidth', 2); -% legend('Expérimental', 'Modèle (Fitted)'); -title('Fitting results'); -xlabel('Omega'); -ylabel('-Z_{im} '); - -subplot(3,1,3); -plot(Z_re_exp, Z_im_exp, 'ro', 'MarkerFaceColor', 'r'); -hold on; -plot(Z_re_exp, Z_im_fit, 'bo', 'LineWidth', 2); -% legend('Expérimental', 'Modèle (Fitted)'); -title('Nyquist'); -xlabel('Z_{re}'); -ylabel('-Z_{im} '); -axis equal; - -grid on; - -text_error = sprintf('Fitting error : %.2e', v_opt); - -subplot(3,1,3); - -text(0.05, 0.90, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); - -function [v, g_norm] = optifunc(p_norm, scales, Z_re_exp, Z_im_exp, omega) - - p = p_norm(:) .* scales(:); - - [Z_re_param, Z_Im_param] = load_nyquist(p, omega); - - Module_Z = sqrt(Z_re_exp.^2 + Z_im_exp.^2); - Module_Z = Module_Z(:); - - err_re = (Z_re_exp(:) - Z_re_param(:)) ./ Module_Z(:); - err_im = (Z_im_exp(:) - Z_Im_param(:)) ./ Module_Z(:); - - v = sum(err_re.^2 + err_im.^2); - - -if nargout > 1 - w = omega(:); - R0 = p(1); - R1 = p(2); - C1 = p(3); - R2 = p(4); - C2 = p(5); - - - g_re_dR0 = -ones(size(w)); - g_re_dR1 = -(1-(R1*C1.*w).^2) ./ (1+(R1*C1.*w).^2).^2; - g_re_dC1 = (2*C1*R1^3.*w.^2) ./ (1+(R1*C1.*w).^2).^2; - g_re_dR2 = -(1-(R2*C2.*w).^2) ./ (1+(R2*C2.*w).^2).^2; - g_re_dC2 = (2*C2*R2^3.*w.^2) ./ (1+(R2*C2.*w).^2).^2; - - J_re = [g_re_dR0, g_re_dR1, g_re_dC1, g_re_dR2, g_re_dC2]; - - - g_im_dR0 = zeros(size(w)); - g_im_dR1 = -(2*R1*C1.*w) ./ (1+(R1*C1.*w).^2).^2; - g_im_dC1 = -(R1^2.*w - C1^2*R1^4.*w.^3) ./ (1+(R1*C1.*w).^2).^2; - g_im_dR2 = -(2*R2*C2.*w) ./ (1+(R2*C2.*w).^2).^2; - g_im_dC2 = -(R2^2.*w - C2^2*R2^4.*w.^3) ./ (1+(R2*C2.*w).^2).^2; - - J_im = [g_im_dR0, g_im_dR1, g_im_dC1, g_im_dR2, g_im_dC2]; - derr_re_dp = J_re ./ Module_Z; - derr_im_dp = J_im ./ Module_Z; - - - g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); - g_norm = g_true .* scales(:); -end - -end - - - From 09b2e430ccbe65d9d9c7f5a5e75762627df05727 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 22 Jun 2026 17:28:24 +0200 Subject: [PATCH 058/119] more changes --- .../specific_calibration/ankExpCalibration.m | 51 ++++++++++++++++++ .../specific_calibration/chenCalibration.m | 34 ++++++++++++ .../specific_calibration/testCalibration.m | 32 +++++++++++ .../calibration/utils/load_chen_data.m | 2 +- .../notebooks/calibrationECM.mlx | Bin 723693 -> 994433 bytes 5 files changed, 118 insertions(+), 1 deletion(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m create mode 100644 Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m create mode 100644 Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m new file mode 100644 index 000000000..0b03911b1 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m @@ -0,0 +1,51 @@ +filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; +% filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; +[Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename) + +params0 = [3.84e-03,... +2.71e-03,... +6.00e+03,... +9.48e-04,... +1.11e+01]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + +figure; + +plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); +hold on; +plot(feis.Z_re_exp, -Z_im_fit, 'b'); +legend('experience', 'fitted model'); +xlabel('Z_{re}'); +ylabel('-Z_{im} '); +axis equal; + +grid on; + +text_error = sprintf('Fitting error : %.2e', fitting_error); + +text(0.05, 0.90, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + +fprintf('\n=== FITTING SCORE ===\n'); +fprintf('Error : %e\n', fitting_error); + +fprintf('\n=== PARAMETERS FOUND ===\n'); +fprintf('R0 = %.2e Ohms\n', best_params(1)); +fprintf('R1 = %.2e Ohms\n', best_params(2)); +fprintf('C1 = %.2e Farads\n', best_params(3)); +fprintf('R2 = %.2e Ohms\n', best_params(4)); +fprintf('C2 = %.2e Farads\n', best_params(5)); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m new file mode 100644 index 000000000..d400dde3f --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m @@ -0,0 +1,34 @@ +[Z_re_exp, Z_im_exp, omega] = load_chen_data(); +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + +figure; + +plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); +hold on; +plot(feis.Z_re_exp, -Z_im_fit, 'b'); +legend('experience', 'fitted model'); +xlabel('Z_{re}'); +ylabel('-Z_{im} '); +axis equal; + +grid on; + +text_error = sprintf('Fitting error : %.2e', fitting_error); + +text(0.05, 0.90, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m new file mode 100644 index 000000000..291ba808d --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m @@ -0,0 +1,32 @@ +omega = logspace(-4, 2, 50); +params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; +[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); + +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); +figure; +plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); +hold on; +plot(Z_re_fit, -Z_im_fit, 'b'); +legend('experience', 'fitted model'); +xlabel('Z_{re}'); +ylabel('-Z_{im} '); +axis equal; +grid on; +text_error = sprintf('Fitting error : %.2e', fitting_error); +text_error = sprintf('Fitting error : %.2e', fitting_error); +text(0.05, 0.85, text_error, 'Units', 'normalized', ... +'BackgroundColor', 'white', ... +'EdgeColor', 'black', ... +'FontSize', 11, ... +'FontWeight', 'bold'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m index a05b021e5..0fe056cb7 100644 --- a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m @@ -28,7 +28,7 @@ if includeDoubleLayer jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 30; end diff --git a/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx b/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx index 7627a120fc8ff220d21cfc8c2564533b0df563b4..b40953879889667d2e062ee0c90c210c835f4357 100644 GIT binary patch delta 349950 zcmV(%K;pmcl`MhTJh1c&3Lsa~a_=hu0J!9n{tFv_>w4QblIZ_D1x~gzmJ;24i5-u7 z*Rh>$&)4qc*vWLZ<3t}sLJ~W?HA&f4dp+Mi#6H0JyZ_EJoOzRdl2cUxNRXmzIND5lfp3>I-PU88JFv0fh~dv1TF2fTm_wsyb7;GR zIElEGRDxdDz8U&NTqHMxu3&hsQOE|u3OvC$vw)5w?y}GkmSDk<30GK24Z3I=F9 za(G@~3zymtLjWdblUNKVZi^iz2$nB!F>!zmdV%Hjk-=yHtD!3{WL!?<{g*n{6E4phUJdro9c0INrY4?rNGY2xDOxPlRWDvE#sM8RY< 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zxVbQmsgpE%o_ybc%bYN~jDK6WJ`J!T2XCcpE6<1UF@}0XI(=y-GGWXxUKx72BCV+c z$NrV87cY(Ha?+0AmXJd|yN_2SXzqnpjGnIb%I@c5mj-mXXYiTCKypnI(@ZTzcug6O zg9+s=uLF!F7ex92`E}(arDMYB>=yw?iAN>_pNhWjjD6ssP*(Tu-^C~Fl6YbQ$NATv zG0`0N{zD|9$+-x%%9kbMZkMRds$+LFfgk7U{fY+L9#Z(0Z zh5%+|euMdOM6ez6+f{oPh~U!ypzk*lc=tbG_E#Rl|b;R50W}fRjQ4le1#e{O_Ghvtkp%^S_{h4Oy|} z;Uizsz?^j0q~K0gY!3J&81(<08Pj58f(h8LS>OX<|Gy<>uss_#4pIah`rDoU53IEj AZvX%Q From 99fcda2c90e295dbb4c961e9cb872d0823a6afa6 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 17:30:43 +0200 Subject: [PATCH 059/119] rename directory --- .../ankExpCalibration.m | 0 .../chenCalibration.m | 0 .../testCalibration.m | 0 3 files changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/calibration/{specific_calibration => specific_calibrations}/ankExpCalibration.m (100%) rename Battery/EquivalentCircuitModel/calibration/{specific_calibration => specific_calibrations}/chenCalibration.m (100%) rename Battery/EquivalentCircuitModel/calibration/{specific_calibration => specific_calibrations}/testCalibration.m (100%) diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibration/ankExpCalibration.m rename to Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibration/chenCalibration.m rename to Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibration/testCalibration.m rename to Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m From 177c961774c5f1f840d8564ba09f0c7b6e44c851 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 23 Jun 2026 10:58:25 +0200 Subject: [PATCH 060/119] update --- .../calibration/specific_calibrations/testCalibration.m | 6 +++++- 1 file changed, 5 insertions(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m index 291ba808d..3e5e16b33 100644 --- a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m @@ -12,6 +12,10 @@ feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); +set(0, 'defaultlinelinewidth', 3); +set(0, 'DefaultAxesFontSize', 16); +set(0, 'defaulttextfontsize', 18); + [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); figure; @@ -29,4 +33,4 @@ 'BackgroundColor', 'white', ... 'EdgeColor', 'black', ... 'FontSize', 11, ... -'FontWeight', 'bold'); \ No newline at end of file +'FontWeight', 'bold'); From 6c0598265fc843c30e5ddfb4a3488a7984247aff Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 23 Jun 2026 14:57:32 +0200 Subject: [PATCH 061/119] double file deleted --- .../specific_calibrations/ankExpCalibration.m | 4 ++++ .../specific_calibrations/chenCalibration.m | 8 +++++++- .../notebooks/calibrationECM.mlx | Bin 994433 -> 999175 bytes 3 files changed, 11 insertions(+), 1 deletion(-) diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m index 0b03911b1..dec9cfb71 100644 --- a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m @@ -14,6 +14,10 @@ pmax = params0 * a; scales = [pmin, pmax]; +set(0, 'defaultlinelinewidth', 3); +set(0, 'DefaultAxesFontSize', 16); +set(0, 'defaulttextfontsize', 18); + feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m index d400dde3f..adc9a48dc 100644 --- a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m @@ -12,7 +12,13 @@ [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); - + + +set(0, 'defaultlinelinewidth', 3); +set(0, 'DefaultAxesFontSize', 16); +set(0, 'defaulttextfontsize', 18); + + figure; plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); diff --git a/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx 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.../{calibration => examples}/pxdParamsImpact/param_dependency.m | 0 .../{calibration => examples}/pxdParamsImpact/porosity_impact.m | 0 .../pxdParamsImpact/reactionRateConstant_impact.m | 0 .../pxdParamsImpact/referenceDiffusionCoefficient_impact.m | 0 .../pxdParamsImpact/saturationConcentration_impact.m | 0 .../pxdParamsImpact/volumefraction_impact.m | 0 .../pxdParamsImpact/volumetricSurfaceArea_impact.m | 0 .../specific_calibrations/ankExpCalibration.m | 0 .../specific_calibrations/chenCalibration.m | 0 .../specific_calibrations/testCalibration.m | 0 16 files changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/{ => calibration}/utils/costFunctionECM.m (100%) rename Battery/EquivalentCircuitModel/calibration/{plotting => utils}/plot_nyquist_params.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/activationEnergyOfReaction_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/bruggeman_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/doubleLayerCapacitance_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/electronicConductivity_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/param_dependency.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/porosity_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/reactionRateConstant_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/referenceDiffusionCoefficient_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/saturationConcentration_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/volumefraction_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/pxdParamsImpact/volumetricSurfaceArea_impact.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/specific_calibrations/ankExpCalibration.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/specific_calibrations/chenCalibration.m (100%) rename Battery/EquivalentCircuitModel/{calibration => examples}/specific_calibrations/testCalibration.m (100%) diff --git a/Battery/EquivalentCircuitModel/utils/costFunctionECM.m b/Battery/EquivalentCircuitModel/calibration/utils/costFunctionECM.m similarity index 100% rename from Battery/EquivalentCircuitModel/utils/costFunctionECM.m rename to Battery/EquivalentCircuitModel/calibration/utils/costFunctionECM.m diff --git a/Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_params.m b/Battery/EquivalentCircuitModel/calibration/utils/plot_nyquist_params.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_params.m rename to Battery/EquivalentCircuitModel/calibration/utils/plot_nyquist_params.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/activationEnergyOfReaction_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/bruggeman_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/doubleLayerCapacitance_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/electronicConductivity_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/param_dependency.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/param_dependency.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/porosity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/porosity_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/reactionRateConstant_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/referenceDiffusionCoefficient_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/saturationConcentration_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumefraction_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumetricSurfaceArea_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibrations/ankExpCalibration.m rename to Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibrations/chenCalibration.m rename to Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/specific_calibrations/testCalibration.m rename to Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m From 62bdd45bde5c9d8b37753076f8e9ee4abf843a54 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Fri, 26 Jun 2026 11:08:20 +0200 Subject: [PATCH 063/119] uselesss function deleted --- .../calibration/utils/costFunctionEIS.m | 15 --------------- 1 file changed, 15 deletions(-) delete mode 100644 Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m diff --git a/Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m b/Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m deleted file mode 100644 index 28a284906..000000000 --- a/Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m +++ /dev/null @@ -1,15 +0,0 @@ -function [total_error, Z_re_exp, Z_im_exp] = costFunctionEIS(best_params) - - - Z_re_exp = plot_nyquist_ank.Z_real; - Z_im_exp = plot_nyquist_ank.Z_imag; - - - omega = logspace(-2, 4, 100) - - Z_re_params = plot_nyquist_params.Z_real(best_params); - Z_im_params = plot_nyquist_params.Z_imag(best_params); - - totalerror = sum((Z_re_exp(omega)-Z_re_params(omega)).^2) + sum((Z_im_exp(omega)-Z_im_params(omega))^2) - -end From 8093641b009739de4e38a18a0d7e73453a9691f8 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 29 Jun 2026 11:22:04 +0200 Subject: [PATCH 064/119] mapEisToEcmTable() added --- .../calibration/mapEisToEcmTable.m | 63 ++++++++++++++ .../calibration/runClassFitting.m | 83 ++++++++++--------- .../{exampleECM.m => RvariationSOC.m} | 0 .../utils/plotExperience.m | 4 +- 4 files changed, 107 insertions(+), 43 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m rename Battery/EquivalentCircuitModel/examples/{exampleECM.m => RvariationSOC.m} (100%) diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m new file mode 100644 index 000000000..3978c8dbe --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m @@ -0,0 +1,63 @@ +function ecm_table = mapEisToEcmTable() + %% 1. Initialisation + json_path = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-params\jp3-opt-1d-full.json'; + jsonstruct = parseBattmoJson(json_path); + [model, inputparams] = setupModelFromJson(jsonstruct); + state_current = setupInitialState(model); + + soc_list = (1.0:-0.05:0.05)'; + N_steps = length(soc_list); + + results_matrix = zeros(N_steps, 6); + + + C_rate = 1; + t_5percent = 3600 * 0.05 / C_rate; + + %% 2. Main loop + for i = 1:N_steps + current_soc = soc_list(i); + fprintf('\n==================================================\n'); + fprintf(' EIS fitting for SOC = %.2f (%d/%d)\n', current_soc, i, N_steps); + fprintf('==================================================\n'); + + %% extraction de l'EIS par computeImpedance() + + %% extraction des paramètres ECM + p = runClassFitting(Z_re, Z_im, omega); + + % Stockage dans la matrice de résultats + results_matrix(i, 1) = current_soc; + results_matrix(i, 2:6) = p; % Insère [R0, R1, C1, R2, C2] + + %% Décharge de 5% pour passer au SOC suivant + if i < N_steps + fprintf(' 5%% discharge...\n'); + inputparams.Control.controlPolicy = 'CCDischarge'; + inputparams.Control.DRate = C_rate; + jsonstruct.TimeStepping.tmax = t_5percent; + + schedule_pulse = model.setupSchedule(jsonstruct); + [~, states_pulse] = simulateBattery(model, state_current, schedule_pulse); + + % Micro-relaxation + inputparams.Control.DRate = 0; + jsonstruct.TimeStepping.tmax = 60; % 1 minute de repos + schedule_rest = model.setupSchedule(jsonstruct); + [~, states_rest] = simulateBattery(model, states_pulse{end}, schedule_rest); + + % L'état courant est mis à jour pour le prochain tour de boucle + state_current = states_rest{end}; + end + end + + %% 3. Printing final table + ecm_table = array2table(results_matrix, 'VariableNames', ... + {'SOC', 'R0', 'R1', 'C1', 'R2', 'C2'}); + + fprintf('\n--- CARTOGRAPHIE DES PARAMÈTRES ECM TERMINÉE ---\n'); + disp(ecm_table); + + % automatic save + save('ecm_map_results.mat', 'ecm_table'); +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m index 59dbedd95..5f58028da 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m +++ b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m @@ -1,44 +1,45 @@ - -%% Main code: - -% filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; -% filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; -% -% [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); -% [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); -[Z_re_exp, Z_im_exp, omega] = load_chen_data(); - -% omega = logspace(-4, 2, 50); -% params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; -% [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); - -params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - -a = 1000; - -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; -scales_w = params0_w*10; %to be changed between lsq and bfgs - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - - -% [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); -% % Lancement avec LSQNONLIN - - -%% Printing results -feis.plotresults_thevenin(best_params, fitting_error); - -feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin - - - +function p = runClassFitting(Z_re_exp, Z_im_exp, omega) + %% Main code: + + % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; + % filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; + % + % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); + % [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); + % [Z_re_exp, Z_im_exp, omega] = load_chen_data(); + + % omega = logspace(-4, 2, 50); + % params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; + % [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); + + params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + + a = 1000; + + pmin = params0 / a; + pmax = params0 * a; + scales = [pmin, pmax]; + + params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; + scales_w = params0_w*10; %to be changed between lsq and bfgs + + feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + + [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + + + % [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); + % % Lancement avec LSQNONLIN + + + %% Printing results + if nargin == 2 + feis.plotresults_thevenin(best_params, fitting_error); + + feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin + end + +end %% Robustness test % for i = 1:5 diff --git a/Battery/EquivalentCircuitModel/examples/exampleECM.m b/Battery/EquivalentCircuitModel/examples/RvariationSOC.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/exampleECM.m rename to Battery/EquivalentCircuitModel/examples/RvariationSOC.m diff --git a/Battery/EquivalentCircuitModel/utils/plotExperience.m b/Battery/EquivalentCircuitModel/utils/plotExperience.m index d18f714cc..597cf60d6 100644 --- a/Battery/EquivalentCircuitModel/utils/plotExperience.m +++ b/Battery/EquivalentCircuitModel/utils/plotExperience.m @@ -21,11 +21,11 @@ inputparams.Control.controlPolicy = 'CCDischarge'; inputparams.Control.DRate = 2; - inputparams.Control.tmax = 30; + % inputparams.Control.tmax = 30; inputparams.Control.rampupTime = 0.1; inputparams.Control.lowerCutoffVoltage = 2.5; - schedule1 = setupSchedule(model, inputparams); + schedule1 = model.setupSchedule(jsonstruct); [~, states1] = simulateBattery(model, state0, schedule1); state_after_pulse = states1{end}; From 573def5215803bf03ddadd59ccf9d9b09648efc5 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 30 Jun 2026 16:26:30 +0200 Subject: [PATCH 065/119] validation program in time domain working --- .../calibration/mapEisToEcmTable.m | 71 ++++++-- .../calibration/runClassFitting.m | 6 +- .../calibration/utils/load_chen_data.m | 2 +- .../examples/validateEcmTime.m | 152 ++++++++++++++++++ Battery/ImpedanceSolver.m | 10 +- 5 files changed, 220 insertions(+), 21 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/examples/validateEcmTime.m diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m index 3978c8dbe..cb9de18a1 100644 --- a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m +++ b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m @@ -1,16 +1,21 @@ function ecm_table = mapEisToEcmTable() %% 1. Initialisation - json_path = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-params\jp3-opt-1d-full.json'; - jsonstruct = parseBattmoJson(json_path); + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + + jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + + [model, inputparams] = setupModelFromJson(jsonstruct); state_current = setupInitialState(model); - soc_list = (1.0:-0.05:0.05)'; + soc_list = (1.0:-0.1:0.1)'; N_steps = length(soc_list); results_matrix = zeros(N_steps, 6); - + freq = logspace(-4, 2, 50)./(2*pi); C_rate = 1; t_5percent = 3600 * 0.05 / C_rate; @@ -22,13 +27,30 @@ fprintf('==================================================\n'); %% extraction de l'EIS par computeImpedance() + options = struct(); + + options.stateInitialization.computeSteadyState = false; + + options.stateInitialization.initializationSetup = 'given state'; + extrastructs.initstate = state_current; + + impsolv = ImpedanceSolver(inputparams, options, extrastructs); + + fprintf('Linearisation...\n'); + Z = impsolv.computeImpedance(freq); + + + Z_re = real(Z)'; + Z_im = imag(Z)'; + omega = (2*pi).*freq; + %% extraction des paramètres ECM p = runClassFitting(Z_re, Z_im, omega); % Stockage dans la matrice de résultats results_matrix(i, 1) = current_soc; - results_matrix(i, 2:6) = p; % Insère [R0, R1, C1, R2, C2] + results_matrix(i, 2:6) = p; %% Décharge de 5% pour passer au SOC suivant if i < N_steps @@ -37,15 +59,40 @@ inputparams.Control.DRate = C_rate; jsonstruct.TimeStepping.tmax = t_5percent; - schedule_pulse = model.setupSchedule(jsonstruct); - [~, states_pulse] = simulateBattery(model, state_current, schedule_pulse); + model.Control = model.setupControl(inputparams.Control); + + % CONVERSIONS MANUELLES DU SCHEDULE (Plus de setupScheduleStep !) + % On découpe les 180s en 10 étapes de 18s pour aider le solveur à converger + N_substeps = 10; + schedule_pulse = struct(); + schedule_pulse.step.val = ones(N_substeps, 1) * (t_5percent / N_substeps); + schedule_pulse.step.control = ones(N_substeps, 1); + % Cette fonction anonyme renvoie le courant Imax calculé par BattMo + schedule_pulse.control.src = @(t, varargin) varargin{end}; + + schedule_pulse.control.Control = struct('stopFunction', @(model, state, state0) false); + + % Simulation du pulse de décharge + % simulateScheduleAD avec l'état en premier argument + [~, states_pulse, ~] = simulateScheduleAD(state_current, model, schedule_pulse); + + % --- Micro-relaxation (Pause de 1 minute) --- + fprintf(' 1 min pause...\n'); + inputparams.Control.DRate = 0; % Courant nul + model.Control = model.setupControl(inputparams.Control); - % Micro-relaxation - inputparams.Control.DRate = 0; - jsonstruct.TimeStepping.tmax = 60; % 1 minute de repos - schedule_rest = model.setupSchedule(jsonstruct); - [~, states_rest] = simulateBattery(model, states_pulse{end}, schedule_rest); + % Construction manuelle du schedule de repos + N_rest_steps = 5; + schedule_rest = struct(); + schedule_rest.step.val = ones(N_rest_steps, 1) * (60 / N_rest_steps); + schedule_rest.step.control = ones(N_rest_steps, 1); + schedule_rest.control.src = @(t, varargin) varargin{end}; + + schedule_rest.control.Control = struct('stopFunction', @(model, state, state0) false); + % Simulation du repos + [~, states_rest, ~] = simulateScheduleAD(states_pulse{end}, model, schedule_rest); + % L'état courant est mis à jour pour le prochain tour de boucle state_current = states_rest{end}; end diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m index 5f58028da..a0db93ddd 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m +++ b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m @@ -1,4 +1,4 @@ -function p = runClassFitting(Z_re_exp, Z_im_exp, omega) +function p = runClassFitting(Z_re_exp, Z_im_exp, omega, print) %print is a boolean, if one gives it to the function it will plot the results. %% Main code: % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; @@ -27,13 +27,13 @@ [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - + p = best_params; % [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); % % Lancement avec LSQNONLIN %% Printing results - if nargin == 2 + if nargin == 4 feis.plotresults_thevenin(best_params, fitting_error); feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin diff --git a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m index 0fe056cb7..a05b021e5 100644 --- a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m @@ -28,7 +28,7 @@ if includeDoubleLayer jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 30; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; end diff --git a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m new file mode 100644 index 000000000..29694f278 --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m @@ -0,0 +1,152 @@ +function validateEcmTime() + %% ==================================================================== + %% STEP 1 : DATA LOADING AND OCV CATCHING + %% ==================================================================== + + if exist('ecm_map_results.mat', 'file') + load('ecm_map_results.mat', 'ecm_table'); + else + error('file not found ecm_map_results.mat. Run mapEisToEcmTable first.'); + end + + % Cathode (Positive) + json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); + json_pe = parseBattmoJson(json_pe_path); + [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); + + % Anode (Negative) + json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); + json_ne = parseBattmoJson(json_ne_path); + [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); + + % 1.3. Generation of the "Ground Truth": Continuous P2D discharge (BattMo) + % We run a constant current discharge WITHOUT any pauses to serve as a temporal reference + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + + [model, inputparams] = setupModelFromJson(jsonstruct); + state_init = setupInitialState(model); + + C_rate = 1; + t_sim = 3200; % Duration in seconds, be careful not to reach the computed SOC limit (here <10%) + + inputparams.Control.controlPolicy = 'CCDischarge'; + inputparams.Control.DRate = C_rate; + model.Control = model.setupControl(inputparams.Control); + + % Continuous schedule construction + dt_step = 10; + N_sim_steps = floor(t_sim / dt_step); + schedule_p2d = struct(); + schedule_p2d.step.val = ones(N_sim_steps, 1) * dt_step; + schedule_p2d.step.control = ones(N_sim_steps, 1); + schedule_p2d.control.src = @(t, varargin) varargin{end}; + schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); + + fprintf('Simulation of the P2D physical model (BattMo) in progress...\n'); + [~, states_p2d, ~] = simulateScheduleAD(state_init, model, schedule_p2d); + + % Extraction of time vectors from the P2D model + N_points = length(states_p2d); + time_vec = zeros(N_points, 1); + V_p2d = zeros(N_points, 1); + I_p2d = zeros(N_points, 1); + + for k = 1:N_points + time_vec(k) = states_p2d{k}.time; + V_p2d(k) = states_p2d{k}.Control.E; + I_p2d(k) = states_p2d{k}.Control.I; + end + + % Coulomb Counting to obtain SOC + total_charge = trapz(time_vec, I_p2d); + soc_p2d = 1 - cumtrapz(time_vec, I_p2d) / total_charge; + + %% ==================================================================== + %% STEP 2 : ECM EQUATIONS IMPLEMENTATION (Simulation) + %% ==================================================================== + fprintf('\n--- Step 2: Time-domain simulation of the ECM model (2-RC) ---\n'); + + V_ecm = zeros(N_points, 1); + + % Initialization of ECM electrical state variables + Uc1 = 0; % Initial voltage across RC branch #1 (V) + Uc2 = 0; % Initial voltage across RC branch #2 (V) + + for k = 1:N_points + % Calculation of the real time-step (dt) + if k == 1 + dt = time_vec(1); + else + dt = time_vec(k) - time_vec(k-1); + end + + I = I_p2d(k); % Current measured at this timestamp (A) + soc = soc_p2d(k); % SOC estimated at this timestamp + + % 2.1. Dynamic interpolation of fitted ECM parameters according to SOC + R0 = interp1(ecm_table.SOC, ecm_table.R0, soc, 'linear', 'extrap'); + R1 = interp1(ecm_table.SOC, ecm_table.R1, soc, 'linear', 'extrap'); + C1 = interp1(ecm_table.SOC, ecm_table.C1, soc, 'linear', 'extrap'); + R2 = interp1(ecm_table.SOC, ecm_table.R2, soc, 'linear', 'extrap'); + C2 = interp1(ecm_table.SOC, ecm_table.C2, soc, 'linear', 'extrap'); + + % 2.2. Evaluation of the exact thermodynamic OCV via setupFunction + % For the Positive Electrode (NMC Cathode) + pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + + % For the Negative Electrode (Graphite Anode) + ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + + % Note: Chen2020 uses stoichiometry (0 to 1) instead of raw SOC. + x_pe = soc * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; + % Translation of SOC into stoichiometry for the anode (Negative) + x_ne = soc * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; + + % 3. Calculation of the true open circuit voltage of the cell + V_ocv = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); + + % 2.3. Solving the Differential Equations of the RC branches (Explicit Euler) + Uc1_next = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2_next = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + + % 2.4. Calculation of the final cell voltage (Kirchhoff's Voltage Law) + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + % Passing states to the next step + Uc1 = Uc1_next; + Uc2 = Uc2_next; + end + + %% ==================================================================== + %% STEP 3 : PLOTTING THE TWO FUNCTIONS (Visualization) + %% ==================================================================== + fprintf('\n--- Step 3: Generating comparison plots ---\n'); + + figure('Color', 'w', 'Name', 'Validation P2D vs ECM', 'Position', [100, 100, 900, 600]); + + % Voltage Plot + subplot(2,1,1); + plot(time_vec, V_p2d, 'b-', 'LineWidth', 2.5); hold on; + plot(time_vec, V_ecm, 'r--', 'LineWidth', 2); + grid on; + ylabel('Cell Voltage (V)', 'FontSize', 11); + title('Time-domain validation: Physical P2D Model vs Reduced ECM', 'FontSize', 13); + legend('Ground Truth : BattMo P2D', 'Reduced Model : ECM (2-RC fitted by EIS)', 'Location', 'SouthWest'); + + % Absolute Voltage Error Plot + subplot(2,1,2); + error_voltage = abs(V_p2d - V_ecm) * 1000; % Conversion to mV + plot(time_vec, error_voltage, 'k-', 'LineWidth', 1.5); + grid on; + xlabel('Time (s)', 'FontSize', 11); + ylabel('Absolute Error (mV)', 'FontSize', 11); + title('Instantaneous error of the equivalent circuit model', 'FontSize', 11); + + % Calculation of the global mean error for the analysis report + rmse = sqrt(mean((V_p2d - V_ecm).^2)) * 1000; + fprintf('*** Analysis complete! Root Mean Square Error (RMSE): %.2f mV ***\n', rmse); +end \ No newline at end of file diff --git a/Battery/ImpedanceSolver.m b/Battery/ImpedanceSolver.m index a76ef5cc7..81b934f32 100644 --- a/Battery/ImpedanceSolver.m +++ b/Battery/ImpedanceSolver.m @@ -71,21 +71,21 @@ end - function Z = computeImpedance(impsolv, omegas) + function Z = computeImpedance(impsolv, freqs) DM = impsolv.DM; DA = impsolv.DA; b = impsolv.b; indUs = impsolv.indUs; - for iomega = 1 : numel(omegas) + for ifreq = 1 : numel(freqs) - omega = omegas(iomega); + freq = freqs(ifreq); - A = (i*2*pi*omega*DM + DA); + A = (i*2*pi*freq*DM + DA); x = A\b; - Z(iomega) = x(indUs(1) : indUs(2)); + Z(ifreq) = x(indUs(1) : indUs(2)); end From c82a35c415be31f744003f2899e9d01a77b77be8 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Wed, 1 Jul 2026 16:45:27 +0200 Subject: [PATCH 066/119] evrything works/ table in right order/ plotEcmSoc added --- .../calibration/mapEisToEcmTable.m | 25 ++-- .../calibration/plotting/plotEcmSoc.m | 55 +++++++++ .../examples/validateEcmTime.m | 113 +++++++++++------- 3 files changed, 141 insertions(+), 52 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m index cb9de18a1..147a18e2b 100644 --- a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m +++ b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m @@ -9,15 +9,16 @@ [model, inputparams] = setupModelFromJson(jsonstruct); state_current = setupInitialState(model); - - soc_list = (1.0:-0.1:0.1)'; + + soc_step = 0.08; + soc_list = (1.0:-soc_step:0.1)'; N_steps = length(soc_list); results_matrix = zeros(N_steps, 6); freq = logspace(-4, 2, 50)./(2*pi); C_rate = 1; - t_5percent = 3600 * 0.05 / C_rate; + t_xpercent = 3600 * soc_step / C_rate; %% 2. Main loop for i = 1:N_steps @@ -54,18 +55,18 @@ %% Décharge de 5% pour passer au SOC suivant if i < N_steps - fprintf(' 5%% discharge...\n'); + fprintf(' %02d %% discharge...\n', soc_step); inputparams.Control.controlPolicy = 'CCDischarge'; inputparams.Control.DRate = C_rate; - jsonstruct.TimeStepping.tmax = t_5percent; + jsonstruct.TimeStepping.tmax = t_xpercent; model.Control = model.setupControl(inputparams.Control); - % CONVERSIONS MANUELLES DU SCHEDULE (Plus de setupScheduleStep !) + % CONVERSIONS MANUELLES DU SCHEDULE % On découpe les 180s en 10 étapes de 18s pour aider le solveur à converger N_substeps = 10; schedule_pulse = struct(); - schedule_pulse.step.val = ones(N_substeps, 1) * (t_5percent / N_substeps); + schedule_pulse.step.val = ones(N_substeps, 1) * (t_xpercent / N_substeps); schedule_pulse.step.control = ones(N_substeps, 1); % Cette fonction anonyme renvoie le courant Imax calculé par BattMo schedule_pulse.control.src = @(t, varargin) varargin{end}; @@ -102,9 +103,13 @@ ecm_table = array2table(results_matrix, 'VariableNames', ... {'SOC', 'R0', 'R1', 'C1', 'R2', 'C2'}); - fprintf('\n--- CARTOGRAPHIE DES PARAMÈTRES ECM TERMINÉE ---\n'); + % ecm_table = sortrows(ecm_table, 'SOC', 'ascend'); + disp(ecm_table); + + file_name = sprintf('ecm_map_results_%02d.mat', soc_step * 100); - % automatic save - save('ecm_map_results.mat', 'ecm_table'); + + save(file_name, 'ecm_table'); + fprintf('Table saved successfully as: %s\n', file_name); end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m new file mode 100644 index 000000000..aad075337 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m @@ -0,0 +1,55 @@ +function plotEcmSoc(file_name) + % Set default file name if no argument is provided + if nargin < 1 + file_name = 'ecm_map_results_10.mat'; + end + + % Check if the file exists and load it + if exist(file_name, 'file') + load(file_name, 'ecm_table'); + else + error(['File not found: ', file_name]); + end + + % Create a clean figure window + figure('Color', 'w', 'Name', 'ECM Parameters vs SOC', 'Position', [100, 100, 1100, 700]); + + % 1. Plot Ohmic Resistance R0 + subplot(2,3,1); + plot(ecm_table.SOC * 100, ecm_table.R0, 'b-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'b'); + grid on; + xlabel('SOC (%)'); ylabel('R0 (\Omega)'); + title('Internal Resistance (R0)'); + + % 2. Plot RC1 Resistance R1 + subplot(2,3,2); + plot(ecm_table.SOC * 100, ecm_table.R1, 'r-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'r'); + grid on; + xlabel('SOC (%)'); ylabel('R1 (\Omega)'); + title('Charge Transfer Resistance (R1)'); + + % 3. Plot RC1 Capacitance C1 + subplot(2,3,3); + plot(ecm_table.SOC * 100, ecm_table.C1, 'm-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'm'); + grid on; + xlabel('SOC (%)'); ylabel('C1 (F)'); + title('Double Layer Capacitance (C1)'); + + % 4. Plot RC2 Resistance R2 + subplot(2,3,4); + plot(ecm_table.SOC * 100, ecm_table.R2, 'g-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'g'); + grid on; + xlabel('SOC (%)'); ylabel('R2 (\Omega)'); + title('Diffusion Resistance (R2)'); + + % 5. Plot RC2 Capacitance C2 + subplot(2,3,5); + plot(ecm_table.SOC * 100, ecm_table.C2, 'k-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'k'); + grid on; + xlabel('SOC (%)'); ylabel('C2 (F)'); + title('Diffusion Capacitance (C2)'); + + % Global title for the entire figure + sgtitle(['Fitted ECM Parameters Evolution across SOC Range - File: ', file_name], ... + 'FontSize', 14, 'FontWeight', 'bold'); +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m index 29694f278..4f8fe3114 100644 --- a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m +++ b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m @@ -1,12 +1,19 @@ -function validateEcmTime() +function validateEcmTime(file_name) + %% ==================================================================== %% STEP 1 : DATA LOADING AND OCV CATCHING %% ==================================================================== - if exist('ecm_map_results.mat', 'file') - load('ecm_map_results.mat', 'ecm_table'); + % Set default file name if no argument is provided + if nargin < 1 + file_name = 'ecm_map_results_10.mat'; + end + + % Check if the file exists and load it + if exist(file_name, 'file') + load(file_name, 'ecm_table'); else - error('file not found ecm_map_results.mat. Run mapEisToEcmTable first.'); + error(['File not found: ', file_name]); end % Cathode (Positive) @@ -20,28 +27,34 @@ function validateEcmTime() [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); % 1.3. Generation of the "Ground Truth": Continuous P2D discharge (BattMo) - % We run a constant current discharge WITHOUT any pauses to serve as a temporal reference jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); [model, inputparams] = setupModelFromJson(jsonstruct); - state_init = setupInitialState(model); - C_rate = 1; - t_sim = 3200; % Duration in seconds, be careful not to reach the computed SOC limit (here <10%) + %% New time-varying current profile setup + custom_time = [0, 100, 600, 800, 1500, 2000]; + custom_current = [0, 5, -2, 0, 6, 0]; % Current profile in Amperes + + t_sim = custom_time(end); - inputparams.Control.controlPolicy = 'CCDischarge'; - inputparams.Control.DRate = C_rate; + % FIX HERE: Keeping CCDischarge ensures the MRST time-stepper steps correctly + inputparams.Control.controlPolicy = 'CCDischarge'; model.Control = model.setupControl(inputparams.Control); - % Continuous schedule construction - dt_step = 10; + % Safe initialization using the standard policy branch + state_init = setupInitialState(model); + + % Building the fine-grained time schedule (2-second steps) + dt_step = 50; N_sim_steps = floor(t_sim / dt_step); schedule_p2d = struct(); schedule_p2d.step.val = ones(N_sim_steps, 1) * dt_step; schedule_p2d.step.control = ones(N_sim_steps, 1); - schedule_p2d.control.src = @(t, varargin) varargin{end}; + + % Dynamically feed the current profile into the simulation via interpolation + schedule_p2d.control.src = @(t, varargin) interp1(custom_time, custom_current, t, 'previous', 0); schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); fprintf('Simulation of the P2D physical model (BattMo) in progress...\n'); @@ -52,6 +65,14 @@ function validateEcmTime() time_vec = zeros(N_points, 1); V_p2d = zeros(N_points, 1); I_p2d = zeros(N_points, 1); + soc_p2d = zeros(N_points, 1); % Pre-allocation du vrai SOC + + + pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + sat_conc_ne = model.NegativeElectrode.Coating.ActiveMaterial.Interface.saturationConcentration; for k = 1:N_points time_vec(k) = states_p2d{k}.time; @@ -60,9 +81,15 @@ function validateEcmTime() end % Coulomb Counting to obtain SOC - total_charge = trapz(time_vec, I_p2d); - soc_p2d = 1 - cumtrapz(time_vec, I_p2d) / total_charge; - + [Q_nominal, ~] = computeCellCapacity(model); + + % Genuine SOC calculation tracking the real capacity depletion + soc_p2d = 1 - cumtrapz(time_vec, I_p2d) / Q_nominal; + + % Security boundary to avoid interpolation out-of-bounds [0, 1] + soc_p2d = max(0, min(1, soc_p2d)); + + %% ==================================================================== %% STEP 2 : ECM EQUATIONS IMPLEMENTATION (Simulation) %% ==================================================================== @@ -75,15 +102,14 @@ function validateEcmTime() Uc2 = 0; % Initial voltage across RC branch #2 (V) for k = 1:N_points - % Calculation of the real time-step (dt) if k == 1 dt = time_vec(1); else dt = time_vec(k) - time_vec(k-1); end - I = I_p2d(k); % Current measured at this timestamp (A) - soc = soc_p2d(k); % SOC estimated at this timestamp + I = I_p2d(k); + soc = soc_p2d(k); % 2.1. Dynamic interpolation of fitted ECM parameters according to SOC R0 = interp1(ecm_table.SOC, ecm_table.R0, soc, 'linear', 'extrap'); @@ -92,21 +118,10 @@ function validateEcmTime() R2 = interp1(ecm_table.SOC, ecm_table.R2, soc, 'linear', 'extrap'); C2 = interp1(ecm_table.SOC, ecm_table.C2, soc, 'linear', 'extrap'); - % 2.2. Evaluation of the exact thermodynamic OCV via setupFunction - % For the Positive Electrode (NMC Cathode) - pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; - pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; - % For the Negative Electrode (Graphite Anode) - ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; - ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; - - % Note: Chen2020 uses stoichiometry (0 to 1) instead of raw SOC. x_pe = soc * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; - % Translation of SOC into stoichiometry for the anode (Negative) x_ne = soc * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; - % 3. Calculation of the true open circuit voltage of the cell V_ocv = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); % 2.3. Solving the Differential Equations of the RC branches (Explicit Euler) @@ -116,37 +131,51 @@ function validateEcmTime() % 2.4. Calculation of the final cell voltage (Kirchhoff's Voltage Law) V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; - % Passing states to the next step Uc1 = Uc1_next; Uc2 = Uc2_next; end - %% ==================================================================== - %% STEP 3 : PLOTTING THE TWO FUNCTIONS (Visualization) + %% ==================================================================== + %% STEP 3 : PLOTTING THE THREE FUNCTIONS (Visualization) %% ==================================================================== fprintf('\n--- Step 3: Generating comparison plots ---\n'); - figure('Color', 'w', 'Name', 'Validation P2D vs ECM', 'Position', [100, 100, 900, 600]); + % Hauteur augmentée à 800 pixels pour accueillir confortablement les 3 subplots + figure('Color', 'w', 'Name', 'Validation P2D vs ECM', 'Position', [100, 100, 900, 800]); - % Voltage Plot - subplot(2,1,1); + % --- SUBPLOT 1: Tension (Axe gauche) & Courant (Axe droit) --- + subplot(3,1,1); + yyaxis left plot(time_vec, V_p2d, 'b-', 'LineWidth', 2.5); hold on; plot(time_vec, V_ecm, 'r--', 'LineWidth', 2); - grid on; ylabel('Cell Voltage (V)', 'FontSize', 11); + ax = gca; ax.YColor = 'k'; + + yyaxis right + plot(time_vec, I_p2d, 'g-', 'LineWidth', 1.5); + ylabel('Current (A)', 'FontSize', 11); + ax.YColor = 'g'; + + grid on; title('Time-domain validation: Physical P2D Model vs Reduced ECM', 'FontSize', 13); - legend('Ground Truth : BattMo P2D', 'Reduced Model : ECM (2-RC fitted by EIS)', 'Location', 'SouthWest'); + legend('Ground Truth: BattMo P2D', 'Reduced Model: ECM (2-RC)', 'Input Current Profile', 'Location', 'SouthWest'); + + % --- SUBPLOT 2: Profil du SOC physique au cours du temps --- + subplot(3,1,2); + plot(time_vec, soc_p2d * 100, 'Color', [0.4660, 0.6740, 0.1880], 'LineWidth', 2); % Tracé en pourcentage + grid on; + ylabel('State of Charge (%)', 'FontSize', 11); + title('Physical State of Charge (SOC) profile extracted from BattMo', 'FontSize', 11); - % Absolute Voltage Error Plot - subplot(2,1,2); - error_voltage = abs(V_p2d - V_ecm) * 1000; % Conversion to mV + % --- SUBPLOT 3: Erreur absolue de tension --- + subplot(3,1,3); + error_voltage = abs(V_p2d - V_ecm) * 1000; plot(time_vec, error_voltage, 'k-', 'LineWidth', 1.5); grid on; xlabel('Time (s)', 'FontSize', 11); ylabel('Absolute Error (mV)', 'FontSize', 11); title('Instantaneous error of the equivalent circuit model', 'FontSize', 11); - % Calculation of the global mean error for the analysis report rmse = sqrt(mean((V_p2d - V_ecm).^2)) * 1000; fprintf('*** Analysis complete! Root Mean Square Error (RMSE): %.2f mV ***\n', rmse); end \ No newline at end of file From 0809fd334dbd3f7ab9bf9407a0ed8e174423f557 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 6 Jul 2026 11:59:03 +0200 Subject: [PATCH 067/119] fittingTime working --- .../calibration/FittingTime.m | 288 ++++++++++++++++++ .../calibration/mapEisToEcmTable.m | 7 +- .../calibration/plotting/plotEcmSoc.m | 24 +- .../calibration/runClassFitting.m | 25 +- .../calibration/runClassFittingTime.m | 29 ++ .../examples/robustnessTest.m | 15 + .../examples/validateEcmTime.m | 27 +- .../utils/loadP2dVoltage.m | 66 ++++ 8 files changed, 433 insertions(+), 48 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/FittingTime.m create mode 100644 Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m create mode 100644 Battery/EquivalentCircuitModel/examples/robustnessTest.m create mode 100644 Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m new file mode 100644 index 000000000..7171dcb41 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -0,0 +1,288 @@ +classdef FittingTime + + properties + params0 + scales + time_vec + current_exp + voltage_exp + ocv_vec + end + + + methods + + function ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec) + + + if istable(params0), params0 = table2array(params0); end + if istable(scales), scales = table2array(scales); end + if istable(time_vec), time_vec = table2array(time_vec); end + if istable(current_exp), current_exp = table2array(current_exp); end + if istable(voltage_exp), voltage_exp = table2array(voltage_exp); end + if istable(ocv_vec), ocv_vec = table2array(ocv_vec); end + + ftime.params0 = double(params0(:)); + ftime.scales = double(scales(:)); + ftime.time_vec = double(time_vec(:)); + ftime.current_exp = double(current_exp(:)); + ftime.voltage_exp = double(voltage_exp(:)); + ftime.ocv_vec = double(ocv_vec(:)); + end + + + function p_norm = unscaled2scaled(ftime, p) + pmin = ftime.scales(1:5); + pmax = ftime.scales(6:10); + p_norm = (p-pmin)./(pmax-pmin); + end + + function p = scaled2unscaled(ftime, p_norm) + pmin = ftime.scales(1:5); + pmax = ftime.scales(6:10); + p = (pmax-pmin).*p_norm +pmin; + end + + + function [min_value, history, best_params, fitting_error] = optimizationBFGS(ftime) + + + f_opt = @(p_norm) ftime.optifunc(scaled2unscaled(ftime, p_norm)); + + params0_norm = unscaled2scaled(ftime, ftime.params0); + % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); + params0_norm = params0_norm(:); + + pmin = ftime.scales(1:5); + pmax = ftime.scales(6:10); + p03min = pmin(3); + p03max = pmax(3); + p05min = pmin(5); + p05max = pmax(5); + + A_custom = [0, 0, -1, 0, 2*(p05max - p05min)/(p03max- p03min)]; + b_custom = (p03min-2*p05min)/(p03max - p03min); + + max_iter = 300; + tol_obj = 1e-15; + tol_grad = 1e-5; + + [min_value, best_params_norm, history] = unitBoxBFGS(... + params0_norm, ... + f_opt, ... + 'maximize', false, ... + 'linIneq', struct('A', A_custom, 'b', b_custom), ... %A*u<=b + 'enforceFeasible', true, ... + 'maxIt', max_iter, ... + 'objChangeTol', tol_obj, ... + 'gradTol', tol_grad, ... + 'lineSearchMaxIt', 100 ... + ); + best_params = scaled2unscaled(ftime, best_params_norm(:) ); + + % explications of why it stopped + fitting_error = ftime.optifunc(best_params); + + it_count = length(history.val) - 1; + final_pg = history.pg(end); + + % Cost function variation + if it_count >= 1 + delta_v = abs(history.val(end) - history.val(end-1)); + else + delta_v = inf; + end + + if it_count >= max_iter + fprintf('Stopped because %d iterations reached.\n', max_iter); + elseif final_pg < tol_grad + fprintf('Stopped because reached gradTol = %e.\n', tol_grad); + elseif delta_v < tol_obj + fprintf('Stopped because reached objChangeTol = %e.\n', tol_obj); + else + fprintf('Unexpected error or relative tolerance reached.\n'); + end + + + end + + function [v, g_norm] = optifunc(ftime, p) + + % Preventing physical values to get too close from 0 + p_safe = max(p, 1e-8); + R0 = p_safe(1); + R1 = p_safe(2); + C1 = p_safe(3); + R2 = p_safe(4); + C2 = p_safe(5); + + N_points = length(ftime.time_vec); + V_ecm = zeros(N_points, 1); + + + Uc1 = 0; + Uc2 = 0; + + % Sensibilities initialisation + + s_R1 = 0; % dUc1 / dR1 + s_C1 = 0; % dUc1 / dC1 + s_R2 = 0; % dUc2 / dR2 + s_C2 = 0; % dUc2 / dC2 + + g_true = zeros(5, 1); + + for k = 1:N_points + if k == 1 + dt = ftime.time_vec(1); + else + dt = ftime.time_vec(k) - ftime.time_vec(k-1); + end + + I = ftime.current_exp(k); + V_ocv = ftime.ocv_vec(k); + + % 1. Tension du modèle au pas k + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + % 2. Erreur instantanée + err = ftime.voltage_exp(k) - V_ecm(k); + + % 3. Si le gradient est demandé (nargout > 1) + if nargout > 1 + % Dérivées partielles de V_ecm par rapport à chaque paramètre + dV_dR0 = -I; + dV_dR1 = -s_R1; + dV_dC1 = -s_C1; + dV_dR2 = -s_R2; + dV_dC2 = -s_C2; + + % Accumulation du gradient de la fonction coût (v = sum(err^2)) + g_true(1) = g_true(1) - 2 * err * dV_dR0; + g_true(2) = g_true(2) - 2 * err * dV_dR1; + g_true(3) = g_true(3) - 2 * err * dV_dC1; + g_true(4) = g_true(4) - 2 * err * dV_dR2; + g_true(5) = g_true(5) - 2 * err * dV_dC2; + + % Mise à jour des sensibilités pour le pas suivant (Euler Explicite) + s_R1 = s_R1 + (-s_R1 / (R1 * C1) + Uc1 / (R1^2 * C1)) * dt; + s_C1 = s_C1 + (-s_C1 / (R1 * C1) + Uc1 / (R1 * C1^2) - I / C1^2) * dt; + s_R2 = s_R2 + (-s_R2 / (R2 * C2) + Uc2 / (R2^2 * C2)) * dt; + s_C2 = s_C2 + (-s_C2 / (R2 * C2) + Uc2 / (R2 * C2^2) - I / C2^2) * dt; + end + + % 4. Mise à jour des variables d'état électriques pour le pas suivant + Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + end + + % Valeur de la fonction objectif (Erreur quadratique totale) + v = sum((ftime.voltage_exp - V_ecm).^2); + + % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé + if nargout > 1 + pmin = ftime.scales(1:5); + pmax = ftime.scales(6:10); + dp_dpnorm = (pmax - pmin); + g_norm = g_true .* dp_dpnorm(:); + end + end + + function plotresults_thevenin(ftime, best_params, fitting_error) + % 1. Recalculate the final voltage trajectory using best_params + p_safe = max(best_params, 1e-8); + R0 = p_safe(1); + R1 = p_safe(2); + C1 = p_safe(3); + R2 = p_safe(4); + C2 = p_safe(5); + + N_points = length(ftime.time_vec); + V_ecm = zeros(N_points, 1); + Uc1 = 0; + Uc2 = 0; + + for k = 1:N_points + if k == 1 + dt = ftime.time_vec(1); + else + dt = ftime.time_vec(k) - ftime.time_vec(k-1); + end + I = ftime.current_exp(k); + V_ocv = ftime.ocv_vec(k); + + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + end + + % 2. Generate time-domain plots + figure('Name', 'ECM Time Domain Fitting Results', 'NumberTitle', 'off'); + + % Subplot 1: Applied Current Profile + subplot(3,1,1); + plot(ftime.time_vec, ftime.current_exp, 'k', 'LineWidth', 1.5); + grid on; + title('Applied Current Profile'); + xlabel('Time (s)'); + ylabel('Current (A)'); + + % Subplot 2: Voltage Comparison (Exp vs Model) + subplot(3,1,2); + plot(ftime.time_vec, ftime.voltage_exp, 'r-', 'MarkerSize', 8); + hold on; + plot(ftime.time_vec, V_ecm, 'b-', 'LineWidth', 1.5); + grid on; + legend('Experimental / P2D', 'Optimized ECM', 'Location', 'best'); + title('Cell Voltage Fitting'); + xlabel('Time (s)'); + ylabel('Voltage (V)'); + + % Subplot 3: Instantaneous Residual Error (V_exp - V_ecm) + subplot(3,1,3); + error_vec = ftime.voltage_exp - V_ecm; + plot(ftime.time_vec, error_vec, 'g', 'LineWidth', 1.2); + grid on; + title('Residual Error (V_{exp} - V_{ecm})'); + xlabel('Time (s)'); + ylabel('Error (V)'); + + % Text box displaying the global fitting score + text_error = sprintf('Fitting Error (SSR): %.2e V²', fitting_error); + text(0.05, 0.15, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + end + + function printResults(ftime, best_params, fitting_error) + % Extraction des paramètres + R0 = best_params(1); + R1 = best_params(2); + C1 = best_params(3); + R2 = best_params(4); + C2 = best_params(5); + + % Calcul des constantes de temps (tau = R * C) + tau1 = R1 * C1; + tau2 = R2 * C2; + + % Calcul de la RMSE pour un affichage plus parlant qu'une simple somme quadratique + rmse_mv = sqrt(fitting_error / length(ftime.time_vec)) * 1000; + + fprintf('\n=======================================\n'); + fprintf(' FITTING RESULTS (TIME DOMAIN) \n'); + fprintf('=======================================\n'); + fprintf('Total Error (SSR) : %.4e V²\n', fitting_error); + + fprintf('R0 : %.4e Ohms\n', R0); + fprintf('R1 : %.4e Ohms\n', R1); + fprintf('C1 : %.4e Farads\n', C1); + fprintf('R2 : %.4e Ohms\n', R2); + fprintf('C2 : %.4e Farads\n', C2); + end + end + +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m index 147a18e2b..1119d7bfe 100644 --- a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m +++ b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m @@ -1,4 +1,4 @@ -function ecm_table = mapEisToEcmTable() +function ecm_table = mapEisToEcmTable(soc_step) %% 1. Initialisation jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); @@ -9,8 +9,9 @@ [model, inputparams] = setupModelFromJson(jsonstruct); state_current = setupInitialState(model); - - soc_step = 0.08; + if nargin < 1 + soc_step = 0.1; + end soc_list = (1.0:-soc_step:0.1)'; N_steps = length(soc_list); diff --git a/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m index aad075337..30fe743a3 100644 --- a/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m +++ b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m @@ -1,7 +1,7 @@ function plotEcmSoc(file_name) % Set default file name if no argument is provided if nargin < 1 - file_name = 'ecm_map_results_10.mat'; + file_name = 'ecm_map_results_08.mat'; end % Check if the file exists and load it @@ -18,38 +18,38 @@ function plotEcmSoc(file_name) subplot(2,3,1); plot(ecm_table.SOC * 100, ecm_table.R0, 'b-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'b'); grid on; - xlabel('SOC (%)'); ylabel('R0 (\Omega)'); - title('Internal Resistance (R0)'); + xlabel('SOC (%)'); ylabel('R_0 (\Omega)'); + title('Internal Resistance (R_0)'); % 2. Plot RC1 Resistance R1 subplot(2,3,2); plot(ecm_table.SOC * 100, ecm_table.R1, 'r-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'r'); grid on; - xlabel('SOC (%)'); ylabel('R1 (\Omega)'); - title('Charge Transfer Resistance (R1)'); + xlabel('SOC (%)'); ylabel('R_1 (\Omega)'); + title('Charge Transfer Resistance (R_1)'); % 3. Plot RC1 Capacitance C1 subplot(2,3,3); plot(ecm_table.SOC * 100, ecm_table.C1, 'm-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'm'); grid on; - xlabel('SOC (%)'); ylabel('C1 (F)'); - title('Double Layer Capacitance (C1)'); + xlabel('SOC (%)'); ylabel('C_1 (F)'); + title('Double Layer Capacitance (C_1)'); % 4. Plot RC2 Resistance R2 subplot(2,3,4); plot(ecm_table.SOC * 100, ecm_table.R2, 'g-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'g'); grid on; - xlabel('SOC (%)'); ylabel('R2 (\Omega)'); - title('Diffusion Resistance (R2)'); + xlabel('SOC (%)'); ylabel('R_2 (\Omega)'); + title('Diffusion Resistance (R_2)'); % 5. Plot RC2 Capacitance C2 subplot(2,3,5); plot(ecm_table.SOC * 100, ecm_table.C2, 'k-o', 'LineWidth', 1.5, 'MarkerFaceColor', 'k'); grid on; - xlabel('SOC (%)'); ylabel('C2 (F)'); - title('Diffusion Capacitance (C2)'); + xlabel('SOC (%)'); ylabel('C_2 (F)'); + title('Diffusion Capacitance (C_2)'); % Global title for the entire figure sgtitle(['Fitted ECM Parameters Evolution across SOC Range - File: ', file_name], ... - 'FontSize', 14, 'FontWeight', 'bold'); + 'FontSize', 14, 'FontWeight', 'bold', 'Interpreter', 'none'); end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m index a0db93ddd..566ba31a5 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m +++ b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m @@ -12,6 +12,9 @@ % params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); + % params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; + % scales_w = params0_w*10; %to be changed between lsq and bfgs + params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 a = 1000; @@ -19,21 +22,16 @@ pmin = params0 / a; pmax = params0 * a; scales = [pmin, pmax]; - - params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; - scales_w = params0_w*10; %to be changed between lsq and bfgs - + feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); p = best_params; - % [min_value, best_params, fitting_error] = feis.optimizationLsqnonlin(); - % % Lancement avec LSQNONLIN %% Printing results - if nargin == 4 + if nargin == 4 || nargin == 1 feis.plotresults_thevenin(best_params, fitting_error); feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin @@ -41,20 +39,7 @@ end -%% Robustness test -% for i = 1:5 - % params0 = pmin + (pmax - pmin) .* rand(1, 5); - % disp(['Tour ', num2str(i), ' - params0 :']); - % disp(params0); - % feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - % - % [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - % feis.plotresults_thevenin(best_params, fitting_error); - % feis.printResults(best_params, fitting_error); - % - % drawnow; -% end %% % result with lsqnonlin: diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m new file mode 100644 index 000000000..5d1a4c9fd --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m @@ -0,0 +1,29 @@ +function p = runClassFittingTime(pr) + +%% Main code: + time_init = (0:100:1000)'; + current_init = ones(size(time_init));[time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(time_init, current_init); + + params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + + a = 1000; + + pmin = params0 / a; + pmax = params0 * a; + scales = [pmin, pmax]; + + ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec); + + [~, ~, best_params, fitting_error] = ftime.optimizationBFGS(); + + p = best_params; + + + %% Printing results + if nargin == 4 || nargin == 1 + ftime.plotresults_thevenin(best_params, fitting_error); + + ftime.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin + end + +end diff --git a/Battery/EquivalentCircuitModel/examples/robustnessTest.m b/Battery/EquivalentCircuitModel/examples/robustnessTest.m new file mode 100644 index 000000000..d9f2f22de --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/robustnessTest.m @@ -0,0 +1,15 @@ +%% Robustness test for fitting programm + +for i = 1:5 + params0 = pmin + (pmax - pmin) .* rand(1, 5); + disp(['Tour ', num2str(i), ' - params0 :']); + disp(params0); + feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + + [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + feis.plotresults_thevenin(best_params, fitting_error); + feis.printResults(best_params, fitting_error); + + drawnow; + +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m index 4f8fe3114..1f6448242 100644 --- a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m +++ b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m @@ -16,17 +16,9 @@ function validateEcmTime(file_name) error(['File not found: ', file_name]); end - % Cathode (Positive) - json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); - json_pe = parseBattmoJson(json_pe_path); - [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); - % Anode (Negative) - json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); - json_ne = parseBattmoJson(json_ne_path); - [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); - % 1.3. Generation of the "Ground Truth": Continuous P2D discharge (BattMo) + % Generation of the "Ground Truth": Continuous P2D discharge (BattMo) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); @@ -65,14 +57,12 @@ function validateEcmTime(file_name) time_vec = zeros(N_points, 1); V_p2d = zeros(N_points, 1); I_p2d = zeros(N_points, 1); - soc_p2d = zeros(N_points, 1); % Pre-allocation du vrai SOC pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; - ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; - sat_conc_ne = model.NegativeElectrode.Coating.ActiveMaterial.Interface.saturationConcentration; + ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; for k = 1:N_points time_vec(k) = states_p2d{k}.time; @@ -117,8 +107,19 @@ function validateEcmTime(file_name) C1 = interp1(ecm_table.SOC, ecm_table.C1, soc, 'linear', 'extrap'); R2 = interp1(ecm_table.SOC, ecm_table.R2, soc, 'linear', 'extrap'); C2 = interp1(ecm_table.SOC, ecm_table.C2, soc, 'linear', 'extrap'); + + % Loading of ocp functions with setupFunction + % Cathode (Positive) + json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); + json_pe = parseBattmoJson(json_pe_path); + [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); - + % Anode (Negative) + json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); + json_ne = parseBattmoJson(json_ne_path); + [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); + + %link between soc and stoechiometry x_pe = soc * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; x_ne = soc * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; diff --git a/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m b/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m new file mode 100644 index 000000000..219c37188 --- /dev/null +++ b/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m @@ -0,0 +1,66 @@ +function [time_sim, I_p2d, V_p2d, ocv_vec] = loadP2dVoltage(time_vec, current_exp) + + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + + [model, inputparams] = setupModelFromJson(jsonstruct); + + inputparams.Control.controlPolicy = 'CCDischarge'; + model.Control = model.setupControl(inputparams.Control); + + state_init = setupInitialState(model); + + time_vec = double(time_vec(:)); + current_exp = double(current_exp(:)); + + dt_steps = diff(time_vec); + N_sim_steps = length(dt_steps); + + schedule_p2d = struct(); + schedule_p2d.step.val = dt_steps; + schedule_p2d.step.control = ones(N_sim_steps, 1); + + schedule_p2d.control.src = @(t, varargin) interp1(time_vec, current_exp, t, 'linear', 0); + schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); + + fprintf('Simulation of the P2D physical model (BattMo) in progress...\n'); + [~, states_p2d, ~] = simulateScheduleAD(state_init, model, schedule_p2d); + + N_points_sim = length(states_p2d); + V_p2d = zeros(N_points_sim, 1); + I_p2d = zeros(N_points_sim, 1); + time_sim = zeros(N_points_sim, 1); % On le nomme distinctement + + pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + + for k = 1:N_points_sim + time_sim(k) = states_p2d{k}.time; + V_p2d(k) = states_p2d{k}.Control.E; + I_p2d(k) = states_p2d{k}.Control.I; + end + + [Q_nominal, ~] = computeCellCapacity(model); + + soc_p2d = 1 - cumtrapz(time_sim, I_p2d) / Q_nominal; + soc_p2d = max(0, min(1, soc_p2d)); + + json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); + json_pe = parseBattmoJson(json_pe_path); + [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); + + json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); + json_ne = parseBattmoJson(json_ne_path); + [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); + + ocv_vec = zeros(N_points_sim, 1); + for idx = 1:N_points_sim + soc_now = soc_p2d(idx); + x_pe = soc_now * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; + x_ne = soc_now * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; + ocv_vec(idx) = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); + end +end \ No newline at end of file From 6c05ebe96004c8cf973f664703f98458c397ec77 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 6 Jul 2026 17:08:27 +0200 Subject: [PATCH 068/119] time simulation enhanced --- .../EquivalentCircuitModel/calibration/FittingTime.m | 11 ++++++++++- .../calibration/runClassFittingTime.m | 11 +++++++++-- 2 files changed, 19 insertions(+), 3 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 7171dcb41..cd766495a 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -178,7 +178,16 @@ % Valeur de la fonction objectif (Erreur quadratique totale) v = sum((ftime.voltage_exp - V_ecm).^2); - + + + if isnan(v) || isinf(v) || (nargout > 1 && (any(isnan(g_true)) || any(isinf(g_true)))) + v = 1e10; % Assigne un coût massif pour rejeter le point instable + if nargout > 1 + g_norm = zeros(5, 1); % Renvoie un gradient plat pour forcer le pas arrière + end + return; + end + % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé if nargout > 1 pmin = ftime.scales(1:5); diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m index 5d1a4c9fd..341c2519f 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m @@ -1,8 +1,15 @@ function p = runClassFittingTime(pr) %% Main code: - time_init = (0:100:1000)'; - current_init = ones(size(time_init));[time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(time_init, current_init); + time_init = (0:10:1000)'; + current_init = ones(size(time_init)); + + current_init(time_init >= 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) + current_init(time_init >= 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) + current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) + current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) + + [time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(time_init, current_init); params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 From 736c08451e3da8565ba740f8eeca26679ee6a8fc Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 13 Jul 2026 11:06:37 +0200 Subject: [PATCH 069/119] cleaning --- .../calibration/FittingEIS.m | 125 +----------------- .../calibration/FittingTime.m | 87 +++++++++++- .../calibration/runClassFittingTime.m | 4 +- .../examples/validateEcmTime.m | 2 +- .../notebooks/calibrationECM.mlx | Bin 999175 -> 951303 bytes .../utils/loadP2dVoltage.m | 4 +- 6 files changed, 93 insertions(+), 129 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m index 53564e67a..b50182043 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m @@ -304,130 +304,7 @@ - %% lsq method - - function residuals = optifunc_lsq(feis, p) - % 1. On empêche physiquement les paramètres de valoir zéro - p = max(p, 1e-8); - - % 2. Chargement du modèle - [Z_re_param, Z_im_param] = load_nyquist(p, feis.omega); - if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end - if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end - - Z_re_param = double(Z_re_param(:)); - Z_im_param = double(Z_im_param(:)); - - % Si le modèle renvoie du NaN (physiquement impossible), on pénalise - if ~isnumeric(Z_re_param) || ~isreal(Z_re_param) || any(isnan(Z_re_param(:))) - residuals = 1e10 * ones(2 * length(feis.omega), 1); - return; - end - - % 3. Calcul du module pour l'erreur relative - Modulus_Z = sqrt(feis.Z_re_exp.^2 + feis.Z_im_exp.^2); - Modulus_Z = Modulus_Z(:); - - % 4. Vecteurs de résidus (Non mis au carré, lsqnonlin s'en charge) - err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z; - err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z; - - % 5. On empile les parties réelles et imaginaires en un seul vecteur colonne - residuals = [err_re; err_im]; - end - - function [min_value, best_params, resnorm] = optimizationLsqnonlin(feis) - % Fonction objectif : renvoie le vecteur de résidus - f_res = @(p_norm) feis.optifunc_lsq(p_norm(:) .* feis.scales(:)); - - % Paramètres initiaux normés - params0_norm = feis.params0(:) ./ feis.scales(:); - - % Bornes (Limites inférieures strictes > 0 pour éviter les crashs) - lb_norm = ones(5,1) * 1e-5; - ub_norm = ones(5,1) * 1e5./ feis.scales(:); - - % Options de lsqnonlin - options = optimoptions('lsqnonlin', ... - 'Display', 'iter-detailed', ... % Affichage très détaillé - 'Algorithm', 'trust-region-reflective', ... % Parfait pour l'EIS - 'MaxFunctionEvaluations', 3000, ... - 'MaxIterations', 500, ... - 'StepTolerance', 1e-8, ... - 'FunctionTolerance', 1e-6); - - % Lancement de l'optimiseur natif MATLAB - [best_params_norm, resnorm, ~, exitflag, output] = lsqnonlin(... - f_res, params0_norm, lb_norm, ub_norm, options); - - % Récupération des vraies valeurs (dénormalisation) - best_params = best_params_norm(:) .* feis.scales(:); - min_value = resnorm; % Erreur finale (somme des carrés des résidus) - - % Affichage du statut de fin - disp('=== RAISON DE FIN DE LSQNONLIN ==='); - disp(output.message); - end - -%% lsq method warburg - function v = optifunclsq_warburg(feis, p) - p_safe = max(p, 1e-15); - - R0 = p_safe(1); R1 = p_safe(2); Q1 = p_safe(3); a1 = p_safe(4); - R2 = p_safe(5); Q2 = p_safe(6); a2 = p_safe(7); Q = p_safe(8); L = p_safe(9); - - w = feis.omega(:); - s = 1i .* w; - - sa1 = s.^a1; - sa2 = s.^a2; - Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); - - Z_re_param = real(Z_param_cplx); - Z_im_param = imag(Z_param_cplx); - - if any(isnan(Z_re_param)) || any(isnan(Z_im_param)) || any(isinf(Z_re_param)) || any(isinf(Z_im_param)) - v = 1e6; % Pénalité forte mais gérable - return; - end - - Modulus_Z = sqrt(Z_re_param.^2 + Z_im_param.^2); - Modulus_Z = Modulus_Z(:); - - err_re = (feis.Z_re_exp(:) - Z_re_param) ./ Modulus_Z; - err_im = (feis.Z_im_exp(:) - Z_im_param) ./ Modulus_Z; - - v = sum(err_re.^2 + err_im.^2); - - end - - - function [min_value, history, best_params, fitting_error] = optimizationlsq_warburg(feis) - f_opt = @(p_norm) feis.optifunclsq_warburg(p_norm .* feis.scales); - - params0_norm = feis.params0 ./ feis.scales; - params0_norm = params0_norm(:); - - if length(params0_norm) ~= 9 - error('feis.params0 should have 9 parameters but it has %d).', length(params0_norm)); - end - - lb_norm = [1e-10; 1e-10; 1e-10; 1e-3; 1e-10; 1e-10; 0.01; 1e-5; 1e-15] ./ feis.scales; - ub_norm = [1e5; 1e5; 1e6; 1.0; 1e5; 1e6; 1.0; 1e15; 1e-2 ] ./ feis.scales; - - options = optimoptions('fmincon', ... - 'Display', 'iter', ... - 'Algorithm', 'sqp', ... % Très bon pour ce type de fitting - 'SpecifyObjectiveGradient', false, ... - 'MaxFunctionEvaluations', 10000, ... - 'MaxIterations', 1000); - - [best_params_norm, min_value] = fmincon(f_opt, params0_norm, [], [], [], [], lb_norm, ub_norm, [], options); - - history = []; % Si vous n'en avez pas besoin - best_params = best_params_norm(:) .* feis.scales(:); - fitting_error = feis.optifunclsq_warburg(best_params); - end + %% showing the results diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index cd766495a..11df71007 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -148,7 +148,7 @@ % 2. Erreur instantanée err = ftime.voltage_exp(k) - V_ecm(k); - % 3. Si le gradient est demandé (nargout > 1) + if nargout > 1 % Dérivées partielles de V_ecm par rapport à chaque paramètre dV_dR0 = -I; @@ -292,6 +292,91 @@ function printResults(ftime, best_params, fitting_error) fprintf('R2 : %.4e Ohms\n', R2); fprintf('C2 : %.4e Farads\n', C2); end + + + function plottest(ftime, best_params) + % 1. Recalculate the final voltage trajectory using best_params + p_safe = max(best_params, 1e-8); + R0 = p_safe(1); + R1 = p_safe(2); + C1 = p_safe(3); + R2 = p_safe(4); + C2 = p_safe(5); + + % Get original training time grid as a column vector + time_vec = ftime.time_vec(:); + + % Define the 3-pulse test current profile + current_test = ones(size(time_vec)); + current_test(time_vec >= 0 & time_vec < 200) = -5; + current_test(time_vec >= 200 & time_vec < 400) = 5; + current_test(time_vec >= 400 & time_vec < 700) = -5; + current_test(time_vec >= 700 & time_vec <= 1000) = 0; + + + [time_test, current_test_p2d, voltage_test, ocv_test] = loadP2dVoltage(time_vec, current_test); + + % Force all outputs to be column vectors to avoid any plot orientation errors + time_test = time_test(:); + current_test_p2d = current_test_p2d(:); + voltage_test = voltage_test(:); + ocv_test = ocv_test(:); + + % Synchronize the simulation length with the actual P2D points (e.g., 99) + N_points = length(time_test); + + % Initialize ECM state variables + V_ecm = zeros(N_points, 1); + Uc1 = 0; + Uc2 = 0; + + + for k = 1:N_points + if k == 1 + dt = time_test(1); + else + dt = time_test(k) - time_test(k-1); + end + I = current_test_p2d(k); % Use the actual simulated current from BattMo + V_ocv = ocv_test(k); % Use the profile-specific OCV from BattMo + + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + end + + % 2. Generate time-domain plots using the synchronized time_test grid + figure('Name', 'ECM Time Domain Validation Results', 'NumberTitle', 'off'); + + % Subplot 1: Applied Current Profile + subplot(3,1,1); + plot(time_test, current_test_p2d, 'k', 'LineWidth', 1.5); + grid on; + title('Applied Current Profile (P2D Simulated Range)'); + xlabel('Time (s)'); + ylabel('Current (A)'); + + % Subplot 2: Voltage Comparison (P2D vs ECM) + subplot(3,1,2); + plot(time_test, voltage_test, 'r-', 'LineWidth', 1.5); + hold on; + plot(time_test, V_ecm, 'b--', 'LineWidth', 1.5); + grid on; + legend('Ground Truth: P2D Model', 'Validated ECM', 'Location', 'best'); + title('Cell Voltage Validation'); + xlabel('Time (s)'); + ylabel('Voltage (V)'); + + % Subplot 3: Instantaneous Residual Error (V_p2d - V_ecm) + subplot(3,1,3); + error_vec = voltage_test - V_ecm; + plot(time_test, error_vec, 'g', 'LineWidth', 1.2); + grid on; + title('Residual Error (V_{p2d} - V_{ecm})'); + xlabel('Time (s)'); + ylabel('Error (V)'); + end end end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m index 341c2519f..6d68fecfe 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m @@ -30,7 +30,9 @@ if nargin == 4 || nargin == 1 ftime.plotresults_thevenin(best_params, fitting_error); - ftime.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin + ftime.printResults(best_params, fitting_error); + + ftime.plottest(best_params) end end diff --git a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m index 1f6448242..869180023 100644 --- a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m +++ b/Battery/EquivalentCircuitModel/examples/validateEcmTime.m @@ -6,7 +6,7 @@ function validateEcmTime(file_name) 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zl+_@cKkU03#Lri0FC{vcgSpSBeF&fanM91fcPgM4mzx#BjhujEurVU_$)wg~ku!1JFdE zhpk{io&cH<6#o{e;Xf5<4RD}a08JQr*ajZN9f&53S6bLe@F-jLMR9b;{V^|2UF!j2W Date: Mon, 13 Jul 2026 12:49:22 +0200 Subject: [PATCH 070/119] changed names --- .../{runClassFitting.m => classFitting.m} | 4 ++-- ...runClassFittingTime.m => runFittingTime.m} | 22 ++++++++++--------- 2 files changed, 14 insertions(+), 12 deletions(-) rename Battery/EquivalentCircuitModel/calibration/{runClassFitting.m => classFitting.m} (91%) rename Battery/EquivalentCircuitModel/calibration/{runClassFittingTime.m => runFittingTime.m} (54%) diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m b/Battery/EquivalentCircuitModel/calibration/classFitting.m similarity index 91% rename from Battery/EquivalentCircuitModel/calibration/runClassFitting.m rename to Battery/EquivalentCircuitModel/calibration/classFitting.m index 566ba31a5..1d1473a34 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFitting.m +++ b/Battery/EquivalentCircuitModel/calibration/classFitting.m @@ -1,4 +1,4 @@ -function p = runClassFitting(Z_re_exp, Z_im_exp, omega, print) %print is a boolean, if one gives it to the function it will plot the results. +function p = classFitting(Z_re_exp, Z_im_exp, omega, print) %print is a boolean, if one gives it to the function it will plot the results. %% Main code: % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; @@ -63,4 +63,4 @@ % 1.0000e-1 ... % 0.0307 ... % 7.0505e+02 ... -% 2.9134e-06 \ No newline at end of file +% 2.9134e-06 diff --git a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m similarity index 54% rename from Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m rename to Battery/EquivalentCircuitModel/calibration/runFittingTime.m index 6d68fecfe..ca5816be7 100644 --- a/Battery/EquivalentCircuitModel/calibration/runClassFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -1,13 +1,13 @@ -function p = runClassFittingTime(pr) +function p = classFittingTime(pr) %% Main code: time_init = (0:10:1000)'; current_init = ones(size(time_init)); - current_init(time_init >= 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) - current_init(time_init >= 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) - current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) - current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) + current_init(time_init > = 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) + current_init(time_init > = 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) + current_init(time_init > = 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) + current_init(time_init > = 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) [time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(time_init, current_init); @@ -28,11 +28,13 @@ %% Printing results if nargin == 4 || nargin == 1 - ftime.plotresults_thevenin(best_params, fitting_error); - - ftime.printResults(best_params, fitting_error); - - ftime.plottest(best_params) + + ftime.plotresults_thevenin(best_params, fitting_error); + + ftime.printResults(best_params, fitting_error); + + ftime.plottest(best_params) + end end From 8c13e375388edbe31cb6fb0a33407fef1d6c9aae Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 14:02:35 +0200 Subject: [PATCH 071/119] update in EquivalentCircuitModel model --- .../models/EquivalentCircuitModel.m | 42 ++++++----- .../utils/createParametersECM.m | 74 ++++++++++--------- 2 files changed, 62 insertions(+), 54 deletions(-) diff --git a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m index ff38ffcc0..6efb43c50 100644 --- a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m @@ -11,8 +11,6 @@ R2 C2 initSOC - initOverpotential2 - lowerVoltageCutoff I totalTime @@ -25,6 +23,7 @@ C1func R2func C2func + end methods @@ -43,8 +42,6 @@ 'R2' , ... 'C2' , ... 'initSOC' , ... - 'initOverpotential2' , ... - 'lowerVoltageCutoff' , ... 'I' , ... 'totalTime'}; @@ -52,11 +49,11 @@ model.OCPfunc = setupFunction(model.OCP); model.Ifunc = setupFunction(model.I); - model.R0func = setupFunction(model.R0); - model.R1func = setupFunction(model.R1); - model.C1func = setupFunction(model.C1); - model.R2func = setupFunction(model.R2); - model.C2func = setupFunction(model.C2); + model.R0func = setupFunction(model.R0); + model.R1func = setupFunction(model.R1); + model.C1func = setupFunction(model.C1); + model.R2func = setupFunction(model.R2); + model.C2func = setupFunction(model.C2); end @@ -72,7 +69,7 @@ % varnames{end + 1} = 'U'; - varnames{end + 1} = 'UR'; + varnames{end + 1} = 'U0'; varnames{end + 1} = 'U1'; varnames{end + 1} = 'U2'; varnames{end + 1} = 'SOC'; @@ -83,9 +80,9 @@ model = model.registerVarNames(varnames); - fn = @EquivalentCircuitModel.updateUR; + fn = @EquivalentCircuitModel.updateU0; inputnames = {'I'}; - model = model.registerPropFunction({'UR', fn, inputnames}); + model = model.registerPropFunction({'U0', fn, inputnames}); fn = @EquivalentCircuitModel.updatedU1dt; inputnames = {'U1', 'I'}; @@ -100,14 +97,18 @@ model = model.registerPropFunction({'dSOCdt', fn, inputnames}); fn = @EquivalentCircuitModel.updateU; - inputnames = {'SOC', 'U1', 'U2', 'UR'}; - model = model.registerPropFunction({'U', fn, inputnames}); + inputnames = {'OCP', 'U1', 'U2', 'U0'}; + model = model.registerPropFunction({'U', fn, inputnames}); + + fn = @EquivalentCircuitModel.updateOCP; + inputnames = {'SOC'}; + model = model.registerPropFunction({'OCP', fn, inputnames}); end - function state = updateUR(model, state) + function state = updateU0(model, state) - state.UR = model.R0func(state.SOC)*state.I; + state.U0 = model.R0func(state.SOC)*state.I; end @@ -133,11 +134,16 @@ function state = updateU(model, state) - OCP = model.OCPfunc(state.SOC); - state.U = OCP - (state.U1 + state.U2 + state.UR); + state.U = state.OCP - (state.U1 + state.U2 + state.U0); end + function state = updateOCP(model, state) + + state.OCP = model.OCPfunc(state.SOC); + + end + function state0 = setupInitialCondition(model, SOC0) state0.U1 = 0; diff --git a/Battery/EquivalentCircuitModel/utils/createParametersECM.m b/Battery/EquivalentCircuitModel/utils/createParametersECM.m index 4e2c35f7d..7e8603649 100644 --- a/Battery/EquivalentCircuitModel/utils/createParametersECM.m +++ b/Battery/EquivalentCircuitModel/utils/createParametersECM.m @@ -1,20 +1,22 @@ -function p = createParametersECM() +function jsonstruct = createParametersECM() + + % create example data set for ECM - p.nominalcellcapacity = 63.7; - p.initSOC = 1.0; - p.lowerVoltageCutoff = 3.0; - p.initOverpotential2 = 0; - p.totalTime = 4200; - - p.I.functionFormat = 'tabulated'; - p.I.argumentList = {'time'}; - p.I.dataX = [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200]; - p.I.dataY = [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0]; - - p.OCP.functionFormat = 'tabulated'; - p.OCP.argumentList = {'SOC'}; - p.OCP.dataX = [0.00, 0.02, 0.04, 0.06, 0.08, 0.10, 0.12, 0.14, 0.16, 0.18, 0.20, 0.22, 0.24, 0.26, 0.28, 0.30, 0.32, 0.34, 0.36, 0.38, 0.40, 0.42, 0.44, 0.46, 0.48, 0.50, 0.52, 0.54, 0.56, 0.58, 0.60, 0.62, 0.64, 0.66, 0.68, 0.70, 0.72, 0.74, 0.76, 0.78, 0.80, 0.82, 0.84, 0.86, 0.88, 0.90, 0.92, 0.94, 0.96, 0.98, 1.00]; - p.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]; + jsonstruct.nominalcellcapacity = 63.7; + jsonstruct.initSOC = 1.0; + jsonstruct.lowerVoltageCutoff = 3.0; + jsonstruct.initOverpotential2 = 0; + jsonstruct.totalTime = 4200; + + jsonstruct.I.functionFormat = 'tabulated'; + jsonstruct.I.argumentList = {'time'}; + jsonstruct.I.dataX = [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200]; + jsonstruct.I.dataY = [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0]; + + jsonstruct.OCP.functionFormat = 'tabulated'; + jsonstruct.OCP.argumentList = {'SOC'}; + jsonstruct.OCP.dataX = [0.00, 0.02, 0.04, 0.06, 0.08, 0.10, 0.12, 0.14, 0.16, 0.18, 0.20, 0.22, 0.24, 0.26, 0.28, 0.30, 0.32, 0.34, 0.36, 0.38, 0.40, 0.42, 0.44, 0.46, 0.48, 0.50, 0.52, 0.54, 0.56, 0.58, 0.60, 0.62, 0.64, 0.66, 0.68, 0.70, 0.72, 0.74, 0.76, 0.78, 0.80, 0.82, 0.84, 0.86, 0.88, 0.90, 0.92, 0.94, 0.96, 0.98, 1.00]; + jsonstruct.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]; R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; @@ -31,29 +33,29 @@ C2 = tau2 ./ R2; - p.R0.functionFormat = 'tabulated'; - p.R0.argumentList = {'SOC'}; - p.R0.dataX = p.OCP.dataX; % same axis as SOC - p.R0.dataY = R0; + jsonstruct.R0.functionFormat = 'tabulated'; + jsonstruct.R0.argumentList = {'SOC'}; + jsonstruct.R0.dataX = jsonstruct.OCP.dataX; % same axis as SOC + jsonstruct.R0.dataY = R0; - p.R1.functionFormat = 'tabulated'; - p.R1.argumentList = {'SOC'}; - p.R1.dataX = p.OCP.dataX; - p.R1.dataY = R1; + jsonstruct.R1.functionFormat = 'tabulated'; + jsonstruct.R1.argumentList = {'SOC'}; + jsonstruct.R1.dataX = jsonstruct.OCP.dataX; + jsonstruct.R1.dataY = R1; - p.C1.functionFormat = 'tabulated'; - p.C1.argumentList = {'SOC'}; - p.C1.dataX = p.OCP.dataX; - p.C1.dataY = C1; + jsonstruct.C1.functionFormat = 'tabulated'; + jsonstruct.C1.argumentList = {'SOC'}; + jsonstruct.C1.dataX = jsonstruct.OCP.dataX; + jsonstruct.C1.dataY = C1; - p.R2.functionFormat = 'tabulated'; - p.R2.argumentList = {'SOC'}; - p.R2.dataX = p.OCP.dataX; - p.R2.dataY = R2; + jsonstruct.R2.functionFormat = 'tabulated'; + jsonstruct.R2.argumentList = {'SOC'}; + jsonstruct.R2.dataX = jsonstruct.OCP.dataX; + jsonstruct.R2.dataY = R2; - p.C2.functionFormat = 'tabulated'; - p.C2.argumentList = {'SOC'}; - p.C2.dataX = p.OCP.dataX; - p.C2.dataY = C2; + jsonstruct.C2.functionFormat = 'tabulated'; + jsonstruct.C2.argumentList = {'SOC'}; + jsonstruct.C2.dataX = jsonstruct.OCP.dataX; + jsonstruct.C2.dataY = C2; end From 65b774c5d0ce2e95caf9b33328ae33bfbca92882 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 13:41:36 +0200 Subject: [PATCH 072/119] some clean-up --- .../calibration/FittingTime.m | 111 +++--------------- .../calibration/mapEisToEcmTable.m | 4 +- .../calibration/plotting/plotEcmSoc.m | 17 +-- .../calibration/runFittingTime.m | 71 +++++------ .../calibration/runMapEisToEcmTable.m | 4 + .../EquivalentCircuitModel/functions/runECM.m | 91 ++++++++++++++ .../utils/loadP2dVoltage.m | 11 +- 7 files changed, 161 insertions(+), 148 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m create mode 100644 Battery/EquivalentCircuitModel/functions/runECM.m diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 11df71007..7945db93e 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -1,12 +1,16 @@ classdef FittingTime properties - params0 - scales - time_vec - current_exp - voltage_exp - ocv_vec + + params0 % initial guess for the parameters to be fitted + scales % scaling for the unit box optimization + + time_vec % time steps for current_exp and voltage_exp + current_exp % experimental current values + voltage_exp % experimental voltage values + + ocv_vec % open circuit voltage values computed from a model + end @@ -106,95 +110,14 @@ end + function [v, g_norm] = optifunc(ftime, p) - + % Preventing physical values to get too close from 0 p_safe = max(p, 1e-8); - R0 = p_safe(1); - R1 = p_safe(2); - C1 = p_safe(3); - R2 = p_safe(4); - C2 = p_safe(5); - - N_points = length(ftime.time_vec); - V_ecm = zeros(N_points, 1); - - - Uc1 = 0; - Uc2 = 0; - - % Sensibilities initialisation - - s_R1 = 0; % dUc1 / dR1 - s_C1 = 0; % dUc1 / dC1 - s_R2 = 0; % dUc2 / dR2 - s_C2 = 0; % dUc2 / dC2 - - g_true = zeros(5, 1); - - for k = 1:N_points - if k == 1 - dt = ftime.time_vec(1); - else - dt = ftime.time_vec(k) - ftime.time_vec(k-1); - end - - I = ftime.current_exp(k); - V_ocv = ftime.ocv_vec(k); - - % 1. Tension du modèle au pas k - V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; - - % 2. Erreur instantanée - err = ftime.voltage_exp(k) - V_ecm(k); - - - if nargout > 1 - % Dérivées partielles de V_ecm par rapport à chaque paramètre - dV_dR0 = -I; - dV_dR1 = -s_R1; - dV_dC1 = -s_C1; - dV_dR2 = -s_R2; - dV_dC2 = -s_C2; - - % Accumulation du gradient de la fonction coût (v = sum(err^2)) - g_true(1) = g_true(1) - 2 * err * dV_dR0; - g_true(2) = g_true(2) - 2 * err * dV_dR1; - g_true(3) = g_true(3) - 2 * err * dV_dC1; - g_true(4) = g_true(4) - 2 * err * dV_dR2; - g_true(5) = g_true(5) - 2 * err * dV_dC2; - - % Mise à jour des sensibilités pour le pas suivant (Euler Explicite) - s_R1 = s_R1 + (-s_R1 / (R1 * C1) + Uc1 / (R1^2 * C1)) * dt; - s_C1 = s_C1 + (-s_C1 / (R1 * C1) + Uc1 / (R1 * C1^2) - I / C1^2) * dt; - s_R2 = s_R2 + (-s_R2 / (R2 * C2) + Uc2 / (R2^2 * C2)) * dt; - s_C2 = s_C2 + (-s_C2 / (R2 * C2) + Uc2 / (R2 * C2^2) - I / C2^2) * dt; - end - - % 4. Mise à jour des variables d'état électriques pour le pas suivant - Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; - Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; - end - - % Valeur de la fonction objectif (Erreur quadratique totale) - v = sum((ftime.voltage_exp - V_ecm).^2); - - if isnan(v) || isinf(v) || (nargout > 1 && (any(isnan(g_true)) || any(isinf(g_true)))) - v = 1e10; % Assigne un coût massif pour rejeter le point instable - if nargout > 1 - g_norm = zeros(5, 1); % Renvoie un gradient plat pour forcer le pas arrière - end - return; - end + output = runECM(p_safe, input, options) - % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé - if nargout > 1 - pmin = ftime.scales(1:5); - pmax = ftime.scales(6:10); - dp_dpnorm = (pmax - pmin); - g_norm = g_true .* dp_dpnorm(:); - end end function plotresults_thevenin(ftime, best_params, fitting_error) @@ -267,6 +190,7 @@ function plotresults_thevenin(ftime, best_params, fitting_error) end function printResults(ftime, best_params, fitting_error) + % Extraction des paramètres R0 = best_params(1); R1 = best_params(2); @@ -295,8 +219,10 @@ function printResults(ftime, best_params, fitting_error) function plottest(ftime, best_params) + % 1. Recalculate the final voltage trajectory using best_params p_safe = max(best_params, 1e-8); + R0 = p_safe(1); R1 = p_safe(2); C1 = p_safe(3); @@ -313,7 +239,6 @@ function plottest(ftime, best_params) current_test(time_vec >= 400 & time_vec < 700) = -5; current_test(time_vec >= 700 & time_vec <= 1000) = 0; - [time_test, current_test_p2d, voltage_test, ocv_test] = loadP2dVoltage(time_vec, current_test); % Force all outputs to be column vectors to avoid any plot orientation errors @@ -329,7 +254,6 @@ function plottest(ftime, best_params) V_ecm = zeros(N_points, 1); Uc1 = 0; Uc2 = 0; - for k = 1:N_points if k == 1 @@ -376,7 +300,8 @@ function plottest(ftime, best_params) title('Residual Error (V_{p2d} - V_{ecm})'); xlabel('Time (s)'); ylabel('Error (V)'); + end end -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m index 1119d7bfe..0b795bf3a 100644 --- a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m +++ b/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m @@ -1,4 +1,6 @@ function ecm_table = mapEisToEcmTable(soc_step) + % soc_step : soc increment between 0 and 1. Start from soc = 1. + %% 1. Initialisation jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); @@ -113,4 +115,4 @@ save(file_name, 'ecm_table'); fprintf('Table saved successfully as: %s\n', file_name); -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m index 30fe743a3..f3f4e1b4c 100644 --- a/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m +++ b/Battery/EquivalentCircuitModel/calibration/plotting/plotEcmSoc.m @@ -1,15 +1,4 @@ -function plotEcmSoc(file_name) - % Set default file name if no argument is provided - if nargin < 1 - file_name = 'ecm_map_results_08.mat'; - end - - % Check if the file exists and load it - if exist(file_name, 'file') - load(file_name, 'ecm_table'); - else - error(['File not found: ', file_name]); - end +function plotEcmSoc(ecm_table) % Create a clean figure window figure('Color', 'w', 'Name', 'ECM Parameters vs SOC', 'Position', [100, 100, 1100, 700]); @@ -50,6 +39,6 @@ function plotEcmSoc(file_name) title('Diffusion Capacitance (C_2)'); % Global title for the entire figure - sgtitle(['Fitted ECM Parameters Evolution across SOC Range - File: ', file_name], ... + sgtitle('Fitted ECM Parameters Evolution across SOC Range', ... 'FontSize', 14, 'FontWeight', 'bold', 'Interpreter', 'none'); -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m index ca5816be7..c8b3af121 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -1,40 +1,45 @@ -function p = classFittingTime(pr) - -%% Main code: - time_init = (0:10:1000)'; - current_init = ones(size(time_init)); - - current_init(time_init > = 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) - current_init(time_init > = 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) - current_init(time_init > = 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) - current_init(time_init > = 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) +%% Time fitting - [time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(time_init, current_init); - params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - - a = 1000; - - pmin = params0 / a; - pmax = params0 * a; - scales = [pmin, pmax]; - - ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec); +%% Setup current input +time_init = (0:10:1000)'; +current_init = ones(size(time_init)); + +current_init(time_init >= 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) +current_init(time_init >= 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) +current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) +current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); +jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + +[time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(jsonstruct, time_init, current_init); + +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec); + +[~, ~, best_params, fitting_error] = ftime.optimizationBFGS(); + +p = best_params; + + +doprint = true; +%% Printing results +if doprint - [~, ~, best_params, fitting_error] = ftime.optimizationBFGS(); + ftime.plotresults_thevenin(best_params, fitting_error); - p = best_params; + ftime.printResults(best_params, fitting_error); + ftime.plottest(best_params) - %% Printing results - if nargin == 4 || nargin == 1 - - ftime.plotresults_thevenin(best_params, fitting_error); - - ftime.printResults(best_params, fitting_error); - - ftime.plottest(best_params) - - end - end + diff --git a/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m new file mode 100644 index 000000000..d5a80d0ef --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m @@ -0,0 +1,4 @@ +soc_step = 0.5; +ecm_table = mapEisToEcmTable(soc_step); +plotEcmSoc(ecm_table); + diff --git a/Battery/EquivalentCircuitModel/functions/runECM.m b/Battery/EquivalentCircuitModel/functions/runECM.m new file mode 100644 index 000000000..5ba0577be --- /dev/null +++ b/Battery/EquivalentCircuitModel/functions/runECM.m @@ -0,0 +1,91 @@ +function output = runECM(params, input, options) + + + R0 = params(1); + R1 = params(2); + C1 = params(3); + R2 = params(4); + C2 = params(5); + + + N_points = length(input.time_vec); + V_ecm = zeros(N_points, 1); + + Uc1 = 0; + Uc2 = 0; + + % Sensibilities initialisation + + s_R1 = 0; % dUc1 / dR1 + s_C1 = 0; % dUc1 / dC1 + s_R2 = 0; % dUc2 / dR2 + s_C2 = 0; % dUc2 / dC2 + + g_true = zeros(5, 1); + + for k = 1:N_points + + if k == 1 + dt = input.time_vec(1); + else + dt = input.time_vec(k) - input.time_vec(k-1); + end + + I = input.current_exp(k); + + V_ocv = input.ocv_vec(k); + + % 1. Tension du modèle au pas k + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + % 2. Erreur instantanée + err = input.voltage_exp(k) - V_ecm(k); + + if nargout > 1 + % Dérivées partielles de V_ecm par rapport à chaque paramètre + dV_dR0 = -I; + dV_dR1 = -s_R1; + dV_dC1 = -s_C1; + dV_dR2 = -s_R2; + dV_dC2 = -s_C2; + + % Accumulation du gradient de la fonction coût (v = sum(err^2)) + g_true(1) = g_true(1) - 2 * err * dV_dR0; + g_true(2) = g_true(2) - 2 * err * dV_dR1; + g_true(3) = g_true(3) - 2 * err * dV_dC1; + g_true(4) = g_true(4) - 2 * err * dV_dR2; + g_true(5) = g_true(5) - 2 * err * dV_dC2; + + % Mise à jour des sensibilités pour le pas suivant (Euler Explicite) + s_R1 = s_R1 + (-s_R1 / (R1 * C1) + Uc1 / (R1^2 * C1)) * dt; + s_C1 = s_C1 + (-s_C1 / (R1 * C1) + Uc1 / (R1 * C1^2) - I / C1^2) * dt; + s_R2 = s_R2 + (-s_R2 / (R2 * C2) + Uc2 / (R2^2 * C2)) * dt; + s_C2 = s_C2 + (-s_C2 / (R2 * C2) + Uc2 / (R2 * C2^2) - I / C2^2) * dt; + end + + % 4. Mise à jour des variables d'état électriques pour le pas suivant + Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + end + + % Valeur de la fonction objectif (Erreur quadratique totale) + v = sum((input.voltage_exp - V_ecm).^2); + + + if isnan(v) || isinf(v) || (nargout > 1 && (any(isnan(g_true)) || any(isinf(g_true)))) + v = 1e10; % Assigne un coût massif pour rejeter le point instable + if nargout > 1 + g_norm = zeros(5, 1); % Renvoie un gradient plat pour forcer le pas arrière + end + return; + end + + % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé + if nargout > 1 + pmin = input.scales(1:5); + pmax = input.scales(6:10); + dp_dpnorm = (pmax - pmin); + g_norm = g_true .* dp_dpnorm(:); + end + +end diff --git a/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m b/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m index cfb4f221e..32f87f115 100644 --- a/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m +++ b/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m @@ -1,8 +1,5 @@ -function [time_sim, I_p2d, V_p2d, ocv_vec] = loadP2dVoltage(time_vec, current_exp) - - jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); - jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); +function [time_sim, I_p2d, V_p2d, ocv_vec] = loadP2dVoltage(jsonstruct, time_vec, current_exp) + %% Load P2D model and simulate voltage response to experimental current profile [model, inputparams] = setupModelFromJson(jsonstruct); @@ -24,7 +21,6 @@ schedule_p2d.control.src = @(t, varargin) interp1(time_vec, current_exp, t, 'linear', 0); schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); - [~, states_p2d, ~] = simulateScheduleAD(state_init, model, schedule_p2d); N_points_sim = length(states_p2d); @@ -63,4 +59,5 @@ x_ne = soc_now * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; ocv_vec(idx) = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); end -end \ No newline at end of file + +end From b4e8bd566d16e5f087c2a915780a7bb951596498 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 14:10:34 +0200 Subject: [PATCH 073/119] more update --- .../calibration/FittingTime.m | 97 ++++++++++++++++++- 1 file changed, 94 insertions(+), 3 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 7945db93e..fb9f93061 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -115,11 +115,102 @@ % Preventing physical values to get too close from 0 p_safe = max(p, 1e-8); + + R0 = p_safe(1); + R1 = p_safe(2); + C1 = p_safe(3); + R2 = p_safe(4); + C2 = p_safe(5); - output = runECM(p_safe, input, options) - end - + N_points = length(ftime.time_vec); + + V_ecm = zeros(N_points, 1); + + Uc1 = 0; + Uc2 = 0; + + % Sensibilities initialisation + + % we do not need s_R0 as it is trivial + s_R1 = 0; % dUc1 / dR1 + s_C1 = 0; % dUc1 / dC1 + s_R2 = 0; % dUc2 / dR2 + s_C2 = 0; % dUc2 / dC2 + + g_true = zeros(5, 1); + + for k = 1:N_points + + if k == 1 + dt = ftime.time_vec(1); + else + dt = ftime.time_vec(k) - ftime.time_vec(k-1); + end + + I = ftime.current_exp(k); + + V_ocv = ftime.ocv_vec(k); + + % 1. Tension du modèle au pas k + V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; + + % 2. Erreur instantanée + err = ftime.voltage_exp(k) - V_ecm(k); + + if options.computeDerivatives + + % Dérivées partielles de V_ecm par rapport à chaque paramètre + dV_dR0 = -I; + dV_dR1 = -s_R1; + dV_dC1 = -s_C1; + dV_dR2 = -s_R2; + dV_dC2 = -s_C2; + + % Accumulation du gradient de la fonction coût (v = sum(err^2)) + g_true(1) = g_true(1) - 2 * err * dV_dR0; + g_true(2) = g_true(2) - 2 * err * dV_dR1; + g_true(3) = g_true(3) - 2 * err * dV_dC1; + g_true(4) = g_true(4) - 2 * err * dV_dR2; + g_true(5) = g_true(5) - 2 * err * dV_dC2; + + % Mise à jour des sensibilités pour le pas suivant (Euler Explicite) + s_R1 = s_R1 + (-s_R1 / (R1 * C1) + Uc1 / (R1^2 * C1)) * dt; + s_C1 = s_C1 + (-s_C1 / (R1 * C1) + Uc1 / (R1 * C1^2) - I / C1^2) * dt; + s_R2 = s_R2 + (-s_R2 / (R2 * C2) + Uc2 / (R2^2 * C2)) * dt; + s_C2 = s_C2 + (-s_C2 / (R2 * C2) + Uc2 / (R2 * C2^2) - I / C2^2) * dt; + + end + + % 4. Mise à jour des variables d'état électriques pour le pas suivant + Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; + Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; + + end + + % Valeur de la fonction objectif (Erreur quadratique totale) + v = sum((ftime.voltage_exp - V_ecm).^2); + + + if isnan(v) || isinf(v) || (nargout > 1 && (any(isnan(g_true)) || any(isinf(g_true)))) + v = 1e10; % Assigne un coût massif pour rejeter le point instable + if nargout > 1 + g_norm = zeros(5, 1); % Renvoie un gradient plat pour forcer le pas arrière + end + return; + end + + % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé + if nargout > 1 + pmin = ftime.scales(1:5); + pmax = ftime.scales(6:10); + dp_dpnorm = (pmax - pmin); + g_norm = g_true .* dp_dpnorm(:); + end + + end + + function plotresults_thevenin(ftime, best_params, fitting_error) % 1. Recalculate the final voltage trajectory using best_params p_safe = max(best_params, 1e-8); From cd31e4a51f59ef4786169819cc6305f6fa52476a Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 14:29:57 +0200 Subject: [PATCH 074/119] update in time fitting calibration --- .../calibration/FittingTime.m | 107 ++++++++++++++---- .../calibration/runFittingTime.m | 22 ++-- .../EquivalentCircuitModel/functions/runECM.m | 91 --------------- .../utils/loadP2dVoltage.m | 63 ----------- 4 files changed, 101 insertions(+), 182 deletions(-) delete mode 100644 Battery/EquivalentCircuitModel/functions/runECM.m delete mode 100644 Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index fb9f93061..60b656590 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -5,20 +5,25 @@ params0 % initial guess for the parameters to be fitted scales % scaling for the unit box optimization - time_vec % time steps for current_exp and voltage_exp + time_vec % time steps for current_exp and voltage_exp + current_exp % experimental current values + jsontruct % input structure for P2D model which gives us the the ocv and the experimental data + + %% helpers + voltage_exp % experimental voltage values + ocv_vec % open circuit voltage values computed from jsonstruct - ocv_vec % open circuit voltage values computed from a model - end - methods - function ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec) + function ftime = FittingTime(jsonstruct, time_vec, current_exp, params0, scales) + ftime.jsonstruct = jsonstruct; + if istable(params0), params0 = table2array(params0); end if istable(scales), scales = table2array(scales); end if istable(time_vec), time_vec = table2array(time_vec); end @@ -30,10 +35,13 @@ ftime.scales = double(scales(:)); ftime.time_vec = double(time_vec(:)); ftime.current_exp = double(current_exp(:)); - ftime.voltage_exp = double(voltage_exp(:)); - ftime.ocv_vec = double(ocv_vec(:)); - end + [V_p2d, ocv_vec] = ftime.setup(ftime.time_vec, ftime.current_exp); + + ftime.voltage_exp = V_p2d; + ftime.ocv_vec = ocv_vec; + + end function p_norm = unscaled2scaled(ftime, p) pmin = ftime.scales(1:5); @@ -47,7 +55,72 @@ p = (pmax-pmin).*p_norm +pmin; end - + + function [V_p2d, ocv_vec] = setupOCP(ftime, time_vec, current_exp) + + jsonstruct = ftime.jsonstruct; + + [model, inputparams] = setupModelFromJson(jsonstruct); + + inputparams.Control.controlPolicy = 'CCDischarge'; + model.Control = model.setupControl(inputparams.Control); + + state_init = setupInitialState(model); + + time_vec = double(time_vec(:)); + current_exp = double(current_exp(:)); + + dt_steps = diff(time_vec); + N_sim_steps = length(dt_steps); + + schedule_p2d = struct(); + schedule_p2d.step.val = dt_steps; + schedule_p2d.step.control = ones(N_sim_steps, 1); + + schedule_p2d.control.src = @(t, varargin) interp1(time_vec, current_exp, t, 'linear', 0); + schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); + + [~, states_p2d, ~] = simulateScheduleAD(state_init, model, schedule_p2d); + + N_points_sim = length(states_p2d); + V_p2d = zeros(N_points_sim, 1); + I_p2d = zeros(N_points_sim, 1); + time_sim = zeros(N_points_sim, 1); + + pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; + ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; + + for k = 1:N_points_sim + time_sim(k) = states_p2d{k}.time; + V_p2d(k) = states_p2d{k}.Control.E; + I_p2d(k) = states_p2d{k}.Control.I; + end + + [Q_nominal, ~] = computeCellCapacity(model); + + soc_p2d = 1 - cumtrapz(time_sim, I_p2d) / Q_nominal; + soc_p2d = max(0, min(1, soc_p2d)); + + json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); + json_pe = parseBattmoJson(json_pe_path); + [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); + + json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); + json_ne = parseBattmoJson(json_ne_path); + [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); + + ocv_vec = zeros(N_points_sim, 1); + + for idx = 1:N_points_sim + soc_now = soc_p2d(idx); + x_pe = soc_now * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; + x_ne = soc_now * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; + ocv_vec(idx) = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); + end + + end function [min_value, history, best_params, fitting_error] = optimizationBFGS(ftime) @@ -122,7 +195,6 @@ R2 = p_safe(4); C2 = p_safe(5); - N_points = length(ftime.time_vec); V_ecm = zeros(N_points, 1); @@ -158,7 +230,7 @@ % 2. Erreur instantanée err = ftime.voltage_exp(k) - V_ecm(k); - if options.computeDerivatives + if nargout > 1 % Dérivées partielles de V_ecm par rapport à chaque paramètre dV_dR0 = -I; @@ -309,8 +381,10 @@ function printResults(ftime, best_params, fitting_error) end - function plottest(ftime, best_params) + function plottest(ftime, best_params, current_test) + % utility function to compare with a given modified current input, see definition below + % 1. Recalculate the final voltage trajectory using best_params p_safe = max(best_params, 1e-8); @@ -323,14 +397,7 @@ function plottest(ftime, best_params) % Get original training time grid as a column vector time_vec = ftime.time_vec(:); - % Define the 3-pulse test current profile - current_test = ones(size(time_vec)); - current_test(time_vec >= 0 & time_vec < 200) = -5; - current_test(time_vec >= 200 & time_vec < 400) = 5; - current_test(time_vec >= 400 & time_vec < 700) = -5; - current_test(time_vec >= 700 & time_vec <= 1000) = 0; - - [time_test, current_test_p2d, voltage_test, ocv_test] = loadP2dVoltage(time_vec, current_test); + [voltage_test, ocv_test] = ftime.setupOCP(time_vec, current_test); % Force all outputs to be column vectors to avoid any plot orientation errors time_test = time_test(:); diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m index c8b3af121..176edd49c 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -5,17 +5,15 @@ time_init = (0:10:1000)'; current_init = ones(size(time_init)); -current_init(time_init >= 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) -current_init(time_init >= 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) -current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) +current_init(time_init >= 0 & time_init < 200) = 2.5; % 1. Décharge (0 à 200s) +current_init(time_init >= 200 & time_init < 400) = -1.5; % 2. Charge (200 à 400s) +current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); -[time_vec, current_exp, voltage_exp, ocv_vec] = loadP2dVoltage(jsonstruct, time_init, current_init); - params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 a = 1000; @@ -24,22 +22,30 @@ pmax = params0 * a; scales = [pmin, pmax]; -ftime = FittingTime(params0, scales, time_vec, current_exp, voltage_exp, ocv_vec); +ftime = FittingTime(jsonstruct, time_vec, current_exp, params0, scales); [~, ~, best_params, fitting_error] = ftime.optimizationBFGS(); p = best_params; -doprint = true; %% Printing results +doprint = true; if doprint ftime.plotresults_thevenin(best_params, fitting_error); ftime.printResults(best_params, fitting_error); + + % Define the 3-pulse test current profile + time_vec = ftime.time_vec(:); + current_test = ones(size(time_vec)); + current_test(time_vec >= 0 & time_vec < 200) = -5; + current_test(time_vec >= 200 & time_vec < 400) = 5; + current_test(time_vec >= 400 & time_vec < 700) = -5; + current_test(time_vec >= 700 & time_vec <= 1000) = 0; - ftime.plottest(best_params) + ftime.plottest(best_params, current_test) end diff --git a/Battery/EquivalentCircuitModel/functions/runECM.m b/Battery/EquivalentCircuitModel/functions/runECM.m deleted file mode 100644 index 5ba0577be..000000000 --- a/Battery/EquivalentCircuitModel/functions/runECM.m +++ /dev/null @@ -1,91 +0,0 @@ -function output = runECM(params, input, options) - - - R0 = params(1); - R1 = params(2); - C1 = params(3); - R2 = params(4); - C2 = params(5); - - - N_points = length(input.time_vec); - V_ecm = zeros(N_points, 1); - - Uc1 = 0; - Uc2 = 0; - - % Sensibilities initialisation - - s_R1 = 0; % dUc1 / dR1 - s_C1 = 0; % dUc1 / dC1 - s_R2 = 0; % dUc2 / dR2 - s_C2 = 0; % dUc2 / dC2 - - g_true = zeros(5, 1); - - for k = 1:N_points - - if k == 1 - dt = input.time_vec(1); - else - dt = input.time_vec(k) - input.time_vec(k-1); - end - - I = input.current_exp(k); - - V_ocv = input.ocv_vec(k); - - % 1. Tension du modèle au pas k - V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; - - % 2. Erreur instantanée - err = input.voltage_exp(k) - V_ecm(k); - - if nargout > 1 - % Dérivées partielles de V_ecm par rapport à chaque paramètre - dV_dR0 = -I; - dV_dR1 = -s_R1; - dV_dC1 = -s_C1; - dV_dR2 = -s_R2; - dV_dC2 = -s_C2; - - % Accumulation du gradient de la fonction coût (v = sum(err^2)) - g_true(1) = g_true(1) - 2 * err * dV_dR0; - g_true(2) = g_true(2) - 2 * err * dV_dR1; - g_true(3) = g_true(3) - 2 * err * dV_dC1; - g_true(4) = g_true(4) - 2 * err * dV_dR2; - g_true(5) = g_true(5) - 2 * err * dV_dC2; - - % Mise à jour des sensibilités pour le pas suivant (Euler Explicite) - s_R1 = s_R1 + (-s_R1 / (R1 * C1) + Uc1 / (R1^2 * C1)) * dt; - s_C1 = s_C1 + (-s_C1 / (R1 * C1) + Uc1 / (R1 * C1^2) - I / C1^2) * dt; - s_R2 = s_R2 + (-s_R2 / (R2 * C2) + Uc2 / (R2^2 * C2)) * dt; - s_C2 = s_C2 + (-s_C2 / (R2 * C2) + Uc2 / (R2 * C2^2) - I / C2^2) * dt; - end - - % 4. Mise à jour des variables d'état électriques pour le pas suivant - Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; - Uc2 = Uc2 + (-Uc2 / (R2 * C2) + I / C2) * dt; - end - - % Valeur de la fonction objectif (Erreur quadratique totale) - v = sum((input.voltage_exp - V_ecm).^2); - - - if isnan(v) || isinf(v) || (nargout > 1 && (any(isnan(g_true)) || any(isinf(g_true)))) - v = 1e10; % Assigne un coût massif pour rejeter le point instable - if nargout > 1 - g_norm = zeros(5, 1); % Renvoie un gradient plat pour forcer le pas arrière - end - return; - end - - % 5. Application de la règle de dérivation en chaîne pour l'espace normalisé - if nargout > 1 - pmin = input.scales(1:5); - pmax = input.scales(6:10); - dp_dpnorm = (pmax - pmin); - g_norm = g_true .* dp_dpnorm(:); - end - -end diff --git a/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m b/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m deleted file mode 100644 index 32f87f115..000000000 --- a/Battery/EquivalentCircuitModel/utils/loadP2dVoltage.m +++ /dev/null @@ -1,63 +0,0 @@ -function [time_sim, I_p2d, V_p2d, ocv_vec] = loadP2dVoltage(jsonstruct, time_vec, current_exp) - %% Load P2D model and simulate voltage response to experimental current profile - - [model, inputparams] = setupModelFromJson(jsonstruct); - - inputparams.Control.controlPolicy = 'CCDischarge'; - model.Control = model.setupControl(inputparams.Control); - - state_init = setupInitialState(model); - - time_vec = double(time_vec(:)); - current_exp = double(current_exp(:)); - - dt_steps = diff(time_vec); - N_sim_steps = length(dt_steps); - - schedule_p2d = struct(); - schedule_p2d.step.val = dt_steps; - schedule_p2d.step.control = ones(N_sim_steps, 1); - - schedule_p2d.control.src = @(t, varargin) interp1(time_vec, current_exp, t, 'linear', 0); - schedule_p2d.control.Control = struct('stopFunction', @(model, state, state0) false); - - [~, states_p2d, ~] = simulateScheduleAD(state_init, model, schedule_p2d); - - N_points_sim = length(states_p2d); - V_p2d = zeros(N_points_sim, 1); - I_p2d = zeros(N_points_sim, 1); - time_sim = zeros(N_points_sim, 1); - - pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; - pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; - ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; - ne_guestStoichiometry100 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; - - for k = 1:N_points_sim - time_sim(k) = states_p2d{k}.time; - V_p2d(k) = states_p2d{k}.Control.E; - I_p2d(k) = states_p2d{k}.Control.I; - end - - [Q_nominal, ~] = computeCellCapacity(model); - - soc_p2d = 1 - cumtrapz(time_sim, I_p2d) / Q_nominal; - soc_p2d = max(0, min(1, soc_p2d)); - - json_pe_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_positive_electrode_interface.json'); - json_pe = parseBattmoJson(json_pe_path); - [fn_ocp_pe, ~] = setupFunction(json_pe.openCircuitPotential); - - json_ne_path = fullfile('ParameterData','ParameterSets','Chen2020','chen2020_negative_electrode_interface.json'); - json_ne = parseBattmoJson(json_ne_path); - [fn_ocp_ne, ~] = setupFunction(json_ne.openCircuitPotential); - - ocv_vec = zeros(N_points_sim, 1); - for idx = 1:N_points_sim - soc_now = soc_p2d(idx); - x_pe = soc_now * (pe_guestStoichiometry100 - pe_guestStoichiometry0) + pe_guestStoichiometry0; - x_ne = soc_now * (ne_guestStoichiometry100 - ne_guestStoichiometry0) + ne_guestStoichiometry0; - ocv_vec(idx) = fn_ocp_pe(x_pe) - fn_ocp_ne(x_ne); - end - -end From 9ba4c45dd64bd209760456a02f56d89bb7820ec2 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 15:23:44 +0200 Subject: [PATCH 075/119] update in runEquivalentCircuitModel --- .../models/EquivalentCircuitModel.m | 1 + .../models/runEquivalentCircuitModel.m | 31 +++++++++++++++++++ 2 files changed, 32 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m diff --git a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m index 6efb43c50..79136595f 100644 --- a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m @@ -210,6 +210,7 @@ SOC = zeros(length(t_out), 1); U = zeros(length(t_out), 1); I = zeros(length(t_out), 1); %gagne du temps en allouant déjà la mémoire + for i = 1:length(t_out) state = model.setupStateFromY(y_out(i, :)); diff --git a/Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m new file mode 100644 index 000000000..90f0f91aa --- /dev/null +++ b/Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m @@ -0,0 +1,31 @@ +jsonstruct = createParametersECM(); +inputparams = EquivalentCircuitModelInputParams(jsonstruct); + +model = EquivalentCircuitModel(inputparams); + +close all +cgit = model.cgit; +cgit.plot; + + +[t, U, I, SOC] = model.solve(); + +%% + +figure +tiledlayout(1, 3) +nexttile +plot(t/hour, I) +title('Current') +xlabel('Time / hour') +ylabel('Current / A'); +nexttile +plot(t/hour, U) +title('Voltage') +xlabel('Time / hour') +ylabel('Voltage / V'); +nexttile +plot(t/hour, SOC) +title('SOC') +xlabel('Time / hour') +ylabel('SOC / -'); From 665fa7deac3f19e4cf011f3696b813e4d9acde4d Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 15:26:45 +0200 Subject: [PATCH 076/119] some clean-up --- .../runEquivalentCircuitModel.m | 0 .../utils/createParametersECM.m | 22 +++--- .../utils/plotExperience.m | 76 ------------------- 3 files changed, 12 insertions(+), 86 deletions(-) rename Battery/EquivalentCircuitModel/{models => examples}/runEquivalentCircuitModel.m (100%) delete mode 100644 Battery/EquivalentCircuitModel/utils/plotExperience.m diff --git a/Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m similarity index 100% rename from Battery/EquivalentCircuitModel/models/runEquivalentCircuitModel.m rename to Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m diff --git a/Battery/EquivalentCircuitModel/utils/createParametersECM.m b/Battery/EquivalentCircuitModel/utils/createParametersECM.m index 7e8603649..690f2edef 100644 --- a/Battery/EquivalentCircuitModel/utils/createParametersECM.m +++ b/Battery/EquivalentCircuitModel/utils/createParametersECM.m @@ -3,10 +3,9 @@ % create example data set for ECM jsonstruct.nominalcellcapacity = 63.7; - jsonstruct.initSOC = 1.0; - jsonstruct.lowerVoltageCutoff = 3.0; - jsonstruct.initOverpotential2 = 0; - jsonstruct.totalTime = 4200; + jsonstruct.initSOC = 1.0; + jsonstruct.lowerVoltageCutoff = 3.0; + jsonstruct.totalTime = 4200; jsonstruct.I.functionFormat = 'tabulated'; jsonstruct.I.argumentList = {'time'}; @@ -19,19 +18,22 @@ jsonstruct.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]; R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; + R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; + tau1_tot=[4.9,11,12,17,15;4.9,11,12,18,17;4.9,13,14,17,18;4.9,13,20,16,19;4.9,12,17,16,18;3.7,13,16,14,15;3.2,14,17,15,14;3.2,16,18,15,15;4.3,16,17,15,15;5.9,16,17,15,13;8.8,17,17,15,15;14,18,17,16,15;18,20,18,16,14;21,23,22,18,16;23,24,24,19,17;23,26,25,20,16;23,26,24,23,21;22,26,23,23,23;22,24,22,24,22;21,23,21,22,20;19,23,20,21,19;19,23,20,20,17;18,23,19,19,16;17,23,19,18,15;16,23,19,18,15;15,24,19,17,14;15,25,20,17,14;17,26,20,18,15;17,27,22,18,14;20,27,24,20,16;25,29,25,26,21;23,27,22,22,23;21,22,20,27,24;21,21,21,24,21;21,23,25,22,18;22,26,26,20,18;24,28,23,21,18;27,27,21,20,18;31,25,21,21,17;31,24,20,21,18;29,23,19,21,17;26,23,20,20,18;24,23,20,21,19;22,23,20,20,19;21,23,20,22,19;19,23,21,23,17;19,24,21,21,18;18,24,20,20,18;17,24,21,23,19;17,23,15,22,19;17,23,14,15,17]; + R2_tot = [0.00465917,0.00296137,0.00671937,0.00670953,0.00638318;0.00465917,0.00296137,0.0049358,0.00369832,0.00345545;0.00465917,0.00360752,0.00337953,0.00232382,0.00217768;0.00465917,0.00385934,0.00299688,0.00165026,0.00141804;0.00465917,0.00279048,0.00167985,0.000868944,0.00062913;0.00344996,0.00198995,0.00127818,0.000602667,0.000490827;0.00243925,0.00173739,0.00100247,0.000502448,0.000400199;0.00195174,0.0016195,0.00117991,0.000653807,0.000522623;0.00196127,0.00143448,0.00090563,0.000593035,0.000515238;0.00210982,0.0013075,0.000808184,0.000489967,0.000453458;0.00266036,0.00121596,0.000742684,0.000416342,0.000378914;0.00344871,0.00125469,0.00074347,0.000401257,0.000350742;0.00389231,0.00126885,0.000696434,0.000379638,0.000337394;0.00392122,0.00188842,0.00105021,0.000512664,0.000344475;0.00377053,0.00200223,0.00129526,0.00051701,0.000287237;0.00349905,0.00192787,0.00134563,0.000629481,0.000378992;0.00314826,0.00181955,0.00130909,0.000850741,0.000526779;0.00285045,0.00175597,0.00125321,0.000856617,0.000718745;0.00255589,0.00161788,0.00119344,0.000887228,0.000640541;0.00227795,0.00154717,0.00113057,0.000748643,0.000532106;0.00204687,0.00150239,0.00108992,0.000741976,0.00046544;0.00179717,0.00147648,0.00104268,0.000650899,0.000408277;0.00166159,0.00146907,0.00104974,0.000648536,0.000425937;0.00154212,0.0014479,0.00100709,0.000584535,0.000365088;0.00142178,0.00147631,0.000971539,0.000574467,0.000359385;0.00138252,0.00149249,0.000966175,0.000567393,0.00034615;0.00135213,0.00150963,0.000946023,0.000509391,0.00032513;0.00161978,0.00157701,0.000973037,0.000512528,0.000321927;0.0018797,0.00176393,0.00107455,0.000552517,0.000360338;0.00233758,0.00204923,0.00128005,0.000575555,0.000345665;0.00303428,0.00251452,0.00155042,0.00101129,0.000740204;0.00397936,0.0023618,0.00194514,0.00167676,0.00124506;0.00494525,0.00268869,0.00239193,0.00146285,0.000987005;0.00575857,0.00294003,0.00244425,0.0011978,0.000867504;0.00596764,0.00278034,0.00213064,0.00106735,0.000733011;0.00569216,0.00241023,0.00177033,0.00095135,0.00066496;0.00494613,0.00199842,0.00153419,0.000885069,0.000648523;0.00403546,0.00176577,0.00135467,0.000898499,0.000675215;0.00326917,0.00161032,0.00130149,0.000889941,0.000633382;0.00274124,0.00153081,0.001227,0.000919164,0.000697074;0.00244927,0.00150333,0.0012413,0.000897664,0.000705495;0.00220336,0.00150596,0.00124922,0.000957534,0.000664272;0.00199516,0.00153147,0.00127479,0.000917949,0.0007466;0.00184088,0.0015754,0.00130798,0.000984517,0.000675919;0.00173782,0.00161791,0.00131662,0.000949267,0.000741;0.0017013,0.00158804,0.00133677,0.000999377,0.000704756;0.00162086,0.00170525,0.00138481,0.000946432,0.000736538;0.00152086,0.00166043,0.00128942,0.00097447,0.000683679;0.00150632,0.00176676,0.00137887,0.00096943,0.000718854;0.00128553,0.00167337,0.0016092,0.000944572,0.000726751;0.00128553,0.00167337,0.00170989,0.00124241,0.000828314]; + tau2_tot = [95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,3.2e+02,6.7e+02,7.2e+02,7.2e+02;95,4.4e+02,7.2e+02,7.2e+02,7.2e+02;95,5.3e+02,7e+02,6.9e+02,7.2e+02;95,5.3e+02,6.4e+02,5.8e+02,6.9e+02;1.2e+02,5.4e+02,5.8e+02,4.5e+02,5.5e+02;1.8e+02,5.8e+02,5.8e+02,4.4e+02,5.4e+02;2.5e+02,6.2e+02,6.2e+02,5.6e+02,6e+02;3.7e+02,6e+02,5.7e+02,5.6e+02,6.2e+02;5.3e+02,5.6e+02,5.1e+02,5e+02,6.4e+02;6.7e+02,5.6e+02,4.8e+02,4.3e+02,6e+02;7.2e+02,5.9e+02,4.6e+02,3.8e+02,5.7e+02;7.2e+02,6.4e+02,4.9e+02,3.7e+02,5.2e+02;7.2e+02,6.9e+02,6.4e+02,4.6e+02,4.3e+02;7.2e+02,7.2e+02,6.9e+02,5e+02,3.9e+02;7.2e+02,7e+02,7e+02,6.4e+02,5.5e+02;7.2e+02,7e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.1e+02,7e+02,6.9e+02,7.1e+02;7.2e+02,7e+02,7e+02,7e+02,6.8e+02;7.1e+02,7e+02,6.9e+02,6.5e+02,6e+02;6.8e+02,7.1e+02,6.8e+02,6.4e+02,5e+02;6.3e+02,7.1e+02,6.6e+02,6.1e+02,4.8e+02;6e+02,7e+02,6.6e+02,5.6e+02,5e+02;5.6e+02,6.9e+02,6.4e+02,5.3e+02,4.3e+02;5.3e+02,6.9e+02,6.1e+02,5.4e+02,4.2e+02;5.2e+02,6.8e+02,6e+02,5.2e+02,4.1e+02;5.7e+02,6.7e+02,5.9e+02,4.6e+02,3.9e+02;7e+02,6.9e+02,6e+02,4.9e+02,4.1e+02;7.2e+02,7.1e+02,6.3e+02,5e+02,4.2e+02;7.2e+02,7.2e+02,6.6e+02,5.9e+02,5.5e+02;7.2e+02,7.2e+02,7e+02,6.3e+02,6.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.1e+02,7.2e+02,7.2e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,7e+02;7.2e+02,7.2e+02,7.2e+02,7.2e+02,6.5e+02;7.2e+02,7.2e+02,7.2e+02,6.9e+02,6.1e+02;7.2e+02,7.2e+02,7.1e+02,6.8e+02,6.3e+02;7.2e+02,7e+02,6.8e+02,6.9e+02,6.6e+02;7e+02,6.7e+02,6.8e+02,7e+02,6.4e+02;6.6e+02,6.5e+02,6.7e+02,7.2e+02,7.1e+02;6e+02,6.4e+02,6.7e+02,7.2e+02,6.9e+02;5.6e+02,6.5e+02,6.7e+02,7.2e+02,6.9e+02;5.4e+02,6.6e+02,6.8e+02,7.2e+02,7.2e+02;5.3e+02,6.7e+02,7e+02,7.2e+02,6.5e+02;5.4e+02,6.7e+02,7e+02,7.2e+02,7.1e+02;5.5e+02,6.5e+02,7.1e+02,7.2e+02,6.4e+02;5.3e+02,6.7e+02,7e+02,6.9e+02,6.8e+02;5.2e+02,6.4e+02,6.3e+02,6.8e+02,5.9e+02;4.9e+02,6.2e+02,6.5e+02,6.7e+02,5.8e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02;4.3e+02,5.6e+02,5.6e+02,6e+02,4.9e+02]; - R0 = R0_tot(:,3)'; - R1 = R1_tot(:,3)'; + R0 = R0_tot(:,3)'; + R1 = R1_tot(:,3)'; tau1 = tau1_tot(:,3)'; - R2 = R2_tot(:,3)'; + R2 = R2_tot(:,3)'; tau2 = tau2_tot(:,3)'; - C1 = tau1 ./ R1; - C2 = tau2 ./ R2; - + C1 = tau1 ./ R1; + C2 = tau2 ./ R2; jsonstruct.R0.functionFormat = 'tabulated'; jsonstruct.R0.argumentList = {'SOC'}; diff --git a/Battery/EquivalentCircuitModel/utils/plotExperience.m b/Battery/EquivalentCircuitModel/utils/plotExperience.m deleted file mode 100644 index 597cf60d6..000000000 --- a/Battery/EquivalentCircuitModel/utils/plotExperience.m +++ /dev/null @@ -1,76 +0,0 @@ -function experience = plotexperience() - - - json_jp3 = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\jp3-params\jp3-opt-1d-full.json'; - jsonstruct = parseBattmoJson(json_jp3); - - % 1. Construction du modèle - [model, inputparams] = setupModelFromJson(jsonstruct); - - model.NegativeElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.argumentList = {'c'}; - model.NegativeElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.numberOfArguments = 1; - - model.PositiveElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.argumentList = {'c'}; - model.PositiveElectrode.Coating.ActiveMaterial.Interface.computeOCPFunc.numberOfArguments = 1; - - model.Electrolyte.computeDiffusionCoefficientFunc.argumentList = {'c', 'T'}; - model.Electrolyte.computeConductivityFunc.argumentList = {'c', 'T'}; - - % 3. Initialisation de l'état (maintenant le modèle sait quoi envoyer !) - state0 = setupInitialState(model); - - inputparams.Control.controlPolicy = 'CCDischarge'; - inputparams.Control.DRate = 2; - % inputparams.Control.tmax = 30; - inputparams.Control.rampupTime = 0.1; - inputparams.Control.lowerCutoffVoltage = 2.5; - - schedule1 = model.setupSchedule(jsonstruct); - [~, states1] = simulateBattery(model, state0, schedule1); - state_after_pulse = states1{end}; - - inputparams.Control.DRate = 0; - inputparams.Control.tmax = 600; - inputparams.Control.rampupTime = 0.1; - - - schedule2 = setupSchedule(model, inputparams); - disp('Simulation du Repos en cours...'); - [~, states2] = simulateBattery(model, state_after_pulse, schedule2); - - all_states = [states1(:); states2(:)]; - N = length(all_states); - - time = zeros(N, 1); - voltage = zeros(N, 1); - current = zeros(N, 1); - - - for i = 1:N - time(i) = all_states{i}.time; - try - % Dans BattMo, les données du circuit extérieur sont dans "Control" - voltage(i) = all_states{i}.Control.E; - current(i) = all_states{i}.Control.I; - catch - % Alternative si les variables sont stockées à la racine - voltage(i) = all_states{i}.voltage; - current(i) = all_states{i}.current; - end - end - - figure; - subplot(2,1,1); - plot(time, voltage); - xlabel('Time (s)'); - ylabel('Voltage (V)'); - title('Voltage vs Time'); - - subplot(2,1,2); - plot(time, current); - xlabel('Time (s)'); - ylabel('Current (A)'); - title('Current vs Time'); - - experience = [current, voltage, time]; -end From eacf9d0dbeec12c878083479a5043578ae5c3b2f Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 15:40:35 +0200 Subject: [PATCH 077/119] more clean-up --- .../examples/runEquivalentCircuitModel.m | 71 +++++++++++++++++-- .../utils/createParametersECM.m | 2 +- 2 files changed, 68 insertions(+), 5 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m index 90f0f91aa..77ade5eb4 100644 --- a/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m @@ -1,12 +1,75 @@ +%% Example script for EquivalentCircuitModel + +%% +% The function createParametersECM setup an example data set for the ECM model. See below +% jsonstruct = createParametersECM(); -inputparams = EquivalentCircuitModelInputParams(jsonstruct); +%% +% Setup the ECM model +% +inputparams = EquivalentCircuitModelInputParams(jsonstruct); model = EquivalentCircuitModel(inputparams); -close all -cgit = model.cgit; -cgit.plot; +%% +% Review of the model parameters + +soc = linspace(0, 1, 100); +figure +tiledlayout(2, 3, 'tileindexing', 'columnmajor'); + +nexttile +plot(soc, model.OCPfunc(soc)) +title('OCP') +xlabel('SOC / -') +ylabel('OCP / V'); + +nexttile +plot(soc, model.R0func(soc)) +title('R0') +xlabel('SOC / -') +ylabel('R0 / Ohm'); + +nexttile +plot(soc, model.R1func(soc)) +title('R1') +xlabel('SOC / -') +ylabel('R1 / Ohm'); + +nexttile +plot(soc, model.C1func(soc)) +title('C1') +xlabel('SOC / -') +ylabel('C1 / Ohm'); + +nexttile +plot(soc, model.R2func(soc)) +title('R2') +xlabel('SOC / -') +ylabel('R2 / Ohm'); + +nexttile +plot(soc, model.C2func(soc)) +title('C2') +xlabel('SOC / -') +ylabel('C2 / Ohm'); + +%% +% The input current has been passed to the model + +figure +totalTime = model.totalTime +t = linspace(0, totalTime, 200); +plot(t/hour, model.Ifunc(t), 'o-'); +title('Input current') +xlabel('time / hour') +ylabel('I / A'); + + +%% +% Solve the model +% [t, U, I, SOC] = model.solve(); diff --git a/Battery/EquivalentCircuitModel/utils/createParametersECM.m b/Battery/EquivalentCircuitModel/utils/createParametersECM.m index 690f2edef..2d796880f 100644 --- a/Battery/EquivalentCircuitModel/utils/createParametersECM.m +++ b/Battery/EquivalentCircuitModel/utils/createParametersECM.m @@ -1,6 +1,6 @@ function jsonstruct = createParametersECM() - % create example data set for ECM + % create example data set for the ECM model jsonstruct.nominalcellcapacity = 63.7; jsonstruct.initSOC = 1.0; From f5a326e7e10f3fe31da1102b2dd44492d5a4c1ce Mon Sep 17 00:00:00 2001 From: Alexandre Date: Mon, 13 Jul 2026 16:01:46 +0200 Subject: [PATCH 078/119] first fixes for fitting time, 4 arguments for setupOCP to ensure same vector sizes --- .../calibration/FittingTime.m | 22 +++++++++++-------- .../calibration/runFittingTime.m | 4 +++- 2 files changed, 16 insertions(+), 10 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 60b656590..5f6fcfd69 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -8,7 +8,7 @@ time_vec % time steps for current_exp and voltage_exp current_exp % experimental current values - jsontruct % input structure for P2D model which gives us the the ocv and the experimental data + jsonstruct % input structure for P2D model which gives us the the ocv and the experimental data %% helpers @@ -28,19 +28,23 @@ if istable(scales), scales = table2array(scales); end if istable(time_vec), time_vec = table2array(time_vec); end if istable(current_exp), current_exp = table2array(current_exp); end - if istable(voltage_exp), voltage_exp = table2array(voltage_exp); end - if istable(ocv_vec), ocv_vec = table2array(ocv_vec); end - ftime.params0 = double(params0(:)); - ftime.scales = double(scales(:)); - ftime.time_vec = double(time_vec(:)); - ftime.current_exp = double(current_exp(:)); + + t_raw = double(time_vec(:)); + i_raw = double(current_exp(:)); + - [V_p2d, ocv_vec] = ftime.setup(ftime.time_vec, ftime.current_exp); + [V_p2d, ocv_vec, time_sim, I_p2d] = ftime.setupOCP(t_raw, i_raw); + + ftime.time_vec = time_sim; + ftime.current_exp = I_p2d; ftime.voltage_exp = V_p2d; ftime.ocv_vec = ocv_vec; + ftime.params0 = double(params0(:)); + ftime.scales = double(scales(:)); + end function p_norm = unscaled2scaled(ftime, p) @@ -56,7 +60,7 @@ end - function [V_p2d, ocv_vec] = setupOCP(ftime, time_vec, current_exp) + function [V_p2d, ocv_vec, time_sim, I_p2d] = setupOCP(ftime, time_vec, current_exp) jsonstruct = ftime.jsonstruct; diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m index 176edd49c..21f9da119 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -10,6 +10,8 @@ current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) + + jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); @@ -22,7 +24,7 @@ pmax = params0 * a; scales = [pmin, pmax]; -ftime = FittingTime(jsonstruct, time_vec, current_exp, params0, scales); +ftime = FittingTime(jsonstruct, time_init, current_init, params0, scales); [~, ~, best_params, fitting_error] = ftime.optimizationBFGS(); From b2bb4aa980cd3c078294cf3b96702a287ad4e995 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 16:41:10 +0200 Subject: [PATCH 079/119] working on runCalibration --- .../calibration/runCalibration.m | 162 ++++++++++++++++++ 1 file changed, 162 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/calibration/runCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibration.m b/Battery/EquivalentCircuitModel/calibration/runCalibration.m new file mode 100644 index 000000000..6086aa1fa --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/runCalibration.m @@ -0,0 +1,162 @@ +%% ECM Fitting for lithium-ion batteries + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); +jsonstruct_base = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + +jsonstruct_base.NegativeElectrode.Coating.ActiveMaterial.Interface.useDoubleLayerCapacity = true; + +c_ne = 29.866*mol/litre; +c_pe = 17.038*mol/litre; + + +%% +% This slider allows logarithmic changes: new_val = val_init * 10^p. + +p_diffusion = 0; +p_reactionRate = 0; +p_doubleLayerCapacitance = 0; +base_diff_anode = 1.3135e-15; +base_rate_anode = 5.031e-11; +base_cdl = 0.2; + +val_diff_anode = base_diff_anode * (10^p_diffusion); +val_rate_anode = base_rate_anode * (10^p_reactionRate); +val_cdl = base_cdl * (10^p_doubleLayerCapacitance); + +jsonstruct = jsonstruct_base; + +jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode; +jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; +jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl; + + +[model, inputparams, ~] = setupModelFromJson(jsonstruct); +initstate = initStateChen2020(model, c_ne, c_pe); +options = []; +options.stateInitialization.initializationSetup = 'given state'; +options.stateInitialization.computeSteadyState = false; + +extrastructs = []; +extrastructs.initstate = initstate; + +impsolv = ImpedanceSolver(inputparams, options, extrastructs); +frequences = logspace(-2, 3, 30); + +Z = impsolv.computeImpedance(frequences); + +figure('Name', 'Nyquist Diagram'); +plot(real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); +grid on; +xlabel('Re(Z)'); +ylabel('-Im(Z)'); +title('Interactive Nyquist Diagram'); + +disp('Calculation succeeded'); + + +%% +% +% The impact of diffusion is mainly seen on the tail at low frequencies. While +% a larger coefficient does not have much of an impact, using a very small one +% shows how strongly the diffusion phenomenon is linked to this tail. +% +% The double-layer capacitance affects the first semicircle, as the frequency +% at its peak is governed by the relation $f_{\max } =\frac{1\;}{2\pi R_{\textrm{CT}} +% C_{\textrm{DL}} }$. A large capacitance will result in a lower $f_{\max }$ (a +% shift to the left, as frequencies are plotted inversely), while a small one +% will shift the center of the first semicircle to the right. +% +% Finally, the influence of the reaction rate on the Nyquist diagram is clearly +% evident. A more facile reaction (i.e., a higher reaction rate) leads to a lower +% charge-transfer resistance. As this parameter dictates the width of the first +% semicircle, it virtually vanishes at high reaction rates and broadens considerably +% at lower ones. + + + + +%% Calibration of ECM parameters +% Impedance is the opposition to alternating current presented by the combined +% effect of resistance and reactance in a circuit. It is obtained with the ratio +% of complex voltage and complex current : $Z=U/I$ . It extends the concept of +% resistance to alternating current (AC) circuits. +% +% We tried through our optimization algorithm to fit different battery models +% to ECM through five parameters, $R_0$, $R_1$, $C_1$, $R_2$ and $C_2$. The aim +% of the study is to obtain the set of parameters as close as possible to the +% real impedance curve with the 2-RC Impedance function $Z = R_0 + \frac{R_1}{1 +% + j R_1 C_1 \omega} + \frac{R_2}{1 + j R_2 C_2 \omega}$. +% +% We chose unitBoxBFGS as optimization algorithm, which allows other constraints. +% As the two RC parallel cells are symetric, we imposed $C_1 > 2*C_2$ to ensure +% robustness and injectivity of the optimization. Thanks this criteria, a particular +% battery state always lead to the same equivalent circuit. +% +% UnitBoxBFGS needs to work in a box between 0 and 1. We chose to work between +% two vectors pmax and pmin, framing initial values, and to normalize them so +% that pmin becomes 0 and pmax becomes 1. + +omega = logspace(-4, 2, 50); +params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; +[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); + +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +feis.plotresults_thevenin(best_params, fitting_error); + +%% Calibration from experimental data +% We use data from the Ank's paper (http://dx.doi.org/10.1149/1945-7111/ad14d0) to calibrate the ECM parameters. + +filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv'); +data = readmatrix(filename); +omega = data(:, 1); +Z_re_exp = data(:, 2); +Z_im_exp = data(:, 3); + +%% +% Initial data +params0 = [3.84e-03,... + 2.71e-03,... + 6.00e+03,... + 9.48e-04,... + 1.11e+01]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +feis.plotresults_thevenin(best_params, fitting_error); + +%% +% We use data from the P2d model using Chen's paper (http://dx.doi.org/10.1149/1945-7111/ab9050) data + +[Z_re_exp, Z_im_exp, omega] = load_chen_data(); +params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 + +a = 1000; + +pmin = params0 / a; +pmax = params0 * a; +scales = [pmin, pmax]; + +feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); + +[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +feis.plotresults_thevenin(best_params, fitting_error); + From 6e9e343769a77bba2b94a0672eb86564dfef825d Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 16:45:14 +0200 Subject: [PATCH 080/119] added ank EIS data --- .../calibration/utils/ank_data.csv | 54 +++++++++++++++++++ 1 file changed, 54 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/calibration/utils/ank_data.csv diff --git a/Battery/EquivalentCircuitModel/calibration/utils/ank_data.csv b/Battery/EquivalentCircuitModel/calibration/utils/ank_data.csv new file mode 100644 index 000000000..ebfc7a057 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/utils/ank_data.csv @@ -0,0 +1,54 @@ +omega,Z_re_exp, Z_im_exp +0.0585167228806873,0.0059037684,-0.0015759115 +0.073145902815461,0.0057388577,-0.0013762877 +0.102404265198282,0.0055251499,-0.0011229047 +0.131662627581104,0.0053971787,-0.00096647855 +0.160920989963925,0.0053179273,-0.00084524695 +0.204808530396565,0.0052275578,-0.00072484021 +0.263325255162208,0.0051419241,-0.00061617774 +0.321841979927851,0.0050863023,-0.00054461212 +0.40961706079313,0.0050385431,-0.00045775058 +0.512021325991412,0.0049994029,-0.00040029659 +0.658313137905519,0.0049494077,-0.00033935858 +0.81923412158626,0.0049303146,-0.00029267545 +1.03867185516538,0.0049035605,-0.00025913521 +1.31662627581104,0.0048818574,-0.00022838252 +1.66772658670578,0.0048576323,-0.00020123593 +2.10660205386403,0.0048366045,-0.00017050178 +2.66251089515534,0.0048242784,-0.00016462906 +3.36471157977669,0.0048125829,-0.00014065423 +4.25709140311648,0.0047928458,-0.00013059085 +5.36890914853095,0.0047881249,-0.00010821626 +6.78793997228361,0.0047618011,-0.00012012554 +8.58732863365019,0.0047471607,-0.00010675551 +10.854851671195,0.0047396827,-0.0001151508 +13.7221713480743,0.0047308835,-0.00011481276 +17.3355784394767,0.0047241068,-0.00010846369 +21.9145125639369,0.00471238,-0.00011203043 +27.6784095700784,0.0046953661,-0.00012770121 +34.992999223306,0.0046865055,-0.00013188807 +44.2093834053107,0.0046605985,-0.00014636198 +55.8980979614515,0.0046593016,-0.00016671699 +70.6589426726556,0.0046344302,-0.00017830553 +89.2526284389301,0.0046159248,-0.00020566618 +112.834868029396,0.0045877914,-0.00022511468 +142.663762487665,0.0045476044,-0.00025920509 +180.20225098155,0.004507428,-0.00029294193 +227.703194735681,0.0044634948,-0.00032793963 +287.829106090345,0.0044142846,-0.00035223772 +363.798452471367,0.0043558846,-0.00039301551 +459.897553780265,0.0042858119,-0.00041878037 +581.422148770899,0.0042147879,-0.00044296851 +734.809096896692,0.0041281688,-0.00045479828 +927.841115903863,0.0040384089,-0.00046610759 +1173.02621189845,0.0039561596,-0.00047885193 +1483.17944396928,0.0038676499,-0.00047028391 +1873.04713387303,0.0037774039,-0.00046054387 +2367.93770069961,0.0036888993,-0.00044175831 +2994.08124399164,0.0036058144,-0.00041262037 +3781.20433025146,0.003509155,-0.00038143093 +4783.01041244106,0.0034532545,-0.00033303836 +6044.66013628319,0.0033818206,-0.00027218863 +7640.35270521185,0.0033192835,-0.00019796912 +9647.60798609585,0.0032685795,-0.00011912013 +12201.9502647725,0.003236911,-3.5926867e-05 From 42ecdb39f17f16930006db8ff470419bb86f921e Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 16:45:37 +0200 Subject: [PATCH 081/119] more in runCalibration --- .../EquivalentCircuitModel/calibration/runCalibration.m | 9 +++------ 1 file changed, 3 insertions(+), 6 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibration.m b/Battery/EquivalentCircuitModel/calibration/runCalibration.m index 6086aa1fa..391df0e0c 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibration.m @@ -9,10 +9,6 @@ c_ne = 29.866*mol/litre; c_pe = 17.038*mol/litre; - -%% -% This slider allows logarithmic changes: new_val = val_init * 10^p. - p_diffusion = 0; p_reactionRate = 0; p_doubleLayerCapacitance = 0; @@ -125,6 +121,7 @@ %% % Initial data + params0 = [3.84e-03,... 2.71e-03,... 6.00e+03,... @@ -143,8 +140,8 @@ feis.plotresults_thevenin(best_params, fitting_error); -%% -% We use data from the P2d model using Chen's paper (http://dx.doi.org/10.1149/1945-7111/ab9050) data +%% Synthetic data from P2D model +% We use impedance data generated from the P2d model with Chen et al's paper (http://dx.doi.org/10.1149/1945-7111/ab9050) parameters [Z_re_exp, Z_im_exp, omega] = load_chen_data(); params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 From c31bef625cefc13b3808e43eac31fb519ad96957 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 16:46:25 +0200 Subject: [PATCH 082/119] added readme file --- .../calibration/utils/README.org | 21 +++++++++++++++++++ 1 file changed, 21 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/calibration/utils/README.org diff --git a/Battery/EquivalentCircuitModel/calibration/utils/README.org b/Battery/EquivalentCircuitModel/calibration/utils/README.org new file mode 100644 index 000000000..8b227b99b --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/utils/README.org @@ -0,0 +1,21 @@ +The Ank data in [[file:ank_data.csv][ank_data.csv]] is taken from + +#+begin_quote +@article{ + title = {Lithium-Ion Cells in Automotive Applications: Tesla 4680 Cylindrical Cell Teardown and + Characterization}, + volume = 170, + ISSN = {1945-7111}, + url = {http://dx.doi.org/10.1149/1945-7111/ad14d0}, + DOI = {10.1149/1945-7111/ad14d0}, + number = 12, + journal = {Journal of The Electrochemical Society}, + publisher = {The Electrochemical Society}, + author = {Ank, Manuel and Sommer, Alessandro and Abo Gamra, Kareem and Schöberl, Jan and Leeb, Matthias and + Schachtl, Johannes and Streidel, Noah and Stock, Sandro and Schreiber, Markus and Bilfinger, Philip and Allgäuer, + Christian and Rosner, Philipp and Hagemeister, Jan and Rößle, Matti and Daub, Rüdiger and Lienkamp, Markus}, + year = 2023, + month = Dec, + pages = 120536 +} +#+end_quote From f0913f50d6f7f330591072a6ce51341e3eeec1fb Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 18:18:23 +0200 Subject: [PATCH 083/119] added class impedance Explore --- .../pxdParamsImpact/ImpedanceExplore.m | 201 ++++++++++++++++++ .../pxdParamsImpact/runImpedanceExplore.m | 21 ++ 2 files changed, 222 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m create mode 100644 Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m new file mode 100644 index 000000000..9a88e7255 --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -0,0 +1,201 @@ +classdef ImpedanceExplore < handle + + properties (SetAccess = private) + + jsonstruct + baseValues + + end + + properties + + %% + % TODO: add option to change soc in slider + soc = 1 + + parameters + parameterLegendNames + + end + + methods + + function impexp = ImpedanceExplore(jsonstruct) + + impexp.jsonstruct = jsonstruct; + impexp.setupDefaultParameters() + impexp.baseValues = impexp.getParameterValues(); + + end + + function setupDefaultParameters(impexp) + + elyte = 'Electrolyte'; + ne = 'NegativeElectrode'; + pe = 'PositiveElectrode'; + co = 'Coating'; + am = 'ActiveMaterial'; + itf = 'Interface'; + sd = 'SolidDiffusion'; + cc = 'CurrentCollector'; + ctrl = 'Control'; + thermal = 'ThermalModel'; + + impexp.parameters = {{ne, co, am, sd, 'referenceDiffusionCoefficient'}, ... + {ne, co, am, itf, 'reactionRateConstant'}, ... + {ne, co, am, itf, 'doubleLayerCapacitance'}}; + + %% + % TODO : setup default way to get legend + impexp.parameterLegendNames = {'Negative Electrode Solid Diffusion Coefficient', ... + 'Negative Electrode Reaction Rate Constant', ... + 'Negative Electrode Double Layer Capacitance'}; + + end + + function updateImpedance(impexp) + + end + + function sld = setupSlider(imexp, fig, ypos, txt) + + uilabel(fig , ... + 'Position', [50, ypos + 20, 500, 40], ... + 'WordWrap', 'on' , ... + 'Text', txt); + + + sld = uislider(fig, ... + 'Position', [50, ypos, 500, 3], ... + 'Limits', [-5, 5] , ... % Définit le minimum et le maximum + 'MajorTicks', -5:0.5:5 , ... % Ajoute une graduation tous les 1 + 'Value', 0); + + end + + function vals = getParameterValues(impexp, jsonstruct) + + if nargin < 2 + jsonstruct = impexp.jsonstruct; + end + + parameters = impexp.parameters; + + for iparam = 1 : numel(parameters) + vals(iparam) = getJsonStructField(jsonstruct, parameters{iparam}); + end + + end + + function jsonstruct = setParameterValues(impexp, vals, jsonstruct) + + if nargin < 3 + jsonstruct = impexp.jsonstruct; + end + + parameters = impexp.parameters; + + for iparam = 1 : numel(parameters) + jsonstruct = setJsonStructField(jsonstruct, parameters{iparam}, vals(iparam), 'handleMisMatch', 'quiet'); + end + + end + + function start(impexp) + + % 2. Création de l'interface graphique (Fenêtre plus haute pour accueillir les curseurs) + fig = uifigure('Name', 'Impedance Explorer', 'Position', [100, 50, 600, 650]); + + % Graphique + ax = uiaxes(fig, 'Position', [50, 350, 500, 250]); + title(ax, 'Nyquist Diagram'); + xlabel(ax, 'Re(Z)'); + ylabel(ax, '-Im(Z)'); + grid(ax, 'on'); + + % Label de statut + lbl = uilabel(fig, 'Position', [50, 310, 500, 22], 'Text', 'Ready, use slider to start.'); + lbl.FontWeight = 'bold'; + + sliders = {}; + + pnames = impexp.parameterLegendNames; + vals = impexp.baseValues; + % TODO : setup logic to get y positions based on number of parameters + yposs = [240, 150, 60]; + + for iparam = 1 : numel(pnames) + txt = sprintf('%d. %s * 10^x (initial value: %g)', iparam, pnames{iparam}, vals(iparam)); + sliders{iparam} = impexp.setupSlider(fig, yposs(iparam), txt); + end + + % 4. Connexion aux événements + % On crée une fonction anonyme qui passe TOUS les curseurs + callback_fcn = @(src, event) impexp.updatePlot(ax, lbl, sliders); + for islider = 1 : numel(sliders) + sliders{islider}.ValueChangedFcn = callback_fcn; + end + % Optionnel : Tracer l'état initial + % updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3); + + end + + function updatePlot(impexp, ax, lbl, sliders) + + jsonstruct = impexp.jsonstruct; + + % Figer l'affichage + lbl.Text = 'Processing... '; + lbl.FontColor = '#D95319'; + drawnow; + + try + + baseValues = impexp.baseValues; + + for ival = 1 : numel(baseValues) + vals(ival) = baseValues(ival)*(10^(sliders{ival}.Value)); + end + + jsonstruct = impexp.setParameterValues(vals); + + % 4. Exécution de BattMo + + [model, inputparams, ~] = setupModelFromJson(jsonstruct); + + %% + % We use a dedicated function to compute the initial state for the given electrode concentrations. + options = []; + options.stateInitialization.initializationSetup = 'soc'; + options.stateInitialization.soc = impexp.soc; + + %% + % setup impedance solver and compute the Impedance for a given set of frequencies + impsolv = ImpedanceSolver(inputparams, options); + + frequences = logspace(-2, 3, 30); + Z = impsolv.computeImpedance(frequences); + + % 5. Tracé + plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); + + % Retour à la normale + lbl.Text = 'Done'; + lbl.FontColor = '#77AC30'; + + catch ME + + lbl.Text = 'Erreur lors du calcul (vérifiez la console).'; + lbl.FontColor = '#A2142F'; + disp('--- ERREUR DANS LE CALCUL ---'); + disp(ME.message); + for k = 1:length(ME.stack) + disp(['Ligne ', num2str(ME.stack(k).line), ' dans ', ME.stack(k).name]); + end + end + end + + end + + +end diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m new file mode 100644 index 000000000..8d06ba7f6 --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m @@ -0,0 +1,21 @@ +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); +jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); +ne = 'NegativeElectrode'; +co = 'Coating'; +am = 'ActiveMaterial'; +itf = 'Interface'; + +includeDoubleLayer = true; + +if includeDoubleLayer + + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + +end + +impexp = ImpedanceExplore(jsonstruct); + +close all +impexp.start(); From dfd5e83f22f54291e8bfb8b839c72b72d7d06475 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 18:19:04 +0200 Subject: [PATCH 084/119] minor changes in runCalibration --- .../calibration/runCalibration.m | 53 ++++++++++++------- 1 file changed, 33 insertions(+), 20 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibration.m b/Battery/EquivalentCircuitModel/calibration/runCalibration.m index 391df0e0c..9173d8391 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibration.m @@ -1,4 +1,8 @@ %% ECM Fitting for lithium-ion batteries +% + +%% Impedance computation +% We setup a P2D model and compute the impedance response jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); @@ -23,23 +27,32 @@ jsonstruct = jsonstruct_base; jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode; -jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; -jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl; - +jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; +jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl; +%% +% Setup P2D model from the parameter set |jsonstruct| [model, inputparams, ~] = setupModelFromJson(jsonstruct); + +%% +% We use a dedicated function to compute the initial state for the given electrode concentrations. initstate = initStateChen2020(model, c_ne, c_pe); options = []; options.stateInitialization.initializationSetup = 'given state'; options.stateInitialization.computeSteadyState = false; +%% +% setup input for |ImpedanceSolver| extrastructs = []; extrastructs.initstate = initstate; + +%% +% setup impedance solver and compute the Impedance for a given set of frequencies impsolv = ImpedanceSolver(inputparams, options, extrastructs); -frequences = logspace(-2, 3, 30); +frequencies = logspace(-2, 3, 30); -Z = impsolv.computeImpedance(frequences); +Z = impsolv.computeImpedance(frequencies); figure('Name', 'Nyquist Diagram'); plot(real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); @@ -48,8 +61,6 @@ ylabel('-Im(Z)'); title('Interactive Nyquist Diagram'); -disp('Calculation succeeded'); - %% % @@ -70,8 +81,6 @@ % at lower ones. - - %% Calibration of ECM parameters % Impedance is the opposition to alternating current presented by the combined % effect of resistance and reactance in a circuit. It is obtained with the ratio @@ -83,15 +92,12 @@ % of the study is to obtain the set of parameters as close as possible to the % real impedance curve with the 2-RC Impedance function $Z = R_0 + \frac{R_1}{1 % + j R_1 C_1 \omega} + \frac{R_2}{1 + j R_2 C_2 \omega}$. -% -% We chose unitBoxBFGS as optimization algorithm, which allows other constraints. -% As the two RC parallel cells are symetric, we imposed $C_1 > 2*C_2$ to ensure -% robustness and injectivity of the optimization. Thanks this criteria, a particular -% battery state always lead to the same equivalent circuit. -% -% UnitBoxBFGS needs to work in a box between 0 and 1. We chose to work between -% two vectors pmax and pmin, framing initial values, and to normalize them so -% that pmin becomes 0 and pmax becomes 1. + +%% Calibration using pertubed initial data +% We compute the impedance response of the ECM model for a given set of parameters and use it as an input in our +% calibration algorithm. We choose a initial guess for the parameters that is perturbed from the true values. The +% optimization algorithm should be able to recover the true parameters. + omega = logspace(-4, 2, 50); params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; @@ -108,19 +114,25 @@ feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); + +%% +% plot the results + feis.plotresults_thevenin(best_params, fitting_error); %% Calibration from experimental data % We use data from the Ank's paper (http://dx.doi.org/10.1149/1945-7111/ad14d0) to calibrate the ECM parameters. +% filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv'); data = readmatrix(filename); + omega = data(:, 1); Z_re_exp = data(:, 2); Z_im_exp = data(:, 3); %% -% Initial data +% We choose the following Initial guess params0 = [3.84e-03,... 2.71e-03,... @@ -141,7 +153,8 @@ feis.plotresults_thevenin(best_params, fitting_error); %% Synthetic data from P2D model -% We use impedance data generated from the P2d model with Chen et al's paper (http://dx.doi.org/10.1149/1945-7111/ab9050) parameters +% We use impedance data generated from the P2d model with Chen et al's paper +% (http://dx.doi.org/10.1149/1945-7111/ab9050) parameters [Z_re_exp, Z_im_exp, omega] = load_chen_data(); params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 From 240db7f6a4aecf5fc5485e615bf23b5c77aecdd3 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 18:19:44 +0200 Subject: [PATCH 085/119] fixes in param_dependency --- .../pxdParamsImpact/param_dependency.m | 28 +++++++++++++------ 1 file changed, 20 insertions(+), 8 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m index 8a44ae62d..d6186307f 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m @@ -1,5 +1,4 @@ -function param_dependency() - mrstModule add ad-core mrst-gui mpfa agmg linearsolvers +function param_dependency(jsonstruct) % 1. Chargement des données (Conservez votre méthode de chargement ici) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); @@ -18,8 +17,6 @@ function param_dependency() jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; end - - c_ne = 29.866*mol/litre; c_pe = 17.038*mol/litre; @@ -103,11 +100,26 @@ function updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3) try % 4. Exécution de BattMo + [model, inputparams, ~] = setupModelFromJson(jsonstruct); + + %% + % We use a dedicated function to compute the initial state for the given electrode concentrations. initstate = initStateChen2020(model, c_ne, c_pe); - - impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); - + options = []; + options.stateInitialization.initializationSetup = 'given state'; + options.stateInitialization.computeSteadyState = false; + + %% + % setup input for |ImpedanceSolver| + extrastructs = []; + extrastructs.initstate = initstate; + + + %% + % setup impedance solver and compute the Impedance for a given set of frequencies + impsolv = ImpedanceSolver(inputparams, options, extrastructs); + frequences = logspace(-2, 3, 30); Z = impsolv.computeImpedance(frequences); @@ -127,4 +139,4 @@ function updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3) disp(['Ligne ', num2str(ME.stack(k).line), ' dans ', ME.stack(k).name]); end end -end \ No newline at end of file +end From 125da03174687a645363d73cdefeb6b45d8ead2b Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 13 Jul 2026 18:34:04 +0200 Subject: [PATCH 086/119] more in ImpedanceExplore --- .../examples/pxdParamsImpact/ImpedanceExplore.m | 15 +++++++++++---- .../pxdParamsImpact/runImpedanceExplore.m | 4 +++- 2 files changed, 14 insertions(+), 5 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index 9a88e7255..69f82d01f 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -3,7 +3,6 @@ properties (SetAccess = private) jsonstruct - baseValues end @@ -24,7 +23,6 @@ impexp.jsonstruct = jsonstruct; impexp.setupDefaultParameters() - impexp.baseValues = impexp.getParameterValues(); end @@ -52,6 +50,15 @@ function setupDefaultParameters(impexp) 'Negative Electrode Double Layer Capacitance'}; end + + function setupDefaultParameterLegendNames(impexp) + + params = impexp.parameters; + for iparam = 1 : numel(params) + impexp.parameterLegendNames{iparam} = strjoin(params{iparam}); + end + + end function updateImpedance(impexp) @@ -120,7 +127,7 @@ function start(impexp) sliders = {}; pnames = impexp.parameterLegendNames; - vals = impexp.baseValues; + vals = impexp.getParameterValues(); % TODO : setup logic to get y positions based on number of parameters yposs = [240, 150, 60]; @@ -151,7 +158,7 @@ function updatePlot(impexp, ax, lbl, sliders) try - baseValues = impexp.baseValues; + baseValues = impexp.getParameterValues(); for ival = 1 : numel(baseValues) vals(ival) = baseValues(ival)*(10^(sliders{ival}.Value)); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m index 8d06ba7f6..91259088f 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m @@ -17,5 +17,7 @@ impexp = ImpedanceExplore(jsonstruct); -close all +% delete(findall(0, 'Type', 'Figure')); +% impexp.parameters{1}{1} = 'PositiveElectrode'; +% impexp.setupDefaultParameterLegendNames(); impexp.start(); From bb438066861d1dfe2f1fbd6128bb28a25c218983 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Tue, 14 Jul 2026 11:05:23 +0200 Subject: [PATCH 087/119] fixes in fittingTime, everything works --- .../calibration/FittingTime.m | 30 +++++++++---------- 1 file changed, 15 insertions(+), 15 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 5f6fcfd69..2a3bcedb0 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -399,18 +399,19 @@ function plottest(ftime, best_params, current_test) C2 = p_safe(5); % Get original training time grid as a column vector - time_vec = ftime.time_vec(:); - - [voltage_test, ocv_test] = ftime.setupOCP(time_vec, current_test); + time_test = ftime.time_vec(:); + current_test = current_test(:); + [voltage_test, ocv_test, time_test_sim, current_test_sim] = ftime.setupOCP(time_test, current_test); + % Force all outputs to be column vectors to avoid any plot orientation errors - time_test = time_test(:); - current_test_p2d = current_test_p2d(:); voltage_test = voltage_test(:); ocv_test = ocv_test(:); + time_test_sim = time_test_sim(:); + current_test_sim = current_test_sim(:); % Synchronize the simulation length with the actual P2D points (e.g., 99) - N_points = length(time_test); + N_points = length(time_test_sim); % Initialize ECM state variables V_ecm = zeros(N_points, 1); @@ -419,13 +420,12 @@ function plottest(ftime, best_params, current_test) for k = 1:N_points if k == 1 - dt = time_test(1); + dt = time_test_sim(1); else - dt = time_test(k) - time_test(k-1); + dt = time_test_sim(k) - time_test_sim(k-1); end - I = current_test_p2d(k); % Use the actual simulated current from BattMo - V_ocv = ocv_test(k); % Use the profile-specific OCV from BattMo - + I = current_test_sim(k); % Courant réel synchronisé simulé par BattMo + V_ocv = ocv_test(k); % OCV réel synchronisé simulé par BattMo V_ecm(k) = V_ocv - R0 * I - Uc1 - Uc2; Uc1 = Uc1 + (-Uc1 / (R1 * C1) + I / C1) * dt; @@ -437,7 +437,7 @@ function plottest(ftime, best_params, current_test) % Subplot 1: Applied Current Profile subplot(3,1,1); - plot(time_test, current_test_p2d, 'k', 'LineWidth', 1.5); + plot(time_test_sim, current_test_sim, 'k', 'LineWidth', 1.5); grid on; title('Applied Current Profile (P2D Simulated Range)'); xlabel('Time (s)'); @@ -445,9 +445,9 @@ function plottest(ftime, best_params, current_test) % Subplot 2: Voltage Comparison (P2D vs ECM) subplot(3,1,2); - plot(time_test, voltage_test, 'r-', 'LineWidth', 1.5); + plot(time_test_sim, voltage_test, 'r-', 'LineWidth', 1.5); hold on; - plot(time_test, V_ecm, 'b--', 'LineWidth', 1.5); + plot(time_test_sim, V_ecm, 'b--', 'LineWidth', 1.5); grid on; legend('Ground Truth: P2D Model', 'Validated ECM', 'Location', 'best'); title('Cell Voltage Validation'); @@ -457,7 +457,7 @@ function plottest(ftime, best_params, current_test) % Subplot 3: Instantaneous Residual Error (V_p2d - V_ecm) subplot(3,1,3); error_vec = voltage_test - V_ecm; - plot(time_test, error_vec, 'g', 'LineWidth', 1.2); + plot(time_test_sim, error_vec, 'g', 'LineWidth', 1.2); grid on; title('Residual Error (V_{p2d} - V_{ecm})'); xlabel('Time (s)'); From 4f8b01b6afbca9b380ebcaf548014e3c5c257a7c Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 11:05:44 +0200 Subject: [PATCH 088/119] added function to list the parameters --- .../pxdParamsImpact/ImpedanceExplore.m | 31 ++++++++++--------- 1 file changed, 16 insertions(+), 15 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index 69f82d01f..4d1443d63 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -1,8 +1,9 @@ classdef ImpedanceExplore < handle - properties (SetAccess = private) + properties (SetAccess = immutable) jsonstruct + model end @@ -13,7 +14,6 @@ soc = 1 parameters - parameterLegendNames end @@ -21,11 +21,22 @@ function impexp = ImpedanceExplore(jsonstruct) + [model, inputparams, jsonstruct] = setupModelFromJson(jsonstruct); impexp.jsonstruct = jsonstruct; + impexp.model = model; + impexp.setupDefaultParameters() end + function viewOptions(impexp) + + fjv = flattenJsonStruct(impexp.jsonstruct, 'doprint', false); + fprintf('\n\n*** List of all the scalar parameters in the model ***\n'); + fjv.print('filter', {'value', @(val) (isnumeric(val) && isscalar(val))}); + + end + function setupDefaultParameters(impexp) elyte = 'Electrolyte'; @@ -42,28 +53,18 @@ function setupDefaultParameters(impexp) impexp.parameters = {{ne, co, am, sd, 'referenceDiffusionCoefficient'}, ... {ne, co, am, itf, 'reactionRateConstant'}, ... {ne, co, am, itf, 'doubleLayerCapacitance'}}; - - %% - % TODO : setup default way to get legend - impexp.parameterLegendNames = {'Negative Electrode Solid Diffusion Coefficient', ... - 'Negative Electrode Reaction Rate Constant', ... - 'Negative Electrode Double Layer Capacitance'}; end - function setupDefaultParameterLegendNames(impexp) + function pnames = setupParameterLegendNames(impexp) params = impexp.parameters; for iparam = 1 : numel(params) - impexp.parameterLegendNames{iparam} = strjoin(params{iparam}); + pnames{iparam} = strjoin(params{iparam}); end end - function updateImpedance(impexp) - - end - function sld = setupSlider(imexp, fig, ypos, txt) uilabel(fig , ... @@ -126,7 +127,7 @@ function start(impexp) sliders = {}; - pnames = impexp.parameterLegendNames; + pnames = impexp.setupParameterLegendNames(); vals = impexp.getParameterValues(); % TODO : setup logic to get y positions based on number of parameters yposs = [240, 150, 60]; From 19d1b787740dd24afa5cbfc2081a83a9c79851de Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 11:18:34 +0200 Subject: [PATCH 089/119] update --- .../examples/pxdParamsImpact/ImpedanceExplore.m | 2 +- .../examples/pxdParamsImpact/runImpedanceExplore.m | 13 ++++++++++--- 2 files changed, 11 insertions(+), 4 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index 4d1443d63..b302c4b6e 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -21,7 +21,7 @@ function impexp = ImpedanceExplore(jsonstruct) - [model, inputparams, jsonstruct] = setupModelFromJson(jsonstruct); + model = setupModelFromJson(jsonstruct); impexp.jsonstruct = jsonstruct; impexp.model = model; diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m index 91259088f..1dc7c6826 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m @@ -17,7 +17,14 @@ impexp = ImpedanceExplore(jsonstruct); -% delete(findall(0, 'Type', 'Figure')); -% impexp.parameters{1}{1} = 'PositiveElectrode'; -% impexp.setupDefaultParameterLegendNames(); +erase_previous_figure = true; +if erase_previous_figure + delete(findall(0, 'Type', 'Figure')); +end + +change_a_parameter = true; +if change_a_parameter + impexp.parameters{1} ={'PositiveElectrode', 'Coating', 'ActiveMaterial', 'Interface', 'volumetricSurfaceArea'}; +end + impexp.start(); From 67ed9909a3b26052a8bb4a8f2f942a6472558267 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 11:24:37 +0200 Subject: [PATCH 090/119] added notebooks --- .../notebooks/runCalibration.ipynb | 586 ++++++++++++++++++ .../calibration/notebooks/runCalibration.mlx | Bin 0 -> 328178 bytes 2 files changed, 586 insertions(+) create mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb create mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.mlx diff --git a/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb new file mode 100644 index 000000000..34e31dbad --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb @@ -0,0 +1,586 @@ +{ + "cells": [ + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "# ECM Fitting for lithium\\-ion batteries\n", + "\n", + "## Impedance computation\n", + "\n", + "We setup a P2D model and compute the impedance response\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json'));\n", + "jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json'));\n", + "jsonstruct_base = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry});\n", + "\n", + "jsonstruct_base.NegativeElectrode.Coating.ActiveMaterial.Interface.useDoubleLayerCapacity = true;\n", + "\n", + "c_ne = 29.866*mol/litre;\n", + "c_pe = 17.038*mol/litre;\n", + "\n", + "p_diffusion = 0;\n", + "p_reactionRate = 0;\n", + "p_doubleLayerCapacitance = 0;\n", + "base_diff_anode = 1.3135e-15;\n", + "base_rate_anode = 5.031e-11;\n", + "base_cdl = 0.2;\n", + "\n", + "val_diff_anode = base_diff_anode * (10^p_diffusion);\n", + "val_rate_anode = base_rate_anode * (10^p_reactionRate);\n", + "val_cdl = base_cdl * (10^p_doubleLayerCapacitance);\n", + "\n", + "jsonstruct = jsonstruct_base;\n", + "\n", + "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode;\n", + "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode;\n", + "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl;" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Setup P2D model from the parameter set jsonstruct\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 2, + "metadata": {}, + "source": [ + "[model, inputparams, ~] = setupModelFromJson(jsonstruct);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "We use a dedicated function to compute the initial state for the given electrode concentrations.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 3, + "metadata": {}, + "source": [ + "initstate = initStateChen2020(model, c_ne, c_pe);\n", + "options = [];\n", + "options.stateInitialization.initializationSetup = 'given state';\n", + "options.stateInitialization.computeSteadyState = false;" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "setup input for ImpedanceSolver\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 4, + "metadata": {}, + "source": [ + "extrastructs = [];\n", + "extrastructs.initstate = initstate;" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "setup impedance solver and compute the Impedance for a given set of frequencies\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 5, + "metadata": {}, + "source": [ + "impsolv = ImpedanceSolver(inputparams, options, extrastructs);\n", + "frequencies = logspace(-2, 3, 30);\n", + "\n", + "Z = impsolv.computeImpedance(frequencies);\n", + "\n", + "figure('Name', 'Nyquist Diagram');\n", + "plot(real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD');\n", + "grid on;\n", + "xlabel('Re(Z)');\n", + "ylabel('-Im(Z)');\n", + "title('Interactive Nyquist Diagram');" + ], + "outputs": [ + { + "data": { + "text/html": [ + "

\"figure_0.png\"
" + ] + }, + "metadata": {}, + "execution_count": 5, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "The impact of diffusion is mainly seen on the tail at low frequencies. While a larger coefficient does not have much of an impact, using a very small one shows how strongly the diffusion phenomenon is linked to this tail.\n", + "\n", + "\n", + "The double\\-layer capacitance affects the first semicircle, as the frequency at its peak is governed by the relation $f_{\\max } =\\frac{1\\;}{2\\pi R_{\\textrm{CT}} C_{\\textrm{DL}} }$ . A large capacitance will result in a lower $f_{\\max }$ (a shift to the left, as frequencies are plotted inversely), while a small one will shift the center of the first semicircle to the right.\n", + "\n", + "\n", + "Finally, the influence of the reaction rate on the Nyquist diagram is clearly evident. A more facile reaction (i.e., a higher reaction rate) leads to a lower charge\\-transfer resistance. As this parameter dictates the width of the first semicircle, it virtually vanishes at high reaction rates and broadens considerably at lower ones.\n", + "\n", + "## Calibration of ECM parameters\n", + "\n", + "Impedance is the opposition to alternating current presented by the combined effect of resistance and reactance in a circuit. It is obtained with the ratio of complex voltage and complex current : $Z=U/I$ . It extends the concept of resistance to alternating current (AC) circuits.\n", + "\n", + "\n", + "We tried through our optimization algorithm to fit different battery models to ECM through five parameters, $R_0$ , $R_1$ , $C_1$ , $R_2$ and $C_2$ . The aim of the study is to obtain the set of parameters as close as possible to the real impedance curve with the 2\\-RC Impedance function $Z=R_0 +\\frac{R_1 }{1+jR_1 C_1 \\omega }+\\frac{R_2 }{1+jR_2 C_2 \\omega }$ .\n", + "\n", + "## Calibration using pertubed initial data\n", + "\n", + "We compute the impedance response of the ECM model for a given set of parameters and use it as an input in our calibration algorithm. We choose a initial guess for the parameters that is perturbed from the true values. The optimization algorithm should be able to recover the true parameters.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 6, + "metadata": {}, + "source": [ + "omega = logspace(-4, 2, 50);\n", + "params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0];\n", + "[Z_re_exp, Z_im_exp] = load_nyquist(params, omega);\n", + "\n", + "params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2\n", + "\n", + "a = 1000;\n", + "\n", + "pmin = params0 / a;\n", + "pmax = params0 * a;\n", + "scales = [pmin, pmax];\n", + "\n", + "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", + "\n", + "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" + ], + "outputs": [ + { + "data": { + "text/plain": [ + "It: 0 | val: 1.373e-31 | ls-its: NaN | pgrad: 1.164e-12\n", + "It: 1 | val: 1.373e-31 | ls-its: 0 | pgrad: 1.152e-12\n", + "Stopped because reached gradTol = 1.000000e-05." + ] + }, + "metadata": {}, + "execution_count": 6, + "output_type": "execute_result" + }, + { + "data": { + "text/html": [ + "
\"figure_1.png\"
" + ] + }, + "metadata": {}, + "output_type": "display_data" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "plot the results\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 7, + "metadata": {}, + "source": [ + "feis.plotresults_thevenin(best_params, fitting_error);" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
\"figure_2.png\"
" + ] + }, + "metadata": {}, + "execution_count": 7, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "## Calibration from experimental data\n", + "\n", + "We use data from the Ank's paper ([http://dx.doi.org/10.1149/1945\\-7111/ad14d0](http://dx.doi.org/10.1149/1945-7111/ad14d0)) to calibrate the ECM parameters.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 8, + "metadata": {}, + "source": [ + "filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv');\n", + "data = readmatrix(filename);\n", + "\n", + "omega = data(:, 1);\n", + "Z_re_exp = data(:, 2);\n", + "Z_im_exp = data(:, 3);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "We choose the following Initial guess\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 9, + "metadata": {}, + "source": [ + "params0 = [3.84e-03,...\n", + " 2.71e-03,...\n", + " 6.00e+03,...\n", + " 9.48e-04,...\n", + "1.11e+01]; % initial condition: C1>2*C2\n", + "\n", + "a = 1000;\n", + "\n", + "pmin = params0 / a;\n", + "pmax = params0 * a;\n", + "scales = [pmin, pmax];\n", + "\n", + "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", + "\n", + "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" + ], + "outputs": [ + { + "data": { + "text/plain": [ + "It: 0 | val: 3.717e-01 | ls-its: NaN | pgrad: 1.563e+02\n", + "It: 1 | val: 3.716e-01 | ls-its: 3 | pgrad: 1.561e+02\n", + "It: 2 | val: 1.870e-01 | ls-its: 8 | pgrad: 1.549e+02\n", + "It: 3 | val: 1.827e-01 | ls-its: 3 | pgrad: 1.616e+03\n", + "It: 4 | val: 1.596e-01 | ls-its: 2 | pgrad: 1.673e+03\n", + "It: 5 | val: 1.419e-01 | ls-its: 2 | pgrad: 4.695e+02\n", + "It: 6 | val: 8.869e-02 | ls-its: 1 | pgrad: 1.096e+03\n", + "It: 7 | val: 6.885e-02 | ls-its: 1 | pgrad: 2.369e+02\n", + "It: 8 | val: 6.869e-02 | ls-its: 1 | pgrad: 1.020e+02\n", + "It: 9 | val: 6.869e-02 | ls-its: 1 | pgrad: 1.253e+01\n", + "It: 10 | val: 6.866e-02 | ls-its: 2 | pgrad: 6.159e+00\n", + "It: 11 | val: 6.864e-02 | ls-its: 1 | pgrad: 3.511e+01\n", + "It: 12 | val: 6.862e-02 | ls-its: 1 | pgrad: 2.040e+01\n", + "It: 13 | val: 6.862e-02 | ls-its: 2 | pgrad: 1.882e+01\n", + "It: 14 | val: 6.862e-02 | ls-its: 1 | pgrad: 3.677e+00\n", + "It: 15 | val: 6.861e-02 | ls-its: 2 | pgrad: 2.463e+00\n", + "It: 16 | val: 6.860e-02 | ls-its: 1 | pgrad: 1.650e+01\n", + "It: 17 | val: 6.860e-02 | ls-its: 1 | pgrad: 5.232e+00\n", + "It: 18 | val: 6.860e-02 | ls-its: 1 | pgrad: 7.828e-01\n", + "It: 19 | val: 6.860e-02 | ls-its: 2 | pgrad: 6.014e-03\n", + "It: 20 | val: 6.860e-02 | ls-its: 1 | pgrad: 8.585e-03\n", + "It: 21 | val: 6.860e-02 | ls-its: 1 | pgrad: 1.911e-03\n", + "It: 22 | val: 6.860e-02 | ls-its: 1 | pgrad: 4.279e-04\n", + "It: 23 | val: 6.860e-02 | ls-its: 1 | pgrad: 2.402e-04\n", + "Stopped because reached objChangeTol = 1.000000e-15." + ] + }, + "metadata": {}, + "execution_count": 9, + "output_type": "execute_result" + }, + { + "data": { + "text/html": [ + "
\"figure_3.png\"
" + ] + }, + "metadata": {}, + "output_type": "display_data" + } + ] + }, + { + "cell_type": "code", + "execution_count": 10, + "metadata": {}, + "source": [ + "\n", + "feis.plotresults_thevenin(best_params, fitting_error);" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
\"figure_4.png\"
" + ] + }, + "metadata": {}, + "execution_count": 10, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "## Synthetic data from P2D model\n", + "\n", + "We use impedance data generated from the P2d model with Chen et al's paper ([http://dx.doi.org/10.1149/1945\\-7111/ab9050](http://dx.doi.org/10.1149/1945-7111/ab9050)) parameters\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 11, + "metadata": {}, + "source": [ + "[Z_re_exp, Z_im_exp, omega] = load_chen_data();\n", + "params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2\n", + "\n", + "a = 1000;\n", + "\n", + "pmin = params0 / a;\n", + "pmax = params0 * a;\n", + "scales = [pmin, pmax];\n", + "\n", + "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", + "\n", + "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" + ], + "outputs": [ + { + "data": { + "text/plain": [ + "It: 0 | val: 5.457e+01 | ls-its: NaN | pgrad: 1.427e+05\n", + "It: 1 | val: 3.954e+01 | ls-its: 1 | pgrad: 1.427e+05\n", + "It: 2 | val: 1.472e+01 | ls-its: 1 | pgrad: 1.126e+05\n", + "Line search at max step size, Wolfe conditions not satisfied for this step.\n", + "Hessian not updated during iteration 3.\n", + "It: 3 | val: 1.177e+01 | ls-its: 4 | pgrad: 1.395e+03\n", + "It: 4 | val: 5.389e+00 | ls-its: 1 | pgrad: 5.470e+04\n", + "It: 5 | val: 5.370e+00 | ls-its: 1 | pgrad: 8.495e+03\n", + "It: 6 | val: 5.190e+00 | ls-its: 1 | pgrad: 8.371e+03\n", + "It: 7 | val: 4.888e+00 | ls-its: 1 | pgrad: 7.419e+03\n", + "It: 8 | val: 4.229e+00 | ls-its: 1 | pgrad: 1.211e+04\n", + "It: 9 | val: 3.452e+00 | ls-its: 1 | pgrad: 1.707e+04\n", + "It: 10 | val: 2.949e+00 | ls-its: 1 | pgrad: 1.621e+04\n", + "It: 11 | val: 2.819e+00 | ls-its: 1 | pgrad: 8.393e+03\n", + "It: 12 | val: 2.810e+00 | ls-its: 1 | pgrad: 1.636e+03\n", + "It: 13 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.247e+02\n", + "It: 14 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", + "It: 15 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", + "It: 16 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", + "It: 17 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", + "It: 18 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", + "It: 19 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", + "It: 20 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.240e+02\n", + "It: 21 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.243e+02\n", + "It: 22 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.639e+02\n", + "It: 23 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.656e+02\n", + "It: 24 | val: 2.809e+00 | ls-its: 1 | pgrad: 2.255e+02\n", + "It: 25 | val: 2.809e+00 | ls-its: 1 | pgrad: 2.258e+02\n", + "It: 26 | val: 2.808e+00 | ls-its: 1 | pgrad: 2.264e+02\n", + "It: 27 | val: 2.808e+00 | ls-its: 1 | pgrad: 3.858e+02\n", + "It: 28 | val: 2.807e+00 | ls-its: 1 | pgrad: 7.234e+02\n", + "It: 29 | val: 2.807e+00 | ls-its: 1 | pgrad: 9.166e+02\n", + "It: 30 | val: 2.806e+00 | ls-its: 1 | pgrad: 9.196e+02\n", + "It: 31 | val: 2.805e+00 | ls-its: 1 | pgrad: 8.062e+02\n", + "It: 32 | val: 2.804e+00 | ls-its: 1 | pgrad: 6.568e+02\n", + "It: 33 | val: 2.801e+00 | ls-its: 1 | pgrad: 2.552e+02\n", + "It: 34 | val: 2.798e+00 | ls-its: 1 | pgrad: 3.681e+02\n", + "It: 35 | val: 2.797e+00 | ls-its: 1 | pgrad: 1.040e+03\n", + "It: 36 | val: 2.795e+00 | ls-its: 1 | pgrad: 1.388e+03\n", + "It: 37 | val: 2.792e+00 | ls-its: 1 | pgrad: 1.385e+03\n", + "It: 38 | val: 2.790e+00 | ls-its: 1 | pgrad: 1.143e+03\n", + "It: 39 | val: 2.783e+00 | ls-its: 1 | pgrad: 8.273e+02\n", + "It: 40 | val: 2.775e+00 | ls-its: 1 | pgrad: 4.889e+02\n", + "It: 41 | val: 2.769e+00 | ls-its: 1 | pgrad: 1.078e+03\n", + "It: 42 | val: 2.767e+00 | ls-its: 1 | pgrad: 1.934e+03\n", + "It: 43 | val: 2.766e+00 | ls-its: 1 | pgrad: 2.103e+03\n", + "It: 44 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.942e+03\n", + "It: 45 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.817e+03\n", + "It: 46 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.716e+03\n", + "It: 47 | val: 2.765e+00 | ls-its: 1 | pgrad: 1.541e+03\n", + "It: 48 | val: 2.765e+00 | ls-its: 1 | pgrad: 1.298e+03\n", + "It: 49 | val: 2.764e+00 | ls-its: 1 | pgrad: 1.016e+03\n", + "It: 50 | val: 2.763e+00 | ls-its: 1 | pgrad: 8.574e+02\n", + "It: 51 | val: 2.761e+00 | ls-its: 1 | pgrad: 9.486e+02\n", + "It: 52 | val: 2.759e+00 | ls-its: 1 | pgrad: 1.330e+03\n", + "It: 53 | val: 2.754e+00 | ls-its: 1 | pgrad: 1.585e+03\n", + "It: 54 | val: 2.750e+00 | ls-its: 1 | pgrad: 2.131e+03\n", + "It: 55 | val: 2.738e+00 | ls-its: 1 | pgrad: 2.181e+03\n", + "It: 56 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.461e+03\n", + "It: 57 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.015e+03\n", + "It: 58 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.077e+03\n", + "It: 59 | val: 2.735e+00 | ls-its: 1 | pgrad: 1.083e+03\n", + "It: 60 | val: 2.726e+00 | ls-its: 1 | pgrad: 1.030e+03\n", + "It: 61 | val: 2.723e+00 | ls-its: 1 | pgrad: 1.042e+03\n", + "It: 62 | val: 2.722e+00 | ls-its: 2 | pgrad: 1.129e+03\n", + "It: 63 | val: 2.721e+00 | ls-its: 1 | pgrad: 1.343e+03\n", + "It: 64 | val: 2.711e+00 | ls-its: 1 | pgrad: 1.515e+03\n", + "It: 65 | val: 2.695e+00 | ls-its: 1 | pgrad: 2.287e+03\n", + "It: 66 | val: 2.658e+00 | ls-its: 1 | pgrad: 2.906e+03\n", + "It: 67 | val: 2.632e+00 | ls-its: 1 | pgrad: 3.567e+03\n", + "It: 68 | val: 2.619e+00 | ls-its: 1 | pgrad: 3.168e+03\n", + "It: 69 | val: 2.613e+00 | ls-its: 1 | pgrad: 2.037e+03\n", + "It: 70 | val: 2.612e+00 | ls-its: 1 | pgrad: 4.564e+02\n", + "It: 71 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.066e+02\n", + "It: 72 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.871e+02\n", + "It: 73 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.986e+02\n", + "It: 74 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.032e+02\n", + "It: 75 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.036e+02\n", + "It: 76 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.072e+02\n", + "It: 77 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.082e+02\n", + "It: 78 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.075e+02\n", + "It: 79 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.041e+02\n", + "It: 80 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.970e+02\n", + "It: 81 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.846e+02\n", + "It: 82 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.225e+02\n", + "It: 83 | val: 2.610e+00 | ls-its: 1 | pgrad: 3.345e+02\n", + "It: 84 | val: 2.610e+00 | ls-its: 1 | pgrad: 4.148e+02\n", + "It: 85 | val: 2.610e+00 | ls-its: 1 | pgrad: 3.974e+02\n", + "It: 86 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.938e+02\n", + "It: 87 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.080e+02\n", + "It: 88 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.614e+01\n", + "It: 89 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.761e+01\n", + "It: 90 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.107e+02\n", + "It: 91 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.801e+01\n", + "It: 92 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.900e+01\n", + "It: 93 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.731e+01\n", + "It: 94 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.538e+01\n", + "It: 95 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.371e+01\n", + "It: 96 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.189e+01\n", + "It: 97 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.062e+01\n", + "It: 98 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.754e+01\n", + "It: 99 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.235e+02\n", + "It: 100 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.047e+02\n", + "It: 101 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.272e+01\n", + "It: 102 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.581e+01\n", + "It: 103 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.677e+01\n", + "It: 104 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.742e+01\n", + "It: 105 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.749e+01\n", + "It: 106 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.786e+01\n", + "It: 107 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.867e+01\n", + "It: 108 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.923e+01\n", + "It: 109 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.918e+01\n", + "It: 110 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.860e+01\n", + "It: 111 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.515e+01\n", + "It: 112 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.549e+01\n", + "It: 113 | val: 2.609e+00 | ls-its: 1 | pgrad: 5.580e+01\n", + "It: 114 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.692e+01\n", + "It: 115 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.067e+01\n", + "It: 116 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.227e+01\n", + "It: 117 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.115e+01\n", + "It: 118 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.161e+01\n", + "It: 119 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.071e+00\n", + "It: 120 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.408e+01\n", + "It: 121 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.767e+01\n", + "It: 122 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.603e+01\n", + "It: 123 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.029e+01\n", + "It: 124 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.346e+01\n", + "It: 125 | val: 2.609e+00 | ls-its: 1 | pgrad: 5.312e+00\n", + "It: 126 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.129e+01\n", + "It: 127 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.024e+01\n", + "It: 128 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.011e+00\n", + "It: 129 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.153e-01\n", + "It: 130 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.984e-01\n", + "It: 131 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.063e-01\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 132 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.214e-01\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 133 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.059e-01\n", + "It: 134 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.800e+00\n", + "It: 135 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.232e+00\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 136 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.554e-01\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 137 | val: 2.609e+00 | ls-its: 2 | pgrad: 3.571e-01\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 138 | val: 2.609e+00 | ls-its: 2 | pgrad: 5.313e-02\n", + "Non-inceasing search direction, trying previous Hessian approximation.\n", + "It: 139 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.891e-01\n", + "It: 140 | val: 2.609e+00 | ls-its: 0 | pgrad: 3.168e-02\n", + "Stopped because reached objChangeTol = 1.000000e-15." + ] + }, + "metadata": {}, + "execution_count": 11, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "code", + "execution_count": 12, + "metadata": {}, + "source": [ + "feis.plotresults_thevenin(best_params, fitting_error);" + ], + "outputs": [] +} + ], + "metadata": { + "kernelspec": { + "display_name": "MATLAB (matlabkernel)", + "language": "matlab", + "name": "matlab" + }, + 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--- a/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb +++ b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb @@ -553,6 +553,15 @@ "metadata": {}, "execution_count": 11, "output_type": "execute_result" + }, + { + "data": { + "text/html": [ + "

\"figure_5.png\"
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Tue, 14 Jul 2026 14:32:10 +0200 Subject: [PATCH 092/119] update in doc --- Documentation/batteryphysics.rst | 5 - Documentation/ecm.rst | 294 +++++++++++++++++++++++++++++++ Documentation/index.rst | 1 + 3 files changed, 295 insertions(+), 5 deletions(-) create mode 100644 Documentation/ecm.rst diff --git a/Documentation/batteryphysics.rst b/Documentation/batteryphysics.rst index 779877add..12b565e5d 100644 --- a/Documentation/batteryphysics.rst +++ b/Documentation/batteryphysics.rst @@ -13,7 +13,6 @@ Battery Physics plating runSwellingExample.ipynb soliddiffusion - runImpedanceScript.nblink .. grid:: 2 @@ -52,9 +51,5 @@ Battery Physics :ref:`Solid Diffusion Models ` - .. grid-item-card:: - :padding: 2 - - :ref:`Battery Impedance Computation ` diff --git a/Documentation/ecm.rst b/Documentation/ecm.rst new file mode 100644 index 000000000..f41b52341 --- /dev/null +++ b/Documentation/ecm.rst @@ -0,0 +1,294 @@ +================================= +EIS and Equivalent Circuit Models +================================= + +.. toctree:: + :maxdepth: 2 + :hidden: + + runImpedanceScript.nblink + runCalibration.nblink + +ECM fitting for lithium-ion batteries +------------------------------------- + +Abstract +^^^^^^^^ + +Batteries become a central piece of electrification of our energy consumption, +especially for transports. To improve their performances, innovation is getting +faster and research is very active. But before building a battery, it is +important to have an idea of how it will react in different conditions, and +modeling appears useful. It is necessary to work on complex models that fit the +best reality, but also to have powerful models that are a lot simpler. This +model could give important information such as State of Charge or State of +Health, without spending a lot of time, with the minimum complexity. + +We present a work on Equivalent Circuit Model to simulate a complete battery +through only a few parameters. The battery management system needs the value of +those parameters to be efficient. ECM are now the most used model for battery +management systems. + +Getting the impedance from PXD Model +^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^ + +ECM parameterisation from PXD model using automatic differentiation. + +Obtaining the impedance is a major part of the work, as we try to fit the +impedance given by our parameters to the synthetic impedance from the PXD +model. + +We work with the state vector :math:`\mathcal{X}(t, x)` containing all the +variables from the PXD model: + +.. math:: + + \mathcal{X}(t, x) = + [c_{\mathrm{ne}}(t, x), \phi_{\mathrm{ne}}(t, x), + c_{\mathrm{elyte}}(t, x), \phi_{\mathrm{elyte}}(t, x), \ldots] + +The generic equation of the system is + +.. math:: + + \frac{\partial \mathcal{M}(\mathcal{X})}{\partial t} + \mathcal{A}(\mathcal{X}) = 0. + +The operators :math:`\mathcal{M}` and :math:`\mathcal{A}` are non-linear, but +we discretize them and :math:`\mathcal{X}(t, x)` becomes :math:`X(t)` +belonging to :math:`\mathbb{R}^{N}`. + +The equation then becomes a non-linear system of *ordinary differential +equations*: + +.. math:: + + \frac{\partial M(X)}{\partial t} + A(X) = I(t)b(X). + +Here :math:`I(t)` is the current and :math:`b` is mostly empty. An implicit +method is then used for the time discretization. One finds :math:`X^{n+1}` +from :math:`X^{n}` at time step :math:`n` by solving the equation for the +unknown :math:`X`: + +.. math:: + + \frac{M(X) - M(X^{n})}{\Delta t} + A(X) = b(X)I(t^{n+1}). + +Then the system is linearized around a state given by :math:`X_{0}` with a +small perturbation :math:`\delta X = X - X_{0}`. The term :math:`A(X)` becomes + +.. math:: + + A(X) = A(X_{0}) + D_{A}(X_{0})\delta X, + +with :math:`D_{A}` the Jacobian of :math:`A`. Applying the same process for +:math:`M` and :math:`b` (:math:`D_{M}` and :math:`D_{b}` being their +Jacobians) gives the following linear system of ordinary differential +equations: + +.. math:: + + D_{M}\frac{\partial}{\partial t}\delta X + A(X_{0}) + D_{A}\delta X + = I(t)b(X_{0}) + I(t)D_{b}\delta X. + +:math:`X_{0}` is a solution to the steady-state problem :math:`I(t) = 0`, which +implies :math:`A(X_{0}) = 0`. Also, :math:`\delta X \ll 1` implies +:math:`I(t)b(X_{0}) \gg I(t)D_{b}(X_{0})\delta X`, so the last term is +neglected. + +The final equation is + +.. math:: + + D_{M}\frac{\partial}{\partial t}\delta X + D_{A}\delta X = I(t)b_{0}. + +It is possible to obtain :math:`D_M` and :math:`D_A` with the Jacobian. Since + +.. math:: + + J(\Delta t) = \frac{D_M}{\Delta t} + D_A, + +this leads to + +.. math:: + + D_M = 2\Delta t \left(J(\Delta t) - J(2\Delta t)\right) + +and + +.. math:: + + D_A = 2\left(J(\Delta t) - J(2\Delta t)\right). + +The Fourier transform of this equation is + +.. math:: + + [i\omega D_{M} + D_{A}]\overline{\delta X} = \bar{I}b_{0}, + +with :math:`I(t) = \bar{I}e^{i\omega t}` and +:math:`\delta X = \overline{\delta X}e^{i\omega t}`. + +So + +.. math:: + + \overline{\delta X} = \left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}\bar{I}. + +There is a certain vector :math:`r` so that :math:`U = r^{t}X`, where +:math:`U` is the voltage response. + +Then + +.. math:: + + U = r^{t}X_{0} + r^{t}\delta X, + +so :math:`U - U_{0} = \bar{U}e^{i\omega t}` with +:math:`U_{0} = r^{t}X_{0}`. + +It follows that + +.. math:: + + \bar{U} = r^{t}\overline{\delta X} + +and therefore + +.. math:: + + \bar{U} = r^{t}\left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}\bar{I}. + +At the end it gives + +.. math:: + + Z(\omega) = r^{t}\left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}. + +ECM Presentation +^^^^^^^^^^^^^^^^ + +Objective +""""""""" + +Effective everyday operation of a battery requires the Battery Management +System (BMS) to continuously monitor its real-time state (State of Charge, +State of Health). Given the practical challenges of measuring this state via +chemical methods, modeling offers a useful alternative. Physics-based models +offer very good approximations, but need thousands of parameters. By +identifying the very few parameters of the Equivalent Circuit Model (ECM) in +real-time, valuable information about the system can be extracted. Because each +set of parameters maps to a specific physical state, the first approach could +be referencing a lookup table to link a particular state to a set of +parameters. Another one, more accurate, could be to train a neural network to +develop a strong state-prediction model. + +Theory +"""""" + +The electrical activity of a battery can be modelled by an Open Circuit Voltage +(OCV), which is a perfect source of current. This is the simplest way to +simulate it. One can realize that it is necessary to go a bit deeper in the +analysis, with the addition of a resistor, which symbolizes the heat +dissipation. This model remains very simple. It is possible to add the +diffusion phenomena with a series of :math:`n` parallel resistor-capacitance +pairs. This is the :math:`n`-Thevenin model. + +Example of a 2-Thevenin Model (`Sun, comprehensive review of ECM `_) + +It is a good compromise to have 2 RC networks, because the model remains simple +but allows two different time-scaled phenomena. However, another flaw of this +model is the symmetry of the two pairs, which makes identifiability much +harder. + +The impedance of this circuit is + +.. math:: + + Z = R_0 + \frac{R_1}{1 + j R_1 C_1 \omega} + + \frac{R_2}{1 + j R_2 C_2 \omega}. + +Another way to model diffusion is with a Warburg component, which has the +impedance :math:`Z_W = \frac{1}{Y_0 \sqrt{j\omega}}` and adds to the Nyquist +diagram a 45° slope for low frequencies. A Warburg element is the equivalent of +an infinity of capacitance/resistor pairs. + +Warburg circuit model (`Analog Devices `_, 2021) + +Some researchers, as Santoni in his `paper `_, +have tried some other similar circuits with more accurate tools, but further +from basic electrical elements. He replaced capacitors by constant phase +elements (CPE), adding an :math:`\alpha` parameter to quantify non-ideality. +The impedance is :math:`Z = \frac{1}{Q\left(j\omega\right)^{\alpha}}`. +:math:`\alpha = 1` would make it an ideal capacitor, while +:math:`\alpha = 0.5` corresponds to a Warburg element. + +A 2nd-Order model with CPE used by Santoni + +Physical Meaning of ECM components (`Analog Devices `_, 2021) +""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""" + +ECM are built after Occam's razor principles, where each component has to be +linked to a physical phenomenon of the battery (`Fletcher `_, 2013): + +*The ohmic resistance* (:math:`R_\Omega`) represents the battery's internal +resistance (of the electrolyte and of the electrode interface for instance) and +accounts for heat generation during operation. This resistance naturally +increases as the battery ages. Experimentally, it can be determined by +observing the battery's voltage drop response to a load. On a Nyquist diagram, +it corresponds to the real part of the impedance where the imaginary component +is zero. + +*The first RC network* is associated with the charge-transfer process at the +electrode-electrolyte interface. The resistance :math:`R_{\textrm{CT}}` +reflects the kinetic barrier electrons must overcome to move from the solid +electrode into the liquid electrolyte. The capacitance +:math:`C_{\textrm{DL}}` represents the double-layer capacitance, formed by two +parallel layers of opposing charges. This RC pair governs the mid-frequency +behavior (typically between 1 Hz and 1 kHz) and manifests as the first +semi-circular arc on the Nyquist plot. + +*The second RC network*, or Warburg element, is associated with a much slower +phenomenon characterized by a significantly larger magnitude: the mass +transport driven by lithium ion diffusion. This dictates the low-frequency +response, appearing as a characteristic 45° phase shift in the Nyquist diagram, +which reflects the fact that diffusion becomes the rate-determining step in +this range. + +Electrochemical processes linked to EIS regions (`Analog Devices `_, 2021) + +Impact on Impedance of physical parameters from PXD model +^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^ + +The PXD BattMo model was developed using parameters derived from the study by +Chen et al. (2020). These parameters were subsequently modified to better +understand their influence on the impedance diagram. + +Experimental impedance data were acquired using Electrochemical Impedance +Spectroscopy (EIS). EIS is a highly sensitive, non-destructive analytical +technique utilized to investigate the internal dynamics of electrochemical +systems, such as lithium-ion batteries. The method involves applying a +small-amplitude alternating current (AC) excitation across a broad frequency +spectrum, ranging from thousands of hertz down to fractions of a hertz, and +recording the subsequent response and phase shift. + +Because the applied variations remain small, EIS assumes the system remains in +a pseudo-steady state, thereby enabling the use of Fourier transform analysis. + +By analyzing the battery's response across distinct frequency bands, its +internal mechanisms can be diagnosed. Specifically, high frequencies reveal the +pure ohmic resistance of the components, mid-frequencies capture the +charge-transfer resistance, and low frequencies reflect mass transport and +diffusion processes, providing insight into the migration rate of lithium ions +through the solid electrode particles. + +.. grid:: 2 + + .. grid-item-card:: + :padding: 2 + + :ref:`Battery Impedance Computation ` + + .. grid-item-card:: + :padding: 2 + + :ref:`ECM calibration ` diff --git a/Documentation/index.rst b/Documentation/index.rst index 205b33e74..8fff40b77 100644 --- a/Documentation/index.rst +++ b/Documentation/index.rst @@ -13,6 +13,7 @@ output geometryinput batteryphysics + ecm elchemsystems optimisation modeling From 162176d13f55b46eb7904e2bb4d2ee356dbb0292 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 14:32:57 +0200 Subject: [PATCH 093/119] added nblink --- Documentation/runCalibration.nblink | 3 +++ 1 file changed, 3 insertions(+) create mode 100644 Documentation/runCalibration.nblink diff --git a/Documentation/runCalibration.nblink b/Documentation/runCalibration.nblink new file mode 100644 index 000000000..075b83087 --- /dev/null +++ b/Documentation/runCalibration.nblink @@ -0,0 +1,3 @@ +{ + "path" : "../Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb" +} \ No newline at end of file From 35eaff6f676888b1c6023cac05f7a2e079e2e353 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 16:32:59 +0200 Subject: [PATCH 094/119] update in FittingEIS --- .../calibration/FittingEIS.m | 278 ++++-------------- 1 file changed, 50 insertions(+), 228 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m index b50182043..cfc59bd2b 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m @@ -1,15 +1,18 @@ -classdef FittingEIS +classdef FittingEIS < handle properties - params0 + + % Observed impedances (array of same lengths) + omega Z_re_exp Z_im_exp - omega + + % initial parameters + params0 + + % scales for unit box search algorithm scales - % best_params_found = [] - % fitting_error = [] - end @@ -17,53 +20,63 @@ methods - function feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega) + function feis = FittingEIS(eisdata, params0, scales) - % feis.params0 = params0; - % feis.scales = scales; - % feis.Z_re_exp = Z_re_exp; - % feis.Z_im_exp = Z_im_exp; - % feis.omega = omega; + feis.Z_re_exp = eisdata.Z_re_exp; + feis.Z_im_exp = eisdata.Z_im_exp; + feis.omega = eisdata.omega; + feis.params0 = params0; + + if nargin < 3 || isempty(scales) + feis.setupDefaultScales(); + end + end - if istable(Z_re_exp), Z_re_exp = table2array(Z_re_exp); end - if istable(Z_im_exp), Z_im_exp = table2array(Z_im_exp); end - if istable(omega), omega = table2array(omega); end - if istable(params0), params0 = table2array(params0); end - if istable(scales), scales = table2array(scales); end + function setupDefaultScales(feis) - % Everything has to be "double" and colon (:) - feis.params0 = double(params0(:)); - feis.scales = double(scales(:)); - feis.Z_re_exp= double(Z_re_exp(:)); - feis.Z_im_exp= double(Z_im_exp(:)); - feis.omega = double(omega(:)); + params0 = feis.params0; - %pb here because the way I take exp data changes a lot the - %result... + a = 1000; + + pmin = params0 / a; + pmax = params0 * a; + scales = [pmin; pmax]; + feis.scales = scales; + end - + function p_norm = unscaled2scaled(feis, p) + pmin = feis.scales(1:5); pmax = feis.scales(6:10); p_norm = (p-pmin)./(pmax-pmin); + end function p = scaled2unscaled(feis, p_norm) + pmin = feis.scales(1:5); pmax = feis.scales(6:10); p = (pmax-pmin).*p_norm +pmin; + end + + function [optparams, fitting_error] = run(feis) + + [~, ~, optparams, fitting_error] = feis.optimizationBFGS(); + + end + %% Thevenin Model function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) - f_opt = @(p_norm) feis.optifunc(scaled2unscaled(feis, p_norm)); - params0_norm = unscaled2scaled(feis, feis.params0); + params0_norm = feis.unscaled2scaled(feis.params0); % best_params_norm = lsqnonlin(deltagap, params0_norm, lb_norm, ub_norm, [0,0,-1,0,10], 0); params0_norm = params0_norm(:); @@ -84,14 +97,13 @@ [min_value, best_params_norm, history] = unitBoxBFGS(... params0_norm, ... f_opt, ... - 'maximize', false, ... - 'linIneq', struct('A', A_custom, 'b', b_custom), ... %A*u<=b - 'enforceFeasible', true, ... - 'maxIt', max_iter, ... - 'objChangeTol', tol_obj, ... - 'gradTol', tol_grad, ... - 'lineSearchMaxIt', 100 ... - ); + 'maximize' , false, ... + 'linIneq' , struct('A', A_custom, 'b', b_custom), ... + 'enforceFeasible', true , ... + 'maxIt' , max_iter, ... + 'objChangeTol' , tol_obj , ... + 'gradTol' , tol_grad, ... + 'lineSearchMaxIt', 100); best_params = scaled2unscaled(feis, best_params_norm(:) ); % explications of why it stopped @@ -117,11 +129,8 @@ fprintf('Unexpected error or relative tolerance reached.\n'); end - end - - function [v, g_norm] = optifunc(feis, p) % Preventing physical values to get too close from 0 @@ -191,124 +200,9 @@ end end - - -%% Warburg Model - - function [min_value, history, best_params, fitting_error] = optimizationBFGS_warburg(feis) - - f_opt = @(p_norm) feis.optifunc_warburg(p_norm.* feis.scales) ; - - params0_norm = feis.params0 ./ feis.scales; - params0_norm = params0_norm(:); - - - - [min_value, best_params_norm, history] = unitBoxBFGS(... - params0_norm, ... - f_opt, ... - 'maximize', false, ... - 'enforceFeasible', true, ... - 'maxIt', 300, ... - 'objChangeTol', 1e-6, ... - 'gradTol', 1e-5, ... - 'lineSearchMaxIt', 200 ... - ); - best_params = best_params_norm(:) .* feis.scales(:); - - fitting_error = feis.optifunc_warburg(best_params); - - end - - function [v, g_norm] = optifunc_warburg(feis, p) - - % Preventing physical values to get too close from 0 - p_safe = max(p, 1e-7); - - - w = feis.omega(:); - R0 = p_safe(1); - R1 = p_safe(2); - Q1 = p_safe(3); - a1 = p_safe(4); - R2 = p_safe(5); - Q2 = p_safe(6); - a2 = p_safe(7); - Q = p_safe(8); - L = p_safe(9); - - s = 1i .* w; - s = s(:); - - sa1 = s.^a1; - sa2 = s.^a2; - - Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); - - Z_re_param = real(Z_param_cplx); - Z_im_param = imag(Z_param_cplx); - - if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end - if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end - - - Z_re_param = double(Z_re_param(:)); - Z_im_param = double(Z_im_param(:)); - - Modulus_Z = sqrt(Z_re_param.^2 + Z_im_param.^2); - Modulus_Z = Modulus_Z(:); - - err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); - err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); - - v = sum(err_re.^2 + err_im.^2); - - - if nargout > 1 - - den1 = (1 + R1 .* Q1 .* sa1).^2; - den2 = (1 + R2 .* Q2 .* sa2).^2; - - - dZ_dR0 = ones(size(s)); % R0 - dZ_dR1 = 1 ./ den1; % R1 - dZ_dR2 = 1 ./ den2; % R2 - - dZ_dQ1 = - (R1^2 .* sa1) ./ den1; % Q1 - dZ_dQ2 = - (R2^2 .* sa2) ./ den2; % Q2 - - dZ_da1 = - (Q1 * R1^2 .* sa1 .* log(s)) ./ den1; % a1 - dZ_da2 = - (Q2 * R2^2 .* sa2 .* log(s)) ./ den2; % a2 - - dZ_dQ = - 1 ./ (Q^2 .* (s.^0.5)); % Q - dZ_dL = s; % L - - J = [dZ_dR0, dZ_dR1, dZ_dQ1, dZ_da1, dZ_dR2, dZ_dQ2, dZ_da2, dZ_dQ, dZ_dL]; - - J_im = imag(J); - J_re = real(J); - - derr_re_dp = -J_re ./ Modulus_Z; - derr_im_dp = -J_im ./ Modulus_Z; - - g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); - g_norm = g_true .* feis.scales(:); - - - if any(isinf(g_norm)) || any(isnan(g_norm)) || isinf(v) || isnan(v) v = 1e10; - g_norm = zeros(9,1); - return; - end - end - end - - - - - %% showing the results - function plotresults_thevenin(feis, best_params, fitting_error) + function plotResults(feis, best_params, fitting_error) [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); @@ -355,69 +249,6 @@ function plotresults_thevenin(feis, best_params, fitting_error) end - function plotresults_warburg(feis, best_params, fitting_error) - - % [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); - w = feis.omega(:); - R0 = best_params(1); - R1 = best_params(2); - Q1 = best_params(3); - a1 = best_params(4); - R2 = best_params(5); - Q2 = best_params(6); - a2 = best_params(7); - Q = best_params(8); - L = best_params(9); - s = 1i .* w; - s = s(:); - - sa1 = s.^a1; - sa2 = s.^a2; - - Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); - - Z_re_fit = real(Z_param_cplx); - Z_im_fit = imag(Z_param_cplx); - - - figure; - subplot(3,1,1); - semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - semilogx(feis.omega, Z_re_fit, 'b'); - legend('experience', 'fitted model'); - title('Fitting results'); - xlabel('Omega'); - ylabel('Z_{re} '); - - subplot(3,1,2); - semilogx(feis.omega, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - semilogx(feis.omega, -Z_im_fit, 'b'); - legend('experience', 'fitted model'); - title('Fitting results'); - xlabel('Omega'); - ylabel('-Z_{im} '); - - subplot(3,1,3); - plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); - hold on; - plot(Z_re_fit, -Z_im_fit, 'b'); - legend('experience', 'fitted model'); - title('Nyquist'); - xlabel('Z_{re}'); - ylabel('-Z_{im} '); - axis equal; - - grid on; - text_error = sprintf('Fitting error : %.2e', fitting_error); - text(0.05, 0.85, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); - end - function printResults(feis, best_params, fitting_error) fprintf('\n=== FITTING SCORE ===\n'); @@ -430,16 +261,7 @@ function printResults(feis, best_params, fitting_error) fprintf('R2 = %.2e Ohms\n', best_params(4)); fprintf('C2 = %.2e Farads\n', best_params(5)); - % fprintf('\n=== PARAMETERS FOUND ===\n'); - % fprintf('R0 = %.4e Ohms\n', best_params(1)); - % fprintf('R1 = %.4e Ohms\n', best_params(2)); - % fprintf('Q1 = %.4e s^a/Ohm\n', best_params(3)); - % fprintf('a1 = %.4f \n', best_params(4)); % %f suffit pour 'a' car il est entre 0 et 1 - % fprintf('R2 = %.4e Ohms\n', best_params(5)); - % fprintf('Q2 = %.4e s^a/Ohm\n', best_params(6)); - % fprintf('a2 = %.4f \n', best_params(7)); - % fprintf('Q = %.4e \n', best_params(8)); - % fprintf('L = %.4e Henrys\n', best_params(9)); end + end end From f5e148301de4266d1eeb512f50d7b46dae60b5aa Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 16:34:33 +0200 Subject: [PATCH 095/119] removed unused files --- .../calibration/classFitting.m | 66 ------------------- .../specific_calibrations/ankExpCalibration.m | 55 ---------------- .../specific_calibrations/chenCalibration.m | 40 ----------- .../specific_calibrations/testCalibration.m | 36 ---------- 4 files changed, 197 deletions(-) delete mode 100644 Battery/EquivalentCircuitModel/calibration/classFitting.m delete mode 100644 Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m delete mode 100644 Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m delete mode 100644 Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m diff --git a/Battery/EquivalentCircuitModel/calibration/classFitting.m b/Battery/EquivalentCircuitModel/calibration/classFitting.m deleted file mode 100644 index 1d1473a34..000000000 --- a/Battery/EquivalentCircuitModel/calibration/classFitting.m +++ /dev/null @@ -1,66 +0,0 @@ -function p = classFitting(Z_re_exp, Z_im_exp, omega, print) %print is a boolean, if one gives it to the function it will plot the results. - %% Main code: - - % filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; - % filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; - % - % [Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename); - % [Z_re_exp, Z_im_exp, omega] = load_santoni_data(); - % [Z_re_exp, Z_im_exp, omega] = load_chen_data(); - - % omega = logspace(-4, 2, 50); - % params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; - % [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); - - % params0_w = [1e-1,1e-1,1e-1,1e-1,1e-2,1,1,1e2,1e-07]; - % scales_w = params0_w*10; %to be changed between lsq and bfgs - - params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - - a = 1000; - - pmin = params0 / a; - pmax = params0 * a; - scales = [pmin, pmax]; - - feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - - [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - - p = best_params; - - - %% Printing results - if nargin == 4 || nargin == 1 - feis.plotresults_thevenin(best_params, fitting_error); - - feis.printResults(best_params, fitting_error); % to be changed btw Warburg and Thevenin - end - -end - - -%% - -% result with lsqnonlin: -% === FITTING SCORE === -% Error : 7.324871e-02 -% -% === PARAMETERS FOUND === -% R0 = 0.05052 Ohms -% R1 = 1.12673 Ohms -% C1 = 59119.9 Farads -% R2 = 0.03155 Ohms -% C2 = 11054.0 Farads - - -% results warburg chen -% 4.7197e-02 ... -% 1.0000e-2 ... -% 2.3392e-03 ... -% 0.0103 ... -% 6.8573e-04 ... -% 1.0000e-1 ... -% 0.0307 ... -% 7.0505e+02 ... -% 2.9134e-06 diff --git a/Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m deleted file mode 100644 index dec9cfb71..000000000 --- a/Battery/EquivalentCircuitModel/examples/specific_calibrations/ankExpCalibration.m +++ /dev/null @@ -1,55 +0,0 @@ -filename = 'C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\data_August\ank_data\Supplementary material\02_Electrical_characterization\EIS\131-828_EIS_01_MB_CD8.txt'; -% filename = '/home/xavier/Matlab/Projects/battmo/Data/131-828_EIS_01_MB_CD8.txt'; -[Z_re_exp, Z_im_exp, omega] = load_experimental_data(filename) - -params0 = [3.84e-03,... -2.71e-03,... -6.00e+03,... -9.48e-04,... -1.11e+01]; % initial condition: C1>2*C2 - -a = 1000; - -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -set(0, 'defaultlinelinewidth', 3); -set(0, 'DefaultAxesFontSize', 16); -set(0, 'defaulttextfontsize', 18); - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); - -figure; - -plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); -hold on; -plot(feis.Z_re_exp, -Z_im_fit, 'b'); -legend('experience', 'fitted model'); -xlabel('Z_{re}'); -ylabel('-Z_{im} '); -axis equal; - -grid on; - -text_error = sprintf('Fitting error : %.2e', fitting_error); - -text(0.05, 0.90, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); - -fprintf('\n=== FITTING SCORE ===\n'); -fprintf('Error : %e\n', fitting_error); - -fprintf('\n=== PARAMETERS FOUND ===\n'); -fprintf('R0 = %.2e Ohms\n', best_params(1)); -fprintf('R1 = %.2e Ohms\n', best_params(2)); -fprintf('C1 = %.2e Farads\n', best_params(3)); -fprintf('R2 = %.2e Ohms\n', best_params(4)); -fprintf('C2 = %.2e Farads\n', best_params(5)); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m deleted file mode 100644 index adc9a48dc..000000000 --- a/Battery/EquivalentCircuitModel/examples/specific_calibrations/chenCalibration.m +++ /dev/null @@ -1,40 +0,0 @@ -[Z_re_exp, Z_im_exp, omega] = load_chen_data(); -params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - -a = 1000; - -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); - - -set(0, 'defaultlinelinewidth', 3); -set(0, 'DefaultAxesFontSize', 16); -set(0, 'defaulttextfontsize', 18); - - -figure; - -plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); -hold on; -plot(feis.Z_re_exp, -Z_im_fit, 'b'); -legend('experience', 'fitted model'); -xlabel('Z_{re}'); -ylabel('-Z_{im} '); -axis equal; - -grid on; - -text_error = sprintf('Fitting error : %.2e', fitting_error); - -text(0.05, 0.90, text_error, 'Units', 'normalized', ... - 'BackgroundColor', 'white', ... - 'EdgeColor', 'black', ... - 'FontSize', 11, ... - 'FontWeight', 'bold'); \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m b/Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m deleted file mode 100644 index 3e5e16b33..000000000 --- a/Battery/EquivalentCircuitModel/examples/specific_calibrations/testCalibration.m +++ /dev/null @@ -1,36 +0,0 @@ -omega = logspace(-4, 2, 50); -params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; -[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); - -params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - -a = 1000; - -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - -set(0, 'defaultlinelinewidth', 3); -set(0, 'DefaultAxesFontSize', 16); -set(0, 'defaulttextfontsize', 18); - -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); -[Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); -figure; -plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); -hold on; -plot(Z_re_fit, -Z_im_fit, 'b'); -legend('experience', 'fitted model'); -xlabel('Z_{re}'); -ylabel('-Z_{im} '); -axis equal; -grid on; -text_error = sprintf('Fitting error : %.2e', fitting_error); -text_error = sprintf('Fitting error : %.2e', fitting_error); -text(0.05, 0.85, text_error, 'Units', 'normalized', ... -'BackgroundColor', 'white', ... -'EdgeColor', 'black', ... -'FontSize', 11, ... -'FontWeight', 'bold'); From 852d5da78d60b9318e74ea4e15387bf164c0a477 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 14 Jul 2026 16:35:27 +0200 Subject: [PATCH 096/119] update --- .../calibration/WarburgFittingEIS.m | 207 ++++++++++++++++++ ...pEisToEcmTable.m => calibrateEcmFromP2D.m} | 19 +- .../calibration/runCalibrateEcmFromP2D.m | 70 ++++++ .../calibration/runMapEisToEcmTable.m | 4 - .../examples/{ => old}/RvariationSOC.m | 0 .../examples/{ => old}/runECMfitting.m | 0 .../examples/{ => old}/validateEcmTime.m | 4 +- .../{ => old}/param_dependency.m | 0 .../notebooks/exampleECM.ipynb | 104 --------- .../notebooks/exampleECM.mlx | Bin 22373 -> 0 bytes 10 files changed, 284 insertions(+), 124 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/WarburgFittingEIS.m rename Battery/EquivalentCircuitModel/calibration/{mapEisToEcmTable.m => calibrateEcmFromP2D.m} (87%) create mode 100644 Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m delete mode 100644 Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m rename Battery/EquivalentCircuitModel/examples/{ => old}/RvariationSOC.m (100%) rename Battery/EquivalentCircuitModel/examples/{ => old}/runECMfitting.m (100%) rename Battery/EquivalentCircuitModel/examples/{ => old}/validateEcmTime.m (99%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => old}/param_dependency.m (100%) delete mode 100644 Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb delete mode 100644 Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx diff --git a/Battery/EquivalentCircuitModel/calibration/WarburgFittingEIS.m b/Battery/EquivalentCircuitModel/calibration/WarburgFittingEIS.m new file mode 100644 index 000000000..af6e635c4 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/WarburgFittingEIS.m @@ -0,0 +1,207 @@ +classdef WarburgFittingEIS < FittingEIS + + methods + + function feis = WarburgFittingEIS(params0, eisdata, scales) + + if nargin < 3 + scales = []; + end + + feis = feis@FittingEIS(params0, eisdata, scales); + + end + + function [min_value, history, best_params, fitting_error] = optimizationBFGS(feis) + + %% Warburg Model + error('not updated....'); + + f_opt = @(p_norm) feis.optifunc(p_norm.* feis.scales) ; + + params0_norm = feis.params0 ./ feis.scales; + params0_norm = params0_norm(:); + + + + [min_value, best_params_norm, history] = unitBoxBFGS(... + params0_norm, ... + f_opt, ... + 'maximize', false, ... + 'enforceFeasible', true, ... + 'maxIt', 300, ... + 'objChangeTol', 1e-6, ... + 'gradTol', 1e-5, ... + 'lineSearchMaxIt', 200 ... + ); + best_params = best_params_norm(:) .* feis.scales(:); + + fitting_error = feis.optifunc(best_params); + + end + + function [v, g_norm] = optifunc(feis, p) + + % Preventing physical values to get too close from 0 + p_safe = max(p, 1e-7); + + + w = feis.omega(:); + R0 = p_safe(1); + R1 = p_safe(2); + Q1 = p_safe(3); + a1 = p_safe(4); + R2 = p_safe(5); + Q2 = p_safe(6); + a2 = p_safe(7); + Q = p_safe(8); + L = p_safe(9); + + s = 1i .* w; + s = s(:); + + sa1 = s.^a1; + sa2 = s.^a2; + + Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); + + Z_re_param = real(Z_param_cplx); + Z_im_param = imag(Z_param_cplx); + + if istable(Z_re_param), Z_re_param = table2array(Z_re_param); end + if istable(Z_im_param), Z_im_param = table2array(Z_im_param); end + + + Z_re_param = double(Z_re_param(:)); + Z_im_param = double(Z_im_param(:)); + + Modulus_Z = sqrt(Z_re_param.^2 + Z_im_param.^2); + Modulus_Z = Modulus_Z(:); + + err_re = (feis.Z_re_exp(:) - Z_re_param(:)) ./ Modulus_Z(:); + err_im = (feis.Z_im_exp(:) - Z_im_param(:)) ./ Modulus_Z(:); + + v = sum(err_re.^2 + err_im.^2); + + + if nargout > 1 + + den1 = (1 + R1 .* Q1 .* sa1).^2; + den2 = (1 + R2 .* Q2 .* sa2).^2; + + + dZ_dR0 = ones(size(s)); % R0 + dZ_dR1 = 1 ./ den1; % R1 + dZ_dR2 = 1 ./ den2; % R2 + + dZ_dQ1 = - (R1^2 .* sa1) ./ den1; % Q1 + dZ_dQ2 = - (R2^2 .* sa2) ./ den2; % Q2 + + dZ_da1 = - (Q1 * R1^2 .* sa1 .* log(s)) ./ den1; % a1 + dZ_da2 = - (Q2 * R2^2 .* sa2 .* log(s)) ./ den2; % a2 + + dZ_dQ = - 1 ./ (Q^2 .* (s.^0.5)); % Q + dZ_dL = s; % L + + J = [dZ_dR0, dZ_dR1, dZ_dQ1, dZ_da1, dZ_dR2, dZ_dQ2, dZ_da2, dZ_dQ, dZ_dL]; + + J_im = imag(J); + J_re = real(J); + + derr_re_dp = -J_re ./ Modulus_Z; + derr_im_dp = -J_im ./ Modulus_Z; + + g_true = 2 * (derr_re_dp' * err_re) + 2 * (derr_im_dp' * err_im); + g_norm = g_true .* feis.scales(:); + + + if any(isinf(g_norm)) || any(isnan(g_norm)) || isinf(v) || isnan(v) v = 1e10; + g_norm = zeros(9,1); + return; + end + end + end + + function plotResults(feis, best_params, fitting_error) + + % [Z_re_fit, Z_im_fit] = load_nyquist(best_params, feis.omega); + w = feis.omega(:); + R0 = best_params(1); + R1 = best_params(2); + Q1 = best_params(3); + a1 = best_params(4); + R2 = best_params(5); + Q2 = best_params(6); + a2 = best_params(7); + Q = best_params(8); + L = best_params(9); + s = 1i .* w; + s = s(:); + + sa1 = s.^a1; + sa2 = s.^a2; + + Z_param_cplx = R0 + s.*L + R1 ./ (1 + R1.*Q1.*sa1) + R2 ./ (1 + R2.*Q2.*sa2) + 1 ./ (Q.*(s.^0.5)); + + Z_re_fit = real(Z_param_cplx); + Z_im_fit = imag(Z_param_cplx); + + + figure; + subplot(3,1,1); + semilogx(feis.omega, feis.Z_re_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, Z_re_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('Z_{re} '); + + subplot(3,1,2); + semilogx(feis.omega, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + semilogx(feis.omega, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Fitting results'); + xlabel('Omega'); + ylabel('-Z_{im} '); + + subplot(3,1,3); + plot(feis.Z_re_exp, -feis.Z_im_exp, 'r', 'MarkerFaceColor', 'r'); + hold on; + plot(Z_re_fit, -Z_im_fit, 'b'); + legend('experience', 'fitted model'); + title('Nyquist'); + xlabel('Z_{re}'); + ylabel('-Z_{im} '); + axis equal; + + grid on; + text_error = sprintf('Fitting error : %.2e', fitting_error); + text(0.05, 0.85, text_error, 'Units', 'normalized', ... + 'BackgroundColor', 'white', ... + 'EdgeColor', 'black', ... + 'FontSize', 11, ... + 'FontWeight', 'bold'); + end + + function printResults(feis, best_params, fitting_error) + + fprintf('\n=== FITTING SCORE ===\n'); + fprintf('Error : %e\n', fitting_error); + + + fprintf('\n=== PARAMETERS FOUND ===\n'); + fprintf('R0 = %.4e Ohms\n', best_params(1)); + fprintf('R1 = %.4e Ohms\n', best_params(2)); + fprintf('Q1 = %.4e s^a/Ohm\n', best_params(3)); + fprintf('a1 = %.4f \n', best_params(4)); % %f suffit pour 'a' car il est entre 0 et 1 + fprintf('R2 = %.4e Ohms\n', best_params(5)); + fprintf('Q2 = %.4e s^a/Ohm\n', best_params(6)); + fprintf('a2 = %.4f \n', best_params(7)); + fprintf('Q = %.4e \n', best_params(8)); + fprintf('L = %.4e Henrys\n', best_params(9)); + + end + end +end diff --git a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m similarity index 87% rename from Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m rename to Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m index 0b795bf3a..5495e2412 100644 --- a/Battery/EquivalentCircuitModel/calibration/mapEisToEcmTable.m +++ b/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m @@ -1,15 +1,10 @@ -function ecm_table = mapEisToEcmTable(soc_step) +function jsonstruct_ecm = calibrateEcmFromP2D(jsonstruct_p2d, soc_step) + % soc_step : soc increment between 0 and 1. Start from soc = 1. %% 1. Initialisation - jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); - jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - - jsonstruct = mergeJsonStructs({jsonstruct_material, ... - jsonstruct_geometry}); - - - [model, inputparams] = setupModelFromJson(jsonstruct); + + [model, inputparams] = setupModelFromJson(jsonstruct_p2d); state_current = setupInitialState(model); if nargin < 1 soc_step = 0.1; @@ -32,7 +27,6 @@ %% extraction de l'EIS par computeImpedance() options = struct(); - options.stateInitialization.computeSteadyState = false; options.stateInitialization.initializationSetup = 'given state'; @@ -42,7 +36,6 @@ fprintf('Linearisation...\n'); Z = impsolv.computeImpedance(freq); - Z_re = real(Z)'; Z_im = imag(Z)'; @@ -50,7 +43,7 @@ omega = (2*pi).*freq; %% extraction des paramètres ECM - p = runClassFitting(Z_re, Z_im, omega); + p = runFitting(Z_re, Z_im, omega); % Stockage dans la matrice de résultats results_matrix(i, 1) = current_soc; @@ -61,7 +54,7 @@ fprintf(' %02d %% discharge...\n', soc_step); inputparams.Control.controlPolicy = 'CCDischarge'; inputparams.Control.DRate = C_rate; - jsonstruct.TimeStepping.tmax = t_xpercent; + jsonstruct_p2d.TimeStepping.tmax = t_xpercent; model.Control = model.setupControl(inputparams.Control); diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m new file mode 100644 index 000000000..fe33973d3 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m @@ -0,0 +1,70 @@ +%% Calibrate ECM model from P2D model +% + +soc_step = 0.5; + +%% +% The results of the calibration is given in a struct where the fields are functions in battmo table format + + +jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); +jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +jsonstruct_p2d = mergeJsonStructs({jsonstruct_material, ... + jsonstruct_geometry}); + +jsonstruct = calibrateEcmFromP2D(jsonstruct_p2d, soc_step); + +%% +% plot the results + +figure +tiledlayout(2, 3, 'tileindexing', 'columnmajor'); + +nexttile +%% +% the function |setupFunction| creates a function handle from the battmo function input format. +fn = setupFunction(jsonstruct.OCP) +plot(soc, fn(soc)) +title('OCP') +xlabel('SOC / -') +ylabel('OCP / V'); + +nexttile +fn = setupFunction(jsonstruct.R0) +plot(soc, fn(soc)) +title('R0') +xlabel('SOC / -') +ylabel('R0 / Ohm'); + +nexttile +fn = setupFunction(jsonstruct.R1) +plot(soc, fn(soc)) +title('R1') +xlabel('SOC / -') +ylabel('R1 / Ohm'); + +nexttile +fn = setupFunction(jsonstruct.C1) +plot(soc, fn(soc)) +title('C1') +xlabel('SOC / -') +ylabel('C1 / Ohm'); + +nexttile +fn = setupFunction(jsonstruct.R2) +plot(soc, fn(soc)) +title('R2') +xlabel('SOC / -') +ylabel('R2 / Ohm'); + +nexttile +fn = setupFunction(jsonstruct.C2) +plot(soc, fn(soc)) +title('C2') +xlabel('SOC / -') +ylabel('C2 / Ohm'); + + + + diff --git a/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m b/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m deleted file mode 100644 index d5a80d0ef..000000000 --- a/Battery/EquivalentCircuitModel/calibration/runMapEisToEcmTable.m +++ /dev/null @@ -1,4 +0,0 @@ -soc_step = 0.5; -ecm_table = mapEisToEcmTable(soc_step); -plotEcmSoc(ecm_table); - diff --git a/Battery/EquivalentCircuitModel/examples/RvariationSOC.m b/Battery/EquivalentCircuitModel/examples/old/RvariationSOC.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/RvariationSOC.m rename to Battery/EquivalentCircuitModel/examples/old/RvariationSOC.m diff --git a/Battery/EquivalentCircuitModel/examples/runECMfitting.m b/Battery/EquivalentCircuitModel/examples/old/runECMfitting.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/runECMfitting.m rename to Battery/EquivalentCircuitModel/examples/old/runECMfitting.m diff --git a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m similarity index 99% rename from Battery/EquivalentCircuitModel/examples/validateEcmTime.m rename to Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m index 869180023..b7e4ba5da 100644 --- a/Battery/EquivalentCircuitModel/examples/validateEcmTime.m +++ b/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m @@ -17,7 +17,6 @@ function validateEcmTime(file_name) end - % Generation of the "Ground Truth": Continuous P2D discharge (BattMo) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); @@ -58,7 +57,6 @@ function validateEcmTime(file_name) V_p2d = zeros(N_points, 1); I_p2d = zeros(N_points, 1); - pe_guestStoichiometry0 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; pe_guestStoichiometry100 = model.PositiveElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry100; ne_guestStoichiometry0 = model.NegativeElectrode.Coating.ActiveMaterial.Interface.guestStoichiometry0; @@ -179,4 +177,4 @@ function validateEcmTime(file_name) rmse = sqrt(mean((V_p2d - V_ecm).^2)) * 1000; fprintf('*** Analysis complete! Root Mean Square Error (RMSE): %.2f mV ***\n', rmse); -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/param_dependency.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m diff --git a/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb b/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb deleted file mode 100644 index 6dafa2118..000000000 --- a/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb +++ /dev/null @@ -1,104 +0,0 @@ -{ - "cells": [ - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "# Equivalent Circuit Model\n", - "\n", - "## Load data set" - ] - }, - { - "cell_type": "code", - "execution_count": 1, - "metadata": {}, - "source": [ - "jsonstruct = parseBattmoJson('exampleECM.json');\n", - "inputparams = EquivalentCircuitModelInputParams(jsonstruct);" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "## Setup model" - ] - }, - { - "cell_type": "code", - "execution_count": 2, - "metadata": {}, - "source": [ - "model = EquivalentCircuitModel(inputparams);" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "## run Simulation" - ] - }, - { - "cell_type": "code", - "execution_count": 3, - "metadata": {}, - "source": [ - "[t, U, I] = model.solve();" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "## Plotting" - ] - }, - { - "cell_type": "code", - "execution_count": 4, - "metadata": {}, - "source": [ - "tiledlayout(1, 2);\n", - "nexttile\n", - "plot(t, U)\n", - "nexttile\n", - "plot(t, I)" - ], - "outputs": [ - { - "data": { - "text/html": [ - "
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z%-gmnOhb++wUl{^jO1x@gmP#RZKaol)Gp&{+LbIA4FV8>5|D2q6B=>yjm`+m# z^{#dN|6tU+Fi`G7`M=}8U{dcJ+-H9NQU0%i_1*1n1kn4!`)td Date: Tue, 14 Jul 2026 16:35:39 +0200 Subject: [PATCH 097/119] update --- .../calibration/runCalibration.m | 74 +++++++++---------- .../doubleLayerCapacitance_impact.m | 16 +++- .../examples/robustnessTest.m | 5 +- 3 files changed, 52 insertions(+), 43 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibration.m b/Battery/EquivalentCircuitModel/calibration/runCalibration.m index 9173d8391..f1631c4f2 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibration.m @@ -49,6 +49,7 @@ %% % setup impedance solver and compute the Impedance for a given set of frequencies + impsolv = ImpedanceSolver(inputparams, options, extrastructs); frequencies = logspace(-2, 3, 30); @@ -99,26 +100,26 @@ % optimization algorithm should be able to recover the true parameters. +%% +% fetch data omega = logspace(-4, 2, 50); -params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; [Z_re_exp, Z_im_exp] = load_nyquist(params, omega); -params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - -a = 1000; +eisdata = struct('omega', omega, ... + 'Z_re_exp', Z_re_exp, ... + 'Z_im_exp', Z_im_exp); -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); +%% +% Initial parameters for the calibration +params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; % initial condition: C1>2*C2 -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); +feis = FittingEIS(eisdata, params0); +[best_params, fitting_error] = feis.run(); %% % plot the results -feis.plotresults_thevenin(best_params, fitting_error); +feis.plotResults(best_params, fitting_error); %% Calibration from experimental data % We use data from the Ank's paper (http://dx.doi.org/10.1149/1945-7111/ad14d0) to calibrate the ECM parameters. @@ -127,46 +128,43 @@ filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv'); data = readmatrix(filename); -omega = data(:, 1); -Z_re_exp = data(:, 2); -Z_im_exp = data(:, 3); +eisdata.omega = data(:, 1); +eisdata.Z_re_exp = data(:, 2); +eisdata.Z_im_exp = data(:, 3); %% % We choose the following Initial guess -params0 = [3.84e-03,... - 2.71e-03,... - 6.00e+03,... - 9.48e-04,... - 1.11e+01]; % initial condition: C1>2*C2 - -a = 1000; +params0 = [3.84e-03; ... + 2.71e-03; ... + 6.00e+03; ... + 9.48e-04; ... + 1.11e+01]; % initial condition: C1>2*C2 -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); +feis = FittingEIS(eisdata, params0); -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - -feis.plotresults_thevenin(best_params, fitting_error); +[best_params, fitting_error] = feis.run(); +feis.plotResults(best_params, fitting_error); +feis.printResults(best_params, fitting_error); %% Synthetic data from P2D model % We use impedance data generated from the P2d model with Chen et al's paper % (http://dx.doi.org/10.1149/1945-7111/ab9050) parameters +%% +% fetch Chen data [Z_re_exp, Z_im_exp, omega] = load_chen_data(); -params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 - -a = 1000; +eisdata = struct('omega', omega, ... + 'Z_re_exp', Z_re_exp, ... + 'Z_im_exp', Z_im_exp); -pmin = params0 / a; -pmax = params0 * a; -scales = [pmin, pmax]; - -feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); +%% +% initial parameters +params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; % initial condition: C1>2*C2 -[~, ~, best_params, fitting_error] = feis.optimizationBFGS(); -feis.plotresults_thevenin(best_params, fitting_error); +feis = FittingEIS(eisdata, params0); +[best_params, fitting_error] = feis.run(); +feis.plotResults(best_params, fitting_error); +feis.printResults(best_params, fitting_error); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m index df5714137..a13efd261 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m @@ -28,9 +28,9 @@ initstate = initStateChen2020(model, c_ne, c_pe); -b = logspace(-2, 2, 20); %change here +b = logspace(-2, 2, 5); %change here -frequences = logspace(-2, 4, 30); +frequences = logspace(-4, 4, 200); figure; @@ -44,7 +44,15 @@ [model, inputparams, ~] = setupModelFromJson(jsonstruct); % inputparams.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); - impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); + + options = []; + options.stateInitialization.initializationSetup = 'given state'; + options.stateInitialization.computeSteadyState = false; + + extrastructs = []; + extrastructs.initstate = initstate; + + impsolv = ImpedanceSolver(inputparams, options, extrastructs); Z = impsolv.computeImpedance(frequences); @@ -58,4 +66,4 @@ end -legend('show'); \ No newline at end of file +legend('show'); diff --git a/Battery/EquivalentCircuitModel/examples/robustnessTest.m b/Battery/EquivalentCircuitModel/examples/robustnessTest.m index d9f2f22de..74bfc9c57 100644 --- a/Battery/EquivalentCircuitModel/examples/robustnessTest.m +++ b/Battery/EquivalentCircuitModel/examples/robustnessTest.m @@ -1,9 +1,12 @@ %% Robustness test for fitting programm +% for i = 1:5 + params0 = pmin + (pmax - pmin) .* rand(1, 5); disp(['Tour ', num2str(i), ' - params0 :']); disp(params0); + feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); @@ -12,4 +15,4 @@ drawnow; -end \ No newline at end of file +end From 06e05d59af1bc58fbc339a0921b93904565a0823 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Thu, 16 Jul 2026 11:58:02 +0200 Subject: [PATCH 098/119] Impedance explorer ready for notebook --- .../pxdParamsImpact/ImpedanceExplore.m | 203 +++++++++++------- .../examples/runEquivalentCircuitModel.m | 2 +- 2 files changed, 126 insertions(+), 79 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index b302c4b6e..023904f8a 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -1,7 +1,5 @@ classdef ImpedanceExplore < handle - properties (SetAccess = immutable) - jsonstruct model @@ -9,8 +7,8 @@ properties - %% - % TODO: add option to change soc in slider + + % done : add option to change soc in slider soc = 1 parameters @@ -18,9 +16,26 @@ end methods - + %% + % Constructor method that initializes the application, auto-loading the physical P2D Chen2020 battery dataset from BattMo files if no input JSON structure is provided. function impexp = ImpedanceExplore(jsonstruct) - + if nargin < 1 + fprintf('Automatic initialization of Chen2020 configuration (BattMo)...\n'); + try + jsonstruct_material = parseBattmoJson(fullfile('ParameterData', 'ParameterSets', 'Chen2020', 'chen2020_lithium_ion_battery.json')); + jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + + jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + if ~isfield(jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface, 'doubleLayerCapacitance') + jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = 0.2; + fprintf('-> default doubleLayerCapacitance, value = 0.2 F/m^2\n'); + end + + catch ME + error('ImpedanceExplore:AutoLoadFailed', ... + ME.message); + end + end model = setupModelFromJson(jsonstruct); impexp.jsonstruct = jsonstruct; impexp.model = model; @@ -28,17 +43,19 @@ impexp.setupDefaultParameters() end - + + %% + % Utility method to flatten the active JSON structure and print all available scalar parameters in the model to the command window. function viewOptions(impexp) - fjv = flattenJsonStruct(impexp.jsonstruct, 'doprint', false); fprintf('\n\n*** List of all the scalar parameters in the model ***\n'); fjv.print('filter', {'value', @(val) (isnumeric(val) && isscalar(val))}); end - + + %% + % Configures the default internal hierarchical paths of the active material parameters to be observed and modified. function setupDefaultParameters(impexp) - elyte = 'Electrolyte'; ne = 'NegativeElectrode'; pe = 'PositiveElectrode'; @@ -53,11 +70,11 @@ function setupDefaultParameters(impexp) impexp.parameters = {{ne, co, am, sd, 'referenceDiffusionCoefficient'}, ... {ne, co, am, itf, 'reactionRateConstant'}, ... {ne, co, am, itf, 'doubleLayerCapacitance'}}; - end - + + %% + % Helper method that generates human-readable parameter names by joining the individual sub-keys of their nested JSON paths. function pnames = setupParameterLegendNames(impexp) - params = impexp.parameters; for iparam = 1 : numel(params) pnames{iparam} = strjoin(params{iparam}); @@ -65,145 +82,175 @@ function setupDefaultParameters(impexp) end - function sld = setupSlider(imexp, fig, ypos, txt) + %% + % Dynamically instantiates a slider control alongside its descriptive label at a specific vertical coordinate. + function sld = setupSlider(impexp, fig, ypos, txt, limits, majorTicks, initVal) + if nargin < 5, limits = [-5, 5]; end + if nargin < 6, majorTicks = -5:0.5:5; end + if nargin < 7, initVal = 0; end - uilabel(fig , ... + uilabel(fig, ... 'Position', [50, ypos + 20, 500, 40], ... - 'WordWrap', 'on' , ... + 'WordWrap', 'on', ... 'Text', txt); - sld = uislider(fig, ... 'Position', [50, ypos, 500, 3], ... - 'Limits', [-5, 5] , ... % Définit le minimum et le maximum - 'MajorTicks', -5:0.5:5 , ... % Ajoute une graduation tous les 1 - 'Value', 0); - + 'Limits', limits, ... + 'MajorTicks', majorTicks, ... + 'Value', initVal); end - + + %% + % Retrieves the current numerical values of targeted active parameters from the application''s JSON model. function vals = getParameterValues(impexp, jsonstruct) - if nargin < 2 jsonstruct = impexp.jsonstruct; end parameters = impexp.parameters; - + vals = zeros(1, numel(parameters)); for iparam = 1 : numel(parameters) - vals(iparam) = getJsonStructField(jsonstruct, parameters{iparam}); + val = getJsonStructField(jsonstruct, parameters{iparam}); + if ~isnumeric(val) || ~isscalar(val) + pathStr = strjoin(parameters{iparam}, '.'); + error('ImpedanceExplore:ParameterNotFound', ... + ['\n\n=== PARAMETER NOT FOUND ===\n' ... + 'The following path is incorrect in the BattMo JSON:\n' ... + ' -> "jsonstruct.%s"\n' ... + 'Received type: %s (instead of a double).\n\n' ... + 'To find the correct path, use the command:\n' ... + ' >> app = ImpedanceExplore(); app.viewOptions();\n\n'], ... + pathStr, class(val)); + end + + vals(iparam) = val; end end + %% + % Updates specific nested fields within the model''s JSON structure using values calculated from the current slider states. function jsonstruct = setParameterValues(impexp, vals, jsonstruct) - if nargin < 3 jsonstruct = impexp.jsonstruct; end parameters = impexp.parameters; - for iparam = 1 : numel(parameters) jsonstruct = setJsonStructField(jsonstruct, parameters{iparam}, vals(iparam), 'handleMisMatch', 'quiet'); end end - + + %% + % Dynamically calculates element positions, builds the graphical user interface, spawns the sliders, and registers event callbacks. function start(impexp) + pnames = impexp.setupParameterLegendNames(); + vals = impexp.getParameterValues(); + + numParams = numel(pnames); + numSliders = numParams + 1; % active parameters + SoC slider + + % --- DYNAMIC GEOMETRIC CONFIGURATION --- + sliderSpacing = 75; % Height allocated to each block (Label + Slider) + bottomOffset = 40; % Margin at the bottom of the window - % 2. Création de l'interface graphique (Fenêtre plus haute pour accueillir les curseurs) - fig = uifigure('Name', 'Impedance Explorer', 'Position', [100, 50, 600, 650]); + % Calculate Y positions for status label and axes + lblY = bottomOffset + numSliders * sliderSpacing + 10; + axY = lblY + 35; - % Graphique - ax = uiaxes(fig, 'Position', [50, 350, 500, 250]); + % Dynamic calculation of the window height + % (axY + 250 pixels for the plot + 40 pixels margin at the top) + figHeight = axY + 250 + 40; + + % 1. Create the user interface at the correct size + fig = uifigure('Name', 'Impedance Explorer', 'Position', [100, 50, 600, figHeight]); + + % 2. Create automatically positioned axes + ax = uiaxes(fig, 'Position', [50, axY, 500, 250]); title(ax, 'Nyquist Diagram'); xlabel(ax, 'Re(Z)'); ylabel(ax, '-Im(Z)'); grid(ax, 'on'); - % Label de statut - lbl = uilabel(fig, 'Position', [50, 310, 500, 22], 'Text', 'Ready, use slider to start.'); + % 3. Create automatically positioned status label + lbl = uilabel(fig, 'Position', [50, lblY, 500, 22], 'Text', 'Ready, use slider to start.'); lbl.FontWeight = 'bold'; - - sliders = {}; - - pnames = impexp.setupParameterLegendNames(); - vals = impexp.getParameterValues(); - % TODO : setup logic to get y positions based on number of parameters - yposs = [240, 150, 60]; - for iparam = 1 : numel(pnames) + sliders = cell(1, numParams); + + % --- CREATE PARAMETER SLIDERS --- + % Stack them from bottom to top. The first parameter will be placed right above the SoC slider. + for iparam = 1 : numParams txt = sprintf('%d. %s * 10^x (initial value: %g)', iparam, pnames{iparam}, vals(iparam)); - sliders{iparam} = impexp.setupSlider(fig, yposs(iparam), txt); + + % Calculate Y position: offsets by "iparam" heights + ypos = bottomOffset + iparam * sliderSpacing; + + sliders{iparam} = impexp.setupSlider(fig, ypos, txt); end - - % 4. Connexion aux événements - % On crée une fonction anonyme qui passe TOUS les curseurs - callback_fcn = @(src, event) impexp.updatePlot(ax, lbl, sliders); - for islider = 1 : numel(sliders) + + % --- CREATE SOC SLIDER (At the very bottom) --- + socTxt = sprintf('State of Charge (SoC) - Current: %g', impexp.soc); + ypos_soc = bottomOffset; % Starting position at the very bottom + socSlider = impexp.setupSlider(fig, ypos_soc, socTxt, [0, 1], 0:0.1:1, impexp.soc); + + % --- EVENT CONNECTIONS --- + callback_fcn = @(src, event) impexp.updatePlot(ax, lbl, sliders, socSlider); + + % Bind callback to all parameter sliders + for islider = 1 : numParams sliders{islider}.ValueChangedFcn = callback_fcn; end - % Optionnel : Tracer l'état initial - % updatePlot(ax, lbl, jsonstruct, c_ne, c_pe, sld1, sld2, sld3); - + % Bind callback to the SoC slider + socSlider.ValueChangedFcn = callback_fcn; end - - function updatePlot(impexp, ax, lbl, sliders) - + + %% + % Core callback method that retrieves current slider values, updates the physical state, runs the BattMo impedance solver, and updates the Nyquist plot. + function updatePlot(impexp, ax, lbl, sliders, socSlider) jsonstruct = impexp.jsonstruct; - - % Figer l'affichage + % Freeze display lbl.Text = 'Processing... '; lbl.FontColor = '#D95319'; drawnow; - try - + impexp.soc = socSlider.Value; baseValues = impexp.getParameterValues(); - for ival = 1 : numel(baseValues) vals(ival) = baseValues(ival)*(10^(sliders{ival}.Value)); end - jsonstruct = impexp.setParameterValues(vals); - % 4. Exécution de BattMo - + % 4. Execute BattMo [model, inputparams, ~] = setupModelFromJson(jsonstruct); - %% % We use a dedicated function to compute the initial state for the given electrode concentrations. options = []; options.stateInitialization.initializationSetup = 'soc'; - options.stateInitialization.soc = impexp.soc; - + options.stateInitialization.soc = impexp.soc; % now the soc is updated %% - % setup impedance solver and compute the Impedance for a given set of frequencies + % Setup impedance solver and compute the Impedance for a given set of frequencies impsolv = ImpedanceSolver(inputparams, options); - frequences = logspace(-2, 3, 30); Z = impsolv.computeImpedance(frequences); - % 5. Tracé + % 5. Plotting plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); - % Retour à la normale + % Return to normal lbl.Text = 'Done'; lbl.FontColor = '#77AC30'; - catch ME - - lbl.Text = 'Erreur lors du calcul (vérifiez la console).'; + lbl.Text = 'Calculation error'; lbl.FontColor = '#A2142F'; - disp('--- ERREUR DANS LE CALCUL ---'); + disp('--- Calculation error ---'); disp(ME.message); for k = 1:length(ME.stack) - disp(['Ligne ', num2str(ME.stack(k).line), ' dans ', ME.stack(k).name]); + disp(['Line ', num2str(ME.stack(k).line), ' in ', ME.stack(k).name]); end end end - end - - -end +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m index 77ade5eb4..34e90fc5f 100644 --- a/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/examples/runEquivalentCircuitModel.m @@ -59,7 +59,7 @@ % The input current has been passed to the model figure -totalTime = model.totalTime +totalTime = model.totalTime; t = linspace(0, totalTime, 200); plot(t/hour, model.Ifunc(t), 'o-'); title('Input current') From 19d4013256438d96a82d01928ecacf9501f39916 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Thu, 16 Jul 2026 15:11:22 +0200 Subject: [PATCH 099/119] runImpedanceexplore modified to suit a notebook --- .../pxdParamsImpact/ImpedanceExplore.m | 181 +++++++----------- .../doubleLayerCapacitance_impact.m | 24 ++- .../pxdParamsImpact/runImpedanceExplore.m | 30 ++- 3 files changed, 109 insertions(+), 126 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index 023904f8a..5e6afce3b 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -1,90 +1,71 @@ classdef ImpedanceExplore < handle properties (SetAccess = immutable) - jsonstruct - model - + jsonstruct % Holds the base P2D model configuration structure + model % Initialized BattMo model object end properties - - - % done : add option to change soc in slider - soc = 1 - - parameters - + soc = 1 % Default State of Charge (0 to 1) + parameters % Cell array storing the hierarchical JSON paths of observed parameters end methods - %% - % Constructor method that initializes the application, auto-loading the physical P2D Chen2020 battery dataset from BattMo files if no input JSON structure is provided. function impexp = ImpedanceExplore(jsonstruct) - if nargin < 1 - fprintf('Automatic initialization of Chen2020 configuration (BattMo)...\n'); + % Constructor: auto-loads Chen2020 P2D model if no structure is provided + if nargin < 1 || isempty(jsonstruct) + fprintf('Initializing default Chen2020 P2D model...\n'); try jsonstruct_material = parseBattmoJson(fullfile('ParameterData', 'ParameterSets', 'Chen2020', 'chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); - if ~isfield(jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface, 'doubleLayerCapacitance') - jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = 0.2; - fprintf('-> default doubleLayerCapacitance, value = 0.2 F/m^2\n'); - end + % Safe default fallback for capacitance + ne = 'NegativeElectrode'; co = 'Coating'; am = 'ActiveMaterial'; itf = 'Interface'; + if ~isfield(jsonstruct.(ne).(co).(am).(itf), 'doubleLayerCapacitance') + jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; + end catch ME - error('ImpedanceExplore:AutoLoadFailed', ... - ME.message); + error('ImpedanceExplore:AutoLoadFailed', 'Failed to auto-load default files: %s', ME.message); end end - model = setupModelFromJson(jsonstruct); - impexp.jsonstruct = jsonstruct; - impexp.model = model; - - impexp.setupDefaultParameters() + impexp.jsonstruct = jsonstruct; + impexp.model = setupModelFromJson(jsonstruct); + impexp.setupDefaultParameters(); end - %% - % Utility method to flatten the active JSON structure and print all available scalar parameters in the model to the command window. function viewOptions(impexp) + % Helper to print all available scalar properties in the model JSON fjv = flattenJsonStruct(impexp.jsonstruct, 'doprint', false); fprintf('\n\n*** List of all the scalar parameters in the model ***\n'); fjv.print('filter', {'value', @(val) (isnumeric(val) && isscalar(val))}); - end - - %% - % Configures the default internal hierarchical paths of the active material parameters to be observed and modified. + function setupDefaultParameters(impexp) - elyte = 'Electrolyte'; - ne = 'NegativeElectrode'; - pe = 'PositiveElectrode'; - co = 'Coating'; - am = 'ActiveMaterial'; - itf = 'Interface'; - sd = 'SolidDiffusion'; - cc = 'CurrentCollector'; - ctrl = 'Control'; - thermal = 'ThermalModel'; + % Defines the default nested JSON paths for the 3 target sliders + ne = 'NegativeElectrode'; + co = 'Coating'; + am = 'ActiveMaterial'; + itf = 'Interface'; + sd = 'SolidDiffusion'; impexp.parameters = {{ne, co, am, sd, 'referenceDiffusionCoefficient'}, ... {ne, co, am, itf, 'reactionRateConstant'}, ... {ne, co, am, itf, 'doubleLayerCapacitance'}}; end - %% - % Helper method that generates human-readable parameter names by joining the individual sub-keys of their nested JSON paths. function pnames = setupParameterLegendNames(impexp) + % Joins path cells into unified text labels for the GUI params = impexp.parameters; + pnames = cell(1, numel(params)); for iparam = 1 : numel(params) - pnames{iparam} = strjoin(params{iparam}); + pnames{iparam} = params{iparam}{end}; end - end - %% - % Dynamically instantiates a slider control alongside its descriptive label at a specific vertical coordinate. function sld = setupSlider(impexp, fig, ypos, txt, limits, majorTicks, initVal) + % Generates a single slider with its associated label if nargin < 5, limits = [-5, 5]; end if nargin < 6, majorTicks = -5:0.5:5; end if nargin < 7, initVal = 0; end @@ -101,9 +82,8 @@ function setupDefaultParameters(impexp) 'Value', initVal); end - %% - % Retrieves the current numerical values of targeted active parameters from the application''s JSON model. function vals = getParameterValues(impexp, jsonstruct) + % Reads parameter values from JSON structure. Error out if path is invalid. if nargin < 2 jsonstruct = impexp.jsonstruct; end @@ -113,25 +93,18 @@ function setupDefaultParameters(impexp) for iparam = 1 : numel(parameters) val = getJsonStructField(jsonstruct, parameters{iparam}); if ~isnumeric(val) || ~isscalar(val) - pathStr = strjoin(parameters{iparam}, '.'); - error('ImpedanceExplore:ParameterNotFound', ... - ['\n\n=== PARAMETER NOT FOUND ===\n' ... - 'The following path is incorrect in the BattMo JSON:\n' ... - ' -> "jsonstruct.%s"\n' ... - 'Received type: %s (instead of a double).\n\n' ... - 'To find the correct path, use the command:\n' ... - ' >> app = ImpedanceExplore(); app.viewOptions();\n\n'], ... - pathStr, class(val)); + pathStr = strjoin(parameters{iparam}, '.'); + error('ImpedanceExplore:ParameterNotFound', ... + ['\n\n=== PARAMETER NOT FOUND ===\n' ... + 'Invalid path in BattMo JSON:\n -> "jsonstruct.%s"\n' ... + 'Check spelling or use app.viewOptions() to debug.\n\n'], pathStr); end - vals(iparam) = val; end - end - %% - % Updates specific nested fields within the model''s JSON structure using values calculated from the current slider states. function jsonstruct = setParameterValues(impexp, vals, jsonstruct) + % Writes updated parameter values back into the JSON structure if nargin < 3 jsonstruct = impexp.jsonstruct; end @@ -140,116 +113,94 @@ function setupDefaultParameters(impexp) for iparam = 1 : numel(parameters) jsonstruct = setJsonStructField(jsonstruct, parameters{iparam}, vals(iparam), 'handleMisMatch', 'quiet'); end - end - %% - % Dynamically calculates element positions, builds the graphical user interface, spawns the sliders, and registers event callbacks. function start(impexp) + % Computes sizes and runs the App Designer UI Window pnames = impexp.setupParameterLegendNames(); vals = impexp.getParameterValues(); numParams = numel(pnames); - numSliders = numParams + 1; % active parameters + SoC slider + numSliders = numParams + 1; % Params + SoC slider - % --- DYNAMIC GEOMETRIC CONFIGURATION --- - sliderSpacing = 75; % Height allocated to each block (Label + Slider) - bottomOffset = 40; % Margin at the bottom of the window + % Layout geometry constants + sliderSpacing = 75; + bottomOffset = 40; - % Calculate Y positions for status label and axes lblY = bottomOffset + numSliders * sliderSpacing + 10; axY = lblY + 35; - - % Dynamic calculation of the window height - % (axY + 250 pixels for the plot + 40 pixels margin at the top) figHeight = axY + 250 + 40; - % 1. Create the user interface at the correct size fig = uifigure('Name', 'Impedance Explorer', 'Position', [100, 50, 600, figHeight]); - % 2. Create automatically positioned axes + % Nyquist plot setup ax = uiaxes(fig, 'Position', [50, axY, 500, 250]); title(ax, 'Nyquist Diagram'); xlabel(ax, 'Re(Z)'); ylabel(ax, '-Im(Z)'); grid(ax, 'on'); - % 3. Create automatically positioned status label - lbl = uilabel(fig, 'Position', [50, lblY, 500, 22], 'Text', 'Ready, use slider to start.'); + % Status bar setup + lbl = uilabel(fig, 'Position', [50, lblY, 500, 22], 'Text', 'Ready, adjust a slider to run simulation.'); lbl.FontWeight = 'bold'; + % Create parameter sliders sliders = cell(1, numParams); - - % --- CREATE PARAMETER SLIDERS --- - % Stack them from bottom to top. The first parameter will be placed right above the SoC slider. for iparam = 1 : numParams - txt = sprintf('%d. %s * 10^x (initial value: %g)', iparam, pnames{iparam}, vals(iparam)); - - % Calculate Y position: offsets by "iparam" heights + txt = sprintf('%d. %s * 10^x (initial: %g)', iparam, pnames{iparam}, vals(iparam)); ypos = bottomOffset + iparam * sliderSpacing; - sliders{iparam} = impexp.setupSlider(fig, ypos, txt); end - % --- CREATE SOC SLIDER (At the very bottom) --- + % Create SoC slider (at the absolute bottom) socTxt = sprintf('State of Charge (SoC) - Current: %g', impexp.soc); - ypos_soc = bottomOffset; % Starting position at the very bottom - socSlider = impexp.setupSlider(fig, ypos_soc, socTxt, [0, 1], 0:0.1:1, impexp.soc); + socSlider = impexp.setupSlider(fig, bottomOffset, socTxt, [0, 1], 0:0.1:1, impexp.soc); - % --- EVENT CONNECTIONS --- + % Wire slider events to the updatePlot method callback_fcn = @(src, event) impexp.updatePlot(ax, lbl, sliders, socSlider); - - % Bind callback to all parameter sliders for islider = 1 : numParams sliders{islider}.ValueChangedFcn = callback_fcn; end - % Bind callback to the SoC slider socSlider.ValueChangedFcn = callback_fcn; end - %% - % Core callback method that retrieves current slider values, updates the physical state, runs the BattMo impedance solver, and updates the Nyquist plot. function updatePlot(impexp, ax, lbl, sliders, socSlider) + % Event handler to recalculate physics and update the plot jsonstruct = impexp.jsonstruct; - % Freeze display - lbl.Text = 'Processing... '; + lbl.Text = 'Computing EIS... Please wait.'; lbl.FontColor = '#D95319'; drawnow; + try + % Read updated GUI values impexp.soc = socSlider.Value; baseValues = impexp.getParameterValues(); + vals = zeros(size(baseValues)); for ival = 1 : numel(baseValues) - vals(ival) = baseValues(ival)*(10^(sliders{ival}.Value)); + vals(ival) = baseValues(ival) * (10^(sliders{ival}.Value)); end jsonstruct = impexp.setParameterValues(vals); - % 4. Execute BattMo - [model, inputparams, ~] = setupModelFromJson(jsonstruct); - %% - % We use a dedicated function to compute the initial state for the given electrode concentrations. + % Setup BattMo Model and state initialization + [~, inputparams, ~] = setupModelFromJson(jsonstruct); options = []; options.stateInitialization.initializationSetup = 'soc'; - options.stateInitialization.soc = impexp.soc; % now the soc is updated - %% - % Setup impedance solver and compute the Impedance for a given set of frequencies + options.stateInitialization.soc = impexp.soc; + + % Execute Impedance Solver impsolv = ImpedanceSolver(inputparams, options); - frequences = logspace(-2, 3, 30); - Z = impsolv.computeImpedance(frequences); + frequencies = logspace(-2, 3, 100); + Z = impsolv.computeImpedance(frequencies); - % 5. Plotting - plot(ax, real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); + % Draw new Nyquist trace + plot(ax, real(Z), -imag(Z), '-', 'LineWidth', 2); - % Return to normal lbl.Text = 'Done'; lbl.FontColor = '#77AC30'; catch ME - lbl.Text = 'Calculation error'; + lbl.Text = 'Calculation failed.'; lbl.FontColor = '#A2142F'; - disp('--- Calculation error ---'); - disp(ME.message); - for k = 1:length(ME.stack) - disp(['Line ', num2str(ME.stack(k).line), ' in ', ME.stack(k).name]); - end + fprintf('\n--- BATTMO CALCULATION ERROR ---\n%s\n', ME.message); end end end diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m index a13efd261..b2b10da25 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m @@ -1,3 +1,13 @@ + +%% Example of variation of one parameter: double layer capacitance +% We offer an example of variations of the EIS spectrum of the P2D model +% when the double layer capacitance changes. + + +%% +% First we take the original model developped by Chen et al. in 2020 + + mrstModule add ad-core mrst-gui mpfa agmg linearsolvers jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); @@ -28,23 +38,27 @@ initstate = initStateChen2020(model, c_ne, c_pe); -b = logspace(-2, 2, 5); %change here +%% +% Then we chose a range of value we evaluate the double layer capacitance +b = logspace(-2, 2, 5); frequences = logspace(-4, 4, 200); +%% +% Finally we plot the comparative results on one chart. figure; hold on; + + for i = 1:length(b) - fprintf('compute impedance for doubleLayerCapacitance = %.2e ... ', b(i)); %change here + fprintf('compute impedance for doubleLayerCapacitance = %.2e ... ', b(i)); tic - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); %change here + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); [model, inputparams, ~] = setupModelFromJson(jsonstruct); - % inputparams.(ne).(co).(am).(itf).doubleLayerCapacitance = b(i); - options = []; options.stateInitialization.initializationSetup = 'given state'; options.stateInitialization.computeSteadyState = false; diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m index 1dc7c6826..ba39d095b 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m @@ -1,30 +1,48 @@ +%% Slider to understand better the impact of physical parameters +% Loading the raw BattMo JSON parameter files for chemistry (Chen2020) and geometry. jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); + +%% +% Merging the chemistry and geometry JSON structures into a unified configuration. jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + +%% +% Enabling and configuring the double layer capacitance on the negative electrode interface. +% By default, the raw Chen2020 dataset does not enable the double-layer capacitance. +% We must set useDoubleLayerCapacity to true so the solver registers the parameter. ne = 'NegativeElectrode'; co = 'Coating'; am = 'ActiveMaterial'; itf = 'Interface'; - includeDoubleLayer = true; if includeDoubleLayer - jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true; - jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; - + jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; % F/m^2 end +%% +% Instantiating the Impedance Explorer application handle with our custom JSON structure. impexp = ImpedanceExplore(jsonstruct); +%% +% Cleaning up the MATLAB workspace by closing any previously opened UI figures. erase_previous_figure = true; if erase_previous_figure delete(findall(0, 'Type', 'Figure')); end +%% +% Dynamically overriding the first observed parameter. +% Because ImpedanceExplore is a handle class, we can swap observed parameters +% at runtime before starting the GUI. Here, we swap the negative electrode diffusion +% coefficient with the positive electrode volumetric surface area. change_a_parameter = true; if change_a_parameter - impexp.parameters{1} ={'PositiveElectrode', 'Coating', 'ActiveMaterial', 'Interface', 'volumetricSurfaceArea'}; + impexp.parameters{1} = {'PositiveElectrode', 'Coating', 'ActiveMaterial', 'Interface', 'volumetricSurfaceArea'}; end -impexp.start(); +%% +% Launching the interactive graphical user interface. +impexp.start(); \ No newline at end of file From ba35450ec5a5cb3293d3bfa9449ab2503d8d4ff4 Mon Sep 17 00:00:00 2001 From: Alexandre Date: Thu, 16 Jul 2026 17:11:37 +0200 Subject: [PATCH 100/119] robustnesstest fixed --- .../examples/robustnessTest.m | 100 +++++++++++++++--- 1 file changed, 87 insertions(+), 13 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/robustnessTest.m b/Battery/EquivalentCircuitModel/examples/robustnessTest.m index 74bfc9c57..6421b01ec 100644 --- a/Battery/EquivalentCircuitModel/examples/robustnessTest.m +++ b/Battery/EquivalentCircuitModel/examples/robustnessTest.m @@ -1,18 +1,92 @@ -%% Robustness test for fitting programm -% +%% ROBUSTNESSTEST for FittingEIS -for i = 1:5 - - params0 = pmin + (pmax - pmin) .* rand(1, 5); - disp(['Tour ', num2str(i), ' - params0 :']); - disp(params0); - - feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega); - [~, ~, best_params, fitting_error] = feis.optimizationBFGS(); - feis.plotresults_thevenin(best_params, fitting_error); - feis.printResults(best_params, fitting_error); +num_runs = 5; + +%% PERTURBATION DISTANCE FACTOR +% Controls the maximum relative deviation from the reference parameters. +% 0.05 = Tight search within +/- 5% of the reference +% 0.20 = Medium search within +/- 20% of the reference +% 0.60 = Wide search within +/- 60% of the reference +perturbation_factor = 0.20; + +% Load the full experimental dataset +[Z_re_exp, Z_im_exp, omegas] = load_chen_data(); + +eisdata = struct('omega', omegas, ... + 'Z_re_exp', Z_re_exp, ... + 'Z_im_exp', Z_im_exp); + +%% +% We define the reference parameters (the center point for our test) + +params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; +feis = FittingEIS(eisdata, params0); +[best_params_ref, fitting_error] = feis.run(); + +% Extract hard boundary constraints from the class properties +pmin = feis.scales(1:5); +pmax = feis.scales(6:10); + +% Pre-allocate logging arrays to store optimization history results +all_best_params = zeros(num_runs, 5); +all_errors = zeros(num_runs, 1); - drawnow; +fprintf('\n==================================================\n'); +fprintf(' STARTING EIS OPTIMIZATION ROBUSTNESS TEST \n'); +fprintf('==================================================\n'); +fprintf('Number of runs: %d | Perturbation Radius: +/-%.1f%%\n', num_runs, perturbation_factor * 100); +% --- MAIN ROBUSTNESS LOOP --- +for i = 1:num_runs + + % Generate a random variation vector between -1 and +1 + rand_deviation = 2 * rand(5, 1) - 1; + + % Scale the reference parameters by the perturbation factor + params0_perturbed = best_params_ref(:) .* (1 + perturbation_factor * rand_deviation); + + % Enforce boundary box constraints so guesses don't breach pmin/pmax + params0_perturbed = max(pmin(:), min(pmax(:), params0_perturbed)); + + fprintf('\n-----------------------------------\n'); + fprintf('Run %d/%d - Perturbed Guess:\n', i, num_runs); + disp(params0_perturbed'); % Displayed horizontally for cleaner logs + + try + % 2. Instantiate the FittingEIS class with the new randomized guess + feis = FittingEIS(eisdata, params0_perturbed); + + % 3. Run the objective optimization process + + % 4. Log the output metrics for the current evaluation run + all_best_params(i, :) = best_params(:)'; + all_errors(i) = fitting_error; + + % Display run metrics inside the console + fprintf('-> Success Run %d! Final Error (SSR): %.4e\n', i, fitting_error); + disp('Optimized parameters found:'); + disp(best_params'); + + catch ME + % If a specific initial guess causes numerical instability, skip it safely + fprintf('-> Run %d failed: %s\n', i, ME.message); + all_best_params(i, :) = NaN; + all_errors(i) = NaN; + end + end + +%% --- GLOBAL PERFORMANCE SUMMARY --- + +fprintf('\n==================================================\n'); +fprintf(' ROBUSTNESS SUMMARY \n'); +fprintf('==================================================\n'); +for i = 1:num_runs + if any(isnan(all_best_params(i, :))) + fprintf('Run %d : FAILED\n', i); + else + fprintf('Run %d : SSR Error = %.4e | R0 = %.2e | R1 = %.2e | C1 = %.2e\n', ... + i, all_errors(i), all_best_params(i,1), all_best_params(i,2), all_best_params(i,3)); + end +end \ No newline at end of file From c29a218508ecf748a49dc53917a4a9b6e0a7019c Mon Sep 17 00:00:00 2001 From: Alexandre Date: Fri, 17 Jul 2026 12:04:28 +0200 Subject: [PATCH 101/119] calibrateEcmFromP2D now returns a jsonfile --- .../calibration/calibrateEcmFromP2D.m | 178 +++++++++++++----- .../calibration/runCalibrateEcmFromP2D.m | 4 +- Documentation/ecm.rst | 22 +-- 3 files changed, 146 insertions(+), 58 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m b/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m index 5495e2412..91129bfaa 100644 --- a/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m +++ b/Battery/EquivalentCircuitModel/calibration/calibrateEcmFromP2D.m @@ -1,111 +1,203 @@ function jsonstruct_ecm = calibrateEcmFromP2D(jsonstruct_p2d, soc_step) - - % soc_step : soc increment between 0 and 1. Start from soc = 1. + % CALIBRATEECMFROMP2D Calibrates a 2-RC Equivalent Circuit Model (ECM) + % from a physics-based P2D model across a range of State of Charge (SOC) points. + % + % Inputs: + % jsonstruct_p2d - P2D model configuration structure + % soc_step - SOC decrement interval (default: 0.1) + % + % Output: + % jsonstruct_ecm - Standardized BattMo ECM configuration structure - %% 1. Initialisation - - [model, inputparams] = setupModelFromJson(jsonstruct_p2d); - state_current = setupInitialState(model); - if nargin < 1 + %% 1. Initialization + if nargin < 2 soc_step = 0.1; end + + [model, inputparams] = setupModelFromJson(jsonstruct_p2d); + state_current = setupInitialState(model); + soc_list = (1.0:-soc_step:0.1)'; N_steps = length(soc_list); - results_matrix = zeros(N_steps, 6); + results_matrix = zeros(N_steps, 6); % Stores [SOC, R0, R1, C1, R2, C2] + ocv_list = zeros(N_steps, 1); % Stores Open Circuit Voltage for each SOC freq = logspace(-4, 2, 50)./(2*pi); C_rate = 1; t_xpercent = 3600 * soc_step / C_rate; - %% 2. Main loop + %% 2. Main Loop for i = 1:N_steps current_soc = soc_list(i); fprintf('\n==================================================\n'); fprintf(' EIS fitting for SOC = %.2f (%d/%d)\n', current_soc, i, N_steps); fprintf('==================================================\n'); - %% extraction de l'EIS par computeImpedance() + % Robustness fallback: ensure the initial state has evaluated terminal voltage (.Control.E) + if i == 1 && (~isfield(state_current, 'Control') || ~isfield(state_current.Control, 'E')) + inputparams.Control.DRate = 0; + model.Control = model.setupControl(inputparams.Control); + schedule_init = struct(); + schedule_init.step.val = 0.001; + schedule_init.step.control = 1; + schedule_init.control.src = @(t, varargin) 0; + schedule_init.control.Control = struct('stopFunction', @(model, state, state0) false); + [~, states_init, ~] = simulateScheduleAD(state_current, model, schedule_init); + state_current = states_init{end}; + end + + % Capture the relaxed terminal voltage as the Open Circuit Voltage (OCV) + ocv_list(i) = state_current.Control.E; + fprintf(' Measured Open Circuit Voltage (OCV): %.4f V\n', ocv_list(i)); + + % Run the Impedance Solver options = struct(); options.stateInitialization.computeSteadyState = false; - options.stateInitialization.initializationSetup = 'given state'; extrastructs.initstate = state_current; impsolv = ImpedanceSolver(inputparams, options, extrastructs); - fprintf('Linearisation...\n'); + fprintf('Linearization...\n'); Z = impsolv.computeImpedance(freq); - Z_re = real(Z)'; Z_im = imag(Z)'; omega = (2*pi).*freq; + + % Run parameter identification + eisdata = struct('omega', omega, ... + 'Z_re_exp', Z_re, ... + 'Z_im_exp', Z_im); + - %% extraction des paramètres ECM - p = runFitting(Z_re, Z_im, omega); + params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; % initial condition: C1>2*C2 - % Stockage dans la matrice de résultats + feis = FittingEIS(eisdata, params0); + [p, ~] = feis.run(); + + + % Store values in the matrix results_matrix(i, 1) = current_soc; results_matrix(i, 2:6) = p; - %% Décharge de 5% pour passer au SOC suivant + % Discharge step to reach the next SOC target if i < N_steps - fprintf(' %02d %% discharge...\n', soc_step); + fprintf(' %02d %% discharge...\n', round(soc_step * 100)); inputparams.Control.controlPolicy = 'CCDischarge'; inputparams.Control.DRate = C_rate; jsonstruct_p2d.TimeStepping.tmax = t_xpercent; model.Control = model.setupControl(inputparams.Control); - % CONVERSIONS MANUELLES DU SCHEDULE - % On découpe les 180s en 10 étapes de 18s pour aider le solveur à converger N_substeps = 10; schedule_pulse = struct(); schedule_pulse.step.val = ones(N_substeps, 1) * (t_xpercent / N_substeps); schedule_pulse.step.control = ones(N_substeps, 1); - % Cette fonction anonyme renvoie le courant Imax calculé par BattMo schedule_pulse.control.src = @(t, varargin) varargin{end}; - schedule_pulse.control.Control = struct('stopFunction', @(model, state, state0) false); - - % Simulation du pulse de décharge - % simulateScheduleAD avec l'état en premier argument + [~, states_pulse, ~] = simulateScheduleAD(state_current, model, schedule_pulse); - - % --- Micro-relaxation (Pause de 1 minute) --- + + % Relaxation step (1 minute) fprintf(' 1 min pause...\n'); - inputparams.Control.DRate = 0; % Courant nul + inputparams.Control.DRate = 0; model.Control = model.setupControl(inputparams.Control); - % Construction manuelle du schedule de repos N_rest_steps = 5; schedule_rest = struct(); schedule_rest.step.val = ones(N_rest_steps, 1) * (60 / N_rest_steps); schedule_rest.step.control = ones(N_rest_steps, 1); schedule_rest.control.src = @(t, varargin) varargin{end}; - schedule_rest.control.Control = struct('stopFunction', @(model, state, state0) false); - % Simulation du repos [~, states_rest, ~] = simulateScheduleAD(states_pulse{end}, model, schedule_rest); - - % L'état courant est mis à jour pour le prochain tour de boucle state_current = states_rest{end}; end end - %% 3. Printing final table - ecm_table = array2table(results_matrix, 'VariableNames', ... - {'SOC', 'R0', 'R1', 'C1', 'R2', 'C2'}); + %% 3. Post-Processing & Sorting (Ascending SOC Order) + % BattMo ECM JSON requires OCP and parameters defined with ascending SOC (0 -> 1) + [~, sort_idx] = sort(soc_list, 'ascend'); + soc_asc = soc_list(sort_idx)'; + ocv_asc = ocv_list(sort_idx)'; - % ecm_table = sortrows(ecm_table, 'SOC', 'ascend'); - + results_matrix_sorted = results_matrix(sort_idx, :); + R0_asc = results_matrix_sorted(:, 2)'; + R1_asc = results_matrix_sorted(:, 3)'; + C1_asc = results_matrix_sorted(:, 4)'; + R2_asc = results_matrix_sorted(:, 5)'; + C2_asc = results_matrix_sorted(:, 6)'; + + %% 4. Build jsonstruct_ecm + jsonstruct_ecm = struct(); + + % Nominal capacity calculation (convert from Ampere-seconds to Ampere-hours) + [Q_nominal, ~] = computeCellCapacity(model); + jsonstruct_ecm.nominalcellcapacity = Q_nominal / 3600; + + jsonstruct_ecm.initSOC = 1.0; + + % Extract lower voltage cutoff if present in the P2D model, otherwise use default + if isfield(jsonstruct_p2d.Control, 'lowerCutoffVoltage') + jsonstruct_ecm.lowerVoltageCutoff = jsonstruct_p2d.Control.lowerCutoffVoltage; + else + jsonstruct_ecm.lowerVoltageCutoff = 3.0; + end + + jsonstruct_ecm.totalTime = 4200; + + % Tabulated input current profiles (aligned with template) + jsonstruct_ecm.I.functionFormat = 'tabulated'; + jsonstruct_ecm.I.argumentList = {'time'}; + jsonstruct_ecm.I.dataX = [0, 100, 100.1, 120, 120.1, 300, 300.1, 3800, 3800.1, 4000, 4000.1, 4020, 4020.1, 4200]; + jsonstruct_ecm.I.dataY = [0, 0, 60, 60, 0, 0, 60, 60, 0, 0, 60, 60, 0, 0]; + + % Tabulated Open Circuit Potential (OCP) + jsonstruct_ecm.OCP.functionFormat = 'tabulated'; + jsonstruct_ecm.OCP.argumentList = {'SOC'}; + jsonstruct_ecm.OCP.dataX = soc_asc; + jsonstruct_ecm.OCP.dataY = ocv_asc; + + % Tabulated R0 + jsonstruct_ecm.R0.functionFormat = 'tabulated'; + jsonstruct_ecm.R0.argumentList = {'SOC'}; + jsonstruct_ecm.R0.dataX = soc_asc; + jsonstruct_ecm.R0.dataY = R0_asc; + + % Tabulated R1 & C1 (First RC branch) + jsonstruct_ecm.R1.functionFormat = 'tabulated'; + jsonstruct_ecm.R1.argumentList = {'SOC'}; + jsonstruct_ecm.R1.dataX = soc_asc; + jsonstruct_ecm.R1.dataY = R1_asc; + + jsonstruct_ecm.C1.functionFormat = 'tabulated'; + jsonstruct_ecm.C1.argumentList = {'SOC'}; + jsonstruct_ecm.C1.dataX = soc_asc; + jsonstruct_ecm.C1.dataY = C1_asc; + + % Tabulated R2 & C2 (Second RC branch) + jsonstruct_ecm.R2.functionFormat = 'tabulated'; + jsonstruct_ecm.R2.argumentList = {'SOC'}; + jsonstruct_ecm.R2.dataX = soc_asc; + jsonstruct_ecm.R2.dataY = R2_asc; + + jsonstruct_ecm.C2.functionFormat = 'tabulated'; + jsonstruct_ecm.C2.argumentList = {'SOC'}; + jsonstruct_ecm.C2.dataX = soc_asc; + jsonstruct_ecm.C2.dataY = C2_asc; + + % Print and save summary + ecm_table = array2table(results_matrix_sorted, 'VariableNames', ... + {'SOC', 'R0', 'R1', 'C1', 'R2', 'C2'}); disp(ecm_table); - - file_name = sprintf('ecm_map_results_%02d.mat', soc_step * 100); + file_name = sprintf('jsonstruct_ecm_calibrated_%02d.mat', round(soc_step * 100)); + save(file_name, 'jsonstruct_ecm'); + fprintf('jsonstruct_ecm structure saved successfully in: %s\n', file_name); - save(file_name, 'ecm_table'); - fprintf('Table saved successfully as: %s\n', file_name); -end + % % Convert the struct to a formatted JSON string and display it + % json_readable = jsonencode(jsonstruct_ecm, 'PrettyPrint', true); + % disp(json_readable); +end \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m index fe33973d3..693c7c85d 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m @@ -17,12 +17,12 @@ %% % plot the results - +soc = linspace(0.1, 1.0, 100); figure tiledlayout(2, 3, 'tileindexing', 'columnmajor'); nexttile -%% + % the function |setupFunction| creates a function handle from the battmo function input format. fn = setupFunction(jsonstruct.OCP) plot(soc, fn(soc)) diff --git a/Documentation/ecm.rst b/Documentation/ecm.rst index f41b52341..5596a0e00 100644 --- a/Documentation/ecm.rst +++ b/Documentation/ecm.rst @@ -15,19 +15,15 @@ ECM fitting for lithium-ion batteries Abstract ^^^^^^^^ -Batteries become a central piece of electrification of our energy consumption, -especially for transports. To improve their performances, innovation is getting -faster and research is very active. But before building a battery, it is -important to have an idea of how it will react in different conditions, and -modeling appears useful. It is necessary to work on complex models that fit the -best reality, but also to have powerful models that are a lot simpler. This -model could give important information such as State of Charge or State of -Health, without spending a lot of time, with the minimum complexity. - -We present a work on Equivalent Circuit Model to simulate a complete battery -through only a few parameters. The battery management system needs the value of -those parameters to be efficient. ECM are now the most used model for battery -management systems. +The simulations tools that are used to monitor battery performances include varying degree of physical +complexity. On one side, we have P2D models based on the Doyle-Fuller-Newman approach but it can be very +computationally demanding and with many parameters difficult to parameterize. On the other side, we have the +Equivalent Circuit Models (ECM) which are used for real-time Battery Management Systems (BMS) due to +their low computational cost. + +In this work, we aim at bridging the two models, that is developing a methodology which allows us to +transfer the parameters between the models. We present an automated calibration workflow in BattMo to extract +2-RC Thevenin parameters from synthetic (P2D) and experimental Electrochemical Impedance Spectroscopy (EIS) data. Getting the impedance from PXD Model ^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^ From 9ae053e5f28ec647e7a105883e6502e432c13f31 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 09:33:02 +0200 Subject: [PATCH 102/119] some clean-up in ecm --- .../calibration/FittingEIS.m | 41 +++++++++++++++++++ .../calibration/FittingTime.m | 34 +++++++++++++++ .../calibration/runFittingTime.m | 2 - Documentation/exampleECM.nblink | 3 -- Documentation/runCalibration.nblink | 2 +- 5 files changed, 76 insertions(+), 6 deletions(-) delete mode 100644 Documentation/exampleECM.nblink diff --git a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m index cfc59bd2b..e6e0f4fd9 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingEIS.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m @@ -1,4 +1,45 @@ classdef FittingEIS < handle +% FittingEIS Fit EIS (Nyquist) data to a two‑RC Thevenin equivalent circuit +% +% feis = FittingEIS(eisdata, params0, scales) constructs an object for +% fitting complex impedance data (Z_re_exp, Z_im_exp) measured at +% frequencies 'omega'. The class fits a 2-RC Thevenin model +% (parameters: R0, R1, C1, R2, C2) by minimizing normalized residuals +% between measured and modelled real and imaginary impedance. +% +% Properties +% omega - vector of angular frequencies (rad/s) +% Z_re_exp - measured real part of impedance +% Z_im_exp - measured imaginary part of impedance +% params0 - initial guess for [R0,R1,C1,R2,C2] +% scales - [pmin; pmax] used to map parameters to unit box +% +% Key methods +% run() - run the optimization and return optimal params +% optimizationBFGS() - internal BFGS optimizer wrapper (unitBoxBFGS) +% optifunc(p) - cost and (optionally) gradient for parameter p +% plotResults(...) - plot fitted vs measured EIS and Nyquist +% printResults(...) - print fitted parameter values and score +% +% Notes +% - The optimizer operates in a normalized unit-box; use scales to +% provide lower/upper bounds. If 'scales' is omitted, sensible +% defaults are created from params0 (factor 1e-3..1e+3). +% - optifunc provides analytic gradients to accelerate optimization. +% - The function load_nyquist(p, omega) must be available and return +% modelled Z_re and Z_im for the current parameters. +% +% Example +% eisdata.omega = omega_vec; +% eisdata.Z_re_exp = Zre_meas; +% eisdata.Z_im_exp = Zim_meas; +% feis = FittingEIS(eisdata, params0); +% [opt, ferr] = feis.run(); +% feis.plotResults(opt, ferr); +% +% See also unitBoxBFGS, load_nyquist + + properties diff --git a/Battery/EquivalentCircuitModel/calibration/FittingTime.m b/Battery/EquivalentCircuitModel/calibration/FittingTime.m index 2a3bcedb0..bf58a5283 100644 --- a/Battery/EquivalentCircuitModel/calibration/FittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/FittingTime.m @@ -1,5 +1,39 @@ classdef FittingTime + % FittingTime - Fit a 2-RC Thevenin ECM to P2D simulated time-domain data + % + % Usage: + % ftime = FittingTime(jsonstruct, time_vec, current_exp, params0, scales) + % + % Inputs: + % jsonstruct - BattMo JSON structure used to setup P2D model and OCV + % time_vec - vector of time instants (s) for experimental current + % current_exp - experimental current vector (A) or experimental voltage + % matched to time_vec (used to generate P2D reference) + % params0 - initial guess [R0; R1; C1; R2; C2] + % scales - normalization bounds vector: [pmin(1:5); pmax(1:5)] + % + % Main methods: + % optimizationBFGS(ftime) - run BFGS optimization in unit box + % optifunc(ftime, p) - objective and gradient for params p + % plotresults_thevenin(...) - plot fitted vs reference voltages + % printResults(...) - print numeric results and diagnostics + % plottest(...) - validate ECM on a new current profile + % + % Notes: + % - The class simulates a BattMo P2D model to produce reference OCV, + % voltage and current traces which are used as the 'experimental' + % data for fitting the equivalent-circuit model parameters. + % - Parameter vector is [R0, R1, C1, R2, C2]. Scales specify lower and + % upper bounds used for normalization between 0 and 1. + % + % Example: + % ftime = FittingTime(jsonstruct, t, Iexp, params0, scales); + % [v, hist, best, err] = ftime.optimizationBFGS(); + % ftime.plotresults_thevenin(best, err); + + + properties params0 % initial guess for the parameters to be fitted diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m index 21f9da119..c613be389 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -10,8 +10,6 @@ current_init(time_init >= 400 & time_init < 700) = 0.0; % 3. Repos (400 à 700s) current_init(time_init >= 700 & time_init <= 1000) = 3.5; % 4. Décharge (700 à 1000s) - - jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); diff --git a/Documentation/exampleECM.nblink b/Documentation/exampleECM.nblink deleted file mode 100644 index dafcad3e0..000000000 --- a/Documentation/exampleECM.nblink +++ /dev/null @@ -1,3 +0,0 @@ -{ - "path" : "../Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb" -} diff --git a/Documentation/runCalibration.nblink b/Documentation/runCalibration.nblink index 075b83087..04e498760 100644 --- a/Documentation/runCalibration.nblink +++ b/Documentation/runCalibration.nblink @@ -1,3 +1,3 @@ { "path" : "../Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb" -} \ No newline at end of file +} From f3a85f9994f26ff7033376faebdd5f1a1cd1b12c Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 10:39:21 +0200 Subject: [PATCH 103/119] update in ecm doc --- Documentation/batteryphysics.rst | 1 - Documentation/conf.py | 39 +++---- Documentation/ecm.rst | 156 ++-------------------------- Documentation/runCalibration.nblink | 3 - 4 files changed, 26 insertions(+), 173 deletions(-) delete mode 100644 Documentation/runCalibration.nblink diff --git a/Documentation/batteryphysics.rst b/Documentation/batteryphysics.rst index 723d907b2..e1d45c1b7 100644 --- a/Documentation/batteryphysics.rst +++ b/Documentation/batteryphysics.rst @@ -13,7 +13,6 @@ Battery Physics plating nblinks/runSwellingExample.ipynb soliddiffusion - nblinks/runImpedanceScript.ipynb .. grid:: 2 diff --git a/Documentation/conf.py b/Documentation/conf.py index e5b9b26eb..379d5c2aa 100644 --- a/Documentation/conf.py +++ b/Documentation/conf.py @@ -110,8 +110,8 @@ # General information about the project. project = 'BattMo' -copyright = '2021-2024' -author = 'Simon Clark' +copyright = '2021-2026' +author = 'Xavier Raynaud, Augut Johansson, Simon Clark' # The version info for the project you're documenting, acts as replacement for # |version| and |release|, also used in various other places throughout the @@ -136,23 +136,24 @@ # directories to ignore when looking for source files. exclude_patterns = ['_build', 'unparsed'] # exclude_patterns += ['*.nblink'] -# exclude_patterns += ["exploreOutput.nblink"] -# exclude_patterns += ["functionInterfaceExample.nblink"] -# exclude_patterns += ["runBolaySEI.nblink"] -# exclude_patterns += ["runCellPlating.nblink"] -# exclude_patterns += ["runControlExamples.nblink"] -# exclude_patterns += ["runGenericStepControlCycle.nblink"] -# exclude_patterns += ["runGenericStepControlSimple.nblink"] -# exclude_patterns += ["runOnlyThermal.nblink"] -# exclude_patterns += ["runSiliconGraphiteBattery.nblink"] -# exclude_patterns += ["runSPMplating.nblink"] -# exclude_patterns += ["runSwellingExample.nblink"] -# exclude_patterns += ["runThermalExample.nblink"] -# exclude_patterns += ["runTimeControlExample.nblink"] -# exclude_patterns += ['publishedExamples'] -# exclude_patterns += ['pynbnotebooks'] -# exclude_patterns += ['pynbnotebooks/part_1_battery_modeling_guide.ipynb'] -# exclude_patterns += ['pynbnotebooks/part_2_battery_modeling_guide.ipynb'] +exclude_patterns += ["tutorials/*"] +exclude_patterns += ["nblinks/exploreOutput.nblink"] +exclude_patterns += ["nblinks/functionInterfaceExample.nblink"] +exclude_patterns += ["nblinks/runBolaySEI.nblink"] +exclude_patterns += ["nblinks/runCellPlating.nblink"] +exclude_patterns += ["nblinks/runControlExamples.nblink"] +exclude_patterns += ["nblinks/runGenericStepControlCycle.nblink"] +exclude_patterns += ["nblinks/runGenericStepControlSimple.nblink"] +exclude_patterns += ["nblinks/runOnlyThermal.nblink"] +exclude_patterns += ["nblinks/runSiliconGraphiteBattery.nblink"] +exclude_patterns += ["nblinks/runSPMplating.nblink"] +exclude_patterns += ["nblinks/runSwellingExample.nblink"] +exclude_patterns += ["nblinks/runThermalExample.nblink"] +exclude_patterns += ["nblinks/runTimeControlExample.nblink"] +exclude_patterns += ['nblinks/publishedExamples'] +exclude_patterns += ['nblinks/pynbnotebooks'] +exclude_patterns += ['modelingGuide/part_1_battery_modeling_guide.ipynb'] +exclude_patterns += ['modelingGuide/part_2_battery_modeling_guide.ipynb'] # The reST default role (used for this markup: `text`) to use for all # documents. diff --git a/Documentation/ecm.rst b/Documentation/ecm.rst index 5596a0e00..54e1c7a83 100644 --- a/Documentation/ecm.rst +++ b/Documentation/ecm.rst @@ -6,14 +6,8 @@ EIS and Equivalent Circuit Models :maxdepth: 2 :hidden: - runImpedanceScript.nblink - runCalibration.nblink - -ECM fitting for lithium-ion batteries -------------------------------------- - Abstract -^^^^^^^^ +======== The simulations tools that are used to monitor battery performances include varying degree of physical complexity. On one side, we have P2D models based on the Doyle-Fuller-Newman approach but it can be very @@ -25,146 +19,8 @@ In this work, we aim at bridging the two models, that is developing a methodolog transfer the parameters between the models. We present an automated calibration workflow in BattMo to extract 2-RC Thevenin parameters from synthetic (P2D) and experimental Electrochemical Impedance Spectroscopy (EIS) data. -Getting the impedance from PXD Model -^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^ - -ECM parameterisation from PXD model using automatic differentiation. - -Obtaining the impedance is a major part of the work, as we try to fit the -impedance given by our parameters to the synthetic impedance from the PXD -model. - -We work with the state vector :math:`\mathcal{X}(t, x)` containing all the -variables from the PXD model: - -.. math:: - - \mathcal{X}(t, x) = - [c_{\mathrm{ne}}(t, x), \phi_{\mathrm{ne}}(t, x), - c_{\mathrm{elyte}}(t, x), \phi_{\mathrm{elyte}}(t, x), \ldots] - -The generic equation of the system is - -.. math:: - - \frac{\partial \mathcal{M}(\mathcal{X})}{\partial t} + \mathcal{A}(\mathcal{X}) = 0. - -The operators :math:`\mathcal{M}` and :math:`\mathcal{A}` are non-linear, but -we discretize them and :math:`\mathcal{X}(t, x)` becomes :math:`X(t)` -belonging to :math:`\mathbb{R}^{N}`. - -The equation then becomes a non-linear system of *ordinary differential -equations*: - -.. math:: - - \frac{\partial M(X)}{\partial t} + A(X) = I(t)b(X). - -Here :math:`I(t)` is the current and :math:`b` is mostly empty. An implicit -method is then used for the time discretization. One finds :math:`X^{n+1}` -from :math:`X^{n}` at time step :math:`n` by solving the equation for the -unknown :math:`X`: - -.. math:: - - \frac{M(X) - M(X^{n})}{\Delta t} + A(X) = b(X)I(t^{n+1}). - -Then the system is linearized around a state given by :math:`X_{0}` with a -small perturbation :math:`\delta X = X - X_{0}`. The term :math:`A(X)` becomes - -.. math:: - - A(X) = A(X_{0}) + D_{A}(X_{0})\delta X, - -with :math:`D_{A}` the Jacobian of :math:`A`. Applying the same process for -:math:`M` and :math:`b` (:math:`D_{M}` and :math:`D_{b}` being their -Jacobians) gives the following linear system of ordinary differential -equations: - -.. math:: - - D_{M}\frac{\partial}{\partial t}\delta X + A(X_{0}) + D_{A}\delta X - = I(t)b(X_{0}) + I(t)D_{b}\delta X. - -:math:`X_{0}` is a solution to the steady-state problem :math:`I(t) = 0`, which -implies :math:`A(X_{0}) = 0`. Also, :math:`\delta X \ll 1` implies -:math:`I(t)b(X_{0}) \gg I(t)D_{b}(X_{0})\delta X`, so the last term is -neglected. - -The final equation is - -.. math:: - - D_{M}\frac{\partial}{\partial t}\delta X + D_{A}\delta X = I(t)b_{0}. - -It is possible to obtain :math:`D_M` and :math:`D_A` with the Jacobian. Since - -.. math:: - - J(\Delta t) = \frac{D_M}{\Delta t} + D_A, - -this leads to - -.. math:: - - D_M = 2\Delta t \left(J(\Delta t) - J(2\Delta t)\right) - -and - -.. math:: - - D_A = 2\left(J(\Delta t) - J(2\Delta t)\right). - -The Fourier transform of this equation is - -.. math:: - - [i\omega D_{M} + D_{A}]\overline{\delta X} = \bar{I}b_{0}, - -with :math:`I(t) = \bar{I}e^{i\omega t}` and -:math:`\delta X = \overline{\delta X}e^{i\omega t}`. - -So - -.. math:: - - \overline{\delta X} = \left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}\bar{I}. - -There is a certain vector :math:`r` so that :math:`U = r^{t}X`, where -:math:`U` is the voltage response. - -Then - -.. math:: - - U = r^{t}X_{0} + r^{t}\delta X, - -so :math:`U - U_{0} = \bar{U}e^{i\omega t}` with -:math:`U_{0} = r^{t}X_{0}`. - -It follows that - -.. math:: - - \bar{U} = r^{t}\overline{\delta X} - -and therefore - -.. math:: - - \bar{U} = r^{t}\left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}\bar{I}. - -At the end it gives - -.. math:: - - Z(\omega) = r^{t}\left[i\omega D_{M} + D_{A}\right]^{-1}b_{0}. - -ECM Presentation -^^^^^^^^^^^^^^^^ - Objective -""""""""" +========= Effective everyday operation of a battery requires the Battery Management System (BMS) to continuously monitor its real-time state (State of Charge, @@ -179,7 +35,7 @@ parameters. Another one, more accurate, could be to train a neural network to develop a strong state-prediction model. Theory -"""""" +====== The electrical activity of a battery can be modelled by an Open Circuit Voltage (OCV), which is a perfect source of current. This is the simplest way to @@ -221,7 +77,7 @@ The impedance is :math:`Z = \frac{1}{Q\left(j\omega\right)^{\alpha}}`. A 2nd-Order model with CPE used by Santoni Physical Meaning of ECM components (`Analog Devices `_, 2021) -""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""""" +========================================================================================================================================================== ECM are built after Occam's razor principles, where each component has to be linked to a physical phenomenon of the battery (`Fletcher `_, 2013): @@ -253,7 +109,7 @@ this range. Electrochemical processes linked to EIS regions (`Analog Devices `_, 2021) Impact on Impedance of physical parameters from PXD model -^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^^ +========================================================= The PXD BattMo model was developed using parameters derived from the study by Chen et al. (2020). These parameters were subsequently modified to better @@ -283,7 +139,7 @@ through the solid electrode particles. :padding: 2 :ref:`Battery Impedance Computation ` - + .. grid-item-card:: :padding: 2 diff --git a/Documentation/runCalibration.nblink b/Documentation/runCalibration.nblink deleted file mode 100644 index 04e498760..000000000 --- a/Documentation/runCalibration.nblink +++ /dev/null @@ -1,3 +0,0 @@ -{ - "path" : "../Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb" -} From 50a822d6c1dd7b736d5d0024d199bf5b51f723aa Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:13:33 +0200 Subject: [PATCH 104/119] fix new syntax --- .../calibration/runCalibrateEcmFromP2D.m | 2 +- .../calibration/runCalibration.m | 2 +- .../calibration/runFittingTime.m | 2 +- .../calibration/utils/load_chen_data.m | 2 +- .../examples/old/validateEcmTime.m | 2 +- .../pxdParamsImpact/ImpedanceExplore.m | 8 +++--- .../activationEnergyOfReaction_impact.m | 2 +- .../pxdParamsImpact/bruggeman_impact.m | 2 +- .../doubleLayerCapacitance_impact.m | 2 +- .../electronicConductivity_impact.m | 2 +- .../pxdParamsImpact/old/param_dependency.m | 2 +- .../pxdParamsImpact/porosity_impact.m | 2 +- .../reactionRateConstant_impact.m | 2 +- .../referenceDiffusionCoefficient_impact.m | 2 +- .../pxdParamsImpact/runImpedanceExplore.m | 28 +++++++++++-------- .../saturationConcentration_impact.m | 2 +- .../pxdParamsImpact/volumefraction_impact.m | 2 +- .../volumetricSurfaceArea_impact.m | 2 +- 18 files changed, 37 insertions(+), 31 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m index 693c7c85d..b6c408502 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m @@ -10,7 +10,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct_p2d = mergeJsonStructs({jsonstruct_material, ... +jsonstruct_p2d = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); jsonstruct = calibrateEcmFromP2D(jsonstruct_p2d, soc_step); diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibration.m b/Battery/EquivalentCircuitModel/calibration/runCalibration.m index f1631c4f2..b3c021502 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibration.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibration.m @@ -6,7 +6,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct_base = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); +jsonstruct_base = mergeStructs({jsonstruct_material, jsonstruct_geometry}); jsonstruct_base.NegativeElectrode.Coating.ActiveMaterial.Interface.useDoubleLayerCapacity = true; diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m index c613be389..13f95348d 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingTime.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingTime.m @@ -12,7 +12,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); +jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry}); params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2 diff --git a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m index a05b021e5..0749ef0ec 100644 --- a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m @@ -18,7 +18,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, ... + jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m b/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m index b7e4ba5da..3729bca12 100644 --- a/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m +++ b/Battery/EquivalentCircuitModel/examples/old/validateEcmTime.m @@ -20,7 +20,7 @@ function validateEcmTime(file_name) % Generation of the "Ground Truth": Continuous P2D discharge (BattMo) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry}); [model, inputparams] = setupModelFromJson(jsonstruct); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m index 5e6afce3b..0517d8152 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m @@ -17,7 +17,7 @@ try jsonstruct_material = parseBattmoJson(fullfile('ParameterData', 'ParameterSets', 'Chen2020', 'chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry}); % Safe default fallback for capacitance ne = 'NegativeElectrode'; co = 'Coating'; am = 'ActiveMaterial'; itf = 'Interface'; @@ -37,7 +37,7 @@ function viewOptions(impexp) % Helper to print all available scalar properties in the model JSON - fjv = flattenJsonStruct(impexp.jsonstruct, 'doprint', false); + fjv = flattenStruct(impexp.jsonstruct, 'doprint', false); fprintf('\n\n*** List of all the scalar parameters in the model ***\n'); fjv.print('filter', {'value', @(val) (isnumeric(val) && isscalar(val))}); end @@ -91,7 +91,7 @@ function setupDefaultParameters(impexp) parameters = impexp.parameters; vals = zeros(1, numel(parameters)); for iparam = 1 : numel(parameters) - val = getJsonStructField(jsonstruct, parameters{iparam}); + val = getStructField(jsonstruct, parameters{iparam}); if ~isnumeric(val) || ~isscalar(val) pathStr = strjoin(parameters{iparam}, '.'); error('ImpedanceExplore:ParameterNotFound', ... @@ -111,7 +111,7 @@ function setupDefaultParameters(impexp) parameters = impexp.parameters; for iparam = 1 : numel(parameters) - jsonstruct = setJsonStructField(jsonstruct, parameters{iparam}, vals(iparam), 'handleMisMatch', 'quiet'); + jsonstruct = setStructField(jsonstruct, parameters{iparam}, vals(iparam), 'handleMisMatch', 'quiet'); end end diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m index 6ff436588..4b5b58bf6 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m @@ -4,7 +4,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m index 1412d6644..f6366355a 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m @@ -4,7 +4,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m index b2b10da25..7ae0d1965 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m @@ -13,7 +13,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); ne = 'NegativeElectrode'; diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m index df70d8b3f..09534a822 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m index d6186307f..3545c67ad 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/old/param_dependency.m @@ -3,7 +3,7 @@ function param_dependency(jsonstruct) % 1. Chargement des données (Conservez votre méthode de chargement ici) jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); - jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); + jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry}); ne = 'NegativeElectrode'; co = 'Coating'; am = 'ActiveMaterial'; diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m index 47d1a7cce..c25c05283 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m index 12baa2706..b18064b96 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m index 88aebd8d1..7faff1798 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m index ba39d095b..ada8cf990 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m @@ -1,20 +1,25 @@ -%% Slider to understand better the impact of physical parameters -% Loading the raw BattMo JSON parameter files for chemistry (Chen2020) and geometry. +%% Exploring the impact of the P2D parameters on EIS output + +%% +% We load the raw BattMo JSON parameter files for chemistry (Chen2020) and geometry. +% jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); %% % Merging the chemistry and geometry JSON structures into a unified configuration. -jsonstruct = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry}); +% +jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry}); %% % Enabling and configuring the double layer capacitance on the negative electrode interface. % By default, the raw Chen2020 dataset does not enable the double-layer capacitance. % We must set useDoubleLayerCapacity to true so the solver registers the parameter. -ne = 'NegativeElectrode'; -co = 'Coating'; -am = 'ActiveMaterial'; +ne = 'NegativeElectrode'; +co = 'Coating'; +am = 'ActiveMaterial'; itf = 'Interface'; + includeDoubleLayer = true; if includeDoubleLayer @@ -24,20 +29,20 @@ %% % Instantiating the Impedance Explorer application handle with our custom JSON structure. +% impexp = ImpedanceExplore(jsonstruct); %% % Cleaning up the MATLAB workspace by closing any previously opened UI figures. +% erase_previous_figure = true; if erase_previous_figure delete(findall(0, 'Type', 'Figure')); end %% -% Dynamically overriding the first observed parameter. -% Because ImpedanceExplore is a handle class, we can swap observed parameters -% at runtime before starting the GUI. Here, we swap the negative electrode diffusion -% coefficient with the positive electrode volumetric surface area. +% We can dynamically override the parameters. Here, as an example, we change the first parameter. +% change_a_parameter = true; if change_a_parameter impexp.parameters{1} = {'PositiveElectrode', 'Coating', 'ActiveMaterial', 'Interface', 'volumetricSurfaceArea'}; @@ -45,4 +50,5 @@ %% % Launching the interactive graphical user interface. -impexp.start(); \ No newline at end of file +% +impexp.start(); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m index ac40f3e89..0c338feeb 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m index 3eff22ccb..724b5ae61 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m index 3e949d075..b0f05fa0d 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m @@ -3,7 +3,7 @@ jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); -jsonstruct = mergeJsonStructs({jsonstruct_material, ... +jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); From 42febbedc95fb3703024d35df011087e1b60343f Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:14:42 +0200 Subject: [PATCH 105/119] moved file --- .../{ => old}/notebooks/calibrationECM.mlx | Bin 1 file changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/{ => old}/notebooks/calibrationECM.mlx (100%) diff --git a/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx b/Battery/EquivalentCircuitModel/old/notebooks/calibrationECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx rename to Battery/EquivalentCircuitModel/old/notebooks/calibrationECM.mlx From 189adbb0640e66042aa35bb29ea897263e54821e Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:14:56 +0200 Subject: [PATCH 106/119] update in doc --- Documentation/ecm.rst | 26 +++++++++++++++++++++----- 1 file changed, 21 insertions(+), 5 deletions(-) diff --git a/Documentation/ecm.rst b/Documentation/ecm.rst index 54e1c7a83..e71062ef7 100644 --- a/Documentation/ecm.rst +++ b/Documentation/ecm.rst @@ -2,10 +2,6 @@ EIS and Equivalent Circuit Models ================================= -.. toctree:: - :maxdepth: 2 - :hidden: - Abstract ======== @@ -133,14 +129,34 @@ charge-transfer resistance, and low frequencies reflect mass transport and diffusion processes, providing insight into the migration rate of lithium ions through the solid electrode particles. +Scripts +======= + +.. toctree:: + :hidden: + + nblinks/runEquivalentCircuitModel.nblink + nblinks/runImpedanceScript.nblink + nblinks/runCalibration.nblink + .. grid:: 2 .. grid-item-card:: :padding: 2 - :ref:`Battery Impedance Computation ` + :ref:`ECM simulation ` + + .. grid-item-card:: + :padding: 2 + + :ref:`Impedance Computation ` .. grid-item-card:: :padding: 2 :ref:`ECM calibration ` + + + + + From 8bd41902b284109f5b1aa4715e2fc53fdf7609bf Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:17:35 +0200 Subject: [PATCH 107/119] update in docs --- .../notebooks/runEquivalentCircuitModel.ipynb | 225 ++++++++++++++++++ .../notebooks/runEquivalentCircuitModel.mlx | Bin 0 -> 154523 bytes .../examples/runEquivalentCircuitModel.m | 8 +- Documentation/nblinks/runCalibration.nblink | 3 + .../nblinks/runEquivalentCircuitModel.nblink | 3 + 5 files changed, 237 insertions(+), 2 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb create mode 100644 Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.mlx create mode 100644 Documentation/nblinks/runCalibration.nblink create mode 100644 Documentation/nblinks/runEquivalentCircuitModel.nblink diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb b/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb new file mode 100644 index 000000000..89e4bc2a0 --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb @@ -0,0 +1,225 @@ +{ + "cells": [ + { + "cell_type": "raw", + "metadata": { +"raw_mimetype": "text/restructuredtext" +}, + "source": [ + "# Time Simulation of an ECM model\n", + "\n", + "The function :battmo:`createParametersECM` setups an data set for the ECM model. The structure `jsonstruct` contains values of the ECM parameters (resistances, capicaties, ...) that depend on the frequency. See below for the plot of the values\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "jsonstruct = createParametersECM();" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Setup the ECM model\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 2, + "metadata": {}, + "source": [ + "inputparams = EquivalentCircuitModelInputParams(jsonstruct);\n", + "model = EquivalentCircuitModel(inputparams);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Review of the model parameters\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 3, + "metadata": {}, + "source": [ + "soc = linspace(0, 1, 100);\n", + "\n", + "\n", + "figure\n", + "tiledlayout(2, 3, 'tileindexing', 'columnmajor');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.OCPfunc(soc))\n", + "title('OCP')\n", + "xlabel('SOC / -')\n", + "ylabel('OCP / V');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.R0func(soc))\n", + "title('R0')\n", + "xlabel('SOC / -')\n", + "ylabel('R0 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.R1func(soc))\n", + "title('R1')\n", + "xlabel('SOC / -')\n", + "ylabel('R1 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.C1func(soc))\n", + "title('C1')\n", + "xlabel('SOC / -')\n", + "ylabel('C1 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.R2func(soc))\n", + "title('R2')\n", + "xlabel('SOC / -')\n", + "ylabel('R2 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "plot(soc, model.C2func(soc))\n", + "title('C2')\n", + "xlabel('SOC / -')\n", + "ylabel('C2 / Ohm');" + ], + "outputs": [ + { + "data": { + "text/html": [ + "

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" + ] + }, + "metadata": {}, + "execution_count": 3, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "The input current has been passed to the model\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 4, + "metadata": {}, + "source": [ + "figure\n", + "totalTime = model.totalTime;\n", + "t = linspace(0, totalTime, 200);\n", + "plot(t/hour, model.Ifunc(t), 'o-');\n", + "title('Input current')\n", + "xlabel('time / hour')\n", + "ylabel('I / A');" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
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" + ] + }, + "metadata": {}, + "execution_count": 4, + "output_type": "execute_result" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Solve the model\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 5, + "metadata": {}, + "source": [ + "[t, U, I, SOC] = model.solve();" + ], + "outputs": [] + }, + { + "cell_type": "code", + "execution_count": 6, + "metadata": {}, + "source": [ + "figure\n", + "tiledlayout(1, 3)\n", + "nexttile\n", + "plot(t/hour, I)\n", + "title('Current')\n", + "xlabel('Time / hour')\n", + "ylabel('Current / A');\n", + "nexttile\n", + "plot(t/hour, U)\n", + "title('Voltage')\n", + "xlabel('Time / hour')\n", + "ylabel('Voltage / V');\n", + "nexttile\n", + "plot(t/hour, SOC)\n", + "title('SOC')\n", + "xlabel('Time / hour')\n", + "ylabel('SOC / -');" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
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z-g@}7khC51ixr#%uhQsk+VH65^x9BHcJYl#WT0tU25ua@kbJkO#x0y>~qWzPl zmGP?&{$8pXLsv|Z07!YlKi7iy?zw1!8p8+Xcb-Wfn3Wwx(}S|xQUgo&x7SK{6Q;Z4jf4iX{zkqN2>}1{GEtbQ)&m5 zC<0bdJI6l}0Sxf5clUPoaR1%O%#$SV_c4Rosthbqd%w8y%7tV8-GBRUNp6uQ0MV;ugy`ET`1xa=#q%;_KT|8oWta5GjRY; zXy04qglz_|#$v^%QyJ$Uu$xG{@txc5K(Xyt8QMhx%*3ET@N+`UzVvjm_-S6rQ{AVP)Sr)L5=YKX9D2Z6sk%ku1Dw zqZwFhbQ-3j3@tDeSYQU)(1#USnYiHr7$b4K^rK=G3B2ABvQk0I%j~-^B4mT7X^&jy z%(qxSc07JDNiqq(_<{G_-Tj_egz$5!Y}s9d$Hx zK8(Mj$-FSwHN>Z8H$GgY)2>=0AQx*;f`u*AIoQfAbW4~-~Rsz(0(DY&V^ED z!~_8F|5F=vK0Sg?UBEswG)Oz@}WR#aqjv-WYdwh^%Nu=RCA zUBG{{>>e+;QK^Lv= Date: Tue, 25 Aug 2026 11:18:59 +0200 Subject: [PATCH 108/119] moved files --- .../{ => selectedParameters}/activationEnergyOfReaction_impact.m | 0 .../pxdParamsImpact/{ => selectedParameters}/bruggeman_impact.m | 0 .../{ => selectedParameters}/doubleLayerCapacitance_impact.m | 0 .../{ => selectedParameters}/electronicConductivity_impact.m | 0 .../pxdParamsImpact/{ => selectedParameters}/porosity_impact.m | 0 .../{ => selectedParameters}/reactionRateConstant_impact.m | 0 .../referenceDiffusionCoefficient_impact.m | 0 .../{ => selectedParameters}/saturationConcentration_impact.m | 0 .../{ => selectedParameters}/volumefraction_impact.m | 0 .../{ => selectedParameters}/volumetricSurfaceArea_impact.m | 0 10 files changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/activationEnergyOfReaction_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/bruggeman_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/doubleLayerCapacitance_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/electronicConductivity_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/porosity_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/reactionRateConstant_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/referenceDiffusionCoefficient_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/saturationConcentration_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/volumefraction_impact.m (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ => selectedParameters}/volumetricSurfaceArea_impact.m (100%) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/activationEnergyOfReaction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/activationEnergyOfReaction_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/activationEnergyOfReaction_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/bruggeman_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/bruggeman_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/bruggeman_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/doubleLayerCapacitance_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/doubleLayerCapacitance_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/doubleLayerCapacitance_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/electronicConductivity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/electronicConductivity_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/electronicConductivity_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/porosity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/porosity_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/porosity_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/reactionRateConstant_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/reactionRateConstant_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/reactionRateConstant_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/referenceDiffusionCoefficient_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/referenceDiffusionCoefficient_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/referenceDiffusionCoefficient_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/saturationConcentration_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/saturationConcentration_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/saturationConcentration_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/volumefraction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumefraction_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/volumefraction_impact.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/volumetricSurfaceArea_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/volumetricSurfaceArea_impact.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/selectedParameters/volumetricSurfaceArea_impact.m From 62fe88b5cd4747bb5ea40dcad0c507d6b1f615cd Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:19:28 +0200 Subject: [PATCH 109/119] changed names --- .../pxdParamsImpact/{ImpedanceExplore.m => ImpedanceExplorer.m} | 0 .../{runImpedanceExplore.m => runImpedanceExplorer.m} | 0 2 files changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{ImpedanceExplore.m => ImpedanceExplorer.m} (100%) rename Battery/EquivalentCircuitModel/examples/pxdParamsImpact/{runImpedanceExplore.m => runImpedanceExplorer.m} (100%) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplore.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplore.m rename to Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m From 126d2b5aa59587746515d019273d7af492c256e7 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:21:00 +0200 Subject: [PATCH 110/119] update after name change --- .../examples/pxdParamsImpact/ImpedanceExplorer.m | 10 +++++----- .../examples/pxdParamsImpact/runImpedanceExplorer.m | 2 +- 2 files changed, 6 insertions(+), 6 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m index 0517d8152..20d835766 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m @@ -1,4 +1,4 @@ -classdef ImpedanceExplore < handle +classdef ImpedanceExplorer < handle properties (SetAccess = immutable) jsonstruct % Holds the base P2D model configuration structure model % Initialized BattMo model object @@ -10,7 +10,7 @@ end methods - function impexp = ImpedanceExplore(jsonstruct) + function impexp = ImpedanceExplorer(jsonstruct) % Constructor: auto-loads Chen2020 P2D model if no structure is provided if nargin < 1 || isempty(jsonstruct) fprintf('Initializing default Chen2020 P2D model...\n'); @@ -26,7 +26,7 @@ jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; end catch ME - error('ImpedanceExplore:AutoLoadFailed', 'Failed to auto-load default files: %s', ME.message); + error('ImpedanceExplorer:AutoLoadFailed', 'Failed to auto-load default files: %s', ME.message); end end @@ -94,7 +94,7 @@ function setupDefaultParameters(impexp) val = getStructField(jsonstruct, parameters{iparam}); if ~isnumeric(val) || ~isscalar(val) pathStr = strjoin(parameters{iparam}, '.'); - error('ImpedanceExplore:ParameterNotFound', ... + error('ImpedanceExplorer:ParameterNotFound', ... ['\n\n=== PARAMETER NOT FOUND ===\n' ... 'Invalid path in BattMo JSON:\n -> "jsonstruct.%s"\n' ... 'Check spelling or use app.viewOptions() to debug.\n\n'], pathStr); @@ -204,4 +204,4 @@ function updatePlot(impexp, ax, lbl, sliders, socSlider) end end end -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m index ada8cf990..6412acca9 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/runImpedanceExplorer.m @@ -30,7 +30,7 @@ %% % Instantiating the Impedance Explorer application handle with our custom JSON structure. % -impexp = ImpedanceExplore(jsonstruct); +impexp = ImpedanceExplorer(jsonstruct); %% % Cleaning up the MATLAB workspace by closing any previously opened UI figures. From cd61762ec5fe85e5be6bd17d1fffad76fbabaf57 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 11:43:42 +0200 Subject: [PATCH 111/119] some update in ImpedanceExplorer --- .../examples/pxdParamsImpact/ImpedanceExplorer.m | 15 +++++++++++---- 1 file changed, 11 insertions(+), 4 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m index 20d835766..f1cd2f447 100644 --- a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/ImpedanceExplorer.m @@ -71,7 +71,7 @@ function setupDefaultParameters(impexp) if nargin < 7, initVal = 0; end uilabel(fig, ... - 'Position', [50, ypos + 20, 500, 40], ... + 'Position', [50, ypos + 10, 500, 40], ... 'WordWrap', 'on', ... 'Text', txt); @@ -116,6 +116,7 @@ function setupDefaultParameters(impexp) end function start(impexp) + % Computes sizes and runs the App Designer UI Window pnames = impexp.setupParameterLegendNames(); vals = impexp.getParameterValues(); @@ -147,14 +148,16 @@ function start(impexp) % Create parameter sliders sliders = cell(1, numParams); for iparam = 1 : numParams - txt = sprintf('%d. %s * 10^x (initial: %g)', iparam, pnames{iparam}, vals(iparam)); - ypos = bottomOffset + iparam * sliderSpacing; + txt = sprintf('%d) %s * 10^x (initial: %g)', iparam, pnames{iparam}, vals(iparam)); + ypos = bottomOffset + (numParams - iparam + 1)*sliderSpacing; sliders{iparam} = impexp.setupSlider(fig, ypos, txt); end % Create SoC slider (at the absolute bottom) - socTxt = sprintf('State of Charge (SoC) - Current: %g', impexp.soc); + socTxt = sprintf('State of Charge (SoC)'); socSlider = impexp.setupSlider(fig, bottomOffset, socTxt, [0, 1], 0:0.1:1, impexp.soc); + + impexp.updatePlot(ax, lbl, sliders, socSlider); % Wire slider events to the updatePlot method callback_fcn = @(src, event) impexp.updatePlot(ax, lbl, sliders, socSlider); @@ -162,6 +165,7 @@ function start(impexp) sliders{islider}.ValueChangedFcn = callback_fcn; end socSlider.ValueChangedFcn = callback_fcn; + end function updatePlot(impexp, ax, lbl, sliders, socSlider) @@ -197,10 +201,13 @@ function updatePlot(impexp, ax, lbl, sliders, socSlider) lbl.Text = 'Done'; lbl.FontColor = '#77AC30'; + catch ME + lbl.Text = 'Calculation failed.'; lbl.FontColor = '#A2142F'; fprintf('\n--- BATTMO CALCULATION ERROR ---\n%s\n', ME.message); + end end end From 560bc9c60be4fc7b704750b8ee7d44e37ff57190 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:09:28 +0200 Subject: [PATCH 112/119] update in explorer --- .../notebooks/runImpedanceExplorer.ipynb | 178 ++++++++++++++++++ .../notebooks/runImpedanceExplorer.mlx | Bin 0 -> 46626 bytes .../pxdParamsImpact/runImpedanceExplorer.m | 4 +- Documentation/ecm.rst | 16 +- .../nblinks/runImpedanceExplorer.nblink | 3 + 5 files changed, 195 insertions(+), 6 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.ipynb create mode 100644 Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.mlx create mode 100644 Documentation/nblinks/runImpedanceExplorer.nblink diff --git a/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.ipynb b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.ipynb new file mode 100644 index 000000000..03322fa31 --- /dev/null +++ b/Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.ipynb @@ -0,0 +1,178 @@ +{ + "cells": [ + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "# Exploring interactively the impact of the P2D parameters on EIS output\n", + "\n", + "We load the raw BattMo JSON parameter files for chemistry (Chen2020) and geometry.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json'));\n", + "jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json'));" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Merging the chemistry and geometry JSON structures into a unified configuration.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 2, + "metadata": {}, + "source": [ + "jsonstruct = mergeStructs({jsonstruct_material, jsonstruct_geometry});" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Enabling and configuring the double layer capacitance on the negative electrode interface. By default, the raw Chen2020 dataset does not enable the double\\-layer capacitance. We must set useDoubleLayerCapacity to true so the solver registers the parameter.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 3, + "metadata": {}, + "source": [ + "ne = 'NegativeElectrode';\n", + "co = 'Coating';\n", + "am = 'ActiveMaterial';\n", + "itf = 'Interface';\n", + "\n", + "\n", + "includeDoubleLayer = true;\n", + "\n", + "\n", + "if includeDoubleLayer\n", + " jsonstruct.(ne).(co).(am).(itf).useDoubleLayerCapacity = true;\n", + " jsonstruct.(ne).(co).(am).(itf).doubleLayerCapacitance = 0.2; % F/m^2\n", + "end" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Instantiating the Impedance Explorer application handle with our custom JSON structure.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 4, + "metadata": {}, + "source": [ + "impexp = ImpedanceExplorer(jsonstruct);" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Cleaning up the MATLAB workspace by closing any previously opened UI figures.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 5, + "metadata": {}, + "source": [ + "erase_previous_figure = true;\n", + "if erase_previous_figure\n", + " delete(findall(0, 'Type', 'Figure'));\n", + "end" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "We can dynamically override the parameters. Here, as an example, we change the first parameter.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 6, + "metadata": {}, + "source": [ + "change_a_parameter = true;\n", + "if change_a_parameter\n", + " impexp.parameters{1} = {'PositiveElectrode', 'Coating', 'ActiveMaterial', 'Interface', 'volumetricSurfaceArea'};\n", + "end" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "Launching the interactive graphical user interface.\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 7, + "metadata": {}, + "source": [ + "impexp.start();" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
\"figure_0.png\"
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zmDhszhY_VzU&XQTZ-?{rM*fHUWCX0FprHewPCEUrCfzfaNa1de`8343C?jYo*JzGa zM3JiGV`3_@;2#pJ1jSbnf>M$E3x_5UmRu4CB)IA;RA_(mXJh0r6Y0l*>gH zh-~SL9||5~FxjQ@Ug< zN=-rVcZV8@U?QI6EsA1t3J?+WTw9|#v{by@6f(j@A0PBN> z|9YK&*Z=?>aXZ_Ov3Az~?qP50r1vlX{|V4?%fChcaWE+~0D$ygtv^1`A w4YghKAE5s2g#0JwKPUQsV@}on2h4v=du2J84^sd2Cj<}R{TQFQx_|Bc9~5O2` - + :ref:`Impedance Computation ` + .. grid-item-card:: :padding: 2 - :ref:`Impedance Computation ` - + :ref:`Interactive EIS parameter exploration ` + + .. grid-item-card:: + :padding: 2 + + :ref:`ECM simulation ` + .. grid-item-card:: :padding: 2 diff --git a/Documentation/nblinks/runImpedanceExplorer.nblink b/Documentation/nblinks/runImpedanceExplorer.nblink new file mode 100644 index 000000000..f9d7b6851 --- /dev/null +++ b/Documentation/nblinks/runImpedanceExplorer.nblink @@ -0,0 +1,3 @@ +{ + "path" : "../../Battery/EquivalentCircuitModel/examples/pxdParamsImpact/notebooks/runImpedanceExplorer.ipynb" +} From 7714c3c671a518345c82979438f9948923feaa55 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:10:05 +0200 Subject: [PATCH 113/119] renamed files --- Documentation/{ecm.rst => equivalentcircuitemodels.rst} | 0 1 file changed, 0 insertions(+), 0 deletions(-) rename Documentation/{ecm.rst => equivalentcircuitemodels.rst} (100%) diff --git a/Documentation/ecm.rst b/Documentation/equivalentcircuitemodels.rst similarity index 100% rename from Documentation/ecm.rst rename to Documentation/equivalentcircuitemodels.rst From baf15c6d1c44ecdbd358a2ba2f13288c3b0e0617 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:10:52 +0200 Subject: [PATCH 114/119] update in doc index --- Documentation/equivalentcircuitemodels.rst | 4 ++-- Documentation/index.rst | 2 +- 2 files changed, 3 insertions(+), 3 deletions(-) diff --git a/Documentation/equivalentcircuitemodels.rst b/Documentation/equivalentcircuitemodels.rst index b7177151b..6c65bc437 100644 --- a/Documentation/equivalentcircuitemodels.rst +++ b/Documentation/equivalentcircuitemodels.rst @@ -129,8 +129,8 @@ charge-transfer resistance, and low frequencies reflect mass transport and diffusion processes, providing insight into the migration rate of lithium ions through the solid electrode particles. -Scripts -======= +Notebooks +========= .. toctree:: :hidden: diff --git a/Documentation/index.rst b/Documentation/index.rst index 0ac3b787d..34248ebdb 100644 --- a/Documentation/index.rst +++ b/Documentation/index.rst @@ -13,7 +13,7 @@ output geometryinput batteryphysics - ecm + equivalentcircuitmodels elchemsystems optimisation modeling From 07417703a34a381134fc6bc56894a3e9c6625377 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:34:46 +0200 Subject: [PATCH 115/119] added missing semi-columns --- .../calibration/runCalibrateEcmFromP2D.m | 13 ++++++------- 1 file changed, 6 insertions(+), 7 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m index b6c408502..04b879124 100644 --- a/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m +++ b/Battery/EquivalentCircuitModel/calibration/runCalibrateEcmFromP2D.m @@ -6,7 +6,6 @@ %% % The results of the calibration is given in a struct where the fields are functions in battmo table format - jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json')); jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json')); @@ -24,42 +23,42 @@ nexttile % the function |setupFunction| creates a function handle from the battmo function input format. -fn = setupFunction(jsonstruct.OCP) +fn = setupFunction(jsonstruct.OCP); plot(soc, fn(soc)) title('OCP') xlabel('SOC / -') ylabel('OCP / V'); nexttile -fn = setupFunction(jsonstruct.R0) +fn = setupFunction(jsonstruct.R0); plot(soc, fn(soc)) title('R0') xlabel('SOC / -') ylabel('R0 / Ohm'); nexttile -fn = setupFunction(jsonstruct.R1) +fn = setupFunction(jsonstruct.R1); plot(soc, fn(soc)) title('R1') xlabel('SOC / -') ylabel('R1 / Ohm'); nexttile -fn = setupFunction(jsonstruct.C1) +fn = setupFunction(jsonstruct.C1); plot(soc, fn(soc)) title('C1') xlabel('SOC / -') ylabel('C1 / Ohm'); nexttile -fn = setupFunction(jsonstruct.R2) +fn = setupFunction(jsonstruct.R2); plot(soc, fn(soc)) title('R2') xlabel('SOC / -') ylabel('R2 / Ohm'); nexttile -fn = setupFunction(jsonstruct.C2) +fn = setupFunction(jsonstruct.C2); plot(soc, fn(soc)) title('C2') xlabel('SOC / -') From 3eaf0df71a55e3112e8cc7cb96950fd041d38d38 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:37:02 +0200 Subject: [PATCH 116/119] update in ecm --- .../notebooks/runCalibrateEcmFromP2D.ipynb | 269 ++++++++ .../notebooks/runCalibrateEcmFromP2D.mlx | Bin 0 -> 239850 bytes .../notebooks/runCalibration.ipynb | 606 ------------------ .../calibration/notebooks/runCalibration.mlx | Bin 464442 -> 0 bytes .../calibration/runCalibration.m | 170 ----- .../notebooks/runEquivalentCircuitModel.ipynb | 70 +- .../notebooks/runEquivalentCircuitModel.mlx | Bin 154523 -> 3471 bytes .../examples/runEquivalentCircuitModel.m | 4 + ...models.rst => equivalentcircuitmodels.rst} | 4 +- ...n.nblink => runCalibrateEcmFromP2D.nblink} | 2 +- 10 files changed, 302 insertions(+), 823 deletions(-) create mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.ipynb create mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.mlx delete mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb delete mode 100644 Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.mlx delete mode 100644 Battery/EquivalentCircuitModel/calibration/runCalibration.m rename Documentation/{equivalentcircuitemodels.rst => equivalentcircuitmodels.rst} (98%) rename Documentation/nblinks/{runCalibration.nblink => runCalibrateEcmFromP2D.nblink} (64%) diff --git a/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.ipynb b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.ipynb new file mode 100644 index 000000000..6ef30c31a --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.ipynb @@ -0,0 +1,269 @@ +{ + "cells": [ + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "# Calibrate ECM model from P2D model" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "soc_step = 0.5;" + ], + "outputs": [] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "The results of the calibration is given in a struct where the fields are functions in battmo table format\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 2, + "metadata": {}, + "source": [ + "jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json'));\n", + "jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json'));\n", + "\n", + "\n", + "jsonstruct_p2d = mergeStructs({jsonstruct_material, ...\n", + " jsonstruct_geometry});\n", + "\n", + "jsonstruct = calibrateEcmFromP2D(jsonstruct_p2d, soc_step);" + ], + "outputs": [ + { + "data": { + "text/plain": [ + "==================================================\n", + " EIS fitting for SOC = 1.00 (1/2)\n", + "==================================================\n", + " Measured Open Circuit Voltage (OCV): 3.8799 V\n", + "Linearization...\n", + "It: 0 | val: 2.621e+00 | ls-its: NaN | pgrad: 8.263e+03\n", + "It: 1 | val: 2.017e+00 | ls-its: 3 | pgrad: 7.736e+03\n", + "It: 2 | val: 1.700e+00 | ls-its: 1 | pgrad: 6.742e+03\n", + "It: 3 | val: 5.475e-01 | ls-its: 2 | pgrad: 3.835e+03\n", + "It: 4 | val: 5.228e-01 | ls-its: 2 | pgrad: 2.868e+03\n", + "It: 5 | val: 4.326e-01 | ls-its: 1 | pgrad: 2.808e+03\n", + "It: 6 | val: 4.081e-01 | ls-its: 1 | pgrad: 9.097e+02\n", + "It: 7 | val: 3.719e-01 | ls-its: 1 | pgrad: 8.472e+02\n", + "It: 8 | val: 2.844e-01 | ls-its: 1 | pgrad: 1.840e+03\n", + "It: 9 | val: 2.010e-01 | ls-its: 1 | pgrad: 3.173e+03\n", + "It: 10 | val: 1.568e-01 | ls-its: 1 | pgrad: 2.809e+03\n", + "It: 11 | val: 1.483e-01 | ls-its: 1 | pgrad: 9.534e+02\n", + "It: 12 | val: 1.470e-01 | ls-its: 1 | pgrad: 2.361e+02\n", + "It: 13 | val: 1.357e-01 | ls-its: 1 | pgrad: 2.783e+02\n", + "It: 14 | val: 1.303e-01 | ls-its: 1 | pgrad: 4.738e+02\n", + "It: 15 | val: 1.207e-01 | ls-its: 1 | pgrad: 7.659e+02\n", + "It: 16 | val: 1.176e-01 | ls-its: 1 | pgrad: 2.781e+02\n", + "It: 17 | val: 1.167e-01 | ls-its: 1 | pgrad: 1.482e+02\n", + "It: 18 | val: 1.156e-01 | ls-its: 1 | pgrad: 9.965e+01\n", + "It: 19 | val: 1.109e-01 | ls-its: 1 | pgrad: 9.822e+01\n", + "It: 20 | val: 1.031e-01 | ls-its: 1 | pgrad: 3.841e+02\n", + "It: 21 | val: 9.081e-02 | ls-its: 1 | pgrad: 5.495e+02\n", + "It: 22 | val: 7.771e-02 | ls-its: 1 | pgrad: 9.180e+02\n", + "It: 23 | val: 7.128e-02 | ls-its: 1 | pgrad: 7.882e+02\n", + "It: 24 | val: 6.887e-02 | ls-its: 1 | pgrad: 2.541e+02\n", + "It: 25 | val: 6.676e-02 | ls-its: 1 | pgrad: 1.989e+02\n", + "It: 26 | val: 6.323e-02 | ls-its: 1 | pgrad: 1.333e+02\n", + "It: 27 | val: 5.939e-02 | ls-its: 1 | pgrad: 1.583e+02\n", + "It: 28 | val: 5.452e-02 | ls-its: 1 | pgrad: 1.735e+02\n", + "It: 29 | val: 5.065e-02 | ls-its: 1 | pgrad: 6.160e+02\n", + "It: 30 | val: 4.898e-02 | ls-its: 1 | pgrad: 1.243e+02\n", + "It: 31 | val: 4.787e-02 | ls-its: 1 | pgrad: 2.180e+02\n", + "It: 32 | val: 4.664e-02 | ls-its: 1 | pgrad: 1.587e+02\n", + "It: 33 | val: 4.598e-02 | ls-its: 1 | pgrad: 8.902e+01\n", + "It: 34 | val: 4.512e-02 | ls-its: 1 | pgrad: 5.662e+01\n", + "It: 35 | val: 4.467e-02 | ls-its: 1 | pgrad: 6.442e+01\n", + "It: 36 | val: 4.361e-02 | ls-its: 1 | pgrad: 3.138e+02\n", + "It: 37 | val: 4.331e-02 | ls-its: 1 | pgrad: 6.196e+01\n", + "It: 38 | val: 4.301e-02 | ls-its: 1 | pgrad: 4.959e+01\n", + "It: 39 | val: 4.299e-02 | ls-its: 2 | pgrad: 5.398e+01\n", + "It: 40 | val: 4.293e-02 | ls-its: 1 | pgrad: 3.661e+01\n", + "It: 41 | val: 4.290e-02 | ls-its: 1 | pgrad: 1.407e+01\n", + "It: 42 | val: 4.287e-02 | ls-its: 1 | pgrad: 8.715e+00\n", + "It: 43 | val: 4.286e-02 | ls-its: 2 | pgrad: 8.915e+00\n", + "It: 44 | val: 4.285e-02 | ls-its: 1 | pgrad: 2.261e+01\n", + "It: 45 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.222e+01\n", + "It: 46 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.236e+01\n", + "It: 47 | val: 4.284e-02 | ls-its: 1 | pgrad: 9.632e+00\n", + "It: 48 | val: 4.284e-02 | ls-its: 1 | pgrad: 4.082e+00\n", + "It: 49 | val: 4.284e-02 | ls-its: 1 | pgrad: 2.898e+00\n", + "It: 50 | val: 4.284e-02 | ls-its: 1 | pgrad: 6.594e+00\n", + "It: 51 | val: 4.284e-02 | ls-its: 1 | pgrad: 4.076e+00\n", + "It: 52 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.116e+00\n", + "It: 53 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.790e+00\n", + "It: 54 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.499e+00\n", + "It: 55 | val: 4.284e-02 | ls-its: 1 | pgrad: 2.878e-01\n", + "It: 56 | val: 4.284e-02 | ls-its: 1 | pgrad: 6.808e-02\n", + "It: 57 | val: 4.284e-02 | ls-its: 1 | pgrad: 7.552e-02\n", + "It: 58 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.240e-01\n", + "It: 59 | val: 4.284e-02 | ls-its: 1 | pgrad: 9.468e-02\n", + "It: 60 | val: 4.284e-02 | ls-its: 1 | pgrad: 5.519e-02\n", + "It: 61 | val: 4.284e-02 | ls-its: 1 | pgrad: 7.811e-03\n", + "It: 62 | val: 4.284e-02 | ls-its: 1 | pgrad: 2.609e-03\n", + "It: 63 | val: 4.284e-02 | ls-its: 1 | pgrad: 1.549e-03\n", + "It: 64 | val: 4.284e-02 | ls-its: 2 | pgrad: 1.176e-03\n", + "It: 65 | val: 4.284e-02 | ls-its: 1 | pgrad: 5.081e-04\n", + "It: 66 | val: 4.284e-02 | ls-its: 2 | pgrad: 5.620e-04\n", + "It: 67 | val: 4.284e-02 | ls-its: 1 | pgrad: 5.226e-04\n", + "It: 68 | val: 4.284e-02 | ls-its: 1 | pgrad: 2.083e-04\n", + "It: 69 | val: 4.284e-02 | ls-its: 1 | pgrad: 4.363e-05" + ] + }, + "metadata": {}, + "execution_count": 2, + "output_type": "execute_result" + }, + { + "data": { + "text/html": [ + "
    \"figure_0.png\"
    " + ] + }, + "metadata": {}, + "output_type": "display_data" + }, + { + "data": { + "text/plain": [ +] + }, + "metadata": {}, + "output_type": "display_data" + }, + { + "data": { + "text/html": [ + "
    \"figure_1.png\"
    " + ] + }, + "metadata": {}, + "output_type": "display_data" + }, + { + "data": { + "text/plain": [ + "Stopped because reached objChangeTol = 1.000000e-15.\n", + " SOC R0 R1 C1 R2 C2 \n", + " ___ ________ ______ _____ ________ ______\n", + " 0.5 0.032452 6.0577 36206 0.0144 3597.1\n", + " 1 0.045339 13.785 24495 0.018915 3215.2\n", + "jsonstruct_ecm structure saved successfully in: jsonstruct_ecm_calibrated_50.mat" + ] + }, + "metadata": {}, + "output_type": "display_data" + } + ] + }, + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "\n", + "plot the results\n", + "" + ] + }, + { + "cell_type": "code", + "execution_count": 3, + "metadata": {}, + "source": [ + "soc = linspace(0.1, 1.0, 100);\n", + "figure\n", + "tiledlayout(2, 3, 'tileindexing', 'columnmajor');\n", + "\n", + "\n", + "nexttile\n", + "\n", + "\n", + "% the function |setupFunction| creates a function handle from the battmo function input format.\n", + "fn = setupFunction(jsonstruct.OCP);\n", + "plot(soc, fn(soc))\n", + "title('OCP')\n", + "xlabel('SOC / -')\n", + "ylabel('OCP / V');\n", + "\n", + "\n", + "nexttile\n", + "fn = setupFunction(jsonstruct.R0);\n", + "plot(soc, fn(soc))\n", + "title('R0')\n", + "xlabel('SOC / -')\n", + "ylabel('R0 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "fn = setupFunction(jsonstruct.R1);\n", + "plot(soc, fn(soc))\n", + "title('R1')\n", + "xlabel('SOC / -')\n", + "ylabel('R1 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "fn = setupFunction(jsonstruct.C1);\n", + "plot(soc, fn(soc))\n", + "title('C1')\n", + "xlabel('SOC / -')\n", + "ylabel('C1 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "fn = setupFunction(jsonstruct.R2);\n", + "plot(soc, fn(soc))\n", + "title('R2')\n", + "xlabel('SOC / -')\n", + "ylabel('R2 / Ohm');\n", + "\n", + "\n", + "nexttile\n", + "fn = setupFunction(jsonstruct.C2);\n", + "plot(soc, fn(soc))\n", + "title('C2')\n", + "xlabel('SOC / -')\n", + "ylabel('C2 / Ohm');" + ], + "outputs": [ + { + "data": { + "text/html": [ + "
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i`oEbe`TvFak8ZD_jE4S~<+G>#^;7#~6g+hp!2bgtpvcYu literal 0 HcmV?d00001 diff --git a/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb b/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb deleted file mode 100644 index f71d7b052..000000000 --- a/Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb +++ /dev/null @@ -1,606 +0,0 @@ -{ - "cells": [ - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "# ECM Fitting for lithium\\-ion batteries\n", - "\n", - "## Impedance computation\n", - "\n", - "We setup a P2D model and compute the impedance response\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 1, - "metadata": {}, - "source": [ - "jsonstruct_material = parseBattmoJson(fullfile('ParameterData','ParameterSets','Chen2020','chen2020_lithium_ion_battery.json'));\n", - "jsonstruct_geometry = parseBattmoJson(fullfile('Examples', 'JsonDataFiles', 'geometryChen.json'));\n", - "jsonstruct_base = mergeJsonStructs({jsonstruct_material, jsonstruct_geometry});\n", - "\n", - "jsonstruct_base.NegativeElectrode.Coating.ActiveMaterial.Interface.useDoubleLayerCapacity = true;\n", - "\n", - "c_ne = 29.866*mol/litre;\n", - "c_pe = 17.038*mol/litre;\n", - "\n", - "p_diffusion = 0;\n", - "p_reactionRate = 0;\n", - "p_doubleLayerCapacitance = 0;\n", - "base_diff_anode = 1.3135e-15;\n", - "base_rate_anode = 5.031e-11;\n", - "base_cdl = 0.2;\n", - "\n", - "val_diff_anode = base_diff_anode * (10^p_diffusion);\n", - "val_rate_anode = base_rate_anode * (10^p_reactionRate);\n", - "val_cdl = base_cdl * (10^p_doubleLayerCapacitance);\n", - "\n", - "jsonstruct = jsonstruct_base;\n", - "\n", - "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode;\n", - "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode;\n", - "jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl;" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "Setup P2D model from the parameter set jsonstruct\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 2, - "metadata": {}, - "source": [ - "[model, inputparams, ~] = setupModelFromJson(jsonstruct);" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "We use a dedicated function to compute the initial state for the given electrode concentrations.\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 3, - "metadata": {}, - "source": [ - "initstate = initStateChen2020(model, c_ne, c_pe);\n", - "options = [];\n", - "options.stateInitialization.initializationSetup = 'given state';\n", - "options.stateInitialization.computeSteadyState = false;" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "setup input for ImpedanceSolver\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 4, - "metadata": {}, - "source": [ - "extrastructs = [];\n", - "extrastructs.initstate = initstate;" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "setup impedance solver and compute the Impedance for a given set of frequencies\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 5, - "metadata": {}, - "source": [ - "impsolv = ImpedanceSolver(inputparams, options, extrastructs);\n", - "frequencies = logspace(-2, 3, 30);\n", - "\n", - "Z = impsolv.computeImpedance(frequencies);\n", - "\n", - "figure('Name', 'Nyquist Diagram');\n", - "plot(real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD');\n", - "grid on;\n", - "xlabel('Re(Z)');\n", - "ylabel('-Im(Z)');\n", - "title('Interactive Nyquist Diagram');" - ], - "outputs": [ - { - "data": { - "text/html": [ - "

    \"figure_0.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 5, - "output_type": "execute_result" - } - ] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "The impact of diffusion is mainly seen on the tail at low frequencies. While a larger coefficient does not have much of an impact, using a very small one shows how strongly the diffusion phenomenon is linked to this tail.\n", - "\n", - "\n", - "The double\\-layer capacitance affects the first semicircle, as the frequency at its peak is governed by the relation $f_{\\max } =\\frac{1\\;}{2\\pi R_{\\textrm{CT}} C_{\\textrm{DL}} }$ . A large capacitance will result in a lower $f_{\\max }$ (a shift to the left, as frequencies are plotted inversely), while a small one will shift the center of the first semicircle to the right.\n", - "\n", - "\n", - "Finally, the influence of the reaction rate on the Nyquist diagram is clearly evident. A more facile reaction (i.e., a higher reaction rate) leads to a lower charge\\-transfer resistance. As this parameter dictates the width of the first semicircle, it virtually vanishes at high reaction rates and broadens considerably at lower ones.\n", - "\n", - "## Calibration of ECM parameters\n", - "\n", - "Impedance is the opposition to alternating current presented by the combined effect of resistance and reactance in a circuit. It is obtained with the ratio of complex voltage and complex current : $Z=U/I$ . It extends the concept of resistance to alternating current (AC) circuits.\n", - "\n", - "\n", - "We tried through our optimization algorithm to fit different battery models to ECM through five parameters, $R_0$ , $R_1$ , $C_1$ , $R_2$ and $C_2$ . The aim of the study is to obtain the set of parameters as close as possible to the real impedance curve with the 2\\-RC Impedance function $Z=R_0 +\\frac{R_1 }{1+jR_1 C_1 \\omega }+\\frac{R_2 }{1+jR_2 C_2 \\omega }$ .\n", - "\n", - "## Calibration using pertubed initial data\n", - "\n", - "We compute the impedance response of the ECM model for a given set of parameters and use it as an input in our calibration algorithm. We choose a initial guess for the parameters that is perturbed from the true values. The optimization algorithm should be able to recover the true parameters.\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 6, - "metadata": {}, - "source": [ - "omega = logspace(-4, 2, 50);\n", - "params = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0];\n", - "[Z_re_exp, Z_im_exp] = load_nyquist(params, omega);\n", - "\n", - "params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2\n", - "\n", - "a = 1000;\n", - "\n", - "pmin = params0 / a;\n", - "pmax = params0 * a;\n", - "scales = [pmin, pmax];\n", - "\n", - "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", - "\n", - "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" - ], - "outputs": [ - { - "data": { - "text/plain": [ - "It: 0 | val: 1.373e-31 | ls-its: NaN | pgrad: 1.164e-12\n", - "It: 1 | val: 1.373e-31 | ls-its: 0 | pgrad: 1.152e-12\n", - "Stopped because reached gradTol = 1.000000e-05." - ] - }, - "metadata": {}, - "execution_count": 6, - "output_type": "execute_result" - }, - { - "data": { - "text/html": [ - "
    \"figure_1.png\"
    " - ] - }, - "metadata": {}, - "output_type": "display_data" - } - ] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "plot the results\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 7, - "metadata": {}, - "source": [ - "feis.plotresults_thevenin(best_params, fitting_error);" - ], - "outputs": [ - { - "data": { - "text/html": [ - "
    \"figure_2.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 7, - "output_type": "execute_result" - } - ] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "## Calibration from experimental data\n", - "\n", - "We use data from the Ank's paper ([http://dx.doi.org/10.1149/1945\\-7111/ad14d0](http://dx.doi.org/10.1149/1945-7111/ad14d0)) to calibrate the ECM parameters.\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 8, - "metadata": {}, - "source": [ - "filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv');\n", - "data = readmatrix(filename);\n", - "\n", - "omega = data(:, 1);\n", - "Z_re_exp = data(:, 2);\n", - "Z_im_exp = data(:, 3);" - ], - "outputs": [] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "\n", - "We choose the following Initial guess\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 9, - "metadata": {}, - "source": [ - "params0 = [3.84e-03,...\n", - " 2.71e-03,...\n", - " 6.00e+03,...\n", - " 9.48e-04,...\n", - "1.11e+01]; % initial condition: C1>2*C2\n", - "\n", - "a = 1000;\n", - "\n", - "pmin = params0 / a;\n", - "pmax = params0 * a;\n", - "scales = [pmin, pmax];\n", - "\n", - "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", - "\n", - "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" - ], - "outputs": [ - { - "data": { - "text/plain": [ - "It: 0 | val: 3.717e-01 | ls-its: NaN | pgrad: 1.563e+02\n", - "It: 1 | val: 3.716e-01 | ls-its: 3 | pgrad: 1.561e+02\n", - "It: 2 | val: 1.870e-01 | ls-its: 8 | pgrad: 1.549e+02\n", - "It: 3 | val: 1.827e-01 | ls-its: 3 | pgrad: 1.616e+03\n", - "It: 4 | val: 1.596e-01 | ls-its: 2 | pgrad: 1.673e+03\n", - "It: 5 | val: 1.419e-01 | ls-its: 2 | pgrad: 4.695e+02\n", - "It: 6 | val: 8.869e-02 | ls-its: 1 | pgrad: 1.096e+03\n", - "It: 7 | val: 6.885e-02 | ls-its: 1 | pgrad: 2.369e+02\n", - "It: 8 | val: 6.869e-02 | ls-its: 1 | pgrad: 1.020e+02\n", - "It: 9 | val: 6.869e-02 | ls-its: 1 | pgrad: 1.253e+01\n", - "It: 10 | val: 6.866e-02 | ls-its: 2 | pgrad: 6.159e+00\n", - "It: 11 | val: 6.864e-02 | ls-its: 1 | pgrad: 3.511e+01\n", - "It: 12 | val: 6.862e-02 | ls-its: 1 | pgrad: 2.040e+01\n", - "It: 13 | val: 6.862e-02 | ls-its: 2 | pgrad: 1.882e+01\n", - "It: 14 | val: 6.862e-02 | ls-its: 1 | pgrad: 3.677e+00\n", - "It: 15 | val: 6.861e-02 | ls-its: 2 | pgrad: 2.463e+00\n", - "It: 16 | val: 6.860e-02 | ls-its: 1 | pgrad: 1.650e+01\n", - "It: 17 | val: 6.860e-02 | ls-its: 1 | pgrad: 5.232e+00\n", - "It: 18 | val: 6.860e-02 | ls-its: 1 | pgrad: 7.828e-01\n", - "It: 19 | val: 6.860e-02 | ls-its: 2 | pgrad: 6.014e-03\n", - "It: 20 | val: 6.860e-02 | ls-its: 1 | pgrad: 8.585e-03\n", - "It: 21 | val: 6.860e-02 | ls-its: 1 | pgrad: 1.911e-03\n", - "It: 22 | val: 6.860e-02 | ls-its: 1 | pgrad: 4.279e-04\n", - "It: 23 | val: 6.860e-02 | ls-its: 1 | pgrad: 2.402e-04\n", - "Stopped because reached objChangeTol = 1.000000e-15." - ] - }, - "metadata": {}, - "execution_count": 9, - "output_type": "execute_result" - }, - { - "data": { - "text/html": [ - "
    \"figure_3.png\"
    " - ] - }, - "metadata": {}, - "output_type": "display_data" - } - ] - }, - { - "cell_type": "code", - "execution_count": 10, - "metadata": {}, - "source": [ - "\n", - "feis.plotresults_thevenin(best_params, fitting_error);" - ], - "outputs": [ - { - "data": { - "text/html": [ - "
    \"figure_4.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 10, - "output_type": "execute_result" - } - ] - }, - { - "cell_type": "markdown", - "metadata": {}, - "source": [ - "## Synthetic data from P2D model\n", - "\n", - "We use impedance data generated from the P2d model with Chen et al's paper ([http://dx.doi.org/10.1149/1945\\-7111/ab9050](http://dx.doi.org/10.1149/1945-7111/ab9050)) parameters\n", - "" - ] - }, - { - "cell_type": "code", - "execution_count": 11, - "metadata": {}, - "source": [ - "[Z_re_exp, Z_im_exp, omega] = load_chen_data();\n", - "params0 = [0.05052, 1.12673, 59119.9, 0.03155, 11054.0]; % initial condition: C1>2*C2\n", - "\n", - "a = 1000;\n", - "\n", - "pmin = params0 / a;\n", - "pmax = params0 * a;\n", - "scales = [pmin, pmax];\n", - "\n", - "feis = FittingEIS(params0, scales, Z_re_exp, Z_im_exp, omega);\n", - "\n", - "[~, ~, best_params, fitting_error] = feis.optimizationBFGS();" - ], - "outputs": [ - { - "data": { - "text/plain": [ - "It: 0 | val: 5.457e+01 | ls-its: NaN | pgrad: 1.427e+05\n", - "It: 1 | val: 3.954e+01 | ls-its: 1 | pgrad: 1.427e+05\n", - "It: 2 | val: 1.472e+01 | ls-its: 1 | pgrad: 1.126e+05\n", - "Line search at max step size, Wolfe conditions not satisfied for this step.\n", - "Hessian not updated during iteration 3.\n", - "It: 3 | val: 1.177e+01 | ls-its: 4 | pgrad: 1.395e+03\n", - "It: 4 | val: 5.389e+00 | ls-its: 1 | pgrad: 5.470e+04\n", - "It: 5 | val: 5.370e+00 | ls-its: 1 | pgrad: 8.495e+03\n", - "It: 6 | val: 5.190e+00 | ls-its: 1 | pgrad: 8.371e+03\n", - "It: 7 | val: 4.888e+00 | ls-its: 1 | pgrad: 7.419e+03\n", - "It: 8 | val: 4.229e+00 | ls-its: 1 | pgrad: 1.211e+04\n", - "It: 9 | val: 3.452e+00 | ls-its: 1 | pgrad: 1.707e+04\n", - "It: 10 | val: 2.949e+00 | ls-its: 1 | pgrad: 1.621e+04\n", - "It: 11 | val: 2.819e+00 | ls-its: 1 | pgrad: 8.393e+03\n", - "It: 12 | val: 2.810e+00 | ls-its: 1 | pgrad: 1.636e+03\n", - "It: 13 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.247e+02\n", - "It: 14 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", - "It: 15 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", - "It: 16 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", - "It: 17 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", - "It: 18 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.238e+02\n", - "It: 19 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.239e+02\n", - "It: 20 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.240e+02\n", - "It: 21 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.243e+02\n", - "It: 22 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.639e+02\n", - "It: 23 | val: 2.810e+00 | ls-its: 1 | pgrad: 2.656e+02\n", - "It: 24 | val: 2.809e+00 | ls-its: 1 | pgrad: 2.255e+02\n", - "It: 25 | val: 2.809e+00 | ls-its: 1 | pgrad: 2.258e+02\n", - "It: 26 | val: 2.808e+00 | ls-its: 1 | pgrad: 2.264e+02\n", - "It: 27 | val: 2.808e+00 | ls-its: 1 | pgrad: 3.858e+02\n", - "It: 28 | val: 2.807e+00 | ls-its: 1 | pgrad: 7.234e+02\n", - "It: 29 | val: 2.807e+00 | ls-its: 1 | pgrad: 9.166e+02\n", - "It: 30 | val: 2.806e+00 | ls-its: 1 | pgrad: 9.196e+02\n", - "It: 31 | val: 2.805e+00 | ls-its: 1 | pgrad: 8.062e+02\n", - "It: 32 | val: 2.804e+00 | ls-its: 1 | pgrad: 6.568e+02\n", - "It: 33 | val: 2.801e+00 | ls-its: 1 | pgrad: 2.552e+02\n", - "It: 34 | val: 2.798e+00 | ls-its: 1 | pgrad: 3.681e+02\n", - "It: 35 | val: 2.797e+00 | ls-its: 1 | pgrad: 1.040e+03\n", - "It: 36 | val: 2.795e+00 | ls-its: 1 | pgrad: 1.388e+03\n", - "It: 37 | val: 2.792e+00 | ls-its: 1 | pgrad: 1.385e+03\n", - "It: 38 | val: 2.790e+00 | ls-its: 1 | pgrad: 1.143e+03\n", - "It: 39 | val: 2.783e+00 | ls-its: 1 | pgrad: 8.273e+02\n", - "It: 40 | val: 2.775e+00 | ls-its: 1 | pgrad: 4.889e+02\n", - "It: 41 | val: 2.769e+00 | ls-its: 1 | pgrad: 1.078e+03\n", - "It: 42 | val: 2.767e+00 | ls-its: 1 | pgrad: 1.934e+03\n", - "It: 43 | val: 2.766e+00 | ls-its: 1 | pgrad: 2.103e+03\n", - "It: 44 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.942e+03\n", - "It: 45 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.817e+03\n", - "It: 46 | val: 2.766e+00 | ls-its: 1 | pgrad: 1.716e+03\n", - "It: 47 | val: 2.765e+00 | ls-its: 1 | pgrad: 1.541e+03\n", - "It: 48 | val: 2.765e+00 | ls-its: 1 | pgrad: 1.298e+03\n", - "It: 49 | val: 2.764e+00 | ls-its: 1 | pgrad: 1.016e+03\n", - "It: 50 | val: 2.763e+00 | ls-its: 1 | pgrad: 8.574e+02\n", - "It: 51 | val: 2.761e+00 | ls-its: 1 | pgrad: 9.486e+02\n", - "It: 52 | val: 2.759e+00 | ls-its: 1 | pgrad: 1.330e+03\n", - "It: 53 | val: 2.754e+00 | ls-its: 1 | pgrad: 1.585e+03\n", - "It: 54 | val: 2.750e+00 | ls-its: 1 | pgrad: 2.131e+03\n", - "It: 55 | val: 2.738e+00 | ls-its: 1 | pgrad: 2.181e+03\n", - "It: 56 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.461e+03\n", - "It: 57 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.015e+03\n", - "It: 58 | val: 2.737e+00 | ls-its: 1 | pgrad: 1.077e+03\n", - "It: 59 | val: 2.735e+00 | ls-its: 1 | pgrad: 1.083e+03\n", - "It: 60 | val: 2.726e+00 | ls-its: 1 | pgrad: 1.030e+03\n", - "It: 61 | val: 2.723e+00 | ls-its: 1 | pgrad: 1.042e+03\n", - "It: 62 | val: 2.722e+00 | ls-its: 2 | pgrad: 1.129e+03\n", - "It: 63 | val: 2.721e+00 | ls-its: 1 | pgrad: 1.343e+03\n", - "It: 64 | val: 2.711e+00 | ls-its: 1 | pgrad: 1.515e+03\n", - "It: 65 | val: 2.695e+00 | ls-its: 1 | pgrad: 2.287e+03\n", - "It: 66 | val: 2.658e+00 | ls-its: 1 | pgrad: 2.906e+03\n", - "It: 67 | val: 2.632e+00 | ls-its: 1 | pgrad: 3.567e+03\n", - "It: 68 | val: 2.619e+00 | ls-its: 1 | pgrad: 3.168e+03\n", - "It: 69 | val: 2.613e+00 | ls-its: 1 | pgrad: 2.037e+03\n", - "It: 70 | val: 2.612e+00 | ls-its: 1 | pgrad: 4.564e+02\n", - "It: 71 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.066e+02\n", - "It: 72 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.871e+02\n", - "It: 73 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.986e+02\n", - "It: 74 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.032e+02\n", - "It: 75 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.036e+02\n", - "It: 76 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.072e+02\n", - "It: 77 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.082e+02\n", - "It: 78 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.075e+02\n", - "It: 79 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.041e+02\n", - "It: 80 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.970e+02\n", - "It: 81 | val: 2.610e+00 | ls-its: 1 | pgrad: 1.846e+02\n", - "It: 82 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.225e+02\n", - "It: 83 | val: 2.610e+00 | ls-its: 1 | pgrad: 3.345e+02\n", - "It: 84 | val: 2.610e+00 | ls-its: 1 | pgrad: 4.148e+02\n", - "It: 85 | val: 2.610e+00 | ls-its: 1 | pgrad: 3.974e+02\n", - "It: 86 | val: 2.610e+00 | ls-its: 1 | pgrad: 2.938e+02\n", - "It: 87 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.080e+02\n", - "It: 88 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.614e+01\n", - "It: 89 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.761e+01\n", - "It: 90 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.107e+02\n", - "It: 91 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.801e+01\n", - "It: 92 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.900e+01\n", - "It: 93 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.731e+01\n", - "It: 94 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.538e+01\n", - "It: 95 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.371e+01\n", - "It: 96 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.189e+01\n", - "It: 97 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.062e+01\n", - "It: 98 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.754e+01\n", - "It: 99 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.235e+02\n", - "It: 100 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.047e+02\n", - "It: 101 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.272e+01\n", - "It: 102 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.581e+01\n", - "It: 103 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.677e+01\n", - "It: 104 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.742e+01\n", - "It: 105 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.749e+01\n", - "It: 106 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.786e+01\n", - "It: 107 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.867e+01\n", - "It: 108 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.923e+01\n", - "It: 109 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.918e+01\n", - "It: 110 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.860e+01\n", - "It: 111 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.515e+01\n", - "It: 112 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.549e+01\n", - "It: 113 | val: 2.609e+00 | ls-its: 1 | pgrad: 5.580e+01\n", - "It: 114 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.692e+01\n", - "It: 115 | val: 2.609e+00 | ls-its: 1 | pgrad: 4.067e+01\n", - "It: 116 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.227e+01\n", - "It: 117 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.115e+01\n", - "It: 118 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.161e+01\n", - "It: 119 | val: 2.609e+00 | ls-its: 1 | pgrad: 9.071e+00\n", - "It: 120 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.408e+01\n", - "It: 121 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.767e+01\n", - "It: 122 | val: 2.609e+00 | ls-its: 1 | pgrad: 2.603e+01\n", - "It: 123 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.029e+01\n", - "It: 124 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.346e+01\n", - "It: 125 | val: 2.609e+00 | ls-its: 1 | pgrad: 5.312e+00\n", - "It: 126 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.129e+01\n", - "It: 127 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.024e+01\n", - "It: 128 | val: 2.609e+00 | ls-its: 1 | pgrad: 3.011e+00\n", - "It: 129 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.153e-01\n", - "It: 130 | val: 2.609e+00 | ls-its: 1 | pgrad: 6.984e-01\n", - "It: 131 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.063e-01\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 132 | val: 2.609e+00 | ls-its: 1 | pgrad: 7.214e-01\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 133 | val: 2.609e+00 | ls-its: 2 | pgrad: 7.059e-01\n", - "It: 134 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.800e+00\n", - "It: 135 | val: 2.609e+00 | ls-its: 1 | pgrad: 1.232e+00\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 136 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.554e-01\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 137 | val: 2.609e+00 | ls-its: 2 | pgrad: 3.571e-01\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 138 | val: 2.609e+00 | ls-its: 2 | pgrad: 5.313e-02\n", - "Non-inceasing search direction, trying previous Hessian approximation.\n", - "It: 139 | val: 2.609e+00 | ls-its: 2 | pgrad: 1.891e-01\n", - "It: 140 | val: 2.609e+00 | ls-its: 0 | pgrad: 3.168e-02\n", - "Stopped because reached objChangeTol = 1.000000e-15." - ] - }, - "metadata": {}, - "execution_count": 11, - "output_type": "execute_result" - }, - { - "data": { - "text/html": [ - "
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-jsonstruct_base.NegativeElectrode.Coating.ActiveMaterial.Interface.useDoubleLayerCapacity = true; - -c_ne = 29.866*mol/litre; -c_pe = 17.038*mol/litre; - -p_diffusion = 0; -p_reactionRate = 0; -p_doubleLayerCapacitance = 0; -base_diff_anode = 1.3135e-15; -base_rate_anode = 5.031e-11; -base_cdl = 0.2; - -val_diff_anode = base_diff_anode * (10^p_diffusion); -val_rate_anode = base_rate_anode * (10^p_reactionRate); -val_cdl = base_cdl * (10^p_doubleLayerCapacitance); - -jsonstruct = jsonstruct_base; - -jsonstruct.NegativeElectrode.Coating.ActiveMaterial.SolidDiffusion.referenceDiffusionCoefficient = val_diff_anode; -jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.reactionRateConstant = val_rate_anode; -jsonstruct.NegativeElectrode.Coating.ActiveMaterial.Interface.doubleLayerCapacitance = val_cdl; - -%% -% Setup P2D model from the parameter set |jsonstruct| -[model, inputparams, ~] = setupModelFromJson(jsonstruct); - -%% -% We use a dedicated function to compute the initial state for the given electrode concentrations. -initstate = initStateChen2020(model, c_ne, c_pe); -options = []; -options.stateInitialization.initializationSetup = 'given state'; -options.stateInitialization.computeSteadyState = false; - -%% -% setup input for |ImpedanceSolver| -extrastructs = []; -extrastructs.initstate = initstate; - - -%% -% setup impedance solver and compute the Impedance for a given set of frequencies - -impsolv = ImpedanceSolver(inputparams, options, extrastructs); -frequencies = logspace(-2, 3, 30); - -Z = impsolv.computeImpedance(frequencies); - -figure('Name', 'Nyquist Diagram'); -plot(real(Z), -imag(Z), '-o', 'LineWidth', 2, 'Color', '#0072BD'); -grid on; -xlabel('Re(Z)'); -ylabel('-Im(Z)'); -title('Interactive Nyquist Diagram'); - - -%% -% -% The impact of diffusion is mainly seen on the tail at low frequencies. While -% a larger coefficient does not have much of an impact, using a very small one -% shows how strongly the diffusion phenomenon is linked to this tail. -% -% The double-layer capacitance affects the first semicircle, as the frequency -% at its peak is governed by the relation $f_{\max } =\frac{1\;}{2\pi R_{\textrm{CT}} -% C_{\textrm{DL}} }$. A large capacitance will result in a lower $f_{\max }$ (a -% shift to the left, as frequencies are plotted inversely), while a small one -% will shift the center of the first semicircle to the right. -% -% Finally, the influence of the reaction rate on the Nyquist diagram is clearly -% evident. A more facile reaction (i.e., a higher reaction rate) leads to a lower -% charge-transfer resistance. As this parameter dictates the width of the first -% semicircle, it virtually vanishes at high reaction rates and broadens considerably -% at lower ones. - - -%% Calibration of ECM parameters -% Impedance is the opposition to alternating current presented by the combined -% effect of resistance and reactance in a circuit. It is obtained with the ratio -% of complex voltage and complex current : $Z=U/I$ . It extends the concept of -% resistance to alternating current (AC) circuits. -% -% We tried through our optimization algorithm to fit different battery models -% to ECM through five parameters, $R_0$, $R_1$, $C_1$, $R_2$ and $C_2$. The aim -% of the study is to obtain the set of parameters as close as possible to the -% real impedance curve with the 2-RC Impedance function $Z = R_0 + \frac{R_1}{1 -% + j R_1 C_1 \omega} + \frac{R_2}{1 + j R_2 C_2 \omega}$. - -%% Calibration using pertubed initial data -% We compute the impedance response of the ECM model for a given set of parameters and use it as an input in our -% calibration algorithm. We choose a initial guess for the parameters that is perturbed from the true values. The -% optimization algorithm should be able to recover the true parameters. - - -%% -% fetch data -omega = logspace(-4, 2, 50); -[Z_re_exp, Z_im_exp] = load_nyquist(params, omega); - -eisdata = struct('omega', omega, ... - 'Z_re_exp', Z_re_exp, ... - 'Z_im_exp', Z_im_exp); - -%% -% Initial parameters for the calibration -params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; % initial condition: C1>2*C2 - -feis = FittingEIS(eisdata, params0); -[best_params, fitting_error] = feis.run(); - -%% -% plot the results - -feis.plotResults(best_params, fitting_error); - -%% Calibration from experimental data -% We use data from the Ank's paper (http://dx.doi.org/10.1149/1945-7111/ad14d0) to calibrate the ECM parameters. -% - -filename = fullfile(battmoDir(), 'Battery', 'EquivalentCircuitModel', 'calibration', 'utils', 'ank_data.csv'); -data = readmatrix(filename); - -eisdata.omega = data(:, 1); -eisdata.Z_re_exp = data(:, 2); -eisdata.Z_im_exp = data(:, 3); - -%% -% We choose the following Initial guess - -params0 = [3.84e-03; ... - 2.71e-03; ... - 6.00e+03; ... - 9.48e-04; ... - 1.11e+01]; % initial condition: C1>2*C2 - - -feis = FittingEIS(eisdata, params0); - -[best_params, fitting_error] = feis.run(); -feis.plotResults(best_params, fitting_error); -feis.printResults(best_params, fitting_error); - -%% Synthetic data from P2D model -% We use impedance data generated from the P2d model with Chen et al's paper -% (http://dx.doi.org/10.1149/1945-7111/ab9050) parameters - -%% -% fetch Chen data -[Z_re_exp, Z_im_exp, omega] = load_chen_data(); -eisdata = struct('omega', omega, ... - 'Z_re_exp', Z_re_exp, ... - 'Z_im_exp', Z_im_exp); - -%% -% initial parameters -params0 = [0.05052; 1.12673; 59119.9; 0.03155; 11054.0]; % initial condition: C1>2*C2 - -feis = FittingEIS(eisdata, params0); - -[best_params, fitting_error] = feis.run(); -feis.plotResults(best_params, fitting_error); -feis.printResults(best_params, fitting_error); diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb b/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb index 89e4bc2a0..a5edddc8d 100644 --- a/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb +++ b/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.ipynb @@ -1,12 +1,27 @@ { "cells": [ + { + "cell_type": "markdown", + "metadata": {}, + "source": [ + "# Time Simulation of an ECM model" + ] + }, + { + "cell_type": "code", + "execution_count": 1, + "metadata": {}, + "source": [ + "clear all" + ], + "outputs": [] + }, { "cell_type": "raw", "metadata": { "raw_mimetype": "text/restructuredtext" }, "source": [ - "# Time Simulation of an ECM model\n", "\n", "The function :battmo:`createParametersECM` setups an data set for the ECM model. The structure `jsonstruct` contains values of the ECM parameters (resistances, capicaties, ...) that depend on the frequency. See below for the plot of the values\n", "" @@ -14,7 +29,7 @@ }, { "cell_type": "code", - "execution_count": 1, + "execution_count": 2, "metadata": {}, "source": [ "jsonstruct = createParametersECM();" @@ -32,7 +47,7 @@ }, { "cell_type": "code", - "execution_count": 2, + "execution_count": 3, "metadata": {}, "source": [ "inputparams = EquivalentCircuitModelInputParams(jsonstruct);\n", @@ -51,7 +66,7 @@ }, { "cell_type": "code", - "execution_count": 3, + "execution_count": 4, "metadata": {}, "source": [ "soc = linspace(0, 1, 100);\n", @@ -102,18 +117,7 @@ "xlabel('SOC / -')\n", "ylabel('C2 / Ohm');" ], - "outputs": [ - { - "data": { - "text/html": [ - "

    \"figure_0.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 3, - "output_type": "execute_result" - } - ] + "outputs": [] }, { "cell_type": "markdown", @@ -126,7 +130,7 @@ }, { "cell_type": "code", - "execution_count": 4, + "execution_count": 5, "metadata": {}, "source": [ "figure\n", @@ -137,18 +141,7 @@ "xlabel('time / hour')\n", "ylabel('I / A');" ], - "outputs": [ - { - "data": { - "text/html": [ - "
    \"figure_1.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 4, - "output_type": "execute_result" - } - ] + "outputs": [] }, { "cell_type": "markdown", @@ -161,7 +154,7 @@ }, { "cell_type": "code", - "execution_count": 5, + "execution_count": 6, "metadata": {}, "source": [ "[t, U, I, SOC] = model.solve();" @@ -170,7 +163,7 @@ }, { "cell_type": "code", - "execution_count": 6, + "execution_count": 7, "metadata": {}, "source": [ "figure\n", @@ -191,19 +184,8 @@ "xlabel('Time / hour')\n", "ylabel('SOC / -');" ], - "outputs": [ - { - "data": { - "text/html": [ - "
    \"figure_2.png\"
    " - ] - }, - "metadata": {}, - "execution_count": 6, - "output_type": "execute_result" - } - ] - } + "outputs": [] +} ], "metadata": { "kernelspec": { diff --git a/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.mlx b/Battery/EquivalentCircuitModel/examples/notebooks/runEquivalentCircuitModel.mlx index 64f0e9452f8a589fabfddc6995939ceb00ea177d..55ed0a8c2bc6c21e794c1d04e46453930f3b6d1b 100644 GIT binary patch delta 1522 zcmVf#j5WVv&roLb#2OBC?6$wO< z+e#d&M3CeXMe1g~1V`&#cXu4ZzwfNE4M`lxA#Ek(kMZuCnfGSK=H&D#lkg~vO|=?( zgMQ?JP+TXex*vO2mp_iadZ&}l$!e5nUSvWc&<15ktFgC4%tv8p`BG%e_H`~4JzHp# zF@L06b04m>NphpPu$J&L84jc9OPH}#c@u)X)5+SM^YU}6VMn=@XMSFORx zgVk!|588CyPDR7(`?>d`+iIz&+Xj0j=w+**)w)X7H(;+C z*lR73-HU^;)w+5Bx5E@6aWAK2mk;8Appwr z&Jv#h000jG000pH003=abZlW_FK=~paCLMpcx`NLkIf3gFc5@aC4c0u(VK^DiXdKl zP#<75ODW{1B%5O1-qaq{;%(;}nAw5$>8zM2rXl!7?zcNB$UlM^eBa31^}IPqkr=%} z8$31A2Ps+&@6aWAK2mk;8Apn~H zRaqC86jcH!e?d=!Fc^mK`xQ;^&;oNI4X}e|CrwPmXuLJ$8*8McX{&7i-VO(Dx`W5& 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index 64% rename from Documentation/nblinks/runCalibration.nblink rename to Documentation/nblinks/runCalibrateEcmFromP2D.nblink index 5c0c6a5b5..429994434 100644 --- a/Documentation/nblinks/runCalibration.nblink +++ b/Documentation/nblinks/runCalibrateEcmFromP2D.nblink @@ -1,3 +1,3 @@ { - "path" : "../../Battery/EquivalentCircuitModel/calibration/notebooks/runCalibration.ipynb" + "path" : "../../Battery/EquivalentCircuitModel/calibration/notebooks/runCalibrateEcmFromP2D.ipynb" } From daca4707b08933c75c8d2e14d1310cda1945e70b Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 12:37:08 +0200 Subject: [PATCH 117/119] added ecm example in test suite --- Tests/TestExamples/TestRunExamples.m | 4 ++++ 1 file changed, 4 insertions(+) diff --git a/Tests/TestExamples/TestRunExamples.m b/Tests/TestExamples/TestRunExamples.m index be4d19c01..000f30331 100644 --- a/Tests/TestExamples/TestRunExamples.m +++ b/Tests/TestExamples/TestRunExamples.m @@ -32,6 +32,10 @@ 'runBatteryP3DMech' , ... 'runBattery1DOptimize' , ... 'runParameterIdentification' , ... + 'runImpedanceExplorer' , ... + 'runEquivalentCircuitModel' , ... + 'runFittingTime' , ... + 'runCalibrateEcmFromP2D' , ... 'runElectrolyser' , ... 'runConductorBlockExample' , ... 'runRegionBruggemanExample' , ... From 508626fe6f7bc6670c0628c148c08d08d968ae3b Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 13:42:38 +0200 Subject: [PATCH 118/119] fix in runImpedanceChen --- Examples/Advanced/Impedance/runImpedanceChen.m | 4 ++-- 1 file changed, 2 insertions(+), 2 deletions(-) diff --git a/Examples/Advanced/Impedance/runImpedanceChen.m b/Examples/Advanced/Impedance/runImpedanceChen.m index 52558925b..b73d4e106 100644 --- a/Examples/Advanced/Impedance/runImpedanceChen.m +++ b/Examples/Advanced/Impedance/runImpedanceChen.m @@ -22,7 +22,7 @@ jsonstruct = mergeStructs({jsonstruct_material, ... jsonstruct_geometry}); -includeDoubleLayer = true; +includeDoubleLayer = false; if includeDoubleLayer @@ -72,7 +72,7 @@ docompare = true; if docompare p = fileparts(mfilename('fullpath')); - data = load('C:\Users\Alexandre Fichter\Documents\stage_3A\contenu stage\matlab\BattMo\Examples\Advanced\Impedance\utils\pybamm_chen_impedances.mat'); + data = load(fullfile(p, 'utils', 'pybamm_chen_impedances.mat')); Zpybamm = data.impedances; plot(real(Zpybamm), -imag(Zpybamm), 'displayname', 'pybamm'); end From 1c7d693bbf33c8ad511199515d93ec0a21b4889d Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Tue, 25 Aug 2026 13:49:35 +0200 Subject: [PATCH 119/119] update in test suite --- Tests/TestExamples/TestRunExamples.m | 2 -- 1 file changed, 2 deletions(-) diff --git a/Tests/TestExamples/TestRunExamples.m b/Tests/TestExamples/TestRunExamples.m index 000f30331..835324a59 100644 --- a/Tests/TestExamples/TestRunExamples.m +++ b/Tests/TestExamples/TestRunExamples.m @@ -15,8 +15,6 @@ 'runChen2020' , ... 'runImpedanceChen' , ... 'runImpedanceScript' , ... - 'exampleECM' , ... - 'runClassFitting' , ... 'runCR' , ... 'runGittTest' , ... 'runJellyRoll' , ...

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.../notebooks/{Notebook.mlx => calibrationECM.mlx} | Bin 1 file changed, 0 insertions(+), 0 deletions(-) rename Battery/EquivalentCircuitModel/notebooks/{Notebook.mlx => calibrationECM.mlx} (100%) diff --git a/Battery/EquivalentCircuitModel/notebooks/Notebook.mlx b/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/notebooks/Notebook.mlx rename to Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx From 0d9e75851f5552d7f41362f4bf6e8e274bc3f27a Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:19:22 +0200 Subject: [PATCH 049/119] update --- .../FittingEIS.m | 0 .../calibration/costFunctionEIS.m | 15 + .../plotting}/plot_nyquist_ank.m | 0 .../plotting}/plot_nyquist_params.m | 0 .../activationEnergyOfReaction_impact.m | 0 .../pxdparams_impact/bruggeman_impact.m | 0 .../doubleLayerCapacitance_impact.m | 0 .../electronicConductivity_impact.m | 0 .../pxdparams_impact/param_dependency.m | 0 .../pxdparams_impact/porosity_impact.m | 0 .../reactionRateConstant_impact.m | 0 .../referenceDiffusionCoefficient_impact.m | 0 .../saturationConcentration_impact.m | 0 .../pxdparams_impact/volumefraction_impact.m | 0 .../volumetricSurfaceArea_impact.m | 0 .../runClassFitting.m} | 0 .../runFittingEIS.m} | 0 .../utils}/load_chen_data.m | 0 .../utils}/load_experimental_data.m | 0 .../utils}/load_nyquist.m | 0 .../utils}/load_santoni_data.m | 0 .../{ => examples}/exampleECM.m | 0 .../notebooks/calibrationECM.mlx | Bin .../{ => examples}/notebooks/exampleECM.ipynb | 0 .../{ => examples}/notebooks/exampleECM.mlx | Bin .../{ => examples}/run_fitting.m | 0 .../{ => models}/EquivalentCircuitModel.m | 0 .../EquivalentCircuitModelInputParams.m | 0 .../spectral_analysis/LimitedMemoryHessian.m | 217 ------- .../spectral_analysis/argmaxCubic.m | 66 -- .../spectral_analysis/cost_function_eis.m | 14 - .../spectral_analysis/lineSearch.m | 147 ----- .../spectral_analysis/unitBoxBFGS.m | 578 ------------------ .../costFunctionECM.m} | 4 +- .../createParametersECM.m} | 0 .../plotExperience.m} | 0 36 files changed, 16 insertions(+), 1025 deletions(-) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/FittingEIS.m (100%) create mode 100644 Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/plotting}/plot_nyquist_ank.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/plotting}/plot_nyquist_params.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/activationEnergyOfReaction_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/bruggeman_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/doubleLayerCapacitance_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/electronicConductivity_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/param_dependency.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/porosity_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/reactionRateConstant_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/referenceDiffusionCoefficient_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/saturationConcentration_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/volumefraction_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration}/pxdparams_impact/volumetricSurfaceArea_impact.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis/runclassfitting.m => calibration/runClassFitting.m} (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis/run_fitting_eis.m => calibration/runFittingEIS.m} (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/utils}/load_chen_data.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/utils}/load_experimental_data.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/utils}/load_nyquist.m (100%) rename Battery/EquivalentCircuitModel/{spectral_analysis => calibration/utils}/load_santoni_data.m (100%) rename Battery/EquivalentCircuitModel/{ => examples}/exampleECM.m (100%) rename Battery/EquivalentCircuitModel/{ => examples}/notebooks/calibrationECM.mlx (100%) rename Battery/EquivalentCircuitModel/{ => examples}/notebooks/exampleECM.ipynb (100%) rename Battery/EquivalentCircuitModel/{ => examples}/notebooks/exampleECM.mlx (100%) rename Battery/EquivalentCircuitModel/{ => examples}/run_fitting.m (100%) rename Battery/EquivalentCircuitModel/{ => models}/EquivalentCircuitModel.m (100%) rename Battery/EquivalentCircuitModel/{ => models}/EquivalentCircuitModelInputParams.m (100%) delete mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m delete mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m delete mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m delete mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m delete mode 100644 Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m rename Battery/EquivalentCircuitModel/{cost_function.m => utils/costFunctionECM.m} (99%) rename Battery/EquivalentCircuitModel/{create_parameters.m => utils/createParametersECM.m} (100%) rename Battery/EquivalentCircuitModel/{plotexperience.m => utils/plotExperience.m} (100%) diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m b/Battery/EquivalentCircuitModel/calibration/FittingEIS.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/FittingEIS.m rename to Battery/EquivalentCircuitModel/calibration/FittingEIS.m diff --git a/Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m b/Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m new file mode 100644 index 000000000..28a284906 --- /dev/null +++ b/Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m @@ -0,0 +1,15 @@ +function [total_error, Z_re_exp, Z_im_exp] = costFunctionEIS(best_params) + + + Z_re_exp = plot_nyquist_ank.Z_real; + Z_im_exp = plot_nyquist_ank.Z_imag; + + + omega = logspace(-2, 4, 100) + + Z_re_params = plot_nyquist_params.Z_real(best_params); + Z_im_params = plot_nyquist_params.Z_imag(best_params); + + totalerror = sum((Z_re_exp(omega)-Z_re_params(omega)).^2) + sum((Z_im_exp(omega)-Z_im_params(omega))^2) + +end diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m b/Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_ank.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_ank.m rename to Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_ank.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m b/Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_params.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/plot_nyquist_params.m rename to Battery/EquivalentCircuitModel/calibration/plotting/plot_nyquist_params.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/activationEnergyOfReaction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/activationEnergyOfReaction_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/activationEnergyOfReaction_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/bruggeman_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/bruggeman_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/bruggeman_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/doubleLayerCapacitance_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/doubleLayerCapacitance_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/doubleLayerCapacitance_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/electronicConductivity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/electronicConductivity_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/electronicConductivity_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/param_dependency.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/param_dependency.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/param_dependency.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/porosity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/porosity_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/porosity_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/reactionRateConstant_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/reactionRateConstant_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/reactionRateConstant_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/referenceDiffusionCoefficient_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/referenceDiffusionCoefficient_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/referenceDiffusionCoefficient_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/saturationConcentration_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/saturationConcentration_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/saturationConcentration_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumefraction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumefraction_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumefraction_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumetricSurfaceArea_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/pxdparams_impact/volumetricSurfaceArea_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumetricSurfaceArea_impact.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m b/Battery/EquivalentCircuitModel/calibration/runClassFitting.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/runclassfitting.m rename to Battery/EquivalentCircuitModel/calibration/runClassFitting.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m b/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/run_fitting_eis.m rename to Battery/EquivalentCircuitModel/calibration/runFittingEIS.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/load_chen_data.m rename to Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_experimental_data.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/load_experimental_data.m rename to Battery/EquivalentCircuitModel/calibration/utils/load_experimental_data.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m b/Battery/EquivalentCircuitModel/calibration/utils/load_nyquist.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/load_nyquist.m rename to Battery/EquivalentCircuitModel/calibration/utils/load_nyquist.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_santoni_data.m similarity index 100% rename from Battery/EquivalentCircuitModel/spectral_analysis/load_santoni_data.m rename to Battery/EquivalentCircuitModel/calibration/utils/load_santoni_data.m diff --git a/Battery/EquivalentCircuitModel/exampleECM.m b/Battery/EquivalentCircuitModel/examples/exampleECM.m similarity index 100% rename from Battery/EquivalentCircuitModel/exampleECM.m rename to Battery/EquivalentCircuitModel/examples/exampleECM.m diff --git a/Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx b/Battery/EquivalentCircuitModel/examples/notebooks/calibrationECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/notebooks/calibrationECM.mlx rename to Battery/EquivalentCircuitModel/examples/notebooks/calibrationECM.mlx diff --git a/Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb b/Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.ipynb similarity index 100% rename from Battery/EquivalentCircuitModel/notebooks/exampleECM.ipynb rename to Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.ipynb diff --git a/Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx b/Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.mlx similarity index 100% rename from Battery/EquivalentCircuitModel/notebooks/exampleECM.mlx rename to Battery/EquivalentCircuitModel/examples/notebooks/exampleECM.mlx diff --git a/Battery/EquivalentCircuitModel/run_fitting.m b/Battery/EquivalentCircuitModel/examples/run_fitting.m similarity index 100% rename from Battery/EquivalentCircuitModel/run_fitting.m rename to Battery/EquivalentCircuitModel/examples/run_fitting.m diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m similarity index 100% rename from Battery/EquivalentCircuitModel/EquivalentCircuitModel.m rename to Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m diff --git a/Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModelInputParams.m similarity index 100% rename from Battery/EquivalentCircuitModel/EquivalentCircuitModelInputParams.m rename to Battery/EquivalentCircuitModel/models/EquivalentCircuitModelInputParams.m diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m b/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m deleted file mode 100644 index b181be464..000000000 --- a/Battery/EquivalentCircuitModel/spectral_analysis/LimitedMemoryHessian.m +++ /dev/null @@ -1,217 +0,0 @@ -classdef LimitedMemoryHessian -% LimitedMemoryHessian: simple implementation of limited memory -% approxiamtion of invere Hessian (for use in L-BFGS) -% see: unitBoxBFGS (option limitedMemory) -properties - initScale % scaling for H0 (defualt 1) - initStrategy % 'static' : H0k = H0 (default) - % 'dynamic': H0k = gamma_k*I - nullspace = []; % nullspace of active subspace -end -properties (SetAccess = private) - m % number of vectors stored (default 5) - S = []; % m recent control/param diffs - Y = []; % m recent gradient diffs - itCount = 0; % update iteration count - sign % sign of Hessian(default 1) -end - -methods - function H = LimitedMemoryHessian(varargin) - opt = struct('initScale', 1, ... - 'initStrategy', 'static', ... - 'm', 5, ... - 'sign', 1); - opt = merge_options(opt, varargin{:}); - fn = fieldnames(opt); - for k = 1:numel(fn) - H.(fn{k}) = opt.(fn{k}); - end - end - % --------------------------------------------------------------------- - - function H = update(H, s ,y) - % store new vectors - H.itCount = H.itCount +1; - pix = ':'; - if H.itCount > H.m - pix = 2:H.m; - end - H.S = [H.S(:, pix), s]; - H.Y = [H.Y(:, pix), y]; - if H.itCount == 1 % limit m to number of vars - if H.m > numel(s) - H.m = numel(s); - dispif(mrstVerbose, 'Resetting ''m'' to number of parameters (%d)\n', H.m); - end - end - end - - % --------------------------------------------------------------------- - function H = reset(H) - [H.S, H.Y] = deal([]); - H.itCount = 0; - H.nullspace = []; - end - - % --------------------------------------------------------------------- - function r = mtimes(H, v) - % apply mulitplication H*v - if isa(v, 'LimitedMemoryHessian') - error('Only right-multiplciation is supported'); - else - if H.itCount == 0 - r = (H.sign*H.initScale)*v; - if ~isempty(H.nullspace) - if islogical(H.nullspace) - r = r.*(~H.nullspace); - else - r = r - H.nullspace*(H.nullspace'*r); - end - end - else - assert(all(size(v)==[size(H.S, 1), 1]), ... - 'Dimension mismatch'); - if isempty(H.nullspace) % do standard L-BFGS - nVec = size(H.S, 2); - [rho, alpha] = deal(nan(1, nVec)); - for k = nVec:-1:1 - rho(k) = 1/(H.S(:,k)'*H.Y(:,k)); - alpha(k) = rho(k)*(H.S(:,k)'*v); - v = v - alpha(k)*H.Y(:,k); - end - r = H.applyInitial(v); - for k = 1:nVec - beta = rho(k)*(H.Y(:,k)'*r); - r = r + (alpha(k)-beta)*H.S(:,k); - end - else % do subspace version - th = H.applyInitial(1); - r = subspaceProd(H.S, H.Y, th, H.nullspace, v); - end - end - end - end - - % --------------------------------------------------------------------- - function H = uminus(H) - H.sign = -H.sign; - end - - % --------------------------------------------------------------------- - function r = applyInitial(H, v) - if strcmp(H.initStrategy, 'static') - r = (H.sign*H.initScale)*v; - elseif strcmp(H.initStrategy, 'dynamic') - [s,y] = deal(H.S(:,end), H.Y(:,end)); - r = ((s'*y)/(y'*y))*v; - else - error('Unknown strategy: %s', H.initStrategy); - end - end - - % --------------------------------------------------------------------- - function H = setNullspace(H, Q) - if nargin < 2 - H.nullspace = []; - else - if H.itCount > 0 && ~islogical(Q) - assert(size(Q,1)==size(H.S, 1), 'Dimension mismatch'); - assert(size(Q,1)>=size(Q,2), ... - 'Number of columns in nullspace matrix exceeds number of rows'); - end - H.nullspace = Q; - end - end - - % --------------------------------------------------------------------- - function M = full(H) - % Create full matrix, only intended for debugging purposes - if H.itCount == 0 - M = H*1; - else - n = size(H.S, 1); - M = zeros(n); - for k = 1:n - ek = zeros(n,1); - ek(k) = 1; - M(:,k) = H*ek; - end - end - end -end -end -% ------------------------------------------------------------------------- -% ------------------------------------------------------------------------- -function r = subspaceProd(S, Y, th, Q, v) -% Perform product restricted to nullspace of Q-colunms, i.e., -% r = Z * (Z'*Hessian*Z)^-1 * Z'*v -% with Z = null(Q') -% Formula from: -% Byrd, R. H., Lu, P., Nocedal, J., & Zhu, C. (1995). -% A limited memory algorithm for bound constrained optimization. -% SIAM Journal on scientific computing, 16(5), 1190-1208. -% -% S : control diffs -% Y : gradient diffs -% th : inverse Hessian scaling -% Q : nullspace of active subspace -% v : vector -if size(Q,1) <= size(Q,2) - % null(Q')=[], return zero; - r = 0*v; -else - n = size(S,2); - W = [Y, S/th]; - tmp = S'*Y; - L = tril(tmp, -1); - D = diag(diag(tmp)); - M = [-D, L'; L, (S'*S)/th]; - % projection onto active subspace (u -> Z*Z'*u) - if islogical(Q) - projSub = @(u)u.*(~Q); - else - projSub = @(u)u-Q*(Q'*u); - end - r = M\(W'*projSub(v)); - r = (eye(2*n) - th*(M\(W'*projSub(W))))\r; - r = projSub(th*v + th^2*(W*r)); -end -end - -%{ -% For reference: -% should be equal to subspaceProd, but at the additional cost of doing null(Q') -Z = null(Q'); -n = size(S,2); -W = [Y, S/th]; -tmp = S'*Y; -L = tril(tmp, -1); -D = diag(diag(tmp)); -M = [-D, L'; L, (S'*S)/th]; -WtZ = W'*Z; -Ztv = Z'*v; -r = M\(WtZ*Ztv); -r = (eye(2*n)-th*(M\(WtZ*WtZ')))\r; -r = th*Ztv + (th^2)*WtZ'*r; -r = Z*r; -%} - -%{ -Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. - -This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). - -MRST is free software: you can redistribute it and/or modify -it under the terms of the GNU General Public License as published by -the Free Software Foundation, either version 3 of the License, or -(at your option) any later version. - -MRST is distributed in the hope that it will be useful, -but WITHOUT ANY WARRANTY; without even the implied warranty of -MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the -GNU General Public License for more details. - -You should have received a copy of the GNU General Public License -along with MRST. If not, see . -%} diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m b/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m deleted file mode 100644 index 3903d6d30..000000000 --- a/Battery/EquivalentCircuitModel/spectral_analysis/argmaxCubic.m +++ /dev/null @@ -1,66 +0,0 @@ -function [xOpt, poly] = argmaxCubic(p1, p2) -% find max of cubic polynomial through p1, p2 -% shift values: -%{ -Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. - -This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). - -MRST is free software: you can redistribute it and/or modify -it under the terms of the GNU General Public License as published by -the Free Software Foundation, either version 3 of the License, or -(at your option) any later version. - -MRST is distributed in the hope that it will be useful, -but WITHOUT ANY WARRANTY; without even the implied warranty of -MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the -GNU General Public License for more details. - -You should have received a copy of the GNU General Public License -along with MRST. If not, see . -%} -shift = p1.a; -p1.a = 0; -p2.a = p2.a-shift; -poly = zeros(4,1); -poly(3:4) = [p1.dv; p1.v]; -a = p2.a; -poly(1:2) = [a^3, a^2; 3*a^2 2*a]\[p2.v-p1.dv*a-p1.v; p2.dv-p1.dv]; -xe = roots(polyder(poly)); -if numel(xe) == 0 - xe = -inf; -elseif any(imag(xe)~=0) - xe = inf; -elseif xe(1) == xe(end) % single root - if poly(1) ~= 0 - xe = inf; - elseif poly(2) < 0 - xe = xe(1); - else - xe = -inf; - end -else % two roots - [~,ix] = max(polyval(poly,xe)); - xe = xe(ix); - if xe < p1.a - xe = -inf; - end -end -xOpt = xe + shift; - -%-------------------------------------------------------------------------- -% % Uncomment for debugging purposes: -% figure(99), clf, hold on -% x1 = p1.a; x2 = p2.a; -% xi = x1/2:(x2-x1)/50:2*x2; -% plot(xi+shift, polyval(poly, xi)); -% plot(xe+shift, polyval(poly, xe), 'o', 'Markersize', 14, 'MarkerEdgeColor', 'r'); -% plot(p1.a+shift, p1.v, 'o', 'Markersize', 14); -% plot(p2.a+shift, p2.v, 'o', 'Markersize', 14); -% l0 = p1.dv*xi + p1.v -p1.dv*p1.a; -% lx = p2.dv*xi + p2.v -p2.dv*p2.a; -% plot(xi+shift, l0, '--k') -% plot(xi+shift, lx, '--k') -% drawnow -end - diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m b/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m deleted file mode 100644 index f4263fe0b..000000000 --- a/Battery/EquivalentCircuitModel/spectral_analysis/cost_function_eis.m +++ /dev/null @@ -1,14 +0,0 @@ - -function [total_error, Z_re_exp, Z_im_exp] = cost_function_eis(best_params) - - -Z_re_exp = plot_nyquist_ank.Z_real; -Z_im_exp = plot_nyquist_ank.Z_imag; - - -omega = logspace(-2, 4, 100) - -Z_re_params = plot_nyquist_params.Z_real(best_params); -Z_im_params = plot_nyquist_params.Z_imag(best_params); - -totalerror = sum((Z_re_exp(omega)-Z_re_params(omega)).^2) + sum((Z_im_exp(omega)-Z_im_params(omega))^2) \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m b/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m deleted file mode 100644 index 9e20938ac..000000000 --- a/Battery/EquivalentCircuitModel/spectral_analysis/lineSearch.m +++ /dev/null @@ -1,147 +0,0 @@ -function [u, v, g, info] = lineSearch(u0, v0, g0, d, f, opt) -% lineSearch -- helper function which performs line search based on -% Wolfe-conditions. -% -% SYNOPSIS: -% [u, v, g, info] = lineSearch(u0, v0, g0, d, f, c, opt) -% -% PARAMETERS: -% u0 : current control vector -% v0 : current objective value -% g0 : current gradient -% d : search direction, returns an error unless d'*g0 > 0 -% f : objective function s.t. [v,g] = f(u) -% c : struct with linear inequality and equality constraints -% opt: struct of parameters for line search -% -% RETURNS: -% u : control vector found along d -% v : objective value for u -% g : gradient for u -% info : struct containing fields: -% flag : 1 for success (Wolfe conditions satisfied) -% -1 max step-length reached without satisfying Wolfe-conds -% -2 line search failed in maxIt iterations (returns most recent -% control without further considerations) -% step : step-length -% nits : number of iterations used - -%{ -Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. - -This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). - -MRST is free software: you can redistribute it and/or modify -it under the terms of the GNU General Public License as published by -the Free Software Foundation, either version 3 of the License, or -(at your option) any later version. - -MRST is distributed in the hope that it will be useful, -but WITHOUT ANY WARRANTY; without even the implied warranty of -MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the -GNU General Public License for more details. - -You should have received a copy of the GNU General Public License -along with MRST. If not, see . -%} -c1 = opt.wolfe1; -c2 = opt.wolfe2; -sgf = opt.safeguardFac; -incTol = opt.stepIncreaseTol; -maxIt = opt.lineSearchMaxIt; -aMax = opt.maxStep; - -% Assert search direction is increasing -assert(d'*g0 <= 0) - -% Define convenience-function to gather info for a "point", where a is the -% step-length, v is the value and dv is the dirctional derivative: -assignPoint = @(a,v,dv)struct('a', a, 'v', v, 'dv', dv); -p0 = assignPoint(0, v0, d'*g0); % 0-point - -% Function handles for wolfe conditions wrt p0 -w1 = @(p) p.v <= p0.v + c1*p.a*p0.dv; -w2 = @(p) abs(p.dv) <= c2*abs(p0.dv); - -% End-points of initial interval -p1 = p0; -p2 = assignPoint(aMax, inf, inf); -% Initial step-length: -a = 1; -lineSearchDone = false; -it = 0; -vals = nan(1, maxIt); -while ~lineSearchDone && it < maxIt - it = it +1; - u = u0 + a*d; - [v, g] = f(u); % function evaluation / simulation - vals(it) = v; - p = assignPoint(a, v, d'*g); % new point - if w1(p) && w2(p) - lineSearchDone = true; - flag = 1; - else - if abs(aMax - p.a) < sqrt(eps) && ... % max step-length reached - (p.v < p0.v) && ... % the step yielded an improvement - (p.dv < 0) % continuing further would improve (but not allowed) - lineSearchDone = true; - flag = -1; - fprintf('Line search at max step size, Wolfe conditions not satisfied for this step.\n'); - else % logic for refining/expanding interval of interest [p1 p2] - if p.a > p2.a - % if we have extrapolated p1.v >= p2.v - [p1, p2] = deal(p2, p); - else - if p.dv >= 0 - p2 = p; - else % keep best - if p1.v <= p2.v - p2 = p; - else - p1 = p; - end - end - end - % Find next candidate-step by interpolation - if p1.v > p2.v && p1.dv >= p2.dv - % Just getting steeper, no need to interpolate - a = inf; - else - a = argmaxCubic(negatePnt(p1), negatePnt(p2)); - end - % Safe-guarding and thresholding: - if a > p2.a - a = max(a, (1+sgf)*p2.a); - a = min(a, min(incTol*p2.a, aMax)); - elseif a > p1.a - a = max(a, p1.a + sgf*(p2.a-p1.a)); - a = min(a, p2.a - sgf*(p2.a-p1.a)); - else - a = (p1.a+p2.a)/2; - fprintf('Cubic interpolation failed, cutting interval in half ...') - end - end - end -end -% Check if line search succeeded -if ~lineSearchDone - flag = -2; - fprintf('Line search unable to succeed in %d iterations ...\n', maxIt); - % Although line search did not succeed in maxIt iterations, we ensure - % to return the greater of p1 and p2's objective value none the less. - if p1.v < p2.v - u = u0 + p1.a*d; - % and we will re-compute the gradients for these controls - [v, g] = f(u); - end -end -info = struct('flag', flag, 'step', a, 'nits', it, 'objVals', vals(1:it)); -end - -function p = negatePnt(p) -[p.v, p.dv] = deal(-p.v, -p.dv); -end - - - - \ No newline at end of file diff --git a/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m b/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m deleted file mode 100644 index 867264599..000000000 --- a/Battery/EquivalentCircuitModel/spectral_analysis/unitBoxBFGS.m +++ /dev/null @@ -1,578 +0,0 @@ -function [v, u, history] = unitBoxBFGS(u0, f, varargin) -% Iterative line search optimization using BFGS intended for scaled -% problems, i.e., 0<=u<=1 and f~O(1) -% -% SYNOPSIS: -% [v, u, history] = unitBoxBFGS(u0, f, ...) -% -% PARAMETERS -% u0 : inital guess nx1 vector with 0<= u0 <= 1 and feasible wrt -% any additional constraints -% f : function handle s.t., [v,g] = f(u) returns -% v : objective value -% g : objective nx1 gradient vector -% KEYWORD ARGUMENTS: -% 'maximize' : Boolean option (false will minimize objective) -% Default: true -% 'stepInit' : Initial step (gradient scaling). If not provided -% (or set to nan), the following scaling will be used: -% stepInit = maxInitialUpdate/max(|initial gradient|) -% 'maxInitialUpdate' : as described above. Default: 0.05 -% 'history' : Option for 'warm starting' based on previous -% optimization (must have been run with option -% 'outputHessian' = true) -% Stopping criteria options -% 'gradTol' : Absolute tollerance of inf-norm of projected gradient. -% Default: 1e-3 -% 'objChangeTol' : Absolute objective update tollerance. Default: 5e-4 -% 'maxIt' : Maximal number of iterations. Default: 25 -% Line-search options -% 'lineSearchMaxIt' : Maximal number of line-search iterations. Default: 5 -% 'stepIncreaseTol' : Maximal step increase factor between line -% search iterations. Deafult: 10 -% 'wolfe1', : Objective improvement condition. Default: 1e-4 -% 'wolfe2', : Gradient reduction condition. Default: 0.9 -% Hessian approximation options -% 'useBFGS' : If false pure gradient search will be used. -% Deafult: true -% 'limitedMemory' : If false, full Hessian approximations will be -% made (in general not recommended), otherwise -% L-BFGS (see LimitedMemoryHessian.m). -% Default: true -% 'lbfgsNum' : Number of vector-pairs stored for L-BFGS. -% : Default: 5 -% 'lbfgsStrategy' : 'static' or 'dynamic' (see LimitedMemoryHessian.m) -% Default: 'dynamic' -% Linear constraints options -% 'linEq' : Linear equality constraints given as structure with -% fields 'A' and 'b' to enforce A*u=b -% 'linIneq' : Linear inequality constraints *in addition to* the default -% box constraints (0 <= u <= 1). Given as structure with -% fields 'A' and 'b' to enforce A*u<=b -% 'enforceFeasible' : If true, will attempt to repair problematic -% constraint handling/violations by projection. A -% NOTE: A non-feasible initial guess, will always be -% attempted to be made feasible. -% Default: false -% Plotting and output options -% 'plotEvolution' : Plot progess of optimization in figure. -% Default: true -% 'logPlot' : Use logarithmic y-axis when plotting objective -% Default: false -% 'outputHessian' : Output Hessian approximation for each iteration -% in history-structure. Deafault: false -% -% RETURNS: -% v : Optimal or best objective value -% u : Control/parameter vector corresponding to v -% history : Structure containing for each iteration: -% 'val' : objective value -% 'u' : control/parameter vector -% 'pg' : norm of projected gradient -% 'alpha' : line-search step length -% 'lsit' : number of line-search iterations -% 'lsfl' : line-search flag -% 'hess' : Hessian inverse approximation (if requested) - -%{ -Copyright 2009-2024 SINTEF Digital, Mathematics & Cybernetics. - -This file is part of The MATLAB Reservoir Simulation Toolbox (MRST). - -MRST is free software: you can redistribute it and/or modify -it under the terms of the GNU General Public License as published by -the Free Software Foundation, either version 3 of the License, or -(at your option) any later version. - -MRST is distributed in the hope that it will be useful, -but WITHOUT ANY WARRANTY; without even the implied warranty of -MERCHANTABILITY or FITNESS FOR A PARTICULAR PURPOSE. See the -GNU General Public License for more details. - -You should have received a copy of the GNU General Public License -along with MRST. If not, see . -%} -opt = struct( 'maximize', true, ... - 'stepInit', nan, ... - 'maxInitialUpdate', 0.05, ... - 'gradTol', 1e-3, ... - 'objChangeTol', 5e-4, ... - 'objChangeTolRel', -inf, ... - 'maxIt', 25, ... - 'lineSearchMaxIt', 5, ... - 'wolfe1', 1e-4, ... - 'wolfe2', 0.9, ... - 'safeguardFac', 1e-5, ... - 'stepIncreaseTol', 10, ... - 'useBFGS', true, ... - 'limitedMemory', true, ... - 'lbfgsNum', 5, ... - 'lbfgsStrategy', 'dynamic', ... - 'linEq', [], ... - 'enforceFeasible', true, ... - 'linIneq', [], ... - 'plotEvolution', true, ... - 'logPlot', false, ... - 'outputHessian', false, ... - 'history', [] ); -opt = merge_options(opt, varargin{:}); -objSign = 1; -if opt.maximize - f = @(u)fNegative(u, f); - objSign = -1; -end -c = getConstraints(u0, opt); -if isempty(opt.history) - % Setup constraint struct - [u0, ~, consOK] = checkFeasible(u0, c, opt.enforceFeasible, 'Initial guess'); - assert(consOK, 'Infeasible initial guess') - - % Perform initial evaluation of objective and gradient: - [v0,g0] = f(u0); - % If not provided, set initial step - step = opt.stepInit; - if isnan(step) || step <= 0 - step = opt.maxInitialUpdate/max(abs(g0)); - end - % Initial Hessian-approximation - if ~opt.limitedMemory - Hi = step; - else - Hi = LimitedMemoryHessian('initScale', step, ... - 'm', opt.lbfgsNum, ... - 'initStrategy', opt.lbfgsStrategy); - end - HiPrev = Hi; - it = 0; - % Setup struct for gathering optimization history - history = gatherInfo([], objSign*v0, u0, norm(g0), nan, nan, nan, Hi, opt.outputHessian); -else - history = opt.history; - it = numel(history.val); - Hi = history.hess{it}; - assert(~isempty(Hi), ... - 'Warm start based on history requires Hessian approximations'); - u0 = history.u{it}; - [v0, g0] = f(u0); - HiPrev = history.hess{max(it-1,1)}; - opt.maxIt = opt.maxIt + it; -end -[v, u] = deal(v0,u0); -if opt.plotEvolution >0 - evFig = figure; - plotInfo(evFig, history, opt.logPlot) -end -printInfo(history, it); - -success = false; -g = g0; -while ~success - it = it+1; - [d, Hi, pg, opt.maxStep] = getSearchDirection(u0, g0, Hi, HiPrev, c); - %if isempty(d), break; end - if ~(norm(pg,inf) < opt.gradTol) && ~isempty(d) - % Perform line-search - [tmp, flag, fixed] = checkFeasible(u0+d, c, opt.enforceFeasible); - if ~flag && fixed - d = tmp - u0; - end - [u, v, g, lsinfo] = lineSearch(u0, v0, g0, d, f, opt); - % Update Hessian approximation - if opt.useBFGS %&& lsinfo.flag == 1 - [du, dg] = deal(u-u0, g-g0); - % if any of the gradient entries are not defined, we set - % the difference to zero - dg(~isfinite(dg)) = 0; - if du'*dg > sqrt(eps)*norm(du)*norm(dg) - HiPrev = Hi; - if isa(Hi, 'LimitedMemoryHessian') - Hi = Hi.update(du, dg); - else - r = 1/(du'*dg); - V = eye(numel(u)) - r*dg*du'; - Hi = V'*Hi*V + r*(du*du'); - end - else - fprintf('Hessian not updated during iteration %d.\n', it) - end - end - % Update history - history = gatherInfo(history, objSign*v, u, norm(pg,inf), lsinfo.step, ... - lsinfo.nits, lsinfo.flag, Hi, opt.outputHessian); - else - history = gatherInfo(history, objSign*v, u, norm(pg,inf), 0, 0, 0, ... - Hi, opt.outputHessian); - end - - %Check stopping criteria - success = (it >= opt.maxIt) || (norm(pg,inf) < opt.gradTol) || ... - (abs(v-v0) < opt.objChangeTol) || ... - (abs((v-v0)./v) < opt.objChangeTolRel); - - [u0, v0, g0] = deal(u, v, g); - if opt.plotEvolution > 0 - plotInfo(evFig, history, opt.logPlot) - end - printInfo(history, it); -end -end -%-------------------------------------------------------------------------- - -function [d, Hi, pg, maxStep] = getSearchDirection(u0, g0, Hi, HiPrev, c) -% Find search-direction which is (sum of) the projection(s) of Hi*g0 -% restricted to directions with non-active constraints. -cnt = 1; -for k = 1:3 - if k==2 - Hi = HiPrev; - elseif k==3 - if isa(Hi, 'LimitedMemoryHessian') - Hi = Hi.reset(); - else - Hi = 1; - end - end - % Project gradient and search direction onto nullspace of equality - % constraints - Q = c.e.Q; - pg = -projQ(g0, Q); - d = -projQ(g0, Q, Hi); - % The following loop(s) should project onto nullspace of additional - % active constraints. First for gradient direction, then for search - % direction which may have additional constraints active. While-loop - % will in most cases only be traversed once, so we don't worry too much - % about efficiency - isActive = false; - for kd = 1:2 - [na, na_prev] = deal(0, -1); - while na > na_prev - if kd == 1 - [~, active_cur] = classifyConstraints(c.i.A, c.i.b, u0, pg); - else - [~, active_cur] = classifyConstraints(c.i.A, c.i.b, u0, d); - end - isActive = isActive | active_cur; - na_prev = na; - na = nnz(isActive); - if na > na_prev % redo projection for all active - [Q, s] = svd([c.i.A(isActive,:)', c.e.A'], 0); - s = diag(s); - Q = Q(:, s > sqrt(eps)*s(1)); - if kd == 1 - pg = -projQ(g0, Q); - else - d = -projQ(g0, Q, Hi); - end - end - end - end - % Check for tiny projected gradient - if norm(pg, inf) <= sqrt(eps)*norm(g0, inf) % nothing more to do - [d, maxStep] = deal([]); - return - end - % Iteratively find all constraints that become active from u0 to u0+d, - % and project remaining line segments accordingly. - [dr, gr] = deal(d, g0); - becomesActive = isActive; - d = 0; - done = false; - while ~done - if norm(dr) > sqrt(eps) - sgn = classifyConstraints(c.i.A, c.i.b, u0+d, dr); - [ix, s] = findNextConstraint(c.i.A, c.i.b, u0+d, dr, sgn<=0 | becomesActive); - else - [ix, s] = deal([], 0); - end - if ~isempty(ix) && s <= 1+sqrt(eps) - becomesActive(ix) = true; - d = d + s*dr; - gr = (1-s)*gr; - Q = expandQ(Q, c.i.A(ix,:)'); - dr = -projQ(gr, Q, Hi); - else - d = d+dr; - done = true; - end - end - % find maximal step length we can take with d before hitting the next - % constraint (should be >= 1) - sgn = classifyConstraints(c.i.A, c.i.b, u0, d); - [~, maxStep] = findNextConstraint(c.i.A, c.i.b, u0, d, sgn<=0); - if maxStep < .95 - warning('Problematic constraint handling, relative step length: %6.5f', maxStep); - end - if maxStep < 1 - [d, maxStep] = deal(maxStep*d, 1); - end - - isDecreasing = d'*g0 <= 0; - isZero = norm(d, inf) <= sqrt(eps)*norm(Hi*g0, inf); - if isDecreasing && ~isZero % decreasing search direction found, exit - break; - else - % retry with other Hessian approx - if ~isZero - str = 'Small norm of search direction'; - else - str = 'Non-inceasing search direction'; - end - switch cnt - case 1 - fprintf('%s, trying previous Hessian approximation.\n', str) - case 2 - fprintf('%s, trying to reset Hessian to identity.\n', str) - case 3 - fprintf('Exiting: %s.\n', str) - [d, maxStep] = deal([]); - end - end -end -end -%-------------------------------------------------------------------------- - -function w = projQ(v, Q, H) -if nargin < 3 - H = 1; -end -if isempty(Q) - w = H*v; -else - if ~isa(H, 'LimitedMemoryHessian') - tmp = H*(v-Q*(Q'*v)); - w = tmp - Q*(Q'*tmp); - else - H = H.setNullspace(Q); - w = H*v; - end -end -end -%-------------------------------------------------------------------------- - -function c = getConstraints(u, opt) -% Box constraints, always 0<= u <= 1 -nu = numel(u); -c.i.A = [diag(-ones(nu,1)); diag(ones(nu,1))]; -c.i.b = [zeros(nu,1); ones(nu,1)]; -% Add general linear constraints -if ~isempty(opt.linIneq) - % scale by norm(A) - sc = norm(opt.linIneq.A); - c.i.A = [c.i.A; opt.linIneq.A/sc]; - c.i.b = [c.i.b; opt.linIneq.b/sc]; -end -% Equality constraints (always active) -if ~isempty(opt.linEq) - sc = norm(opt.linEq.A); - c.e.A = opt.linEq.A/sc; - c.e.b = opt.linEq.b/sc; - [Q, s] = svd(c.e.A', 0); - s = diag(s); - c.e.Q = Q(:, s> sqrt(eps) * s(1)); -else - c.e.A = zeros(0, nu); - c.e.b = []; - c.e.Q = zeros(nu, 0); -end -end -%-------------------------------------------------------------------------- - -function [u, flag, fixed] = checkFeasible(u, c, enforce, nm) -% Check that u is feasible. If not and enforce == true, try to fix. Ideally -% should be solved as ||u-u*|| st c.e and c.i, but since we don't have a -% QP-solver resort to (costly) iterative projections in active subspaces. -% Intended for fixing mild violations. -if nargin < 4 - nm = 'Vector u'; -end -if nargin < 3 - enforce = false; -end -hasEC = ~isempty(c.e.A); -hasIC = ~isempty(c.i.A); -[ecOK, icOK] = deal(true); - -if hasEC - [Ae, be] = deal(c.e.A, c.e.b); - if any(abs(c.e.A*u-c.e.b) > sqrt(eps)) - % find closest u that fulfills c.e. - u = u + Ae'*((Ae*Ae')\(be-Ae*u)); - ecOK = false; %now OK, but warn - end -end - -flag = ecOK; -fixed = false; -maxIt = 100; -for it = 1:maxIt - if hasIC - icOK = ~any(c.i.A*u-c.i.b > sqrt(eps)); - flag = flag && icOK; - end - if ~enforce - break - else - if ~icOK - Q = zeros(numel(u), 0); - proj = @(v)v; - if hasEC - Q = c.e.Q; - proj = @(v)v-Q*(Q'*v); - end - % Loop through each violating and project. If there are no more - % availabe directions, restart while-loop from current point - done = false; - cnt = 0; - while ~done - if cnt == 0 - icIx = find(c.i.A*u-c.i.b > sqrt(eps)); - icIx = circshift(icIx, it); - end - if isempty(icIx) || cnt == numel(icIx) - done = true; - else - % - ix = icIx(cnt+1); - [a, b] = deal(c.i.A(ix,:)', c.i.b(ix)); - pa = proj(a); - if norm(pa) < sqrt(eps)*norm(a) - % skip - cnt = cnt +1; - else - cnt = 0; - u = u + pa*((b-a'*u)/(a'*pa)); - if size(Q,2) < size(Q,1)-1 - Q = expandQ(Q, pa); - proj = @(v)v-Q*(Q'*v); - else - % possibly restart while-loop - done = true; - end - end - end - end - else - fixed = true; - break - end - end -end - - -if it == maxIt - warning('Failed attempt to fix feasibility of %s, continuing anyway ...', nm); -elseif ~flag - if ~enforce - warning('%s is not feasible within tollerance. %s', nm, ... - 'Consider running with option ''enforceFeasible''=true'); - else - warning('%s was not feasible, fixed feasibility in %d iteration(s)', ... - nm, it-1); - end -end -end -%-------------------------------------------------------------------------- -function [sgn, act] = classifyConstraints(A, b, u, v) -% classify inequality constraints for point u with direction v -% sgn: -1: in, 0: parallell, 1: out -% act: true for active -sgn = A*v; -sgn(abs(sgn) -sqrt(eps) & sgn > 0; -end -%-------------------------------------------------------------------------- - -function [ix, s] = findNextConstraint(A, b, u, d, ac) -s = (b-A*u)./(A*d); -s(ac) = inf; -s(s sqrt(eps) - Q = [Q, v/norm(v)]; -else - fprintf('Newly active constraint is linear combination of other active constraints ??!!\n') -end -end -%-------------------------------------------------------------------------- - -function [v, g] = fNegative(u, f) -if nargout == 1 - v = -f(u); -elseif nargout == 2 - [v, g] = f(u); - [v, g] = deal(-v, -g); -end -end -%-------------------------------------------------------------------------- - -function [] = plotInfo(fig, hst, logPlot) -if ~ishandle(fig) - figure(fig) -else - % Avoid stealing focus if figure already exists - set(0, 'CurrentFigure', fig); -end -xt = 0:(numel(hst.val)-1); -xlim = [-.2, xt(end)+.5]; -ch = abs(hst.val(2:end)-hst.val(1:end-1)); -popt = {'o-', 'LineWidth', 2, 'MarkerSize', 6, ... - 'MarkerFaceColor', [1 1 1]}; -subplot(5,1,1), -if ~logPlot - plot(xt, hst.val, popt{:}); -else - semilogy(xt, abs(hst.val), popt{:}); -end -title('Objective'); -set(gca, 'XLim', xlim) -subplot(5,1,2), semilogy(xt,hst.pg, popt{:}), title('Gradient norm'); -set(gca, 'XLim', xlim) -subplot(5,1,3), semilogy(xt(2:end)-.5,ch, popt{:}), title('Objective change'); -set(gca, 'XLim', xlim) -subplot(5,1,4), bar(xt,hst.lsit), title('Line search iterations'); -set(gca, 'XLim', xlim) -subplot(5,1,5), col = [0.8500 0.3250 0.0980]; -if numel(hst.u{end}) < 50 - bar(hst.u{end}, 'FaceColor', col); -else - plot(hst.u{end}, '.-', 'Color', col); -end -title('Current scaled controls'); -set(gca, 'YLim', [0, 1]) -drawnow -end -%-------------------------------------------------------------------------- - -function hst = gatherInfo(hst, val, u, pg, alpha, lsit, lsfl, hess, outputH) -% obj.val | contr | norm proj.grad | ls-step | ls-its | ls-flag | hessian -if ~outputH - hess = []; -end -if isempty(hst) - hst = struct('val', val, 'u', {{u}}, 'pg', pg, ... - 'alpha', alpha, 'lsit', lsit, 'lsfl', lsfl, ... - 'hess', {{hess}}); -else - hst.val = [hst.val , val ]; - hst.u = [hst.u , {u} ]; - hst.pg = [hst.pg , pg ]; - hst.alpha = [hst.alpha, alpha]; - hst.lsit = [hst.lsit , lsit ]; - hst.lsfl = [hst.lsfl , lsfl ]; - hst.hess = [hst.hess ,{hess}]; -end -end -%-------------------------------------------------------------------------- - -function printInfo(history, it) -fprintf('It: %2.1d | val: %4.3e | ls-its: %3.1d | pgrad: %4.3e\n', ... - it, history.val(end), history.lsit(end), ... - history.pg(end)); -end diff --git a/Battery/EquivalentCircuitModel/cost_function.m b/Battery/EquivalentCircuitModel/utils/costFunctionECM.m similarity index 99% rename from Battery/EquivalentCircuitModel/cost_function.m rename to Battery/EquivalentCircuitModel/utils/costFunctionECM.m index 1bb8d6a18..e92753dbe 100644 --- a/Battery/EquivalentCircuitModel/cost_function.m +++ b/Battery/EquivalentCircuitModel/utils/costFunctionECM.m @@ -7,7 +7,6 @@ parameters.R2 = abs(params_test(4)); parameters.C2 = max(abs(params_test(5)), 0.1); - inputparams = EquivalentCircuitModelInputParams(parameters); model = EquivalentCircuitModel(inputparams); [t_sim, V_sim, ~] = model.solve(); @@ -15,7 +14,6 @@ % Time synchronization V_sim_aligne = interp1(t_sim, V_sim, t_exp, 'linear', 'extrap'); - voltage_error = sum((V_exp - V_sim_aligne).^2); lambda = 0.5; @@ -26,4 +24,4 @@ total_error = voltage_error + tikhonov_error; -end \ No newline at end of file +end diff --git a/Battery/EquivalentCircuitModel/create_parameters.m b/Battery/EquivalentCircuitModel/utils/createParametersECM.m similarity index 100% rename from Battery/EquivalentCircuitModel/create_parameters.m rename to Battery/EquivalentCircuitModel/utils/createParametersECM.m diff --git a/Battery/EquivalentCircuitModel/plotexperience.m b/Battery/EquivalentCircuitModel/utils/plotExperience.m similarity index 100% rename from Battery/EquivalentCircuitModel/plotexperience.m rename to Battery/EquivalentCircuitModel/utils/plotExperience.m From b36f505b1345c3d0cd11397ee4ae126248192e98 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:23:13 +0200 Subject: [PATCH 050/119] update --- Battery/EquivalentCircuitModel/examples/exampleECM.m | 4 ++-- .../examples/{run_fitting.m => runECMfitting.m} | 0 .../EquivalentCircuitModel/models/EquivalentCircuitModel.m | 2 +- Battery/EquivalentCircuitModel/utils/createParametersECM.m | 4 ++-- 4 files changed, 5 insertions(+), 5 deletions(-) rename Battery/EquivalentCircuitModel/examples/{run_fitting.m => runECMfitting.m} (100%) diff --git a/Battery/EquivalentCircuitModel/examples/exampleECM.m b/Battery/EquivalentCircuitModel/examples/exampleECM.m index 31a5d82f8..e555eb2c0 100644 --- a/Battery/EquivalentCircuitModel/examples/exampleECM.m +++ b/Battery/EquivalentCircuitModel/examples/exampleECM.m @@ -2,7 +2,7 @@ % Load data set -params = create_parameters(); +params = createParametersECM(); inputparams = EquivalentCircuitModelInputParams(params); % Setup model @@ -35,4 +35,4 @@ title('SOC') xlabel('Time /s') ylabel('SOC') -grid on \ No newline at end of file +grid on diff --git a/Battery/EquivalentCircuitModel/examples/run_fitting.m b/Battery/EquivalentCircuitModel/examples/runECMfitting.m similarity index 100% rename from Battery/EquivalentCircuitModel/examples/run_fitting.m rename to Battery/EquivalentCircuitModel/examples/runECMfitting.m diff --git a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m index ab2715ac3..ff38ffcc0 100644 --- a/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m +++ b/Battery/EquivalentCircuitModel/models/EquivalentCircuitModel.m @@ -1,4 +1,4 @@ -calassdef EquivalentCircuitModel < BaseModel +classdef EquivalentCircuitModel < BaseModel properties diff --git a/Battery/EquivalentCircuitModel/utils/createParametersECM.m b/Battery/EquivalentCircuitModel/utils/createParametersECM.m index 8fa694884..4e2c35f7d 100644 --- a/Battery/EquivalentCircuitModel/utils/createParametersECM.m +++ b/Battery/EquivalentCircuitModel/utils/createParametersECM.m @@ -1,4 +1,4 @@ -function p = create_parameters() +function p = createParametersECM() p.nominalcellcapacity = 63.7; p.initSOC = 1.0; @@ -14,7 +14,7 @@ p.OCP.functionFormat = 'tabulated'; p.OCP.argumentList = {'SOC'}; p.OCP.dataX = [0.00, 0.02, 0.04, 0.06, 0.08, 0.10, 0.12, 0.14, 0.16, 0.18, 0.20, 0.22, 0.24, 0.26, 0.28, 0.30, 0.32, 0.34, 0.36, 0.38, 0.40, 0.42, 0.44, 0.46, 0.48, 0.50, 0.52, 0.54, 0.56, 0.58, 0.60, 0.62, 0.64, 0.66, 0.68, 0.70, 0.72, 0.74, 0.76, 0.78, 0.80, 0.82, 0.84, 0.86, 0.88, 0.90, 0.92, 0.94, 0.96, 0.98, 1.00]; - p.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000] + p.OCP.dataY = [3.126000, 3.273000, 3.380000, 3.447000, 3.470000, 3.480000, 3.489000, 3.500000, 3.515000, 3.533000, 3.551000, 3.567000, 3.582000, 3.594000, 3.602000, 3.609000, 3.614000, 3.620000, 3.625000, 3.631000, 3.637000, 3.643000, 3.649000, 3.657000, 3.665000, 3.674000, 3.684000, 3.696000, 3.710000, 3.727000, 3.750000, 3.775000, 3.798000, 3.818000, 3.838000, 3.858000, 3.877000, 3.897000, 3.917000, 3.937000, 3.958000, 3.979000, 4.000000, 4.022000, 4.044000, 4.066000, 4.089000, 4.112000, 4.135000, 4.159000, 4.182000]; R0_tot = [0.0074814,0.00375135,0.00199926,0.000808379,0.000529892;0.0074814,0.00375135,0.00185474,0.000738337,0.00049771;0.0074814,0.00373265,0.00151744,0.000673703,0.000468303;0.0074814,0.00342697,0.00130825,0.000635903,0.000448193;0.0074814,0.00272078,0.00117717,0.000611909,0.000432971;0.0069826,0.00229452,0.00109773,0.00058627,0.000423262;0.00612671,0.00206227,0.00105217,0.000571475,0.000417812;0.00536849,0.00193337,0.00101405,0.000562212,0.000409251;0.00480278,0.00185103,0.000983687,0.000549631,0.000410476;0.00440167,0.00178588,0.000957044,0.000543895,0.000405368;0.00411575,0.00172477,0.000934531,0.000533558,0.0003994;0.00390187,0.00167949,0.000914869,0.000526768,0.000397983;0.00374658,0.00164546,0.000905014,0.000521591,0.000396355;0.0036334,0.00160835,0.000895256,0.000517151,0.000393944;0.00353281,0.00158063,0.0008793,0.000516464,0.000391954;0.00344791,0.0015608,0.000869252,0.00051227,0.000391406;0.00338977,0.00154377,0.000859461,0.000509065,0.000390664;0.00333872,0.00152388,0.000857998,0.000507685,0.00038969;0.00329657,0.00150926,0.000852066,0.000501813,0.000385995;0.00326141,0.00149673,0.000846844,0.000505136,0.000388294;0.00322799,0.00149188,0.00084232,0.00050115,0.000384211;0.00320237,0.00148102,0.000839376,0.00050073,0.000386191;0.00318137,0.00147045,0.000836217,0.000500865,0.000386833;0.00315527,0.00146685,0.000833235,0.000497888,0.000386251;0.00311928,0.00145992,0.000832092,0.000498747,0.000382866;0.00310424,0.00145576,0.000832276,0.000494884,0.000386295;0.00309834,0.00144722,0.000829437,0.000496968,0.000386992;0.00307867,0.00144351,0.000828243,0.000495848,0.000387399;0.00306673,0.00144798,0.000830089,0.000500481,0.000387638;0.00305254,0.00144507,0.000828833,0.000496636,0.000382113;0.00304161,0.00144131,0.000827309,0.000497478,0.000382439;0.0030343,0.00143125,0.00082455,0.000492916,0.000389673;0.00302615,0.00142702,0.000818782,0.000500463,0.00038546;0.00302297,0.0014205,0.000814619,0.000491503,0.0003858;0.00301535,0.00141463,0.000814864,0.000492482,0.000383651;0.00300786,0.00140957,0.000816839,0.000493931,0.000382345;0.00299892,0.00140604,0.000813864,0.000493379,0.000386187;0.00299335,0.00140043,0.000808475,0.000490454,0.000383351;0.0029867,0.00139212,0.000804998,0.00048877,0.000377422;0.00298272,0.00138903,0.000800962,0.000487252,0.000380367;0.00298442,0.00138775,0.000805805,0.000489012,0.000381427;0.00297911,0.00138254,0.000802961,0.000485793,0.000382455;0.0029803,0.00137618,0.000800822,0.000484924,0.000378882;0.00299019,0.0013734,0.000797575,0.000489591,0.000378052;0.00300121,0.00137477,0.000797567,0.00048441,0.000379647;0.00301775,0.00136948,0.000800597,0.000486859,0.000378768;0.00304181,0.00136736,0.000799303,0.000482635,0.000384018;0.00307807,0.00136092,0.000796617,0.000485164,0.000379421;0.00313868,0.00136725,0.000791133,0.000485946,0.000378392;0.00319877,0.00136795,0.000797194,0.000486639,0.000378749;0.00319877,0.00136795,0.000798674,0.000488616,0.00038044]; R1_tot = [0.0109518,0.00514849,0.00241913,0.000853767,0.000473136;0.0109518,0.00514849,0.00220007,0.000747948,0.000445283;0.0109518,0.00501759,0.00156633,0.000667537,0.000418055;0.0109518,0.00370479,0.00129477,0.000664379,0.000438201;0.0109518,0.00216514,0.00106482,0.000640611,0.000507597;0.00728213,0.00153036,0.000911211,0.000570174,0.000443806;0.00408898,0.00127121,0.000813038,0.000536964,0.000411202;0.00271216,0.00113093,0.000750563,0.000509078,0.00039686;0.00214054,0.00103047,0.000707957,0.00049128,0.000367506;0.00183948,0.000958516,0.000681101,0.000487984,0.000367436;0.00161631,0.000900906,0.00065605,0.000471902,0.000371049;0.00143562,0.000870054,0.000636391,0.000458368,0.000371823;0.00131615,0.000855439,0.000624021,0.000446287,0.000361092;0.00125805,0.000850114,0.000654326,0.000460409,0.000374051;0.00124731,0.000866505,0.000676043,0.000473626,0.000375777;0.00125896,0.000869833,0.00068294,0.000483716,0.000367479;0.00126551,0.000878883,0.000685236,0.000493259,0.000394196;0.00126671,0.000886034,0.000680167,0.000500364,0.000410745;0.00126922,0.000890457,0.000679576,0.00050932,0.000430389;0.00126189,0.000899098,0.000680305,0.000511495,0.000425145;0.00124402,0.000907082,0.000684716,0.000517428,0.000411099;0.00121491,0.000919332,0.000686495,0.00051921,0.000407804;0.00118622,0.000932087,0.000694829,0.000514845,0.000406396;0.00115509,0.000939311,0.000704886,0.000514129,0.000393472;0.00114401,0.000955183,0.000713811,0.000514671,0.000395118;0.00112723,0.000972638,0.00072264,0.000515396,0.000390676;0.00112656,0.000993509,0.000733566,0.000513148,0.000391352;0.00115195,0.00101087,0.000750226,0.000523251,0.000395854;0.0011324,0.00100369,0.000766549,0.000531557,0.000404817;0.00109983,0.000968004,0.000760227,0.000547237,0.000416704;0.00106196,0.000866661,0.000703058,0.000514665,0.000397599;0.00103714,0.000801982,0.000640288,0.00051886,0.000418776;0.00103666,0.000804728,0.000635207,0.000576802,0.000470891;0.00106092,0.000845936,0.000689149,0.000600804,0.00046715;0.00114402,0.000924794,0.000766016,0.000589737,0.000446383;0.00127793,0.00100958,0.000815813,0.000568085,0.000426063;0.0014493,0.00106102,0.000822573,0.000544546,0.00040995;0.00160054,0.001059,0.000798524,0.000529874,0.000401881;0.00167306,0.00102742,0.000775283,0.000512792,0.000385689;0.0016553,0.000997881,0.000747467,0.000499305,0.000378046;0.0015888,0.000969107,0.0007177,0.000486984,0.000365287;0.00153194,0.000943878,0.000695967,0.000473997,0.000353817;0.00148159,0.000922603,0.000676232,0.000464284,0.000347846;0.0014293,0.00090407,0.000661561,0.000451668,0.00033672;0.00138895,0.000883109,0.000647176,0.000443648,0.00033387;0.00135019,0.000864676,0.000632936,0.000434683,0.000323263;0.00130261,0.000848781,0.000617294,0.00042993,0.000315138;0.00125322,0.000834973,0.00060042,0.000418737,0.000311007;0.00119786,0.000809893,0.000597469,0.000413424,0.000304475;0.00114129,0.000782067,0.000524998,0.000399362,0.000286744;0.00114129,0.000782067,0.000511038,0.000349277,0.000271429]; From 11bde03d8bc7e8a7c2c602d52748036992b234a8 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:25:04 +0200 Subject: [PATCH 051/119] update --- Battery/EquivalentCircuitModel/examples/runECMfitting.m | 6 +++--- Battery/EquivalentCircuitModel/utils/costFunctionECM.m | 2 +- 2 files changed, 4 insertions(+), 4 deletions(-) diff --git a/Battery/EquivalentCircuitModel/examples/runECMfitting.m b/Battery/EquivalentCircuitModel/examples/runECMfitting.m index 6b7d6747d..7f908d14d 100644 --- a/Battery/EquivalentCircuitModel/examples/runECMfitting.m +++ b/Battery/EquivalentCircuitModel/examples/runECMfitting.m @@ -6,7 +6,7 @@ I_exp = ones(1001, 1); % Courant expérimental -parameters = create_parameters(); +parameters = createParametersECM(); % Remplacer le courant du modèle par le courant expérimental parameters.I.dataX = t_exp; @@ -19,7 +19,7 @@ disp('beginning of optimization'); % Optimization with fminsearch -best_params = fminsearch(@(p) cost_function(p, parameters, initial_values, t_exp, V_exp), initial_values, options); +best_params = fminsearch(@(p) costFunctionECM(p, parameters, initial_values, t_exp, V_exp), initial_values, options); fprintf('\n=== PARAMETERS FOUND ===\n'); fprintf('R0 = %.5f Ohms\n', best_params(1)); @@ -45,4 +45,4 @@ plot(t_exp, V_exp, 'k', 'LineWidth', 2); hold on; plot(t_sim, V_sim, 'r--', 'LineWidth', 2); legend('Expérimental', 'Modèle (Fitted)'); -title('Résultat du Fitting'); \ No newline at end of file +title('Résultat du Fitting'); diff --git a/Battery/EquivalentCircuitModel/utils/costFunctionECM.m b/Battery/EquivalentCircuitModel/utils/costFunctionECM.m index e92753dbe..0c12089f5 100644 --- a/Battery/EquivalentCircuitModel/utils/costFunctionECM.m +++ b/Battery/EquivalentCircuitModel/utils/costFunctionECM.m @@ -1,4 +1,4 @@ -function total_error = cost_function(params_test, parameters, initial_values, t_exp, V_exp) +function total_error = costFunctionECM(params_test, parameters, initial_values, t_exp, V_exp) parameters.R0 = abs(params_test(1)); From a6f79bb3a18b3b228ab410948e3569e14967d2a9 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:27:26 +0200 Subject: [PATCH 052/119] update --- .../activationEnergyOfReaction_impact.m | 0 .../{pxdparams_impact => pxdParamsImpact}/bruggeman_impact.m | 0 .../doubleLayerCapacitance_impact.m | 0 .../electronicConductivity_impact.m | 0 .../{pxdparams_impact => pxdParamsImpact}/param_dependency.m | 0 .../{pxdparams_impact => pxdParamsImpact}/porosity_impact.m | 0 .../reactionRateConstant_impact.m | 0 .../referenceDiffusionCoefficient_impact.m | 0 .../saturationConcentration_impact.m | 0 .../volumefraction_impact.m | 0 .../volumetricSurfaceArea_impact.m | 0 Battery/EquivalentCircuitModel/calibration/runFittingEIS.m | 4 +--- .../calibration/{ => utils}/costFunctionEIS.m | 0 13 files changed, 1 insertion(+), 3 deletions(-) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/activationEnergyOfReaction_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/bruggeman_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/doubleLayerCapacitance_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/electronicConductivity_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/param_dependency.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/porosity_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/reactionRateConstant_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/referenceDiffusionCoefficient_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/saturationConcentration_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/volumefraction_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{pxdparams_impact => pxdParamsImpact}/volumetricSurfaceArea_impact.m (100%) rename Battery/EquivalentCircuitModel/calibration/{ => utils}/costFunctionEIS.m (100%) diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/activationEnergyOfReaction_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/activationEnergyOfReaction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/activationEnergyOfReaction_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/activationEnergyOfReaction_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/bruggeman_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/bruggeman_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/bruggeman_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/bruggeman_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/doubleLayerCapacitance_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/doubleLayerCapacitance_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/doubleLayerCapacitance_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/doubleLayerCapacitance_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/electronicConductivity_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/electronicConductivity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/electronicConductivity_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/electronicConductivity_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/param_dependency.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/param_dependency.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/param_dependency.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/param_dependency.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/porosity_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/porosity_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/porosity_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/porosity_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/reactionRateConstant_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/reactionRateConstant_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/reactionRateConstant_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/reactionRateConstant_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/referenceDiffusionCoefficient_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/referenceDiffusionCoefficient_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/referenceDiffusionCoefficient_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/referenceDiffusionCoefficient_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/saturationConcentration_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/saturationConcentration_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/saturationConcentration_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/saturationConcentration_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumefraction_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumefraction_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumefraction_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumefraction_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumetricSurfaceArea_impact.m b/Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumetricSurfaceArea_impact.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/pxdparams_impact/volumetricSurfaceArea_impact.m rename to Battery/EquivalentCircuitModel/calibration/pxdParamsImpact/volumetricSurfaceArea_impact.m diff --git a/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m b/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m index 9a6a0ab46..33c8d940a 100644 --- a/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m +++ b/Battery/EquivalentCircuitModel/calibration/runFittingEIS.m @@ -5,11 +5,9 @@ params0 = [3e-3, 0.00260, 100, 0.00132, 1]; - [Z_re_exp, Z_im_exp, omega] = load_experimental_data(); - -%lengthZ = length(Z_im_exp); +% lengthZ = length(Z_im_exp); % synthetic data % opti_params = [0.00341, 0.00260, 5663.9, 0.00132, 0.9]; % params with diff --git a/Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m b/Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m similarity index 100% rename from Battery/EquivalentCircuitModel/calibration/costFunctionEIS.m rename to Battery/EquivalentCircuitModel/calibration/utils/costFunctionEIS.m From c233414f2143fc7e9b20f641509f3b99c6d6791d Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:32:44 +0200 Subject: [PATCH 053/119] fix in load_chen_data --- .../calibration/utils/load_chen_data.m | 12 +++++++++--- 1 file changed, 9 insertions(+), 3 deletions(-) diff --git a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m index 45b210d80..a05b021e5 100644 --- a/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m +++ b/Battery/EquivalentCircuitModel/calibration/utils/load_chen_data.m @@ -38,13 +38,19 @@ c_pe = 17.038*mol/litre; % initial concentration at positive electrode initstate = initStateChen2020(model, c_ne, c_pe); + + options = []; + options.stateInitialization.initializationSetup = 'given state'; + options.stateInitialization.computeSteadyState = false; + + extrastructs = []; + extrastructs.initstate = initstate; - impsolv = ImpedanceSolver(inputparams, 'initstate', initstate, 'computeSteadyState', false); - + impsolv = ImpedanceSolver(inputparams, options, extrastructs); omegas = logspace(-4, 2, 50); Z = impsolv.computeImpedance(omegas); Z_real = real(Z); Z_imag = imag(Z); -end \ No newline at end of file +end From 3a97d0caf97528df049a5bd7b22850236bdd4003 Mon Sep 17 00:00:00 2001 From: Xavier Raynaud Date: Mon, 22 Jun 2026 13:34:29 +0200 Subject: [PATCH 054/119] added ECM tests in testsuite --- Tests/TestExamples/TestRunExamples.m | 2 ++ 1 file changed, 2 insertions(+) diff --git a/Tests/TestExamples/TestRunExamples.m b/Tests/TestExamples/TestRunExamples.m index 8cc100900..be4d19c01 100644 --- a/Tests/TestExamples/TestRunExamples.m +++ b/Tests/TestExamples/TestRunExamples.m @@ -15,6 +15,8 @@ 'runChen2020' , ... 'runImpedanceChen' , ... 'runImpedanceScript' , ... + 'exampleECM' , ... + 'runClassFitting' , ... 'runCR' , ... 'runGittTest' , ... 'runJellyRoll' , ... 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